Interfacial electronic structure of Cl6SubPc non-fullerene acceptors in organic photovoltaics using soft X-ray spectroscopies
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99 GENERAL AND MISCELLANEOUS↗
Engineering topics
Smith, K.
Publications and source records attributed to Smith, K..
Quenching of single-particle strengths in direct reactions
A discrepancy in the asymmetry dependence of spectroscopic factors extracted with different reaction probes calls into question whether the corresponding reaction models are properly understood. In this work, we present extracted spectroscopic factors from the Ar 46 , 34 ( p , d ) Ar 45 , 33 transfer reactions in inverse kinematics at a beam energy of 70 MeV/nucleon. The results are consistent with previous measurements of these reactions at a lower beam energy [Lee et al. , Phys. Rev. Lett. 104 , 112701 (2010) ], indicating that the transfer reaction is a reliable probe for the nuclear structure of exotic nuclei across a wide energy range. Results from a large body of transfer reaction measurements, ( p , p N ) measurements, and theoretical nuclear structure studies make a compelling case for much weaker asymmetry dependence than what is observed with single-nucleon knockout reactions on beryllium or carbon targets.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
High power coupler development for EIC
The synchrotron radiation loss in EIC Electron Storage Ring is as high as up to 10 MW. This energy loss will be compensated by 17 2K 591 MHz single-cell SRF cavities with a combined total of 34 high power fundamental power couplers. Each power coupler will operate 92% of revolution time CW and ~8% of revolution time with 400 kW forward power due to the beam abort gap. To satisfy the EIC needs, we developed two 500 kW standing-wave FPC designs at BNL based on either a BeO and an Al 2 O 3 RF window. This paper will briefly summarize test results of the BeO window FPC , and describe the design development of the Al 2 O 3 window based FPC.
43 PARTICLE ACCELERATORS↗
Steel Corrosion Impacts on Radionuclide Immobilization
This progress report (Level 4 Milestone Number M4SF-21LL010302052) summarizes research conducted at Lawrence Livermore National Laboratory (LLNL) within the Crystalline Activity Number SF-21LL01030205. The research is focused on actinide and radionuclide sequestration in steel corrosion products. Fuel matrix degradation models suggest that the near field is likely to be reducing at the time of canister breaching, steel corrosion, and radionuclide release, but more oxidizing conditions may prevail in the far field. The incorporation of radionuclides into corrosion phases may limit the rate of radionuclide release by sequestering a portion of the radionuclide source term. For these reasons there is a need to evaluate the incorporation of Pu and other radionuclides into various Fe-oxide phases, and to understand the behavior of coprecipitated phases during mineral recrystallization processes and during re-oxidation events. Radionuclide coprecipitation with Fe minerals may impact long-term repository performance and is an ongoing research focus at Lawrence Livermore National Laboratory.
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
HIGH POWER COUPLER DEVELOPMENT FOR EIC
The synchrotron radiation loss in EIC Electron Storage Ring is as high as up to 10 MW. This energy loss will be compensated by 17 2K 591 MHz single-cell SRF cavities with a combined total of 34 high power fundamental power couplers. Each power coupler will operate 92% of revolution time CW and ~8% of revolution time with 400 kW forward power due to the beam abort gap. To satisfy the EIC needs, we developed two 500 kW standing-wave FPC designs at BNL based on either a BeO and an Al2O3 RF window. This paper will briefly summarize test results of the BeO window FPC, and describe the design development of the Al2O3 window based FPC.
43 PARTICLE ACCELERATORS↗
Investigation of secondary γ -ray angular distributions using the N 15 ( p , α 1 γ ) C * 12 reaction
The observation of secondary γ-rays provides an alternative method of measuring cross sections that populate excited final states in nuclear reactions. The angular distributions of these γ-rays also provide information on the underlying reaction mechanism. Despite a large amount of data of this type in the literature, publicly available R-matrix codes do not have the ability to calculate these types of angular distributions. In this report, the mathematical formalism derived in Brune and deBoer is implemented in the R-matrix code AZURE2 and calculations are compared with previous data from the literature for the 15 N( p, α1γ ) 12 C* reaction. In addition, new measurements, made at the University of Notre Dame Nuclear Science Laboratory using the Hybrid Array of Gamma Ray Detectors (HAGRiD), are reported that span an energy range from E p = 0.88 to 4.0 MeV. Excellent agreement between data and the phenomenological fit is obtained up to the limit of the previous fit at E p = 2.0 MeV and the R-matrix fit is extended from E x ≈ 13.5 up to E x ≈ 15.3 MeV, where 15 N+p and 12 C+α reactions are fit simultaneously for the first time. An excellent reproduction of the 15 N( p, α1γ ) 12 C* and 12 C(α, α) 12 C data is achieved, but inconsistencies and difficulty in fitting other data is encountered and discussed.
