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Travis Knepp

Publications and source records attributed to Travis Knepp.

Evidence for Systematic Changes in the Stratospheric Aerosol Size Following Volcanic Eruptions of Diverse Magnitudes Using Space-Based Instruments

An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption’s main aerosol layer and an apparent change in aerosol size distribution that spans multiple orders of magnitude in the stratospheric impact of an volcanic event. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. In this respect, it may be a unique tool to verify the performance of interactive aerosol models used in GCMs and ESMs and may suggest an avenue for improving aerosol extinction coefficient measurements from single channel observations such the Optical Spectrograph and Infrared Imager System. We note limitations on this analysis including that the presence of significant amounts of ash in the main aerosol layer may significantly modulate these results.

Larry Thomason↗

Evidence for the predictability of changes in the stratosphericaerosol size following volcanic eruptions of diverse magnitudesusing space-based instruments

An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption’s main aerosol layer and the wavelength dependence of that perturbation. This relationship spans multiple orders of magnitude in the aerosol extinction coefficient of stratospheric impact of volcanic events. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main sulfuric acid aerosol layer and other factors may significantly modulate these results. Despite these limitations, the findings suggest an avenue for improving aerosol extinction coefficient measurements from single-channel observations such as the Optical Spectrograph and Infrared Imager System as they rely on a prior assumptions about particle size. They may also represent a distinct avenue for the comparison of observations with interactive aerosol models used in global climate models and Earth system models.

Larry W Thomason↗

TPSAS-NF1676L-32936-DND

The Stratospheric Aerosol and Gas Experiment III (SAGE III) instrument, installed on the International Space Station (ISS), has completed over a year of data collection and production of science data products. The SAGE III/ISS is a solar and lunar occultation instrument, scanning the light from the sun and moon, through the limb of the Earth’s atmosphere. It was launched in February 2017 and provides data from June 2017 to the present. It continues SAGE's legacy of ozone, aerosol and water vapor profile measurements and extends the lengthy records for monitoring constituents important for understanding stratospheric ozone trends. This presentation shows the preliminary validation results of comparing SAGE III/ISS ozone and water vapor vertical profiles with those of NOAA ESRL/GMD and NIWA mission-funded ozonesondes and frost point hygrometers, and comparisons with other correlative data.

Susan Kizer↗

TPSAS-NF1676L-30290-DND

The Summer 2017 Ozone Water Land Environmental Transition Study (OWLETS) mission set out to compare the differences in ozone concentrations between inland measurements of air quality, specifically at Langley Research Center (LaRC), and measurements taken over water, specifically on the Chesapeake Bay Bridge Tunnel (CBBT), as well as the vertical profiles above each location. Current weather models often predict a gradient in ozone concentration between land and ocean and this campaign attempted to capture this difference using hand-held Personal Ozone Monitors (POMs) in correspondence to ozonesondes and LIDAR measurements. The Tropospheric Emissions: Monitoring of Pollution (TEMPO) is the first geostationary satellite that will take hourly measurements to monitor air pollutants across North America using solar backscatter. The small footprint allows for higher spatial resolution readings of many parameters including O3, NO2 , and aerosol. TEMPO’s higher resolution readings would benefit from validation techniques on the ground. Validation methods usually include comparison to air quality monitoring stations, but they could also incorporate other forms of validation such as comparison to small sensors. In cooperation with TEMPO, OWLETS aims to provide the user community high resolution temporal and spatial, both horizontal and vertical, variability of O3 simultaneously over the land and water during various air quality events to improve forecast models and air quality satellite retrievals. Together, these missions will improve spatial resolution and capture temporal variability of air quality over North America.

