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Taylor, S.

Publications and source records attributed to Taylor, S..

At least 19 records

Decay studies of the 𝛽-delayed neutron emitters 87 Br and 88 Br measured by means of the Modular Total Absorption Spectrometer at ORNL HRIBF

The Ξ² decays of 87 Br, 88 Br, and 87 Kr were measured with the Modular Total Absorption Spectrometer (MTAS) at Oak Ridge National Laboratory’s Holifield Radioactive Ion Beam Facility (HRIBF). Both bromine isotopes are Ξ²-delayed neutron emitters that have large cumulative fission yields and were identified as top-priority cases for total absorption study by the Nuclear Energy Agency in 2007. Our investigations corroborate that the decay schemes of 87 Br and 88 Br suffer from the so-called pandemonium effect. Unique MTAS properties enable direct neutron measurements. Here, we present MTAS-derived Ξ²-delayed neutron spectra, Ξ²-delayed neutron emission probabilities of P n ( 87 Br) = 2.36(24)%, and P n ( 88 Br) = 6.4(6)%, and the Ξ²-delayed neutron transitions intensity of 4(2)% to the first excited 87 Kr state, populated in the Ξ²-neutron decay of 88Br. Incorporating new data into calculations of the electromagnetic decay heat component emitted during thermal neutron fission of 235 U and 239 Pu improves agreement with experimental data up to approximately 80 s after fission. The estimation of the nuclear reactor $\bar{Ξ½}_e$ flux results in changes of up to 1% in the expected $\bar{Ξ½}_e$ interactions with the detector material for 235 U, 238 U, 239Pu, and 241 Pu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Solar System Ephemerides, Pulsar Timing, Gravitational Waves, & Navigation

In-spiraling supermassive black holes should emit gravitational waves, which would produce characteristic distortions in the pulse time of arrival residuals from millisecond pulsars. There are multiple national and regional consortia that have constructed pulsar timing arrays by precise timing of different sets of millisecond pulsars. An essential aspect of precision timing is the transfer of the pulsar times of arrival to a (quasi-)inertial reference frame, conventionally taken to be the solar system barycenter. The solar system barycenter is determined from the knowledge of the planetary masses and orbits, which has been re ned over the course of the past 50 years by multiple spacecraft missions. Within the North American Nanohertz Observatory for Gravitational Waves (NANOGrav), uncertainties on the solar system barycenter are emerging as an important element of the overall NANOGrav noise budget. We describe what is known about the solar system barycenter, touch upon how uncertainties in it affect gravitational wave studies with pulsar timing arrays, and consider future trends in spacecraft navigation.

Vallisneri, M.β†—

C/N and other Elemental Ratios of Chondritic Porous IDPS and a Fluffy Concordia Micrometeorite

Chondritic porous interplanetary dust particles (CP-IDPs) may be cometary in origin [1], as may ultracarbona-ceous (UCAMMs) [2] and 'fluffy' [3] micrometeorites from the Concordia collection. They are all rich in organics, which can rim grains and may have helped glue grains together during accretion [4]. The organics also contain nitrogen the input of which to Earth has potential biological importance. We report C/N ratios, and other properties of CP-IDPs and a Concordia fluffy microme-teorite.

Smith, T.β†—

Coordinated Analyses of Mineral-organic Matter Associations in Interplanetary Dust Particles

Little is known about the timing and processes involved in the incorporation of organic matter with inorganic materials in early Solar System bodies. Recently, X-ray absorption near-edge spectroscopy (XANES) studies showed carbon-rich rims surrounding individual mineral grains in anhydrous IDPs [1,2]. These carbonaceous rims are believed to have formed prior to parent body formation and likely served to bond mineral grains during accretion into larger aggregates. We are exploring the nature of these carbonaceous rims through coordinated analyses of their chemistry, mineralogy, spectroscopy and isotopic characteristics. Here we report our preliminary mineralogical observations.

Nakamura-Messenger, K.β†—

Characterization of 81P/Wild 2 Particles C2067,1,111,6.0 and C2067,1,111,8.0

The concentrations of C and N in cometary particles are of interest in characterizing the regions where comets formed. One aim of this work is to analyze enough Stardust particles to draw meaningful statistical conclusions about their inventories of C and N. Toward that end we report recent studies of Stardust particles and related materials.

