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Roscilde, Tommaso

Publications and source records attributed to Roscilde, Tommaso.

9 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Reconstructing the spatial structure of quantum correlations in materials

Quantum correlations are a fundamental property of quantum many-body states. Yet they remain experimentally elusive, hindering certification of genuine quantum behavior, especially in quantum materials. Here we show that the momentum-dependent dynamical susceptibility measured via inelastic neutron scattering enables the systematic reconstruction of a general family of quantum correlation functions, which express the degree of quantum coherence in the fluctuations of two spins at an arbitrary mutual distance. Using neutron scattering data for the compound KCuF 3 —a system of weakly coupled S = 1 / 2 Heisenberg chains—and numerically exact quantum Monte Carlo data, we show that quantum correlations possess a radically different spatial structure with respect to conventional correlations. Indeed, they exhibit a different emergent length scale—the quantum coherence length—which is finite at any finite temperature (including when long-range magnetic order develops). Moreover, we show theoretically that coupled Heisenberg spin chains exhibit a form of quantum monogamy, with a trade-off between quantum correlations along and transverse to the spin chains. These results highlight real-space quantum correlators as an informative, model-independent means of probing the underlying quantum state of real quantum materials. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗
DOE OSTI2013

Dirty-boson physics with magnetic insulators

We report on recent theoretical and experimental efforts aimed at the investigation of the physics of interacting disordered bosons (so-called dirty bosons) in the context of quantum magnetism. The physics of dirty bosons is relevant to a wide variety of condensed matter systems, encompassing helium in porous media, granular superconductors, and ultracold atoms in disordered optical potentials, to cite a few. Nevertheless, the understanding of the transition from a localized, Bose-glass phase to an ordered, superfluid condensate phase still represents a fundamentally open problem. Still to be constructed is also a quantitative description of the highly inhomogeneous and strongly correlated phases connected by the transition. We observe how disordered magnetic insulators in a strong magnetic field can provide a well-controlled realization of the above transition. Combining numerical simulations with experiments on real materials can demonstrate some fundamental properties of the critical behavior, such as the scaling of the critical temperature to condensation close to the quantum critical point.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

Quantum critical scaling at a Bose-glass/superfluid transition: Theory and experiment for a model quantum magnet

Here, we investigate the quantum phase transition from magnetic Bose Glass to magnetic Bose-Einstein condensation induced by a magnetic field in NiCl 2 ∙4SC(NH 2 ) 2 (dichloro-tetrakis-thiourea-nickel, or DTN), doped with Br (Br-DTN) or site diluted. Quantum Monte Carlo simulations for the quantum phase transition of the model Hamiltonian for Br-DTN, as well as for site-diluted DTN, are consistent with conventional scaling at the quantum critical point and with a critical exponent $z$ verifying the prediction $z = d$; moreover the correlation length exponent is found to be $ν = 0.75(10)$, and the order parameter exponent to be $β = 0.95(10)$. We investigate the low-temperature thermodynamics at the quantum critical field of Br-DTN both numerically and experimentally, and extract the power-law behavior of the magnetization and of the specific heat. Our results for the exponents of the power laws, as well as previous results for the scaling of the critical temperature to magnetic ordering with the applied field, are incompatible with the conventional crossover-scaling Ansatz proposed by Fisher et al. [Phys. Rev. B 40, 546 (1989)]. However they can all be reconciled within a phenomenological Ansatz in the presence of a dangerously irrelevant operator.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Bose glass and Mott glass of quasiparticles in a doped quantum magnet

The low-temperature states of bosonic fluids exhibit fundamental quantum effects at the macroscopic scale: the best-known examples are Bose–Einstein condensation and superfluidity, which have been tested experimentally in a variety of different systems. When bosons interact, disorder can destroy condensation, leading to a ‘Bose glass’. This phase has been very elusive in experiments owing to the absence of any broken symmetry and to the simultaneous absence of a finite energy gap in the spectrum. Here we report the observation of a Bose glass of field-induced magnetic quasiparticles in a doped quantum magnet (bromine-doped dichloro-tetrakis-thiourea-nickel, DTN). The physics of DTN in a magnetic field is equivalent to that of a lattice gas of bosons in the grand canonical ensemble; bromine doping introduces disorder into the hopping and interaction strength of the bosons, leading to their localization into a Bose glass down to zero field, where it becomes an incompressible Mott glass. The transition from the Bose glass (corresponding to a gapless spin liquid) to the Bose–Einstein condensate (corresponding to a magnetically ordered phase) is marked by a universal exponent that governs the scaling of the critical temperature with the applied field, in excellent agreement with theoretical predictions. Our study represents a quantitative experimental account of the universal features of disordered bosons in the grand canonical ensemble.

