Engineering topics
Singh, D. K.
Publications and source records attributed to Singh, D. K..
Chemically induced ferromagnetism near room temperature in single crystal (Zn 1− x Cr x )Te half-metal
Microscopic origin of ferromagnetism in Cr-doped ZnTe. Figure shows parallel spins with large magnetic moment in a – c plane on Zn/Cr site. The ordered moment is due to orbital overlap between Te and Zn/Cr sites, highlighted by transparent circles.
Various facets of magnetic charge correlation: Micromagnetic and distorted-wave Born approximation simulations study
The emergent concept of the magnetic charge quasiparticle provides a new realm to study the evolution of magnetic properties in two-dimensional artificially frustrated magnets. Here we report on the exploration of magnetic phases due to various magnetic charge correlation using the complementary numerical techniques of micromagnetic and distorted-wave Born approximation simulations in artificial permalloy honeycomb lattice. The honeycomb element length varies between 10 nm and 100 nm, while the width and thickness are kept within the single domain limit. In addition to the charge ordered loop state, we observe disordered charge arrangement, characterized by the random distribution of ±Q charges, in single domain size honeycomb lattice. As the length of the honeycomb element increases, low multiplicity magnetic charges tend to form contiguous bands in thinner lattice. Thin honeycomb lattice with 100 nm element length exhibits a perfect spin ice pattern, which remains unaffected by the modest increase in the width of element size. We simulate scattering profiles under the pretext of distorted-wave Born approximation formalism for the micromagnetic phases. The results are expected to provide useful guidance in the experimental investigation of magnetic phases in an artificial honeycomb magnet.
C-FOG: Life of Coastal Fog
C-FOG is a comprehensive bi-national project dealing with the formation, persistence, and dissipation (life cycle) of fog in coastal areas (coastal fog) controlled by land, marine, and atmospheric processes. Given its inherent complexity, coastal-fog literature has mainly focused on case studies, and there is a continuing need for research that integrates across processes (e.g., air–sea–land interactions, environmental flow, aerosol transport, and chemistry), dynamics (two-phase flow and turbulence), microphysics (nucleation, droplet characterization), and thermodynamics (heat transfer and phase changes) through field observations and modeling. Central to C-FOG was a field campaign in eastern Canada from 1 September to 8 October 2018, covering four land sites in Newfoundland and Nova Scotia and an adjacent coastal strip transected by the Research Vessel Hugh R. Sharp . An array of in situ, path-integrating, and remote sensing instruments gathered data across a swath of space–time scales relevant to fog life cycle. Satellite and reanalysis products, routine meteorological observations, numerical weather prediction model (WRF and COAMPS) outputs, large-eddy simulations, and phenomenological modeling underpin the interpretation of field observations in a multiscale and multiplatform framework that helps identify and remedy numerical model deficiencies. An overview of the C-FOG field campaign and some preliminary analysis/findings are presented in this paper.
Perovskite magnet with quantum mechanical glassiness
Magnetic materials of strongly correlated origin are at the forefront of research in the exploration of new quantum mechanical properties involving spin and charges. Quantum magnetic material with certain intrinsic functionalities, such as continuously fluctuating spins to the lowest accessible temperature - reminiscing a liquid pattern, is argued to form a new phase of matter. Envisaging a phenomenon where the continuously fluctuating spins are also randomly frozen in space, can diminish the distinction between the two opposite extremes of quantum and classical magnetism. Here, we report new evidence in this regard where the coexistence of quantum spin continuum with a spin glass order in Co-doped CaRuO3 perovskite is demonstrated. In experimental investigations of Co-doped CaRuO3 perovskite, we find that (a) a continuum spectrum in the energy-momentum space, due to the uncorrelated spin fluctuations, persists across the weak spin glass transition at T G ≃ 23 K and (b) the quantum fluctuation of magnetic moment is spatially confined to individual sites only, thereby making it an extremely local event. Thus, the fluctuating spins, at a given time, are also randomly frozen macroscopically. The experimental observations suggest the discovery of a new magnetic phase at the cross-road of classical and quantum physics in strongly correlated perovskite materials.
