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Thamizhavel, A.

Publications and source records attributed to Thamizhavel, A..

Spin correlation in trigonal EuMn 2 As 2

The trigonal structure of EuMn 2 As 2 is an anomaly in the tetragonal 122-type pnictide family. Here, we report a detailed investigation of the underlying magnetic correlations in single crystal EuMn 2 As 2 using high-resolution elastic neutron-scattering measurements. The system undergoes two successive antiferromagnetic transitions at T = 135 K and 14.4 K, respectively. Numerical modeling of the experimental data reveals the long-range antiferromagnetic correlation of Mn-ions in the a - b plane below T N 1 = 135 K . Mn spins are aligned closer to the diagonal axis of the unit cell. The lower temperature transition, below T N 2 = 14.4 K , is discovered to arise due to the long-range antiferromagnetic correlation of Eu spins that are rotated by θ = 55 ° from the c axis of the unit cell.

36 MATERIALS SCIENCE↗

Electronic structure of Co-Ni-Ga Heusler alloys studied by resonant photoemission

The electronic structures of Co{sub 2.01}Ni{sub 1.05}Ga{sub 0.94} and Co{sub 1.76}Ni{sub 1.46}Ga{sub 0.78} Heusler alloys have been investigated by resonant photoemission spectroscopy across the 3p-3d transition of Co and Ni. For the Ni excess composition Co{sub 1.76}Ni{sub 1.46}Ga{sub 0.78}, the valence band peak shows a shift of 0.25 eV as compared to the near stoichiometric composition Co{sub 2.01}N1{sub 1.05}Ga{sub 0.94}. Also an enhancement is observed in the Ni related satellite features in the valence band for the Ni excess composition. Due to hybridization of Co and Ni 3d states in these systems, the Co and Ni 3p-3d resonance energies are found to be higher as compared to Co and Ni metals. Theoretical first principle calculation is performed to understand the features in the valence band and the shape of the resonance profile.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Temperature dependent tunneling study of CaFe{sub 1.96}Ni{sub 0.04}As{sub 2} single crystals

We report on temperature dependent scanning tunneling microscopy and spectroscopy studies on CaFe{sub 1.96}Ni{sub 0.04}As{sub 2} single crystals in 5.4 – 19.7 K temperature range across the normal metal - superconductor transition temperature, T{sub C} = 14K. The in-situ cleaved crystals show reasonably flat surface with signatures of atomic resolution. The tunnel spectra show significant spatial inhomogeneity below T{sub C}, which reduces significantly as the temperature goes above the T{sub C}. We discuss these results in terms of an inhomogeneous electronic phase that may exist due to the vicinity of this composition to the quantum critical point.

36 MATERIALS SCIENCE↗

Complex temperature evolution of the electronic structure of CaFe{sub 2}As{sub 2}

Employing high resolution photoemission spectroscopy, we investigate the temperature evolution of the electronic structure of CaFe{sub 2}As{sub 2}, which is a parent compound of high temperature superconductors—CaFe{sub 2}As{sub 2} exhibits superconductivity under pressure as well as doping of charge carriers. Photoemission results of CaFe{sub 2}As{sub 2} in this study reveal a gradual shift of an energy band, α away from the chemical potential with decreasing temperature in addition to the spin density wave (SDW) transition induced Fermi surface reconstruction across SDW transition temperature. The corresponding hole pocket eventually disappears at lower temperatures, while the hole Fermi surface of the β band possessing finite p orbital character survives till the lowest temperature studied. These results, thus, reveal signature of complex charge redistribution among various energy bands as a function of temperature.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