Search NASA⌕ Search

Engineering topics

Valiente-Dobón, J. J.

Publications and source records attributed to Valiente-Dobón, J. J..

18 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Quest for Cooper Pair Transfer in Heavy-Ion Reactions: The 206 Pb + 118 Sn Case

In this Letter we report on effects of nucleon-nucleon correlations probed in nucleon transfer reactions with heavy ions. We measured with high efficiency and resolution a complete set of observables for neutron transfer channels in the ²⁰⁶Pb + ¹¹⁸Sn system employing a large solid angle magnetic spectrometer, which allowed us to study a wide range of internuclear distances via a detailed excitation function. The coupled channel theory, based on an independent particle transfer mechanism, follows the experimental transfer probabilities for one- and two-neutron pick-up and stripping channels. The experimental two-neutron transfer cross sections indicate that in reactions between pair-vibrational (closed shell) and pair-rotational (open shell) nuclei, correlations manifest via pair-addition and pair-removal modes, which constitute one of the elementary modes of excitations in nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Further investigation on the fusion of 6 Li with 209 Bi target at near-barrier energies

The complete and incomplete fusion cross sections for 6 Li+ 209 Bi were measured using the in-beam γ-ray method around the Coulomb barrier. The cross sections of (deuteron captured) incomplete fusion (ICF) products were re-quantified experimentally for this reaction system. Here, the results reveal that the ICF cross section is equivalent to that of complete fusion (CF) above the Coulomb barrier and dominant near or below the Coulomb barrier. A theoretical calculation based on the continuum discretized coupled channel (CDCC) method was performed for the aforementioned CF and ICF cross sections; the result is consistent with the experiments. The universal fusion function (UFF) was also compared with the measured CF cross section for different barrier parameters, demonstrating that the CF suppression factor is significantly influenced by the choice of potential, which can reflect both dynamic and static effects of breakup on the fusion process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

High-Precision Spectroscopy of 20 O Benchmarking Ab Initio Calculations in Light Nuclei

The excited states of unstable 20 O were investigated via γ-ray spectroscopy following the 19 O(d, p) ⁢20 O reaction at 8 A⁢ MeV. By exploiting the Doppler shift attenuation method, the lifetimes of the $2^+_2$ and $3^+_1$ states were firmly established. From the γ-ray branching and E⁢2/M⁢1 mixing ratios for transitions deexciting the $2^+_2$ and $3^+_1$ states, the B⁡(E⁢2) and B⁡(M⁢1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of γ-ray transition probabilities with the valence space in medium similarity renormalization group ab initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab initio approaches using chiral effective field theory forces are challenged by detailed high-precision spectroscopic properties of nuclei. Finally, the reduced transition probabilities were found to be a very constraining test of the performance of the ab initio models.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Shape evolution in even-mass 98-104 Zr isotopes via lifetime measurements using the $\gamma \gamma $-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first 2 + state and the increase in the transition strength B(E2; 2$^+_1$ →0$^+_1$) going from 98 Zr to 100 Zr has been the first example of “quantum phase transition” in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the γγ-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. Here this work reports the results of lifetime measurements for the first yrast excited states in 98-104 Zr carried out to extract reduced transition probabilities. The new lifetime values in γγ-coincidence and γ-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree–Fock–Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

An alternative viewpoint on the nuclear structure towards 100 Sn: Lifetime measurements in 105 Sn

This work aims at presenting an alternative approach to the long standing problem of the B(E2) values in Sn isotopes in the vicinity of the N=Z double-magic nucleus 100 Sn, until now predominantly measured with relativistic and intermediate-energy Coulomb excitation reactions. The direct measurement of the lifetime of low-lying excited states in odd-even Sn isotopes provides a new and precise guidance for the theoretical description of the nuclear structure in this region. Lifetime measurements have been performed in 105 Sn for the first time with the coincidence Recoil Distance Doppler Shift technique. The lifetime results for the $7/2^+_1$ first excited state and the $11/2^+_1$ state, $2^+ (^{104}$Sn) Ⓧ $v1g_{7/2}$ multiplet member, are discussed in comparison with state-of-the-art shell model and mean field calculations, highlighting the crucial contribution of proton excitation across the core of 100 Sn. The reduced transition probability B(E2) of the $11/2^+_1$ core-coupled state points out an enhanced staggering with respect to the B(E2; $2^+_1$ → $0^+_1$) in the even-mass 104 Sn and 106 Sn isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Nuclear structure advancements with multi-nucleon transfer reactions