Relaxing Kondo-screened Kramers doublets in CeRhSi 3
${\mathrm{CeRhSi}}_{3}$ is a superconductor under pressure coexisting with a weakly antiferromagnetic phase characterized by a Bragg peak at q → 0 = (~ 0.2,0,0.5) [N. Aso et al., J. Magn. Magn. Mater. 310, 602 (2007)]. The compound is also a heavy-fermion material with a large specific heat coefficient ${\gamma}=110$ mJ ${\mathrm{mol}}^{{-}1}{\mathrm{K}}^{{-}2}$ and a high Kondo temperature of ${T}_{K}=50$ K, indicating ${\mathrm{CeRhSi}}_{3}$ is in a strongly Kondo screened state. We apply high-resolution neutron spectroscopy to investigate the magnetic fluctuations in the normal phase, at ambient pressures, and at low temperatures. We measure a commensurate dynamic response centered around the Q → = (0,0,2) position that gradually evolves to $H{\sim}0.2$ with decreasing temperature and/or energy transfers. The response is broadened both in momentum and energy and is not reminiscent of sharp spin wave excitations found in insulating magnets where the electrons are localized. We parametrize the excitation spectrum and temperature dependence using a heuristic model utilizing the random-phase approximation to couple relaxing ${\mathrm{Ce}}^{3+}$ ground-state Kramers doublets with a Kondo-like dynamic response. With a Ruderman-Kittel-Kasuya-Yosida exchange interaction within the $ab$ plane and an increasing single-site susceptibility, we can qualitatively reproduce the neutron spectroscopic results in ${\mathrm{CeRhSi}}_{3}$ and, namely, the trade-off between scattering at commensurate and incommensurate positions. We suggest that the antiferromagnetic phase in ${\mathrm{CeRhSi}}_{3}$ is driven by weakly correlated relaxing localized Kramers doublets and that ${\mathrm{CeRhSi}}_{3}$ at ambient pressures is on the border between a Rudderman-Kittel-Yosida antiferromagnetic state and a Kondo-screened phase where static magnetism is predominately absent.
Spin correlation in trigonal EuMn 2 As 2
The trigonal structure of EuMn 2 As 2 is an anomaly in the tetragonal 122-type pnictide family. Here, we report a detailed investigation of the underlying magnetic correlations in single crystal EuMn 2 As 2 using high-resolution elastic neutron-scattering measurements. The system undergoes two successive antiferromagnetic transitions at T = 135 K and 14.4 K, respectively. Numerical modeling of the experimental data reveals the long-range antiferromagnetic correlation of Mn-ions in the a - b plane below T N 1 = 135 K . Mn spins are aligned closer to the diagonal axis of the unit cell. The lower temperature transition, below T N 2 = 14.4 K , is discovered to arise due to the long-range antiferromagnetic correlation of Eu spins that are rotated by θ = 55 ° from the c axis of the unit cell.
From Ising Resonant Fluctuations to Static Uniaxial Order in Antiferromagnetic and Weakly Superconducting CeCo ( In 1 - x Hg x ) 5 ( x = 0.01 )
CeCo (In 0.990 Hg 0.010 ) 5 is a charge doped variant of the d-wave CoCoIn 5 superconductor with coexistent antiferromagnetic and superconducting transitions occurring at T N = 3.4 and T c = 1.4 K, respectively. We use neutron diffraction and spectroscopy to show that the magnetic resonant fluctuations present in the parent superconducting phase are replaced by collinear c -axis magnetic order with three-dimensional Ising critical fluctuations. No low-energy transverse spin fluctuations are observable in this doping-induced antiferromagnetic phase and the dynamic resonant spectral weight predominately shifts to the elastic channel. Static (τ > 0.2 ns) collinear Ising order is proximate to superconductivity in CeCoIn 5 and is stabilized through hole doping with Hg.
