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Sachse, Glen W.

Publications and source records attributed to Sachse, Glen W..

At least 37 records · Page 2

Observations of Convective and Dynamical Instabilities in Tropopause Folds and their Contribution to Stratosphere-Troposphere Exchange

With aircraft-mounted in-situ and remote sensing instruments for dynamical, thermal. and chemical measurements, we studied two cases of tropopause folding. In both folds we found Kelvin-Helmholtz billows with horizontal wavelength of about 900 m and thickness of about 120 m. In one case the instability was effectively mixing the bottomside of the fold, leading to the transfer of stratospheric air into the troposphere. Also we discovered in both cases small-scale secondary ozone maxima shortly after the aircraft ascended past the topside of the fold that corresponded to regions of convective instability. We interpreted this phenomenon as convectively breaking gravity waves. Therefore, we posit that convectively breaking gravity waves acting on tropopause folds must be added to the list of important irreversible mixing mechanisms leading to stratosphere-troposphere exchange.

Cho, John Y. N.↗

Distribution and Seasonality of Selected Hydrocarbons and Halocarbons over the Western Pacific Basin During PEM-West A and PEM-West B

Nonmethane hydrocarbons (NMHCs) and halocarbons were measured in the troposphere over the northwestern Pacific as part of the airborne component of NASA's Pacific Exploratory Mission-West Phase B (PEM-West B). This study took place in late winter of 1994, a period characterized by maximum outflow from the Asian continent. The results are compared to those from Pacific Exploratory Mission-West Phase A (PEM-West A), which was flown in the same region during late summer of 1991, when flow from the subtropical western Pacific dominated the lower troposphere. Mixing ratios of NMHCs, tetrachloroethene (C2Cl4), and methyl bromide (CH3Br) were significantly higher during PEM-West B than during PEM-West A, particularly at latitudes north of 25 deg N and altitudes lower than 6 km. The primary reasons for these higher ambient concentrations were the seasonal increase in the atmospheric lifetimes of trace gases controlled by HO radical reactions, and the more frequent input of continental air masses. During PEM-West B, air masses of continental origin observed north of 25 deg N latitude were augmented with urban signature gases such as C2Cl4. By contrast, more southerly continental outflow had characteristics associated with combustion sources such as biomass burning, including wood fuel burning. During the summer PEM-West A period, the spatial distribution of methyl iodide (CH3I) was consistent with effective oceanic sources at all latitudes, being especially strong in tropical and subtropical regions. At low latitudes, PEM-West B CH3I mixing ratios in the lower troposphere were similar to PEM-West A, but at latitudes greater than about 25 deg N PEM-West B concentrations were significantly reduced. Equatorial regions exhibited enhanced CH3I mixing ratios extending into the upper tropical troposphere, consistent with fast vertical transport of air from the tropical marine boundary layer.

Blake, Nicola J.↗

Atmospheric Layers Measured from the NASA DC-8 During PEM-West B and Comparison with PEM-West A

The Pacific Exploratory Mission-West B (PEM-West B) explored atmospheric layer structure using measurements of O3, H2O, CO, and CH4 from the NASA DC-8 fast-response instruments. The mission took place in February-March 1994 over the western Pacific, mainly in the northern hemisphere. Results were compared with similar measurements made during the Pacific Exploratory Mission-West A (PEM-West A) in September-October 1991. PEM-West B sampled 94 vertical profiles, with an average atmospheric depth per profile of 6.4 km, and this sampling yielded 254 discrete layers. PEM-West A sampled 105 profiles, also with a 6.4 km average depth, yielding 538 layers. Both missions revealed that layers containing high ozone and low water vapor were the most abundant, and low ozone and high water vapor layers were the next most abundant. Lidar images and potential vorticity cross sections showed the former associated with subsidence from the stratosphere in middle latitudes, spreading into the tropics. The latter was associated with convection from the boundary layer. The partition among different types of layers only changed slightly in the two missions, although PEM-West B had half as many layers. Compared to PEM-West A, PEM-West B showed only one-third the number of layers associated with polluted continental air. However, PEM-West B revealed significantly more layers showing characteristics of descended clean marine air. In some cases these layers originated from the southern hemisphere. For ozone- and water-vapor-rich layers, the ozone deviation amplitude was higher in low latitudes and lower in high latitudes in PEM-West B. The mean thickness of layers increased from about 450 m in PEM-West A to 680 in in PEM-West B. Layers also existed in the Intertropical Convergence Zone. CO2 measurements had sufficient vertical resolution to show layer structure as well.

