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Rosenfeld, D.

Publications and source records attributed to Rosenfeld, D..

Tracking Aerosol Convection Interactions Experiment (TRACER) Field Campaign Report

Convective clouds serve a critical role in the Earth’s energy and water cycles through their transport of heat, moisture, momentum, and chemical species through the troposphere driving the global circulation (e.g., Hartmann et al. 1984, Del Genio et al. 2012, Su et al. 2014). On more local scales, convective clouds impact the atmospheric heating profile through diabatic heating effects, removal of water from the atmospheric column through precipitation, and conditioning of the local environment impacting further development of clouds (e.g., Sullivan and Voigt 2021). These critical roles underscore the importance of realistic representation of convective processes across scales of models from large-eddy simulation (LES), to convection-permitting models (CPM; e.g., Kendon et al. 2020, Marinescu et al. 2021), to numerical weather prediction (NWP) models used for operational weather forecasting, to Earth system models used to predict climate sensitivity (Sanderson et al. 2011, Sherwood et al. 2014, Tomassini et al. 2014, Zhao et al. 2016, Cronin et al. 2017). A key component of improving model representation of convective clouds is better quantification and parameterization of updraft microphysics and dynamics, including their interactions with the surrounding environment and storm organization (Bony et al. 2015, Hagos and Houze 2016, Donner et al. 2016, Morrison et al. 2020). Aerosol is an important environmental factor that could affect convective clouds and precipitation since cloud droplet and ice formation processes are initiated by it. Andrae et al. (2004) hypothesized that aerosols associated with increased biomass burning particles acting as cloud condensation nuclei (CCN) result in smaller and more monodisperse cloud droplets leading to suppression of warm rain formation, ultimately leading to more cloud water being lofted above the freezing level based on observations in the Amazon region. The subsequent increase in latent heat release increases the buoyancy of rising convective parcels invigorating the deep convection. This work was followed by a description of the theoretical basis for this “cold-phase invigoration” by Rosenfeld et al. (2008), who argued that it could have a significant effect for deep convective clouds with warm cloud-bases. Several modeling studies (e.g., Khain et al. 2005, 2009, van den Heever et al. 2006, Fan et al. 2007, 2009, 2012, Lee et al. 2008, Storer et al. 2010, Lebo et al. 2012, Storer and van den Heever 2013, Chen et al. 2020, Dagan et al. 2022) have investigated these aerosol-convection interactions and the environmental factors that influence their relative importance and magnitude. More recently, several studies have indicated that “warm-phase invigoration”, the enhancement of convection through condensational heating, also appears to play a role in enhancing both shallow cumuli (Seiki and Nakajima 2014, Saleeby et al 2015) and deeper tropical convection (Lebo and Seinfeld 2011, Khain et al. 2012, Sheffield et al 2015, Fan et al. 2018, Igel and van den Heever 2021), as well as Houston thunderstorms (Fan et al. 2007, 2020). However, still other studies have provided additional evidence of systematic biases in simulated convective outflow ice size distribution properties, which are consistent with a lack of poorly understood secondary ice production within convective updrafts (e.g., Fridlind et al. 2017). To help address these critical gaps in our understanding of cloud processes, aerosol processes and aerosol-cloud interactions, the Tracking Aerosol Convection Interactions Experiment was designed building upon efforts by the Aerosol, Cloud, Precipitation and Climate (ACPC) Initiative (http://acpcintiative.org/), a joint effort of the International Geosphere-Biosphere Programme (IGBP) and the World Climate Research Program (WCRP) that focused on resolving uncertainties in the interactions between aerosol and clouds towards better understanding the role that these interactions play in the climate system. The TRACER campaign was motivated by recommendations from a number of pilot studies undertaken by ACPC (van den Heever et al. 2017, Fridlind et al. 2019, Hu et al. 2019, Fan et al. 2020, Marinescu et al. 2021, Hernandez-Deckers et al. 2022) that pointed towards the southeastern Texas region as a locale where aerosol-convection interactions could be studied owing to the copious occurrence of isolated convection during the summer months accompanied by diverse and significant sources of aerosols from both anthropogenic and natural sources. The TRACER campaign began on 01 October 2021 and extended through 30 September 2022 with an intensive operational period (IOP) during June-September 2022. Three main sites (Table 1) were managed by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility.