Scaling of nonlinear susceptibilities in an artificial permalloy honeycomb lattice
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Fractional electrical dimensionality in the spin solid phase of artificial honeycomb lattice
Two-dimensional artificial magnetic honeycomb lattices are at the forefront of research on unconventional magnetic materials. Among the many emergent magnetic phases that are predicted to arise as a function of temperature, the low temperature spin solid phase with zero magnetization and entropy is of special importance. Here, we report an interesting perspective to the consequence of spin solid order in an artificial honeycomb lattice of ultra-small connected elements using electrical dimensionality analysis. At low temperature, T ≤ 30 K, the system exhibits a very strong insulating characteristic. The electrical dimensionality analysis of the experimental data reveals a fractional dimensionality of d = 0.6(0.04) in the spin solid phase of honeycomb lattice at low temperature. The much smaller electrical dimension in the spin solid phase, perhaps, underscores the strong insulating behavior in this system. Furthermore, the fractional dimensionality in an otherwise two-dimensional system suggests a non-surface-like electrical transport at low temperature in an artificial honeycomb lattice.
Temperature-dependent magnetism in artificial honeycomb lattice of connected elements
Artificial magnetic honeycomb lattices are expected to exhibit a broad and tunable range of novel magnetic phenomena that would be difficult to achieve in natural materials, such as long-range spin ice, entropy-driven magnetic charge-ordered states, and spin order due to the spin chirality. Eventually, the spin correlation is expected to develop into a unique spin-solid-state-density ground state, manifested by the distribution of the pairs of vortex states of opposite chirality. In this paper we report the creation of an artificial permalloy honeycomb lattice of ultrasmall connecting bonds, with a typical size of ${\simeq}12$ nm. Detailed magnetic and neutron-scattering measurements on the newly fabricated honeycomb lattice demonstrate the evolution of magnetic correlation as a function of temperature. Finally, at low enough temperature, neutron-scattering measurements and micromagnetic simulation suggest the development of a loop state of vortex configuration in this system.
New Description of Evolution of Magnetic Phases in Artificial Honeycomb Lattice
Artificial magnetic honeycomb lattice provides a two-dimensional archetypal system to explore novel phenomena of geometrically frustrated magnets. According to theoretical reports, an artificial magnetic honeycomb lattice is expected to exhibit several phase transitions to unique magnetic states as a function of reducing temperature. Experimental investigations of permalloy artificial honeycomb lattice of connected ultra-small elements, ≃ 12 nm, reveal a more complicated behavior. First, upon cooling the sample to intermediate temperature, T≃ 175 K, the system manifests a non-unique state where the long range order co-exists with short-range magnetic charge order and weak spin ice state. Second, at much lower temperature, T≃ 6 K, the long-range spin solid state exhibits a re-entrant behavior. Both observations are in direct contrast to the present understanding of this system. New theoretical approaches are needed to develop a comprehensive formulation of this two dimensional magnet.
Gapped excitation in dense Kondo lattice CePtZn
In this work, we report on neutron scattering and muon spin relaxation measurements of dense Kondo lattice CePtZn. The system develops long-range incommensurate magnetic order as the temperature is reduced below TN=1.75 K. Interestingly, a Q-independent gap at E=0.65 meV in the energy spectrum is found to co-exist with the long-range magnetic order. The gap persists to a very high temperature of T≃100 K. The Q-independent characteristic and its persistence to high temperature hint that the gapped excitation may be manifesting the excited state of the ground-state doublet of the crystal-field energy levels. However, the observed broadness in the linewidth with distinct temperature and field dependencies makes it a nontrivial phenomenon. Qualitative analysis of the experimental data suggests the possible co-existence of a local critical behavior, which is onset near the critical field of H≃3 T, with the crystal-field excitation in the dynamic properties.
Fragile antiferromagnetism in the heavy-fermion compound YbBiPt
We report results from neutron scattering experiments on single crystals of YbBiPt that demonstrate antiferromagnetic order characterized by a propagation vector, τAFM = (121212), and ordered moments that align along the [1 1 1] direction of the cubic unit cell. We describe the scattering in terms of a two-Gaussian peak fit, which consists of a narrower component that appears below TN≈0.4 K and corresponds to a magnetic correlation length of ξn≈ 80 Å, and a broad component that persists up to T*≈ 0.7 K and corresponds to antiferromagnetic correlations extending over ξb≈ 20 Å. Our results illustrate the fragile magnetic order present in YbBiPt and provide a path forward for microscopic investigations of the ground states and fluctuations associated with the purported quantum critical point in this heavy-fermion compound.