Wu, Zhongxiang↗

Remote Sensing from Geostationary Orbit: GEO TROPSAT, A New Concept for Atmospheric Remote Sensing

The Geostationary Tropospheric Pollution Satellite (GEO TROPSAT) mission is a new approach to measuring the critical constituents of tropospheric ozone chemistry: ozone, carbon monoxide, nitrogen dioxide, and aerosols. The GEO TROPSAT mission comprises a constellation of three instruments flying as secondary payloads on geostationary communications satellites around the world. This proposed approach can significantly reduce the cost of getting a science payload to geostationary orbit and also generates revenue for the satellite owners. The geostationary vantage point enables simultaneous high temporal and spatial resolution measurement of tropospheric trace gases, leading to greatly improved atmospheric ozone chemistry knowledge. The science data processing, conducted as a research (not operational) activity, will provide atmospheric trace gas data many times per day over the same region at better than 25 km ground footprint. The high temporal resolution identifies short time scale processes, diurnal variations, seasonal trends, and interannual variation.

Little, Alan D.↗

Airborne boundary layer flux measurements of trace species over Canadian boreal forest and northern wetland regions

Airborne heat, moisture, O3, CO, and CH4 flux measurements were obtained over the Hudson Bay lowlands (HBL) and northern boreal forest regions of Canada during July - August 1990. The airborne flux measurements were an integral part of the NASA/Arctic Boundary Layer Expedition (ABLE) 3B field experiment executed in collaboration with the Canadian Northern Wetlands Study (NOWES). Airborne CH4 flux measurements were taken over a large portion of the HBL. The surface level flux of CH4 was obtained from downward extrapolations of multiple-level CH4 flux measurements. Methane source strengths ranged from -1 to 31 mg m(exp -2)/d, with the higher values occurring in relatively small, isolated areas. Similar measurements of the CH4 source strength in the boreal forest region of Schefferville, Quebec, ranged from 6 to 27 mg m(exp -2)/d and exhibited a diurnal dependence. The CH4 source strengths found during the ABLE 3B expedition were much lower than the seasonally averaged source strength of 51 mg m(exp -2)/d found for the Yukon-Kuskokwim delta region of Alaska during the previous ABLE 3A study. Large positive CO fluxes (0.31 to 0.53 parts per billion by volume (ppbv) m/s) were observed over the inland, forested regions of the HBL study area, although the mechanism for the generation of these fluxes was not identified. Repetitive measurements along the same ground track at various times of day near the Schefferville site also suggested a diurnal dependence for CO emissions. Measurements of surface resistance to the uptake of O3 (1.91 to 0.80 s/cm) for the HBL areas investigated were comparable to those observed near the Schefferville site (3.40 to 1.10 s/cm). Surface resistance values for the ABLE 3B study area were somewhat less than those observed over the Yukon-Kuskokwim delta during the previous ABLE 3A study. The budgets for heat, moisture, O3, CO, and CH4 were evaluated. The residuals from these budget studies indicated, for the cases selected, a moderate net photochemical production of O3 present in the boundary layer over the HBL that coincided with an in situ destruction of CO, although the mechanism responsible for the destruction of CO was not identified. Results from the O3 budget analysis indicate the importance of in situ photochemical production and its possible dominance over surface deposition to the local O3 budget at the Schefferville site. Measurements of the in situ production of O3 indicated a direct relationship between the presence of biomass burning or large-scale pollution effects. Residuals from budget calculations for conserved quantities (heat, moisture, and CH4) were compared with their respective surface fluxes to provide a measure of the internal self-consistency of the flux measurements.

Ritter, John A.↗

Airborne eddy correlation gas flux measurements - Design criteria for optical techniques

Although several methods exist for the determination of the flux of an atmospheric species, the airborne eddy correlation method has the advantage of providing direct flux measurements that are representative of regional spatial domains. The design criteria pertinent to the construction of chemical instrumentation suitable for use in airborne eddy correlation flux measurements are discussed. A brief overview of the advantages and limitations of the current instrumentation used to obtain flux measurements for CO, CH4, O3, CO2, and water vapor are given. The intended height of the measurement within the convective boundary layer is also shown to be an important design criteria. The sensitivity, or resolution, which is required in the measurement of a scalar species to obtain an adequate species flux measurement is discussed. The relationship between the species flux resolution and the more commonly stated instrumental resolution is developed and it is shown that the standard error of the flux estimate is a complicated function of the atmospheric variability and the averaging time that is used. The use of the recently proposed intermittent sampling method to determine the species flux is examined. The application of this technique may provide an opportunity to expand the suite of trace gases for which direct flux measurements are possible.

