eagles-project/haero
A toolbox for constructing performance portable aerosol packages
Engineering topics
Publications and source records attributed to Schmidt, Michael.
A toolbox for constructing performance portable aerosol packages
SAND2024-11300O TChem-atm is a software library that was developed to solve complex kinetic models for atmospheric chemistry applications. TChem-atm interface employs a hierarchical parallelism design to exploit the massive parallelism available from modern computing platforms. It also supports gas atmospheric chemistry applications, e.g., the energy exascale earth system model. TChem can be used as a box model or coupled with a climate model to compute the time evolution of gas tracer species. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525.
Today, tailored laser beams are rarely used and thus an opportunity to optimize existing or introduce new processes is missed. New methods of dynamic beam shaping have the potential to change that in future. This keynote paper deals with methods allowing a transient energy input into the workpiece at such time scales that the underlying interaction processes are guided towards the desired result. It shows principles, categorizes necessary system technology, and gives application examples to familiarize the reader with the topic. It postulates that time-scale-dependent coupling between transient energy input and addressed process features is key for achieving the optimum.
Abstract not provided.
Abstract not provided.
SAND2021-15059 O Haero is a software library for representing aerosol size distributions, chemical species, and parameterized processes to use with a coupled atmospheric dynamics model or as a standalone tool. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525.
Subsoils below 20 cm are an important reservoir in the global carbon cycle, but little is known about their vulnerability under climate change. We measured subsoil carbon in warmed vs control plots of a conifer forest after 4.5 years of whole-soil warming (4°C). We also measured soil CO2 efflux at the surface and soil CO2 concentrations along the soil profile. Over the 4.5 years we observed that warming resulted in a loss of subsoil carbon stocks (−33 ± 11%), primarily from unprotected particulate organic matter. Warming also stimulated a sustained 30 ± 4% increase in soil CO2 efflux due to increased CO2 production through the whole-soil profile. The observed in situ decline in subsoil carbon stocks with warming is now definitive evidence of a positive soil carbon-climate feedback, which could not be concluded based on increases in CO2 effluxes alone. This dataset comprises (1) 13C and C recovery in 2014, 2016, and 2018 1m soil cores sampled in 10cm increments. (2) Monthly surface CO2 fluxes from 2014 to 2018. (3) Monthly gas well sample [CO2] and production data. And (4) density fraction data for three depths of cores recovered in 2017.
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The synthesis of chemically clean and environmentally friendly nanoparticles through pulsed laser ablation in liquids has shown a number of advantages over conventional chemical synthesis methods and has evolved into a thriving research field attracting laboratory and industrial applications. The fundamental understanding of processes leading to the nanoparticle generation, however, still remains elusive. In particular, the origin of bimodal nanoparticle size distributions in femto- and picosecond laser ablation in liquids, where small nanoparticles (several nanometers) with narrow size distribution are commonly observed to coexist with larger (tens to hundreds of nanometers) ones, has not been explained so far. In this paper, joint computational and experimental efforts are applied to understand the mechanisms of nanoparticle formation in picosecond laser ablation in liquids and to explain the bimodal nanoparticle size distributions. The results of a large-scale atomistic simulation reveal the critical role of the dynamic interaction between the ablation plume and the liquid environment, leading to the generation of large nanoparticles through a sequence of hydrodynamic instabilities at the plume-liquid interface and a concurrent nucleation and growth of small nanoparticles in an expanding metal-liquid mixing region. The computational predictions are supported by a series of stroboscopic videography experiments showing the emergence of small satellite bubbles surrounding the main cavitation bubble generated in single pulse experiments. Lastly, carefully timed double pulse irradiation triggers expansion of secondary cavitation bubbles indicating, in accord with the simulation results, the presence of localized sites of laser energy deposition (possibly large nanoparticles) injected into the liquid at the early stage of the bubble formation.
