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Selkirk, Henry

Publications and source records attributed to Selkirk, Henry.

Near-Saturation Conditions at the Tropical Tropopause: Results from Ticosonde

The TTL lies between the neutral buoyancy level (NBL) at ~350 K and the tropopause. Within the the TTL radiative heating drives ascent and air parcel supersaturation. Ticosonde measurements since 2005 show that the incidence ofsupersaturation in the TTL over Costa Rica is ~60%. This is due to diabatic ascent. The frequency is highest (68%) in summer, when convection is frequent. The TSL was defined by Selkirk et al. (2010) as the upper edge of the TTL. It isIn this layer that the final saturation of air parcels rising into the stratosphere occurs and thus the water vapor minima which define the so-called "writehead" of the Atmospheric Tape Recorder.

Selkirk, Henry↗

Profiling the SO2 Plume from Volcan Turrialba: Ticosonde Balloon Measurements Compared with OMI and OMPS Retrievals

The summit of Volcan Turrialba (elev. 3340 m) lies less than 50 km upstream in the prevailing easterlies from the Ticosonde balloon launch site at San Jose, Costa Rica, where ECC ozone sondes have been launched regularly since 2005. In 2006 we began to see telltale notches in the ozone profiles in the altitude range between 2 and 6 km. Given the proximity of Turrialba, it seemed likely that SO2 in the volcano's plume was interfering in the chemical reaction in the ECC ozone sonde used to detect ozone. In early 2010, fumarolic activity in the Turrialba crater increased strongly, and the profile notches in our soundings increased in frequency as well, consistent with this hypothesis. In February 2012 we tested a dual ECC sonde system, where an additional sonde is flown on the same payload using a selective SO2 filter. The difference of the measurements in the dual sonde is a direct measure of the amount of SO2 encountered. This first dual sonde passed through the plume, and the data indicated a tropospheric SO2 column of 1.4 DU, comparing favorably with a total column of 1.7 DU in the OMI 3-km linear fit (LF) product at the sonde profile location and at nearly the same time. We are now launching dual sondes on a regular basis with 18 launches in the first 12 months through July 2014; 11 of these have detectable SO2 signals. These soundings have great potential for validation of the Aura OMI and the Suomi-NPP OMPS retrievals of SO2. Here we present the sonde measurements and compare them with two satellite datasets: the Aura OMI Linear Fit (LF) product and the Suomi-NPP OMPS Principal Components Analysis (PCA) boundary layer product. The PCA algorithm reduces retrieval noise and artifacts by more accurately accounting for various interferences in SO2 retrievals such as O3 absorption and rotational Raman scattering. The comparisons with the in situ observations indicate a significant improvement of the PCA algorithm in capturing relatively weak volcanic SO2 signals.

sondes↗

Dehydration in the Winter Arctic Tropopause Region

Recent work has shown that limited amounts of tropospheric air can penetrate as much as 1 km into the middleworld stratosphere during the arctic winter. This, coupled with temperatures that are cold enough to produce saturation mixing ratios of less than 5 ppmv at the tropopause, results in stratospheric cloud formation and upper tropospheric dehydration. Even though these "cold outbreaks" occupy only a small portion of the area in the arctic (1-2%), their importance is magnified by an order of magnitude because of the air flow through them. This is reinforced by evidence of progressive drying through the winter measured during SOLVE-1. The significance of this process lies in its effect on the upper tropospheric water content of the middle and high latitude tropopause region, which plays an important role in regulating the earth's radiative balance. There appears to be significant year-to-year variability in the incidence of the cold outbreaks. This work has two parts. First, we describe case studies of dehydration taken from the SOLVE and SOLVE2 aircraft sampling missions during the Arctic winters of 2000 and 2003 respectively. Trajectory based microphysical modeling is employed to examine the sensitivity of the dehydration to microphysical parameters and the nature of sub-grid scale temperature fluctuations. We then examine the year-to-year variations in potential dehydration using a trajectory climatology.

