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Rotureau, J.

Publications and source records attributed to Rotureau, J..

9 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Density matrix renormalization group description of the island of inversion isotopes F 28 – 33

Recent experiments have confirmed that the neutron-rich isotopes 28,29 F belong to the so-called island of inversion (IOI), a region of the nuclear chart around Z = 10 and N = 20 where nuclear structure deviates from the standard shell model predictions due to deformation and continuum effects. However, while the general principles leading to the IOI are relatively well understood, the details of the low-lying structure of the exotic fluorine isotopes 28–33 F are basically unknown. In this study, we perform large-scale shell model calculations including continuum states to investigate the properties of the neutron-rich isotopes 25–33 F, from a core of 24 O and using an effective two-body interaction with a small number of adjustable parameters in the central and tensor channels. We develop two models adjusted on experimentally confirmed states in 25,26 O and 25–27 F based on different assumptions concerning the positions of the neutron 0d 3/2 and 1p 3/2 shells, and solve the many-body problem using the density matrix renormalization group (DMRG) method for open quantum systems in an sd–fp model space. We obtain the first detailed spectroscopy of 25–33F in the continuum and show how the interplay between continuum effects and deformation explains the recent data on 28,29 F. Several deformed one- and two-neutron halo states are predicted in 29,31 F, and we provide some information about the possible structure of the heaviest fluorine isotopes. We also suggest several experimental studies of interest to constraint models and test the present predictions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Gamow-shell-model description of Li isotopes and their mirror partners

Background: Weakly bound and unbound nuclei close to particle drip lines are laboratories of new nuclear structure physics at the extremes of neutron/proton excess. The comprehensive description of these systems requires an open quantum system framework that is capable of treating resonant and nonresonant many-body states on equal footing. Purpose: In this work, we develop the complex-energy configuration interaction approach to describe binding energies and spectra of selected 5 ≤ $\textit{A}$ ≤ 11 nuclei. Method: We employ the complex-energy Gamow shell model (GSM) assuming a rigid 4 He core. The effective Hamiltonian, consisting of a core-nucleon Woods-Saxon potential and a simplified version of the Furutani-Horiuchi-Tamagaki interaction with the mass-dependent scaling, is optimized in the $\textit{sp}$ space. To diagonalize the Hamiltonian matrix, we employ the Davidson method and the Density Matrix Renormalization Group technique. Results: We report our optimized GSM Hamiltonian offers a good reproduction of binding energies and spectra with the root-mean-square (rms) deviation from experiment of 160 keV. Since the model performs well when used to predict known excitations that have not been included in the fit, it can serve as a reliable tool to describe poorly known states. A case in point is our prediction for the pair of unbound mirror nuclei 10 Li – 10 N in which a huge Thomas-Ehrman shift dramatically alters the pattern of low-energy excitations. Conclusion: The new model will enable comprehensive studies of structure and reactions aspects of light drip-line nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Merging ab initio theory and few-body approach for (d, p) reactions

A framework for A(d, p)B reactions is introduced by merging the microscopic approach to computing the properties of the nucleon-target systems and the three-body n + p + A reaction formalism, thus providing a consistent link between the reaction cross sections and the underlying microscopic structure. In this first step toward a full microscopic description, we focus on the inclusion of the neutron-target microscopic properties. The properties of the neutron-target subsystem are encapsulated in the Green's function which is computed with the coupled Cluster theory using a chiral nucleon-nucleon and three-nucleon interactions. Subsequently, this many-body information is introduced in the few-body Green's Function Transfer approach to (d, p) reactions. Our benchmarks on stable targets 40,48 Ca show an excellent agreement with the data. We then proceed to make specific predictions for (d, p) on neutron rich 52,54 Ca isotopes. These predictions are directly relevant to testing the new magic numbers N = 32, 34 and are expected to be feasible in the first campaign of the projected FRIB facility.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Energy spectrum of neutron-rich helium isotopes: Complex made simple

We demonstrate herein that the intricate energy spectrum of neutron-rich helium isotopes can be straightforwardly described by taking advantage of the low-energy properties of neutron-neutron interaction and the scale separation that is present in diluted drip-line systems. By using arguments based on the halo effective field theory, we further carry out a parameter reduction of the complex-energy configuration interaction framework in the s p d space, including resonant and scattering states. By constraining the core potential to α - n scattering phase shifts and adjusting the strength of the spin-singlet central neutron-neutron interaction, we reproduce experimental energies and widths of 5 – 8 He within tens of keV precision. We predict a parity inversion of narrow resonances in He 9 and show that the ground state of He 10 is an s -wave-dominated configuration that could decay through two-neutron emission. This threshold state can be viewed as a “double-halo” structure in an analogy to the atomic He 3 4 He 2 trimer.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Search for excited states in O 25