Spaceborne SAR interferometry (InSAR) has the potential ofdetecting forest change on a global scale with fine (meter-level)spatial resolution as well as on a monthly/weekly basis under allweather conditions. This is significant to characterize the land usechange and its impact on climate change. In this paper, bothsingle-pass and repeat-pass SAR interferometry from spacebornesensors are combined in order to detect and quantify (withNormalized RMSE 30%) forest disturbance at a large scale(dozens of kilometers) however with a fine spatial resolution (<1 hectare) based on two newly developed approaches. The singlepassInSAR approach is not only able to detect forest disturbancebut also capable of characterizing meter (or even sub-meter)level change of forest phase-center (mean) height due to forestgrowth and/or degradation. The methodology described in thispaper can be considered as complimentary tools and thus can becombined with the existing PolInSAR technique (that has beenwidely used for retrieving forest height from single-pass SARinterferometry). These methods are extensively validated with thepast and current spaceborne single-pass and repeat-pass InSARmissions (i.e. JAXA’s ALOS-1, ALOS-2 and DLR’s TanDEM-X)over subtropical forests in Australia as well as tropical forestsin Brazil. Such techniques also serve as observing prototypes forthe fusion of the future spaceborne InSAR missions (such asNASA-ISRO’s NISAR and DLR’s TanDEM-L).
We construct long-term time series of Greenland and Antarctic ice sheet mass change from satellite gravity measurements. A statistical reconstruction approach is developed based on a principal component analysis (PCA) to combine high-resolution spatial modes from the Gravity Recovery and Climate Experiment (GRACE) mission with the gravity information from conventional satellite tracking data. Uncertainties of this reconstruction are rigorously assessed; they include temporal limitations for short GRACE measurements, spatial limitations for the low-resolution conventional tracking data measurements, and limitations of the estimated statistical relationships between low- and high-degree potential coefficients reflected in the PCA modes. Trends of mass variations in Greenland and Antarctica are assessed against a number of previous studies. The resulting time series for Greenland show a higher rate of mass loss than other methods before 2000, while the Antarctic ice sheet appears heavily influenced by interannual variations.
With advances in nanolithography and dry etching, top-down methods of nanostructuring have become a widely used tool for improving the efficiency of optoelectronics. These nano dimensions can offer various benefits to the device performance in terms of light extraction and efficiency, but often at the expense of emission color quality. Broadening of the target emission peak and unwanted yellow luminescence are characteristic defect-related effects due to the ion beam etching damage, particularly for III–N based materials. In this article we focus on GaN based nanorods, showing that through thermal annealing the surface roughness and deformities of the crystal structure can be “self-healed”. Correlative electron microscopy and atomic force microscopy show the change from spherical nanorods to faceted hexagonal structures, revealing the temperature-dependent surface morphology faceting evolution. The faceted nanorods were shown to be strain- and defect-free by cathodoluminescence hyperspectral imaging, micro-Raman, and transmission electron microscopy (TEM). In-situ TEM thermal annealing experiments allowed for real time observation of dislocation movements and surface restructuring observed in ex-situ annealing TEM sampling. This thermal annealing investigation gives new insight into the redistribution path of GaN material and dislocation movement post growth, allowing for improved understanding and in turn advances in optoelectronic device processing of compound semiconductors.
This CCSDS paper presents a reference architecture and service framework for spacecraft monitoring and control. It has been prepared by the Spacecraft Monitoring and Control working group of the CCSDS Mission Operations and Information Management Systems (MOIMS) area. In this context, Spacecraft Monitoring and Control (SM&C) refers to end-to-end services between on- board or remote applications and ground-based functions responsible for mission operations. The scope of SM&C includes: 1) Operational Concept: definition of an operational concept that covers a set of standard operations activities related to the monitoring and control of both ground and space segments. 2) Core Set of Services: definition of an extensible set of services to support the operational concept together with its information model and behaviours. This includes (non exhaustively) ground systems such as Automatic Command and Control, Data Archiving and Retrieval, Flight Dynamics, Mission Planning and Performance Evaluation. 3) Application-layer information: definition of the standard information set to be exchanged for SM&C purposes.