Pfister, Leonhard↗

Clouds in the Winter Arctic Tropopause Region

Water vapor in the winter arctic tropopause region is important because, after the tropical tropopause region, the winter arctic tropopause has the coldest temperatures in the tropospheric northern hemisphere. This suggests the potential for cloud formation that can remove water vapor from a part of the atmosphere where radiatively active gases (such as water) exert a disproportionate influence on the earth's radiation budget. Previous work by the same authors has shown that this cloud formation extends into the stratosphere, with 20% of the parcels having ozone values of 300-350 ppbv experiencing ice saturation in any given 10 day period period during the late winter. In fact, temperatures are cold enough that 5-10% of the parcels experience saturation even if the water content is below the prevailing stratospheric value of 5 ppmv. This work describes a case study of clouds observed by aircraft near the winter arctic tropopause during the SAGE Ozone Loss and Validation Experiment (SOLVE). This provided a unique opportunity to examine dehydration processes in this region since in situ water, tracer, cloud particle, and meteorological data were all available simultaneously. During this period, temperatures were cold enough at the tropopause to produce saturation mixing ratios of 3-4 ppmv. Thus, clouds were actually observed within the stratosphere. Back trajectories indicate that the air in these clouds came from lower latitudes and altitudes. The study describes the nature of the clouds, the history of the air, and the possible implications for the upper tropospheric water budget.

Pfister, Leonhard↗

Processes Controlling Water Vapor in the Winter Arctic Stratospheric Middleworld

Water vapor in the winter arctic stratospheric middleworld is import-an: for two reasons: (1) the arctic middleworld is a source of air for the upper Troposphere because of the generally downward motion, and thus its water vapor content helps determine upper tropospheric water, a critical part of the earth's radiation budget; and (2) under appropriate conditions, relative humidities will be large, even to the point of stratospheric cirrus cloud formation, leading to the production of active chlorine species that could destroy ozone. On a number of occasions during SOLVE, clouds were observed in the stratospheric middleworld by the DC-8 aircraft. These tended to coincide with regions of low temperatures, though some cases suggest water vapor enhancements due to troposphere-to-stratosphere transport. The goal of this work is to understand the importance of processes in and at the edge of the arctic stratospheric middleworld in determining water vapor at these levels. Specifically, is water vapor at these levels determined largely by the descent of air from above, or are clouds both within and at the edge of the stratospheric middleworld potentially important? How important is troposphere-to-stratosphere transport of air in determining stratospheric middleworld water vapor content? To this end, we will first examine the minimum saturation mixing ratios along theta/EPV tubes during the SOLVE winter and compare these with DC-8 water vapor observations. This will be a rough indicator of how high relative humidities can get, and the likelihood of cirrus cloud formation in various parts of the stratospheric middleworld. We will then examine saturation mixing ratios along both diabatic and adiabatic trajectories, comparing these values with actual aircraft water vapor observations, both in situ and remote. Finally, we will attempt to actually predict water vapor using minimum saturation mixing ratios along trajectories, cloud injection (derived from satellite imagery) along trajectories, and suitable initial conditions.

Pfister, Leonhard↗

Occurrence of Ice Supersaturations, Ice Clouds, and Ternary Aerosols in the Arctic Lowermost Stratosphere

Relative humidity, aerosol concentration, and ice crystals all have important impacts on chemistry and radiative transfer in the lowermost stratosphere. In this study, we have combined SOLVE measurements with meteorological analyses to investigate the statistics of humidity, aerosols, and clouds in the arctic lower stratosphere. First, we will present a statistical analysis of relative humidity with respect to ice in the lowermost stratosphere, used on the DC-8 in situ measurements. We will show examples of ice supersaturation well within the stratosphere. Generally, these cases were associated with extremely low temperatures near the tropopause. Next, we will discuss the climatological occurrence frequency of tropopause temperatures low enough for ice saturation even with typically low stratospheric water vapor mixing ratios. Really, we will examine case studies of ice clouds observed in the lowermost stratosphere during SOLVE. We will discuss the possible origin of these clouds (i.e., precipitation from higher type II PSCs, injection of tropospheric air into the lower stratosphere, etc.).

Jensen, Eric↗

Tropopause Structure as Revealed by the Satellite Water Vapor Channel During STRAT: The Relationship to Small and Mesoscale Structure as Shown in Aircraft Measurements

This paper examines the use of 6.5 micron geostationary satellite imagery during the Stratospheric Radiation And Transport (STRAT) field mission, the first pha:ie of which is during May, 1995. The 6.5 micron imagery is being us4!d to define the horizontal structure of areas where the tropopause is particularly low. Regions of high PV on, say, a 350K surface have been shown to coincide roughly with regions of enhanced radiance. These regions of enhanced 6.5 micron radiance coincide with dryness in the 5-10 km region, since the dryness enables radiation from lower (and warmer) levels to penetrate through the atmosphere into space. Such dryness is associated with downward penetrations of dry stratospheric, high potential vorticity air. We explore the extent to which such regions of high radiance are related to stratospheric intrusions into the troposphere as observed by aircraft data.

Pfister, Leonhard↗