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Sauer, Kirsten

Publications and source records attributed to Sauer, Kirsten.

Disposal Concepts for a High-Temperature Repository in Shale.

Disposal of large, heat-generating waste packages containing the equivalent of 21 pressurized water reactor (PWR) assemblies or more is among the disposal concepts under investigation for a future repository for spent nuclear fuel (SNF) in the United States. Without a long (>200 years) surface storage period, disposal of 21-PWR or larger waste packages (especially if they contain high-burnup fuel) would result in in-drift and near-field temperatures considerably higher than considered in previous generic reference cases that assume either 4-PWR or 12-PWR waste packages (Jové Colón et al. 2014; Mariner et al. 2015; 2017). Sevougian et al. (2019c) identified high-temperature process understanding as a key research and development (R&D) area for the Spent Fuel and Waste Science and Technology (SFWST) Campaign. A two-day workshop in February 2020 brought together campaign scientists with expertise in geology, geochemistry, geomechanics, engineered barriers, waste forms, and corrosion processes to begin integrated development of a high-temperature reference case for disposal of SNF in a mined repository in a shale host rock. Building on the progress made in the workshop, the study team further explored the concepts and processes needed to form the basis for a high-temperature shale repository reference case. The results are described in this report and summarized..

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Hydrothermal reactivity of neutron absorber composites

The stability of neutron absorber composite materials at hydrothermal conditions was tested in a series of two-week experiments to mimic spent nuclear fuel disposal. Coupons, composed of boron carbide (B 4 C) sintered with and encased in aluminum, were increasingly altered in experiments at 150, 230, and 300 °C and pressures of 150 bar. Alteration of aluminum to boehmite (γ-AlO(OH)) and hydrogen gas generation occurred over the range of investigated temperatures, but is most significant at 300 °C. We found that the formation of boron-bearing mineral phases was not detected; however, aqueous boron was present in the reaction fluids.

36 MATERIALS SCIENCE↗