Emily Gargulinski↗

TPSAS-NF1676L-30150-DND

Validation of science data products from the Stratospheric Aerosol and Gas Experiment (SAGE) III, installed on the International Space Station (ISS) in March 2017, requires intercomparison with validated data sources. The SAGE III/ISS mission is actively utilizing in-situ profile measurements from balloon packages, consisting of a standard meteorological radiosonde, ozonesonde, and frost-point hygrometer, that were launched coincident with SAGE III/ISS overpass opportunities. Some packages have included an aerosol sonde. This provides regional correlations of ozone, water vapor and aerosol extinction between the in-situ measurement data and the SAGE III/ISS profile products. In addition, ground-based LIDAR measurements and aircraft-based measurements of ozone, water vapor, aerosol extinction and nitrogen dioxide will provide additional validation data for correlation with the SAGE III/ISS data products. Initial results of the mission directed validation program will be presented. When possible, operation and launch times were modified to improve the temporal and spatial coincidence between the measurements. Results and progress utilizing LIDAR and balloon-borne aerosol observations are discussed herein, while intercomparisons that make use of ozone sondes is are presented in the companion poster by Kizer et al.

Travis Knepp↗

TPSAS-NF1676L-32505-DND

The Stratospheric Aerosol and Gas Experiment III (SAGE III) instrument, installed on the International Space Station (ISS), has completed over a year of data collection and production of science data products, including the newly released version 5.1 data product. The SAGE III/ISS is a solar and lunar occultation instrument, scanning the light from the sun and moon, through the limb (edge) of the Earth's atmosphere. It was launched in February 2017 and provides data from June 2017 to the present. It continues SAGE's legacy of ozone, aerosol and water vapor profile measurements and extends the lengthy records for monitoring constituents important for understanding stratospheric ozone trends. This presentation shows the preliminary validation results of comparing SAGE III/ISS ozone vertical profiles with those of mission funded ozone sondes, associated lidar, and comparisons with other correlative data.

Susan Kizer↗

Stratospheric Aerosol and Gas Experiment III on the International Space Station(SAGE III/ISS) Validation of Three Years of Ozone and Water Vapor Data

The Stratospheric Aerosol and Gas Experiment III (SAGE III) instrument installed on the International Space Station (ISS) has completed three years of data collection and production of science data products. The SAGE III/ISS is a solar and lunar occultation instrument that scans the light from the Sun and Moon through the limb of the Earth’s atmosphere to produce vertical profiles of aerosol, ozone, water vapor, and other trace gases. It continues the legacy of previous SAGE instruments dating back to the 1970s to provide data continuity of stratospheric constituents critical for assessing trends in the ozone layer. This presentation shows the validation results of comparing SAGE III/ISS ozone and water vapor vertical profiles with those of in situ and satellite data.

SAGE III ISS ozone water vapor validation↗

Revisiting GloSSAC Using Space Based Measurements

We revisit Global Space-based stratospheric aerosol climatology (GloSSAC) and extend the dataset through 2021 in the latest version (version 2.2). Several space-based measurements have been used to construct GloSSAC. For version 2.2, important changes include implementation of a revised aerosol/cloud categorization for The Stratospheric Aerosol and Gas Experiment (SAGE III/ISS). SAGE III/ISS began its mission in June 2017. While SAGEIII/ISS makes reliable and robust solar occultation measurements in stratosphere—similar to its predecessors, interpreting aerosol extinction measurements in the vicinity of tropopause and in the troposphere have been a challenge for all SAGE measurements. Here, we study the challenges associated with the discrimination of aerosols and clouds from the extinction measurements. Here, we describe the methods implemented to categorize Clouds and aerosols using available SAGEIII/ISS aerosol measurements. We use version 5.2 of SAGE III/ISS extinction coefficients for the analysis. The current algorithm now classifies standard (background) and non-standard (enhanced) aerosols in the stratosphere and identify enhanced aerosols and aerosol/cloud mixture in the tropopause region. Extinction coefficient measurements from SAGE series of observations make an important contribution in the GloSSAC data base and therefore, the impact of cloud-filtered aerosol extinction coefficient measurements on the latest version of GloSSAC (version 2.2) is also discussed. Additionally, we discuss minor version changes occurred in other space-based measurements that include Optical Spectrograph and InfraRed Imaging System(OSIRIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation(CALIPSO). We also plan on evaluating and using aerosol extinction profiles from other satellite data sets such as Ozone Mapping Profiler Suite (OMPS) in a future version.