Ritter, John A.↗

Carbon monoxide and methane in the North American Arctic and Subarctic troposphere - July-August 1988

Enhanced concentrations of CH4 in the unpolluted atmospheric mixed layer over both Arctic and subarctic tundra landscapes are documented here using data from the NASA Arctic Boundary Layer Expedition (ABLE 3A). The CH4 concentration gradients were determined mainly by interactions of biogenic emission from wet tundra and turbulent mixing proceses. The gradient were most frequently associated with intrusion of upper tropospheric or stratospheric air into the midtroposphere, emissions from forest and tundra fires, and long-range transport of enhanced concentration of these gases from unidentified sources. Summertime haze layers exhibited midtropospheric enhancements of CH4 similar to those measured in winter Arctic events. The observations confirm the importance of Arctic and Subarctic wetland environments as a regional source of global atmospheric CH4.

Harriss, Robert C.↗

Airborne flux measurements of trace species in an Arctic boundary layer

In situ airborne flux values for O3, CO, an CH4 over selected wetlands of Alaska are reported, and airborne CH4 flux measurements are presented for the first time. The source/sink distribution over the Yukon-Kuskokwim Delta (YKD) is qualitatively correlated with surface vegetation type. The CH4 source strength over the YKD ranged from 25 to 85 mg/sq m/d. A spatially averaged, seasonally adjusted source strength of 51 mg/sq m/d was established for the YKD. Indirect CH4 flux estimates obtained over the Alaskan North Slope indicate a much lower source strength. The global CH4 emission from tundra are estimated to be 44 Tg/a at an upper limit. Airborne CO flux measurements over the YKD indicate low negative flux values over the coastal areas, while some positive fluxes were observed in the inland sparsely forested regions. An inspection of the cospectrum of CO with vertical velocity for sample runs in coastal areas indicate the possibility of in situ photochemical destruction/production of CO.

Ritter, John A.↗

Non-mechanical optical path switching and its application to dual beam spectroscopy including gas filter correlation radiometry

A non-mechanical optical switch is developed for alternately switching a monochromatic or quasi-monochromatic light beam along two optical paths. A polarizer polarizes light into a single, e.g., vertical component which is then rapidly modulated into vertical and horizontal components by a polarization modulator. A polarization beam splitter then reflects one of these components along one path and transmits the other along the second path. In the specific application of gas filter correlation radiometry, one path is directed through a vacuum cell and one path is directed through a gas correlation cell containing a desired gas. Reflecting mirrors cause these two paths to intersect at a second polarization beam splitter which reflects one component and transmits the other to recombine them into a polarization modulated beam which can be detected by an appropriate single sensor.

Sachse, Glen W.↗

Venturi air-jet vacuum ejectors for high-volume atmospheric sampling on aircraft platforms

Documentation of the installation and use of venturi air-jet vacuum ejectors for high-volume atmospheric sampling on aircraft platforms is presented. Information on the types of venturis that are useful for meeting the pumping requirements of atmospheric-sampling experiments is also presented. A description of the configuration and installation of the venturi system vacuum line is included with details on the modifications that were made to adapt a venturi to the NASA Electra aircraft at GSFC, Wallops Flight Facility. Flight test results are given for several venturis with emphasis on applications to the Differential Absorption Carbon Monoxide Measurement (DACOM) system at LaRC. This is a source document for atmospheric scientists interested in using the venturi systems installed on the NASA Electra or adapting the technology to other aircraft.

Hill, Gerald F.↗

A comparison of wet and dry season ozone and CO over Brazil using in situ and satellite measurements

A comparison conducted between direct measurements of Brazilian ozone and NO concentrations and space-based measurements has indicated a strong correlation between the two environmental sensing methods and indicated the seasonality of both ozone and CO concentrations in this region. Dry season increases appear to be due to both increased local biomass burning and the transport of CO and ozone from Africa. The coincident high values of both CO and ozone suggest photochemical sources, rather than a stratospheric source, for the African and South American ozone.