Smith, T.β†—

Estimation of Smoothing Error in SBUV Profile and Total Ozone Retrieval

Data from the Nimbus-4, Nimbus-7 Solar Backscatter Ultra Violet (SBUV) and seven of the NOAA series of SBUV/2 instruments spanning 41 years are being reprocessed using V8.6 algorithm. The data are scheduled to be released by the end of August 2011. An important focus of the new algorithm is to estimate various sources of errors in the SBUV profiles and total ozone retrievals. We discuss here the smoothing errors that describe the components of the profile variability that the SBUV observing system can not measure. The SBUV(/2) instruments have a vertical resolution of 5 km in the middle stratosphere, decreasing to 8 to 10 km below the ozone peak and above 0.5 hPa. To estimate the smoothing effect of the SBUV algorithm, the actual statistics of the fine vertical structure of ozone profiles must be known. The covariance matrix of the ensemble of measured ozone profiles with the high vertical resolution would be a formal representation of the actual ozone variability. We merged the MLS (version 3) and sonde ozone profiles to calculate the covariance matrix, which in general case, for single profile retrieval, might be a function of the latitude and month. Using the averaging kernels of the SBUV(/2) measurements and calculated total covariance matrix one can estimate the smoothing errors for the SBUV ozone profiles. A method to estimate the smoothing effect of the SBUV algorithm is described and the covariance matrixes and averaging kernels are provided along with the SBUV(/2) ozone profiles. The magnitude of the smoothing error varies with altitude, latitude, season and solar zenith angle. The analysis of the smoothing errors, based on the SBUV(/2) monthly zonal mean time series, shows that the largest smoothing errors were detected in the troposphere and might be as large as 15-20% and rapidly decrease with the altitude. In the stratosphere above 40 hPa the smoothing errors are less than 5% and between 10 and 1 hPa the smoothing errors are on the order of 1%. We validate our estimated smoothing errors by comparing the SBUV ozone profiles with other ozone profiling sensors.

Kramarova, N. A.β†—

Characterization of Three Carbon- and Nitrogen-Rich Particles from Comet 81P/WILD

Comets may sample the early solar system s complement of volatile-forming elements - including C and N - more fully and reliably than do the terrestrial planets or asteroids. Until recently, all elemental analyses of unambiguously cometary material were carried out remotely. The return of the Stardust mission makes it possible to analyze documented material from P81/Wild 2 in the laboratory Wild 2 particles fragmented when they stopped in the aerogel collectors. We have studied three fragments thought to be rich in C and N by using several techniques: FTIR to characterize organic matter; synchrotron-induced x-ray fluorescence (SXRF) to determine Fe and certain element/Fe ratios; SEM to image sample morphology and to detect semiquantitatively Mg, Al, Si, Ca, and Fe; and nuclear reaction analysis (NRA) to measure C, N, O, and Si.

Gallien, J.-P.β†—

Elemental Compositions of Comet 81P/Wild 2 Samples Collected by Stardust

We measured the chemical compositions of material from 23 particles in aerogel and residue in 7 craters in aluminum foil, collected during passage of the Stardust spacecraft through the coma of Comet 81P/Wild 2. These particles are chemically heterogeneous at the largest size-scale analyzed, ~180 nanograms. The mean chemical composition of this Wild 2 material agrees with the CI meteorite composition for the refractory elements Mg, Si, Cr, Fe, and Ni to 35%, and for Ca and Mn to 50%. The data suggest the moderately volatile elements Cu, Zn, and Ga may be enriched in this Wild 2 material.

Flynn, G. J.β†—

Distributed Sensing of Carbon-Epoxy Composites and Filament Wound Pressure Vessels Using Fiber-Bragg Gratings

Multiple Fiber Bragg-gratings are embedded in carbon-epoxy laminates as well as in composite wound pressure vessel. Structural properties of such composites are investigated. The measurements include stress-strain relation in laminates and Poisson's ratio in several specimens with varying orientation of the optical fiber Bragg-sensor with respect to the carbon fiber in an epoxy matrix. Additionally, fiber Bragg gratings are bonded on the surface of these laminates and cylinders fabricated out of carbon-epoxy composites and multiple points are monitored and compared for strain measurements at several locations.