stratospheric aerosol↗

A New Level 3 Aerosol Product for SAGE III/ISS

- A new Level 3 SAGE III/ISS aerosol product is produced that now includes aerosol/cloud flags. - Cloud screening algorithm is developed based on a method proposed by Thomason and Vernier (2013) with some modifications. - Frequent volcanic and PyroCb events during SAGE III/ISS era (2017-present) makes it challenging to implement a cloud screening algorithm. - We use version 5.2 of SAGE III/ISS for all our analyses.

Mahesh Kovilakam↗

Model Evaluation and Intercomparison Using Data Collected by the Langley Mobile Ozone Lidar in Hampton, Virginia

Throughout the year 2022, the Langley Mobile Ozone Lidar (LMOL) has been frequently collecting ozone and aerosol measurements in the lower troposphere. The lidar is located in the parking lot behind the Atmospheric Sciences building at NASA Langley in Hampton, Virginia, approximately 37.095 N, -76.389 W. The data was collected during a range of several distinct atmospheric conditions, including stratospheric intrusions, surface frontal passages, and long-range transported wildfire smoke plumes. We use this data to evaluate and intercompare the forecast accuracy of two atmospheric chemistry models: the GEOS Composition Forecasting model (GEOS-CF) and the Weather Research and Forecasting model with Chemistry (WRF-Chem). Both models make daily three-dimensional forecasts of many trace gases and species for the contiguous United States. Over a range of ten distinct collection events, each spanning 36 hours to nearly seven days, the forecast models predict tropospheric ozone at NASA Langley with reasonable accuracy. The models best predict the timing and shape of the observed stratospheric intrusions in the middle troposphere but often vary in the magnitude of the ozone mixing ratios. For other atmospheric conditions, there is more variability in the model accuracy. Here, we summarize the accuracy of the models for all events and investigate reasons for differences between the models and the lidar.

Daniel B. Phoenix↗

Quantifying Uncertainty in Particle Size Distribution Parameters Inferred from SAGE III/ISS Extinction Spectra

Stratospheric aerosols play key roles in the chemistry and radiation balance of the atmosphere and are a key input parameter for global chemistry and climate models. The degree to which aerosols impact chemistry and radiation balance depends primarily on their microphysical properties such as particle size distribution (PSD). The PSD is a mathematical description of the relative abundance of different sized particles within a sampling volume. If the PSD is accurately known then other key modeling parameters (e.g., surface area density) can be derived. Occultation observations from orbital instruments such as SAGE III/ISS have been used to infer these PSD parameters by inverting the extinction coefficient spectra. However, past efforts failed to address two key issues with this methodology: 1. The measurement uncertainty was not accounted for; 2. They assumed the PSDs to be single-mode only, while “real-world” PSDs are predominantly bi-modal. Accounting for both issues in the retrieval will yield an expanded solution space to the inferred PSD parameters; the question is “by how much?” To address this knowledge gap, we propose to carry out a series of simulations and, for every valid SAGE III/ISS data point, determine the range of PSD parameters that yield extinction spectra that are indistinguishable from the SAGE III/ISS data, within the limits of the reported uncertainty. Further, we will expand the solution space, for the first time, to include bimodal distributions. The results of this work will advance Earth system modeling/prediction capability through identifying the uncertainty of PSD parameter estimates using SAGE III/ISS data. The key benefits of this study over previous studies are twofold: 1. we will provide PSD estimates that include bimodal distributions in the solution space, 2. we will provide an uncertainty estimate for these parameters. The results of this study may be used directly in current and future climate and chemistry models.

SAGE III/ISS↗