Sustainable marine fuel production through mild hydrotreating of catalytic fast pyrolysis bio-oil
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Engineering topics
Publications and source records attributed to Tan, Eric C. D..
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Bioprocess development enhanced muconate titers and productivities from mixed sugars, leading to reduced production costs and a significant decrease in GHG emissions compared to fossil carbon-based adipic acid production. Created with BioRender.com.
A membrane-based emulsion separator can enable continuous solvent extraction in bioprocessing separations with substantially improved demulsification and mass transfer rates, including where emulsion formation is a challenge.
Improve overall economics and sustainability of biofuels production by making the best use of byproducts from biomass pyrolytic processes towards energy utilities by leveraging locational consumers and available infrastructure.
This study analyzes catalytic fast pyrolysis as a conversion technology for mixed plastic waste, highlighting key economic and environmental drivers and potential opportunities for process improvements.
Bioconversion of a heterogeneous mixture of lignin-related aromatic compounds (LRCs) to a single product via microbial biocatalysts is a promising approach to valorize lignin. Here, Pseudomonas putida KT2440 was engineered to convert mixed p-coumaroyl– and coniferyl-type LRCs to β-ketoadipic acid, a precursor for performance-advantaged polymers. Expression of enzymes mediating aromatic O-demethylation, hydroxylation, and ring-opening steps was tuned, and a global regulator was deleted. β-ketoadipate titers of 44.5 and 25 grams per liter and productivities of 1.15 and 0.66 grams per liter per hour were achieved from model LRCs and corn stover-derived LRCs, respectively, the latter representing an overall yield of 0.10 grams per gram corn stover-derived lignin. Technoeconomic analysis of the bioprocess and downstream processing predicted a β-ketoadipate minimum selling price of $\$2.01$ per kilogram, which is cost competitive with fossil carbon-derived adipic acid ($\$1.10$ to 1.80 per kilogram). Overall, this work achieved bioproduction metrics with economic relevance for conversion of lignin-derived streams into a performance-advantaged bioproduct.
This work examines the feasibility of a greenfield mixed plastics waste gasification facility with process modeling, TEA, and LCA.
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