6 ≤ A ≤ 19↗
DESIGN AND MEASUREMENT OF THE 1.4 GHZ CAVITY FOR LEReC LINAC
The Low Energy RHIC electron Cooler (LEReC) is the first electron cooler based on rf acceleration of electron bunches. To further improve RHIC luminosity for heavy ion beam energies below 10 GeV/nucleon, a normal conducting RF cavity at 1.4 GHz was designed and fabricated for the LINAC that will provide longer electron bunches for the LEReC. It is a single cell cavity with effective cavity length shorter than half of the 1.4 GHz wavelength. This cavity was fabricated and tested on site at BNL to verify RF properties, i.e. the resonance frequency, fundamental power coupler (FPC) coupling strength, tuner system performance, and high-power tests. In this paper, we report the RF test results for this cavity.
43 PARTICLE ACCELERATORS↗
OPERATIONAL EXPERIENCE AND REDESIGN OF THE TUNER WITH-OUT SPRING FINGERS FOR THE LEReC WARM CAVITY
A folded coaxial tuner without spring fingers was de-signed for the Low Energy Relativistic Heavy Ion Collider (RHIC) electron Cooler (LEReC) 2.1 GHz warm cavity. During RHIC run 2019, this tuner was found to cause cavity trips via different failure modes. After analyzing these failure modes, a new straight coaxial tuner without spring fingers was proposed and was installed. We show the operational experience of the new tuner in this paper.
43 PARTICLE ACCELERATORS↗
Long lifetime of bialkali photocathodes operating in high gradient superconducting radio frequency gun
Abstract High brightness, high charge electron beams are critical for a number of advanced accelerator applications. The initial emittance of the electron beam, which is determined by the mean transverse energy (MTE) and laser spot size, is one of the most important parameters determining the beam quality. The bialkali photocathodes illuminated by a visible laser have the advantages of high quantum efficiency (QE) and low MTE. Furthermore, Superconducting Radio Frequency (SRF) guns can operate in the continuous wave (CW) mode at high accelerating gradients, e.g. with significant reduction of the laser spot size at the photocathode. Combining the bialkali photocathode with the SRF gun enables generation of high charge, high brightness, and possibly high average current electron beams. However, integrating the high QE semiconductor photocathode into the SRF guns has been challenging. In this article, we report on the development of bialkali photocathodes for successful operation in the SRF gun with months-long lifetime while delivering CW beams with nano-coulomb charge per bunch. This achievement opens a new era for high charge, high brightness CW electron beams.
43 PARTICLE ACCELERATORS↗
Developing the Pressure-Temperature-Magnetic Field Phase Diagram of Multiferroic [(CH3)2NH2]Mn(HCOO)3
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99 GENERAL AND MISCELLANEOUS↗
Life Performance Prediction Approach and Update for the Potential eMMRTG
No abstract provided
Wefers, K.↗
19 Ne level structure for explosive nucleosynthesis
Ne 19 is an important isotope in nuclear astrophysics due to its role in both the F 18 ( p , α ) O 15 and O 15 ( α , γ ) Ne 19 reactions in novae and Type I x-ray bursts, respectively. The energy levels of Ne 19 near the α and proton thresholds ( S α = 3529 keV, S p = 6410 keV) correspond to resonances in both of these reactions. Previous measurements to study the structure of Ne 19 have focused on both regions in an effort to constrain these reaction rates. Discrepancies in the energies, spins, and parities for levels in Ne 19 from previous measurements contribute to the reaction-rate uncertainties. Gamma rays from the depopulation of excited states in Ne 19 were measured to reduce the level-energy uncertainties and inconsistencies in previous spin-parity assignments.The F 19 ( He 3 , t ) Ne 19 reaction was used to elucidate the structure of Ne 19 levels up to E x = 6.9 MeV. The reaction products were measured using Gammasphere ORRUBA: Dual Detectors for Experimental Structure Studies—a coupling of the Oak Ridge Rutgers University Barrel Array and Gammasphere at Argonne National Laboratory. Tritons produced in the reaction were measured in coincidence with γ rays from the deexcitation of Ne 19 energy levels. Previously unobserved transitions allowed for discrepancies in the resonance properties relevant to these two reactions to be resolved. In total, 41 transitions from 21 energy levels were measured in Ne 19 , with 21 of those transitions being previously unobserved. Of particular importance, transitions from two 3 / 2 + states with energies of 6423(3) and 6441(3) keV, crucial for accurate estimations of the F 18 ( p , α ) O 15 reaction rate, were found. Energies and spin-parities of important energy levels near the proton and α thresholds were measured and some of the discrepancies in previous measurements were resolved. Overall, measurement of the two near-threshold 3 / 2 + states reduced the calculated upper limit of the F 18 ( p , α ) O 15 reaction rate by factors of 1.5–17 in the nova temperature range.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Cross-section measurements to low-lying excited final states in the 24 M(α,p) 27 Al*(γ) reaction as an energy source for x-ray bursts