54 ENVIRONMENTAL SCIENCES↗

Influence of biogenic emissions from boreal forests on aerosol–cloud interactions

Boreal forest acts as a carbon sink and contributes to the formation of secondary organic aerosols via emission of aerosol precursor compounds. However, these influences on the climate system are poorly quantified. Here we show direct observational evidence that aerosol emissions from the boreal forest biosphere influence warm cloud microphysics and cloud-aerosol interactions in a scale-dependent and highly dynamic manner. Analyses of in situ and ground-based remote-sensing observations from the SMEAR II station in Finland, conducted over eight months in 2014, reveal substantial increases in aerosol load over the forest one to three days after aerosol-poor marine air enters the forest environment. We find that these changes are consistent with secondary organic aerosol formation and, together with water-vapour emissions from evapotranspiration, are associated with changes in the radiative properties of warm, low-level clouds. Here, the feedbacks between boreal forest emissions and aerosol-cloud interactions and the highly dynamic nature of these interactions in air transported over the forest over timescales of several days suggest boreal forests have the potential to mitigate climate change on a continental scale. Our findings suggest that even small changes in aerosol precursor emissions, whether due to changing climatic or anthropogenic factors, may substantially modify the radiative properties of clouds in moderately polluted environments. Emissions from the boreal forest biosphere can substantially increase aerosol load above the forest and influence the radiative properties of clouds, according to analysis of observations from a monitoring station in Finland.

54 ENVIRONMENTAL SCIENCES↗

Tracking Aerosol Convective Interactions Experiment (TRACER) Science Plan

Convective clouds play an important role in the Earth's climate system as a driver of large-scale circulations and a primary mechanism for the transport of heat, moisture, aerosols, and momentum throughout the troposphere. Despite their climatic importance, multi-scale models continue to have persistent biases produced by insufficient representation of convective clouds. This is the result of an incomplete understanding of key processes such as convective initiation, updraft and downdraft dynamics, cloud and precipitation microphysics, and aerosol-convection interactions.The Aerosol-Cloud-Precipitation-Climate Initiative, an international research group dedicated to advancing understanding of aerosol impacts on clouds relevant to climate, has identified the Houston, Texas region as an optimal location for targeted studies of aerosol-convection interactions within frequently developing isolated deep convection. Houston lies within a humid subtropical climate regime, where onshore flow and sea-breeze convection interact with a range of aerosol conditions associated with Houston's urban and industrial emissions. Pilot studies have suggested that convective clouds in this region are potentially significantly impacted by the varying aerosol conditions.

Jensen, M.↗

Remote Sensing the Vertical Profile of Cloud Droplet Effective Radius, Thermodynamic Phase, and Temperature

Cloud-aerosol interaction is a key issue in the climate system, affecting the water cycle, the weather, and the total energy balance including the spatial and temporal distribution of latent heat release. Information on the vertical distribution of cloud droplet microphysics and thermodynamic phase as a function of temperature or height, can be correlated with details of the aerosol field to provide insight on how these particles are affecting cloud properties and their consequences to cloud lifetime, precipitation, water cycle, and general energy balance. Unfortunately, today's experimental methods still lack the observational tools that can characterize the true evolution of the cloud microphysical, spatial and temporal structure in the cloud droplet scale, and then link these characteristics to environmental factors and properties of the cloud condensation nuclei. Here we propose and demonstrate a new experimental approach (the cloud scanner instrument) that provides the microphysical information missed in current experiments and remote sensing options. Cloud scanner measurements can be performed from aircraft, ground, or satellite by scanning the side of the clouds from the base to the top, providing us with the unique opportunity of obtaining snapshots of the cloud droplet microphysical and thermodynamic states as a function of height and brightness temperature in clouds at several development stages. The brightness temperature profile of the cloud side can be directly associated with the thermodynamic phase of the droplets to provide information on the glaciation temperature as a function of different ambient conditions, aerosol concentration, and type. An aircraft prototype of the cloud scanner was built and flew in a field campaign in Brazil.

Martins, J. V.↗

"Weekend-effect" evidence for intensification of storms by pollution over U.S.