Science & Technology - Other Topics↗
DOE OSTI2010

Localization of Cold Atoms in State-Dependent Optical Lattices via a Rabi Pulse

We propose a novel realization of Anderson localization in nonequilibrium states of ultracold atoms in an optical lattice. A Rabi pulse transfers part of the population to a different internal state with infinite effective mass. These frozen atoms create a quantum superposition of different disorder potentials, localizing the mobile atoms. For weakly interacting mobile atoms, Anderson localization is obtained. The localization length increases with increasing disorder and decreasing interaction strength, contrary to the expectation for equilibrium localization.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2010

Magnetic Bose glass phases of coupled antiferromagnetic dimers with site dilution

We numerically investigate the phase diagram of two-dimensional site-diluted coupled dimer systems in an external magnetic field. We show that this phase diagram is characterized by the presence of an extended Bose glass, not accessible to mean-field approximation, and stemming from the localization of two distinct species of bosonic quasiparticles appearing in the ground state. On the one hand, nonmagnetic impurities doped into the dimer-singlet phase of a weakly coupled dimer system are known to free up local magnetic moments. The deviations of these local moments from full polarization along the field can be mapped onto a gas of bosonic quasiparticles, which undergo condensation in zero and very weak magnetic fields, corresponding to transverse long-range antiferromagnetic order. An increasing magnetic field lowers the density of such quasiparticles to a critical value at which a quantum phase transition occurs, corresponding to the quasiparticle localization on clusters of local magnets (dimers, trimers, etc.) and to the onset of a Bose glass. Strong finite-size quantum fluctuations hinder further depletion of quasiparticles from such clusters, and thus lead to the appearance of pseudoplateaus in the magnetization curve of the system. On the other hand, site dilution hinders the field-induced Bose-Einstein condensation of triplet quasiparticles on the intact dimers, and it introduces instead a Bose glass of triplets. A thorough numerical investigation of the phase diagram for a planar system of coupled dimers shows that the two above-mentioned Bose glass phases are continuously connected, and they overlap in a finite region of parameter space, thus featuring a two-species Bose glass. The quantum phase transition from Bose glass to magnetically ordered phases in two dimensions is marked by novel universal exponents (z{approx_equal}2, {beta}{approx_equal}0.9, and {nu}{approx_equal}1). Hence we conclude that doped quantum antiferromagnets in a field represent an ideal setting for the study of fundamental dirty-boson physics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2010

Exploring the grand-canonical phase diagram of interacting bosons in optical lattices by trap squeezing

In this article, we theoretically discuss how quantum simulators based on trapped cold bosons in optical lattices can explore the grand-canonical phase diagram of homogeneous lattice boson models, via control of the trapping potential independent of all other experimental parameters (trap squeezing). Based on quantum Monte Carlo, we establish the general scaling relation linking the global chemical potential to the Hamiltonian parameters for the Bose-Hubbard model in a parabolic trap, describing cold bosons in optical lattices; we find that this scaling relation is well captured by a modified Thomas-Fermi scaling behavior - corrected for quantum fluctuations - in the case of sufficiently high density and/or sufficiently weak interactions, and by a mean-field Gutzwiller ansatz over a much larger parameter range. This scaling relation allows us to control experimentally the chemical potential, independent of all other Hamiltonian parameters, via trap squeezing; given that the global chemical potential coincides with the local chemical potential in the trap center, measurements of the central density as a function of the chemical potential give access to the information on the bulk compressibility of the Bose-Hubbard model. Supplemented with time-of-flight measurements of the coherence properties, the measurement of compressibility enables one to discern among the various possible phases realized by bosons in an optical lattice with or without external (periodic or random) potentials - for example, superfluid, Mott insulator, band insulator, and Bose glass. We theoretically demonstrate the trap-squeezing investigation of these phases in the case of bosons in a one-dimensional optical lattice and in a one-dimensional incommensurate superlattice.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