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Smith, A. G.

Publications and source records attributed to Smith, A. G..

At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Excited levels in odd-A silver isotopes populated rn fission of {sup 252}Cf

Excited levels in 111−121 Ag , odd-𝐴 isotopes populated following spontaneous fission of 252 Cf have been studied using high-fold 𝛾 coincidences measured with Gammasphere array of Compton-suppressed Ge spectrometers at Argonne National Laboratory. The experimental information on these nuclei reported before has been corrected and extended. In the work we discuss the evolution of triaxiality in odd-Ag nuclei. Relative positions of the 𝜋⁢𝑝1/2 and 𝜋⁢𝑔9/2 shells defining the 𝑍=40 gap when approaching the 𝑁=82 closure, the 𝜋⁢1/2+⁢[431] intruder bands, the three-quasiparticle configurations, and the so called 𝑗−1 anomaly in odd-Ag nuclei are also discussed.

Urban, W.↗
DOE OSTI2021

Structure of even-even Sr isotopes with 50 ≤ N ≤ 58 neutrons

Excited levels in Sr 90 , Sr 92 , Sr 94 , and Sr 96 nuclei were reinvestigated using high-statistics multiple- γ coincidence data from neutron-induced fission of U 235 and spontaneous fission of Cf 252 , measured using Exogam at Institut Laue Langevin and Gammasphere arrays, respectively. The experimental goal was the search for new excited levels and firm spin-parity assignments to known levels. A total of 23 new levels with 30 new or corrected decays and 39 new or improved spin-parity assignments were obtained in the four nuclei. Negative-parity structures on top of 3 - excitation were firmly identified and extended to higher spins. New positive-parity structures in Sr 94 and Sr 96 were observed with 3 + excitations characteristic of γ collectivity. The 277.7-keV, E 2 decay from the 1507.0-keV level to the second 0 + level in Sr 96 , found in this paper, completes the coexisting deformed band in this nucleus. To learn about the microscopic structure of levels in the Sr 88 - 96 nuclei, we performed large-scale shell-model calculations. The calculations compared to the experiment, helped the discussion of the evolution of collectivity in strontium isotopes, highlighting the important role of various single-particle excitations in phase transitions and shape coexistence in the region. The special role of the neutron 9 / 2 + [ 404 ] extruder as a catalyst of the deformation change in the region is highlighted.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

First observation of excited states in the 154 Ce 96 nucleus: Rigid rotation at Z = 58

We report new analysis of the data from measurements of γ radiation following spontaneous fission of 248 Cm and 252 Cf, performed using Eurogam2 and Gammashpere arrays, respectively, has revealed, for the first time, excited states in the neutron-rich nucleus, 154 Ce 96 . Using these fission data we have also improved uncertainties on γ-ray energies in the ground-state bands of several neutron-rich nuclei of the A≈150 mass region. The improved data provided precise systematics of the E exc (4+)/E exc (2+) ratio in the region, which indicates that in the Ce isotopic chain the rigid-rotation limit is reached at the neutron number N=96, two neutrons “later” than in the chain of Nd isotopes. The new results suggest the involvement of the proton 9/2 + [404] extruder orbital in generating nuclear deformation in the A≈150 region, analogous to the known role played by the neutron 11/2 – [505] extruder in this region. The catalytic-type action of both extruders is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

New, low-energy excitations in 107 Mo and 109 Mo

New ground-state level with spin-parity 1/2 + is established in 109 Mo, 69.8 keV below the previously reported 5/2(+) ground state in this nucleus, based on precise spectroscopy measurements of gamma radiation following spontaneous fission of 248 Cm performed using the Eurogam2 array of anti-Compton spectrometers. Analogous measurement of gamma radiation following spontaneous fission of 252 Cf, performed using the Gammasphere array, confirms the new 1/2 + ground state of 107 Mo, proposed recently and establishes the isomeric character of the 5/2 + first excited state in 107 Mo. Two beta-decaying isomers are suggested in 111 Mo nucleus based on regular energy systematics, supporting previous predictions. Low-energy excitations in Mo isotopes are interpreted and compared to calculations reported in the literature. The results suggest shape transition from prolate to oblate deformation at N >= 67.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