Aerosols change the way precipitating clouds evolve, due to their effect on condensation and ice formation. The net effect of aerosols on precipitation varies depending on the local environment and synoptic situation, the types of aerosols, and also on how far downstream one looks for effects. Repeated experiments with controlled release of aerosols would be helpful in unraveling how aerosols affect precipitation. The weekly variation in human activity may provide just such a set of experiments. Using the rainfall estimates from the passive microwave instrument on the Tropical Rainfall Measuring Mission (TRMM), which has been orbiting for over eight years and can view areas as far north as about 40 degs, we find that there is indeed a weekly variation in summer (JJA) rainfall over the southeastern U.S. land area, with the average rain rate peaking in the middle of the week (Tue-Thu). Rainfall over nearby oceanic areas, on the other hand, seems to peak on weekends. A bootstrap statistical test indicates that the variations are unlikely to be due to chance. Physically related weekly variations in the statistics of ground-based measurements and model reanalysis data are found. The midweek peak in rainfall over land coincides with the well documented midweek peak in pollution around much of the U.S., and is unlikely to be due to other weekly variations in human influence. The midweek increase is also unlikely to be a consequence of the radiative heating or cooling of the atmosphere by the aerosols.

Bell, T. L.↗

Midweek Intensification of Rain in the U.S.: Does Air Pollution Invigorate Storms?

The effect of pollution on rainfall has been observed to depend both on the type of pollution and the precipitating environment. The climatological consequences of pollution for rainfall are uncertain. In some urban areas, pollution varies with the day of the week because of weekly variations in human activity, in effect providing a repeated experiment on the effects of pollution. Weekly variations in temperature, pressure, cloud characteristics, hails and lightning are observed in many areas. Observing a weekly cycle in rainfall statistics has proven to be more difficult, although there is some evidence for it. Here we examine rainfall statistics from the Tropical Rainfall Measuring Mission (TRMM) satellite over the southern U.S. and adjacent waters, and find that there is a distinct, statistically significant weekly cycle in summertime rainfall over the southeast U.S., as well as weekly variations in rainfall over the nearby Atlantic and the Gulf of Mexico. Rainfall over land peaks in the middle of the week, suggesting that summer rainfall on large scales may increase as pollution levels rise. Both rain statistics over land and what appear to be compensating effects over adjacent seas support the suggestion that air pollution invigorates convection and outflow aloft.

Bell, T. L.↗

Thermodynamic Conditions Favorable to Superlative Thunderstorm Updraft, Mixed Phase Microphysics and Lightning Flash Rate

Satellite observations of lightning flash rate have been merged with proximal surface station thermodynamic observations toward improving the understanding of the response of the updraft and lightning activity in the tropical atmosphere to temperature. The tropical results have led in turn to an examination of thermodynamic climatology over the continental United States in summertime and its comparison with exceptional electrical conditions documented in earlier studies. The tropical and mid-latitude results taken together support an important role for cloud base height in regulating the transfer of Convective Available Potential Energy (CAPE) to updraft kinetic energy in thunderstorms. In the tropics, cloud base height is dominated by the dry bulb temperature over the wet bulb temperature as the lightning-regulating temperature in regions characterized by moist convection. In the extratropics, an elevated cloud base height may enable larger cloud water concentrations in the mixed phase region, a favorable condition for the positive charging of large ice particles that may result in thunderclouds with a reversed polarity of the main cloud dipole. The combined requirements of instability and cloud base height serve to confine the region of superlative electrification to the vicinity of the ridge in moist entropy in the western Great Plains.

Williams, E.↗

Hurricane Erin September 10, 2001: Comparison of TRMM, AMSU-A and QUIKSCAT Data with an Extensive Aircraft Data Set, and Some Preliminary Results

A main purpose of this study is to compare satellite products from TRMM, AMSU-A and QuikSCAT with a unique, extensive aircraft data set in Category 3 Hurricane Erin on September 10,2001, and to draw some preliminary conclusions from the data. For the first time, dropwinsondes were obtained by the NASA ER-2 aircraft. There were 8 soundings in the eye, core and surroundings radially out to the edge of the Central Dense Overcast (CDO). Additionally, 11 dropwinsondes from the DC-8 aircraft at about 12 km documented the storm outskirts and environment. TRMM made a direct overpass of the eye as did both NOAA-15 and NOM-16 with AMSU on board. Among the most interesting results: Contours of the tropopause height (a first). As expected from earlier fragmentary results, the tropopause was approximately 1 km higher in the core than in the environment. The highest tropopause was about 2 km above the tallest towers in the eyewall, south-southeast of the eye center, suggesting that earlier convective towers had been higher than those measured by EDOP and TRMM during the flights. Surprisingly, the heaviest precipitation was on the opposite side of the eyewall from the tallest convective towers. The warm core was elongated in the vertical, and poorly retrieved from the AMSU-A data by the NESDIS profile retrieval algorithm. The eye of Erin was "dirty". A CCN/CN counter flown on the NOAA P3 at 14.3 km showed a concentration of 1500 aerosol particles per cubic centimeter. This is an order of magnitude higher than a sample in the hurricane environment. TRMM data are used to hypothesize an explanation.