Theoretical calculations suggest the presence of low-lying excited states in 25 O. Previous experimental searches by means of proton knockout on 26 F produced no evidence for such excitations. We search for excited states in 25 O using the 24 O(d,p) 25 O reaction. The theoretical analysis of excited states in unbound 25,27 O is based on the configuration interaction approach that accounts for couplings to the scattering continuum. We use invariant-mass spectroscopy to measure neutron-unbound states in 25 O. For the theoretical approach, we use the complex-energy Gamow Shell Model and Density Matrix Renormalization Group method with a finite-range two-body interaction optimized to the bound states and resonances of 23–26 O, assuming a core of 22 O. Here we predict energies, decay widths, and asymptotic normalization coefficients. Our calculations in a large spdf space predict several low-lying excited states in 25 O of positive and negative parity, and we obtain an experimental limit on the relative cross section of a possible J π = 1/2 + state with respect to the ground state of 25 O at σ 1/2+ /σ g.s. = 0.25$^{+1.0}_{-0.25}$. We also discuss how the observation of negative parity states in 25 O could guide the search for the low-lying negative parity states in 27 O. Previous experiments based on the proton knockout of 26 F suffered from the low cross sections for the population of excited states in 25 O because of low spectroscopic factors. In this respect, neutron transfer reactions carry more promise.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Toward a complete theory for predicting inclusive deuteron breakup away from stability

We present an account of the current status of the theoretical treatment of inclusive (d, p) reactions in the breakup-fusion formalism, pointing to some applications and making the connection with current experimental capabilities. Three independent implementations of the reaction formalism have been recently developed, making use of different numerical strategies. The codes also originally relied on two different but equivalent representations, namely the prior (Udagawa-Tamura, UT) and the post (Ichimura-Austern-Vincent, IAV) representations. The different implementations have been benchmarked for the first time, and then applied to the Ca isotopic chain. The neutron-Ca propagator is described in the Dispersive Optical Model (DOM) framework, and the interplay between elastic breakup (EB) and non-elastic breakup (NEB) is studied for three Ca isotopes at two different bombarding energies. The accuracy of the description of different reaction observables is assessed by comparing with experimental data of (d, p) on 40,48Ca. We discuss the predictions of the model for the extreme case of an isotope (60Ca) currently unavailable experimentally, though possibly available in future facilities (nominally within production reach at FRIB). We explore the use of (d, p) reactions as surrogates for (n,γ) processes, by using the formalism to describe the compound nucleus formation in a (d,pγ) reaction as a function of excitation energy, spin, and parity. The subsequent decay is then computed within a Hauser-Feshbach formalism. Comparisons between the (d,pγ) and (n,γ) induced gamma decay spectra are discussed to inform efforts to infer neutron captures from (d,pγ) reactions. Finally, we identify areas of opportunity for future developments, and discuss a possible path toward a predictive reaction theory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Optical potential from first principles

Here, we develop a method to construct a microscopic optical potential from chiral interactions for nucleon-nucleus scattering. The optical potential is constructed by combining the Green’s function approach with the coupled-cluster method. To deal with the poles of the Green’s function along the real energy axis we employ a Berggren basis in the complex energy plane combined with the Lanczos method. Using this approach, we perform a proof-of-principle calculation of the optical potential for the elastic neutron scattering on 16 O. For the computation of the ground-state of 16 O, we use the coupled-cluster method in the singles-and-doubles approximation, while for the A ±1 nuclei we use particle-attached/removed equation-of-motion method truncated at two-particle-one-hole and one-particle-two-hole excitations, respectively. We verify the convergence of the optical potential and scattering phase shifts with respect to the model-space size and the number of discretized complex continuum states. We also investigate the absorptive component of the optical potential (which reflects the opening of inelastic channels) by computing its imaginary volume integral and find an almost negligible absorptive component at low-energies. To shed light on this result, we computed excited states of 16 O using equation-of-motion coupled-cluster method with singles-and- doubles excitations and we found no low-lying excited states below 10 MeV. Furthermore, most excited states have a dominant two-particle-two-hole component, making higher-order particle-hole excitations necessary to achieve a precise description of these core-excited states. We conclude that the reduced absorption at low-energies can be attributed to the lack of correlations coming from the low-order cluster truncation in the employed coupled-cluster method.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