First observation of γ -soft and triaxial bands in Zr isotopes

New results obtained in this work from measurements of γ radiation following fission of 248 Cm and 252 Cf, performed using Eurogam2 and Gammasphere arrays, respectively, reveal excitations corresponding to γ vibrations and triaxial deformation present in 100 Zr and 102 Zr nuclei. This is the first observation of nonaxial bands in Zr isotopes. Such excitations probably occur due to competing prolate and oblate configurations, identified recently in these nuclei. Evolution of γ softness and triaxiality in Zr isotopes is observed in the function of the neutron number.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Structure of 0 + excitations in the mass A ≈ 100 region: 0 2 + bands in Sr 98 and Zr 100

0 + 2 bands in 98 Sr and 100 Zr, populated in spontaneous fission of 248 Cm and 252 Cf, have been studied using the Eurogam2 and Gammasphere arrays. Phenomenological classification of excited 0 + levels in even-even nuclei of the A ≈ 100 region into four categories is presented and an interpretation for each category is proposed. Highly deformed 0 + 1 ground states and low-energy 0 + 2 levels in both nuclei are probably due to the 2p-2h excitation of two neutrons from the 9/2 + [404] extruder to the low-Ω prolate and the 11/2 – [505] oblate orbitals originating from the h 11/2 shell, respectively. As a result, candidates for 0 + , β vibrational states in A ≈ 100 region are suggested at N > 60.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Parity-Doublet Structure in the $147\atop{57}$La 90 nucleus

Excited states in 147 La, populated in spontaneous fission of 252 Cf have been reinvestigated by means of γ spectroscopy, using high-fold γ coincidences measured with Gammasphere array of Ge detectors. The 229.5-keV level, which has been assigned spin-parity 9/2 - in a recent evaluation, is shown to have spin-parity 11/2 - . Consequently, the ground state has spin-parity 5/2 + . Excited levels in 147 La have been arranged into a parity-doublet structure, showing that at medium excitation energy the 147 La nucleus may have octupole deformation. In conclusion, the B ( E 1) rates in 147 La, which are factor four lower than in 145 La, suggest that the electric dipole moment in 147 La is depresses by an extra mechanism, probably connected with the population of particular neutron orbitals.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

New excitations in Ba 142 and Ce 144 : Evolution of γ bands in the N = 86 isotones

New excited states in 142 Ba and 144 Ce are investigated by means of prompt γ-ray spectroscopy of the radiation following spontaneous fission of 252 Cf. Measurements of angular correlations and the observed branchings allowed the assignment of spins and parities with confidence. The new measurements are reinforced by shell-model calculations where energy levels, electric transitions, and magnetic moments are consistent with experimental data. Lastly, the presence of collectivity in the N = 86 isotones is confirmed by clear signatures of soft triaxial γ bands in both nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Anomalies in the Charge Yields of Fission Fragments from the U ( n , f ) 238 Reaction

Fast-neutron-induced fission of 238 U at an energy just above the fission threshold is studied with a novel technique which involves the coupling of a high-efficiency γ-ray spectrometer (MINIBALL) to an inverse-kinematics neutron source (LICORNE) to extract charge yields of fission fragments via γ-γ coincidence spectroscopy. Experimental data and fission models are compared and found to be in reasonable agreement for many nuclei; however, significant discrepancies of up to 600% are observed, particularly for isotopes of Sn and Mo. This indicates that these models significantly overestimate the standard 1 fission mode and suggests that spherical shell effects in the nascent fission fragments are less important for low-energy fast-neutron-induced fission than for thermal neutron-induced fission. Finally, this has consequences for understanding and modeling the fission process, for experimental nuclear structure studies of the most neutron-rich nuclei, for future energy applications (e.g., Generation IV reactors which use fast-neutron spectra), and for the reactor antineutrino anomaly.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2017

Production and Study of Neutron-rich Nuclei Using the LICORNE Directional Neutron Source