Energy production in Type Ia x-ray bursts depends on a number of nuclear reactions that become efficient in a hot environment (up to 2 GK). Model sensitivity studies have been performed in an effort to better identify the reactions that have the largest effect, but these efforts are hampered by the high level of complexity of the astrophysical model and large nuclear physics uncertainties. In a recent study, the 24 Mg(α,p) 27 Al reaction was found to significantly affect the energy generation in x-ray bursts. This manuscript reports the first study of the 24 Mg(α,p 1,2 γ) 27 Al reaction at energies relevant for x-ray bursts. In conclusion, the branches to the 27 Al excited states increase to a small degree the estimates of the total astrophysical 24 Mg(α,p) 27 Al reaction rate.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Interfacial Electronic Structure of C60/ClAlPc on a MoO3 Layer After Thermal Treatment
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99 GENERAL AND MISCELLANEOUS↗
New 13 C(α,n) 16 O Cross Section with Implications for Neutrino Mixing and Geoneutrino Measurements
Precise antineutrino measurements are very sensitive to proper background characterization. Here, we present an improved measurement of the 13 C(α,n) 16 O reaction cross section which constitutes significant background for large v¯ detectors. We greatly improve the precision and accuracy by utilizing a setup that is sensitive to the neutron energies while making measurements of the excited state transitions via secondary γ-ray detection. Our results shows a 54% reduction in the background contributions from the 16 O(3–, 6.13 MeV) state used in the KamLAND analysis.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
M4SF-20LL010302042: Process Model for Radionuclide Incorporation into Corrosion Products
This progress report (Level 4 Milestone Number M4SF-20LL010302042) summarizes research conducted at Lawrence Livermore National Laboratory (LLNL) within the Crystalline Activity Number SF-20LL010302041. The research is focused on actinide and radionuclide sequestration in steel corrosion products. Fuel matrix degradation models suggest that the near field is likely to be reducing at the time of canister breaching, steel corrosion, and radionuclide release, but more oxidizing conditions may prevail in the far field. The incorporation of radionuclides into corrosion phases may limit the rate of radionuclide release by sequestering a portion of the radionuclide source term. For these reasons there is a need to evaluate the incorporation of Pu and other radionuclides into various Fe-oxide phases, and to understand the behavior of coprecipitated phases during mineral recrystallization processes and during re-oxidation events. Radionuclide coprecipitation with Fe minerals may impact long-term repository performance and is an ongoing research focus at Lawrence Livermore National Laboratory.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
High-Brightness Continuous-Wave Electron Beams from Superconducting Radio-Frequency Photoemission Gun
Continuous-wave photoinjectors operating at high accelerating gradients promise to revolutionize many areas of science and applications. They can establish the basis for a new generation of monochromatic x-ray free electron lasers, high-brightness hadron beams, or a new generation of microchip production. In this Letter we report on the record-performing superconducting rf electron gun with CsK 2 Sb photocathode. The gun is generating high charge electron bunches (up to 10 nC / bunch ) and low transverse emittances, while operating for months with a single photocathode. As such, this achievement opens a new era in generating high-power beams with a very high average brightness.
43 PARTICLE ACCELERATORS↗
Nuclear mass measurements map the structure of atomic nuclei and accreting neutron stars
We introduce here mass excesses (ME) of neutron-rich isotopes of Ar through Fe, obtained via time of flight B ρ mass spectrometry at the National Superconducting Cyclotron Laboratory. Our new results have significantly reduced systematic uncertainties relative to a prior analysis, enabling the first determination of ME for Ti 58 , 59 , V 62 , Cr 65 , Mn 67 , 68 , and Fe 69 , 70 . Our results show the N = 34 subshell weaken at Sc and vanish at Ti, along with the absence of an N = 40 subshell at Mn. This further leads to a cooler accreted neutron star crust, highlighting the connection between the structure of nuclei and neutron stars.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