Grant, J.β†—

Investigation of Carbon-Polymer Structures with Embedded Fiber-Optic Bragg Gratings

Several Bragg-grating sensors fabricated within the same optical fiber are buried within multiple-ply carbon-epoxy planar and cylindrical structures. Effect of different orientation of fiber-sensors with respect to carbon fibers in the composite structure is investigated. This is done for both fabric and uni-tape material samples. Response of planar structures to axial and transverse strain up to 1 millistrain is investigated with distributed Bragg-grating sensors. Material properties like Young's Modulus and Poisson ratio is measured. A comparison is made between response measured by sensors in different ply-layers and those bonded on the surface. The results from buried fiber- sensors do not completely agree with surface bonded conventional strain gauges. A plausible explanation is given for observed differences. The planar structures are subjected to impacts with energies up to 10 ft-lb. Effect of this impact on the material stiffness is also investigated with buried fiber-optic Bragg sensors. The strain response of such optical sensors is also measured for cylindrical carbon-epoxy composite structures. The sensors are buried within the walls of the cylinder as well as surface bonded in both the axial as well as hoop directions. The response of these fiber-optic sensors is investigated by pressurizing the cylinder up to its burst pressure of around 1500 psi. This is done at both room temperature as well as cryogenic temperatures. The recorded response is compared with that from a conventional strain gauge.

Grant, Joseph↗

Investigation of Structural Properties of Carbon-Epoxy Composites Using Fiber-Bragg Gratings

Fiber Bragg-gratings are embedded in carbon-epoxy laminates as well as bonded on the surface of cylindrical structures fabricated out of such composites. Structural properties of such composites is investigated. The measurements include stress-strain relation in laminates and Poisson's ratio in several specimens with varying orientation of the optical fiber Bragg-sensor with respect to the carbon fiber in an epoxy matrix. Additionally, Bragg gratings are bonded on the surface of cylinders fabricated out of carbon-epoxy composites and longitudinal and hoop strain on the surface is measured.

Grant, J.β†—

Earth Probe Total Ozone Mapping Spectrometer (TOMS) Data Product User's Guide

Two data products from the Earth Probe Total Ozone Mapping Spectrometer (EP/TOMS) have been archived at the Distributed Active Archive Center, in the form of Hierarchical Data Format files. The EP/ TOMS began taking measurements on July 15, 1996. The instrument measures backscattered Earth radiance and incoming solar irradiance; their ratio is used in ozone retrievals. Changes in the reflectivity of the solar diffuser used for the irradiance measurement are monitored using a carousel of three diffusers, each exposed to the degrading effects of solar irradiation at different rates. The algorithm to retrieve total column ozone compares measured Earth radiances at sets of three wavelengths with radiances calculated for different total ozone values. The initial error in the absolute scale for TOMS total ozone is 3 percent, the one standard deviation random error is 2 percent, and the drift is less than 0.5 percent over the first year of data. The Level-2 product contains the measured radiances, the derived total ozone amount, and reflectivity information for each scan position. The Level-3 product contains daily total ozone and reflectivity in a 1-degree latitude by 1.25 degrees longitude grid. Level-3 files containing estimates of LTVB at the Earth surface and tropospheric aerosol information are also available, Detailed descriptions of both HDF data-files and the CD-ROM product are provided.

McPeters, R.β†—

ADEOS Total Ozone Mapping Spectrometer (TOMS) Data Products User's Guide

Two data products from the Total Ozone Mapping Spectrometer (ADEOS/TOMS) have been archived at the Distributed Active Archive Center, in the form of Hierarchical Data Format files. The ADEOS/ TOMS began taking measurements on September 11, 1996, and ended on June 29, 1997. The instrument measured backscattered Earth radiance and incoming solar irradiance; their ratio was used in ozone retrievals. Changes in the reflectivity of the solar diffuser used for the irradiance measurement were monitored using a carousel of three diffusers, each exposed to the degrading effects of solar irradiation at different rates. The algorithm to retrieve total column ozone compares measured Earth radiances at sets of three wavelengths with radiances calculated for different total ozone values, solar zenith angles, and optical paths. The initial error in the absolute scale for TOMS total ozone is 3 percent, the one standard deviation random error is 2 percent, and the drift is less than 0.5 percent over the 9-month data record. The Level 2 product contains the measured radiances, the derived total ozone amount, and reflectivity information for each scan position. The Level 3 product contains daily total ozone and reflectivity in a 1-degree latitude by 1.25 degrees longitude grid. The Level 3 files containing estimates of UVB at the Earth surface and tropospheric aerosol information will also be available. Detailed descriptions of both HDF data files and the CDROM product are provided.