We have recently successfully demonstrated a new technique for production and study of many of the most exotic neutron-rich nuclei at moderate spins. LICORNE, a newly developed directional inverse-kinematic fast neutron source at the IPN Orsay, was coupled to the MINIBALL high resolution γ-ray spectrometer to study nuclei the furthest from stability using the 238 U(n,f)reaction. This reaction and 232 Th(n,f)are the most neutron-rich fission production mechanisms achievable and can be used to simultaneously populate hundreds of neutron-rich nuclei up to spins of ≈ 16h. High selectivity in the experiment was achieved via tripleγ-ray coincidences and the use of a 400 ns period pulsed neutron beam,a technique which is unavailable to other population mechanisms such as 235 U(nth,f) and 252 Cf(SF). The pulsing allows time correlations to be exploited to separate delayedγrays from isomeric states in the hundreds of nuclei produced, which are then used to cleanly select a particular nucleus and its exotic binary partners. In the recent experiment, several physics cases are simultaneously addressed such as shape coexistence, the evolution of shell closures far from stability, and the spectroscopy of nuclei in the r-process path near N= 82. Overall, preliminary physics results on anomalies in the 238 U(n,f) fission yields and the structure of the 138 Te and100Sr nuclei will soon be published. A future project,ν-ball, to couple LICORNE with a hybrid escape-suppressed spectrometer to refine further the technique and achieve a large increase in the observational limit is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1994

Optical and ultraviolet observations of 3C 279 during outburst

An ongoing program of photometric monitoring of selected active galactic nuclei has revealed a significant outburst in the optically violently variable (OVV) quasi-steller object (QSO) 3C 279. The event occurred during May and June of 1992, and was characterized by a peak amplitude of 2.3 mag in the R band. We obtained nearly simultaneous optical and ultraviolet spectroscopy from 1150 to 8600 A of the source at the approximate midpoint of the outburst. The outburst spectrum is well represented by a power law with index alpha = -1.77 (where F(sub nu) varies as nu (exp alpha) which is relatively flat in comparison with typical quiescent spectra for this source. No emission features are discernable in our data, nor is there any significant Lyman-edge absorption. The observations and data analysis procedures are described, and the resulting photometric light curves and spectra are presented. We also present a long baseline photometric light curve for context. Comparisons with previously published optical-UV outburst and quiescent spectra are made, and luminosity-dependent spectral variations are discussed.

Shrader, C. R.↗
NASA NTRS1994

The multifrequency spectral evolution of blazar 3C 345

The blazar 3C 345 underwent a 2.5 mag optical outburst between 1990 November and 1991 May. We have obtained 10 nearly simultaneous multifrequency spectra during the course of the outburst in order to study the multifrequency spectral variations of 3C 345 as a function of time. Although our observations were not sampled frequently enough to completely resolve the variations in every frequency band, the general rise and decline of the outburst were seen in the UV through radio with differing rise times. Simulations of an electron distribution injected into a tangled magnetic field show a relationship between frequency and characteristic timescale that was also observed in the radio variations of 3C 345. The two X-ray observations made during the monitoring period showed no evidence of variability. The multifrequency spectrum was modeled with two major components: a relativistic jet and a relativistic thermal accretion disk. Models calculated for each spectrum indicate that the outburst can be explained in terms of these models by varying the high-energy cutoff of the injected electron distribution in the jet model, while also varying the mass accretion rate in the disk model. There is marginal evidence that the inferred accretion rate varies with the jet luminosity.

Webb, J. R.↗
NASA NTRS1983

Multifrequency observations of the flaring quasar 1156+295

A report is presented on the optically violent variable quasar 1156+295, known also as 4C 29.45 and Ton 599. A large outburst of this quasar was discovered in April 1981 in the course of a program to obtain simultaneous multifrequency spectra of variable quasars. Ultraviolet observations taken with the International Ultraviolet Explorer satellite were coordinated with ground-based observations at radio, infrared, and optical wavelengths. Measurements were made at four epochs starting immediately after the outburst was discovered, when the B-magnitude was 14.0, and at intervals of 4 days, 60 days and 1 year. The luminosity integrated only over observed wavelength bands was approximately 3 x 10 to the 48th ergs/sec on the first epoch of observation. Modeling of the source with a synchrotron self-Compton model suggests that the core of the source has a linear dimension of 0.01 pc, a magnetic field strength in the range 0.1-30 gauss, and a bulk relativistic motion in the quasar rest frame characterized by a Lorentz factor in the range 2-8.

Glassgold, A. E.↗