Simpson, J.↗

The Role of Boundary Layer Aerosol in the Vertical Development of Precipitation and Electrification: Another Look at the Contrast Between Lightning over Land and Over Ocean

Comparisons are made between the cloud condensation nuclei (CCN) concentration in the boundary layer and radar/electrical observations of the vertical development of precipitation and lightning in both the 'break period' and 'monsoon' regimes in tropical Brazil. The initial radar echoes and the maximum flash rates are found to be higher when the CCN concentration is higher, characteristic of the 'break period' conditions. One possible explanation for both observations is the survival of cloud droplets against coalescence and their attainment of the mixed phase region aloft.

Williams, E.↗

Optimal Empirical Z-R Relations

We attempt to mathematically justify the two empirical approaches to the problem of deriving Z-R relations, namely the power-law regression and the 'probability matching method'.

mathematical assumptions power-law Z-R relation pr↗

The Effect of Strain on the Base Resistance and Transit Time of Ungraded and Compositional-Graded SiGe HBTs

A theoretical study of the effects of the strain on the base properties of ungraded and compositional-graded n-p-n SiGe Heterojunction Bipolar Transistors (HBT) is presented. The dependencies of the transverse hole mobility and longitudinal electron mobility upon strain, composition and doping, are formulated using published Monte-Carlo data and, consequently, the base resistance and transit time are modeled and calculated. The results are compared to results obtained using common formulas that ignore these dependencies. The differences between the two sets of results are shown. The paper's conclusion is that for the design, analysis and optimization of high frequency SiGe HBTs the strain effects on the base properties cannot be ignored.

Rosenfeld, D.↗

The effects of strain on the microwave performance of SiGe HBTs

Theoretical study results are presented for the effects of strain on the cutoff frequencies of SiGe heterojunction bipolar transistors. The positive role played by the strain on the base resistance and transit time is shown to have a further effect on high-frequency performance.

Rosenfeld, D.↗

Effects of strain on the microwave performance of SiGe HBTs

The results of a theoretical study of the effects of the strain on the cutoff frequencies of SiGe HBTs are presented. The influence of the strain on the base resistance and transit time, and through them on high-frequency performance, was taken into account. The positive role played by the strain is demonstrated.

BASE RESISTANCE↗

The quantum efficiency of HgCdTe photodiodes in relation to the direction of illumination and to their geometry

A theoretical study of the effect of the direction of the incident light on the quantum efficiency of homogeneous HgCdTe photodiodes suitable for sensing infrared radiation in the 8-12 microns atmospheric window is presented. The probability of an excess minority carrier to reach the junction is derived as a function of its distance from the edge of the depletion region. Accordingly, the quantum efficiency of photodiodes is presented for two geometries. In the first, the light is introduced directly to the area in which it is absorbed (opaque region), while in the second, the light passes through a transparent region before it reaches the opaque region. Finally, the performance of the two types of diodes is analyzed with the objective of finding the optimal width of the absorption area. The quantum efficiency depends strongly on the way in which the light is introduced. The structure in which the radiation is absorbed following its crossing the transparent region is associated with both higher quantum efficiency and homogeneity. In addition, for absorption region widths higher than a certain minimum, the quantum efficiency in this case is insensitive to the width of the absorption region.

Rosenfeld, D.↗

High frequency performance of Si(1-x)Ge(x)/Si(1-y)Ge(y)/Si(1-x)Ge(x) HBTs

The results of a theoretical study of the performance of high speed SiGe HBTs is presented. The study includes a group of SiGe HBTs in which the Ge concentration in the base is 20 percent higher than that in the emitter and collector (i.e., y = x + 0.2). It is shown that the composition dependences of f(T) and the f(max) are nonmonotonic. As the Ge composition in the emitter and collector layers is increased, f(T) and f(max) first decrease, then remain constant and finally increase to attain their highest values.

Rosenfeld, D.↗