Krueger, A.β†—

Signal processing for ION mobility spectrometers

Signal processing techniques for systems based upon Ion Mobility Spectrometry will be discussed in the light of 10 years of experience in the design of real-time IMS. Among the topics to be covered are compensation techniques for variations in the number density of the gas - the use of an internal standard (a reference peak) or pressure and temperature sensors. Sources of noise and methods for noise reduction will be discussed together with resolution limitations and the ability of deconvolution techniques to improve resolving power. The use of neural networks (either by themselves or as a component part of a processing system) will be reviewed.

Taylor, S.β†—

Application of the Langley plot method to the calibration of the solar backscattered ultraviolet instrument on the Nimbus 7 satellite

The concept of the well-known Langley plot technique, used for the calibration of ground-based instruments, has been generalized for application to satellite instruments. In polar regions, near summer solstice, the solar backscattered ultraviolet (SBUV) instrument on the Nimbus 7 satellite samples the same ozone field at widely different solar zenith angles. These measurements are compared to assess the long-term drift in the instrument calibration. Although the technique provides only a relative wavelength-to-wavelength calibration, it can be combined with existing techniques to determine the drift of the instrument at any wavelength. Using this technique, we have generated a 12-year data set of ozone vertical profiles from SBUV with an estimated accuracy of +/- 5% at 1 mbar and +/- 2% at 10 mbar (95% confidence) over 12 years. Since the method is insensitive to true changes in the atmospheric ozone profile, it can also be used to compare the calibrations of similar SBUV instruments launched without temporal overlap.

Bhartia, P. K.β†—

Calibration of the NOAA 11 solar backscatter ultraviolet (SBUV/2) ozone data set from 1989 to 1993 using in-flight calibration data and SSBUV

Total ozone and ozone profiles are currently being measured by solar backscatter ultraviolet (SBUV/2) instruments onboard NOAA polar orbiting spacecraft using the backscattered ultraviolet technique. The NOAA 11 SBUV/2 operational data set, reprocessed from January 1989 to May 1993 (version 6), includes an updated algorithm and revised prelaunch and postlaunch calibrations of the geometrical albedo observations used to derive ozone values. The postlaunch calibration revisions remove time dependent errors in the ozone amounts due to instrument drift, while the revised prelaunch calibration corrects the absolute value of retrieved ozone. The prelaunch corrections are a result of calibration checks from in-orbit comparisons of ultraviolet geometric albedos measured by shuttle SBUV (SSBUV) and the NOAA 11 SBUV/2. Geometric albedo comparison data are further corrected using a radiative transfer code to account for the small difference in observing conditions between the two spacecraft. The postlaunch corrections rely on in-flight calibration and solar irradiance data to account for time dependent changes in instrument gain, thermal response, and instrument diffuser degradation over time. Comparison of data from three SSBUV flights, which occurred about one year apart, with concurrent SBUV/2 data provided an independent check of the time dependent change derived from the in-flight calibration data. Time independent corrections result in an increase of about 1% for total ozone, 5% for ozone at 1 mbar, and near 0% at 15 mbar. The time dependent corrections amount to an increase of 2% for total ozone, 10% for ozone near 1 mbar, and 3% at 15 mbar at the end of the current record in May 1993. Recent laboratory studies indicate that the absolute radiance calibrations may still be in error by a few percent which results in ozone profile values that are too low. The SBUV/2 total and ozone profile data are compared to the Nimbus SBUV data during the period when the data overlapped. Total ozone values agree to about 1%, while ozone profile differences range from -4% to +6%, depending on latitude and altitude, relative to SBUV. These differences are not statistically significant given the uncertainties of the two data sets.

Hilsenrath, E.β†—