Multi-Nucleon Transfer (MNT) reactions have been used for decades as a reaction mechanism, in order to populate excited states in nuclei far from stability and to perform nuclear structure studies. Nevertheless, the development of set-ups involving high acceptance tracking magnetic spectrometers (mainly existing in Europe), coupled with the Advanced GAmma Tracking Array (AGATA) opens new possibilities, especially if they are used in conjunction with high-intensity stable beams or ISOL RIBs. In this article, we will discuss the capabilities of such set-ups aiming at different goals, including complete information in high-resolution spectroscopy as well as lifetime measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Level scheme study of Mo 91 : Weak-coupling approximation in the N = 50 region

The level scheme of 91 Mo has been studied using the GALILEO γ-ray spectrometer at Laboratori Nazionali di Legnaro, INFN. Five transitions together with four levels are identified for the first time by the γ-γ coincidence measurement, considerably enriching the negative band in 91 Mo. Furthermore, the discrepancy in the previous parity assignments for the states higher than 3807.5 keV has been clarified with the help of new experimental results. A shell-model calculation employing the JUN45 interaction is performed in order to get a further understanding of the level structure of 91 Mo. Being close to N=50 shell closure, the weak-coupling approximation between the valence g 9/2 neutron-hole with the even-even core ( 92 Mo) is discussed in 91Mo.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

First spectroscopic study of odd-odd Cu 78

Nuclei in the vicinity of 78 Ni are important benchmarks for nuclear structure, which can reveal changes in the shell structure far from stability. Spectroscopy of the odd-odd isotope 78 CU was performed for the first time in an experiment with the EURICA setup at the Radioactive Isotope Beam Factory at RIKEN Nishina Center. Excited states in the neutron-rich isotope were populated following the β decay of 78 Ni produced by in-flight fission and separated by the BigRIPS separator. A level scheme based on the analysis of $\gamma$-$\gamma$ coincidences is presented. Tentative spin and parity assignments were made when possible based on the β -decay feeding intensities and $\gamma$-decay properties of the excited states. Time correlations between β and $\gamma$ decay show clear indications of an isomeric state with a half-life of 3.8(4) ms. Large-scale Monte Carlo shell-model calculations were performed using the A3DA-m interaction and a valence space comprising the full f p shell and the 1⁢g 9/2 and 2⁢d 5/2 orbitals for both protons and neutrons. The comparison of the experimental results with the shell-model calculations allows interpreting the excited states in terms of spin multiplets arising from the proton-neutron interaction. In conclusion, the results provide further insight into the evolution of the proton single-particle orbitals as a function of neutron number, and quantitative information about the proton-neutron interaction outside the doubly magic 78 Ni core.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Transfer reactions in 206 $\mathrm{Pb}$ + 118 $\mathrm{Sn}$: From quasielastic to deep-inelastic processes

Here, we measured multinucleon transfer reactions for the 206 Pb+ 118 Sn system at E lab =1200 MeV by employing the large solid angle magnetic spectrometer PRISMA. Differential and total cross sections and Q-value distributions have been obtained for a variety of neutron and proton pick-up and stripping channels. The Q-value distributions show how the quasi-elastic and deep inelastic processes depend on the mass and charge of the transfer products. The corresponding cross sections have been compared with calculations performed with the GRAZING code. An overall good agreement is found for most of the few nucleon transfer channels. The underestimation of the data for channels involving a large number of transferred nucleons indicates that more complicated processes populate the given isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Level scheme study of 92 Mo: Searching for evidence of core excitation