Watson, Catherine E.↗

Venturi Air-Jet Vacuum Ejector For Sampling Air

Venturi air-jet vacuum ejector pump light in weight, requires no electrical power, does not contribute heat to aircraft, and provides high pumping speeds at moderate suctions. High-pressure motive gas required for this type of pump bled from compressor of aircraft engine with negligible effect on performance of engine. Used as source of vacuum for differential-absorption CO-measurement (DACOM), modified to achieve in situ measurements of CO at frequency response of 10 Hz. Provides improvement in spatial resolution and potentially leads to capability to measure turbulent flux of CO by use of eddy-correlation technique.

Hill, Gerald F.↗

Airborne flux measurements and budget estimates of trace species over the Amazon Basin during the GTE/ABLE 2B expedition

In situ airborne measurements of turbulent heat, moisture, momentum, ozone, and carbon monoxide fluxes in a convective boundary layer were obtained over a tropical rain forest between 1100 and 1630 LT on May 4, 1987. The aircraft flight path was chosen so as to fly over the tower site at the Ducke Forest Reserve near Manaus, Amazonas, Brazil. Both turbulence statistics and mean quantities were used to study the budgets of heat, water vapor, ozone, and carbon monoxide. The ozone budget study shows an accumulation rate in the boundary layer of 0.3 + or - 0.2 ppbv/h. The surface resistance to ozone during this flight was determined to be 0.06 + or - 0.03 s/cm, while the aerodynamic resistance was 0.14-0.17 s/cm. Results from the CO budget analysis show a midday accumulation rate of 0.6 + or - 0.3 ppbv/h in the Amazonian boundary layer. The evidence suggests production of CO in the PBL. A source of CO may exist below the lowest flight level (about 150 m), although it was not possible to determine what part of the flux at flight level was due to chemical production and what part may be due to surface emission.

Ritter, John A.↗

Cloud draft structure and trace gas transport

During the second Amazon Boundary Layer Experiment (ABLE 2B), meteorological observations, chemical measurements, and model simulations are utilized in order to interpret convective cloud draft structure and to analyze its role in transport and vertical distribution of trace gases. One-dimensional photochemical model results suggest that the observed poststorm changes in ozone concentration can be attributed to convective transports rather than photochemical production and the results of a two-dimensional time-dependent cloud model simulation are presented for the May 6, 1987 squall system. The mesoscale convective system exhibited evidence of significant midlevel detrainment in addition to transports to anvil heights. Chemical measurements of O3 and CO obtained in the convective environment are used to predict photochemical production within the troposphere and to corroborate the cloud model results.

Scala, John R.↗

Optical fringe reduction technique for FM laser spectroscopy

A simple fringe reduction method for FM diode laser spectroscopy is discussed. The fringes can be effectively suppressed by using a modulation frequency that is an integral multiple of the free spectral range of the fringes. The technique is experimentally confirmed by two-tone FM spectroscopy of water vapor absorption lines. A factor of 20 fringe reduction is observed.

Chou, Nee-Yin↗

NO and NO2 in the troposphere - Technique and measurements in regions of a folded tropopause

Measurements of NO, NO2, O3, and CO were obtained for tropopause fold events encountered during two flights of the NASA global tropospheric experiment aircraft in 1984. The results suggest that NO(x) may not always be a good tracer of air of recent stratospheric origin. It is suggested that the stratospheric source of NO(x) acts to introduce NO(x) over a short period and through a large vertical region of the troposphere.

Ridley, Brian A.↗

Single-tone and two-tone AM-FM spectral calculations for tunable diode laser absorption spectroscopy

A generalized theory for optical heterodyne spectroscopy with phase modulated laser radiation is used which allows the calculation of signal line shapes for frequency modulation spectroscopy of Lorentzian gas absorption lines. In particular, synthetic spectral line shapes for both single-tone and two-tone modulation of lead-salt diode lasers are presented in which the contributions from both amplitude and frequency modulations are included.

Chou, Nee-Yin↗

Operational overview of NASA GTE/CITE 1 airborne instrument intercomparisons - Carbon monoxide, nitric oxide, and hydroxyl instrumentation

An overview of the airborne intercomparisons of CO, NO, and OH instrumentation is presented in this first paper of the series on the NASA Global Tropospheric Experiment/Chemical Instrumentation Test and Evaluation (GTE/CITE 1). This paper provides the reader with background information about several important characteristics of the project. These include the overall objectives and approach, the measurements taken, the intercomparison protocol, aircraft platform, profiles of each aircraft flight, and the participants. A synopsis of the overall results of the CO, NO, and OH instrument intercomparisons is also included. Companion papers discuss the detailed results of the CO and NO intercomparison tests as well as pertinent scientific findings.

Beck, Sherwin M.↗