Excited states in 92 Mo are populated via the 89 Y( 6 Li, 3$\textit{n}$) 92 Mo reaction at the tandem of XTU, INFN-LNL. The level scheme of 92 Mo is revised and expanded considerably by the γ-γ coincidence measurement. The newly observed level structures are compared with different shell-model calculations performed in various model spaces. In this work, the results show that the several high-energy (≈2 MeV) transitions, observed for the first time in the current work, could be a presumable signature of $\textit{N}$ = 50 core-breaking effect. The measured strengths of $\textit{E}$1 transitions between the low-lying positive and negative bands indicate an important contribution from $\textit{Z}$ = 28 proton core-excitation

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Lifetime measurements of states of S 35 , S 36 , S 37 , and S 38 using the AGATA γ -ray tracking spectrometer

Lifetimes or lifetime limits of a small number of excited states of the sulfur isotopes with mass numbers A = 35 , 36, 37, and 38 have been measured using the differential recoil-distance method. The isotopes of sulfur were populated in binary grazing reactions initiated by a beam of 36 S ions of energy 225 MeV incident on a thin 208 Pb target which was mounted in the Cologne plunger apparatus. The combination of the PRISMA magnetic spectrometer and an early implementation of the AGATA γ-ray tracking array was used to detect γ rays in coincidence with projectile-like nuclear species. Lifetime measurements of populated states were measured within the range from about 1 to 100 ps. The number of states for which lifetime measurements or lifetime limits were possible was limited by statistics. For 35 S, the lifetime was determined for the first 1/2 + state at 1572 keV; the result is compared with a previous published lifetime value. The lifetime of the 3 - state of 36 S at 4193 keV was determined and compared with earlier measurements. No previous lifetime information exists for the (6 + ) state at 6690 keV; a lifetime measurement with large associated error was made in the present work. For 37 S, the states for which lifetime limits were established were those at 646 keV with J π = 3/2 - and at 2776 keV with J π = 11/2 - ; there are no previously published lifetime values for excited states of 37 S. Finally, a lifetime limit was established for the J π =(6 + ) state of 38 S at 3675 keV; no lifetime information exists for this state in the literature. Measured lifetime values were compared with the results of state-of-the-art shell-model calculations based on the PSDPF, SDPF-U, and FSU effective interactions. In addition, nuclear magnetic-dipole and electric-quadrupole moments, branching ratios, mixing ratios, and electromagnetic transition rates, where available, have been compared with shell-model values. The current work suffers from poor statistics; nevertheless, lifetime values and limits have been possible, allowing a useful discussion of the ability of state-of-the-art shell-model calculations to reproduce the experimental results.

electromagnetic transitions↗
DOE OSTI2021

Signature splitting of the g 7 / 2 [ 404 ] 7 / 2 + bands in Ba 131 and Ce 133

Excited states in Ba 131 and Ce 133 were studied using in-beam γ -ray spectroscopy through the Sn 122 ( C 13 , 4 n ) Ba 131 and Te 125 ( C 12 , 4 n ) Ce 133 reactions, respectively. A strongly coupled band, associated with the ν g 7 / 2 [ 404 ] 7 / 2 + configuration, was identified in Ba 131 and Ce 133 . It is the first time to observe the ν g 7 / 2 [ 404 ] 7 / 2 + bands in the N = 75 isotones. The signature partners exhibit considerable energy splitting in comparison with those in the π g 7 / 2 [ 404 ] 7 / 2 + bands in the odd- A Ta and Re isotopes. Here, extensive cranked shell model and quasiparticle-plus-triaxial-rotor model calculations reveal the origin of the signature splitting, which depends not only on the triaxiality, but also on the configuration mixing with nearby low- j orbitals.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Lifetime measurements in the even-even Cd 102 – 108 isotopes

The heaviest T z = 0 doubly-magic nucleus, Sn 100 , and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction. For instance, the structure of light-Sn nuclei has been shown to be affected by the delicate balance between nuclear-interaction components, such as pairing and quadrupole correlations. From Cd to Te, many common features and phenomena have been observed experimentally along the isotopic chains, leading to theoretical studies devoted to a more general and comprehensive study of the region. In this context, having only two proton holes in the Z = 50 shell, the Cd isotopes are expected to present properties similar to those found in the Sn isotopic chain. The aim of this work was to measure lifetimes of excited states in neutron-deficient nuclei in the vicinity of Sn 100 . Here, the neutron-deficient nuclei in the N ≈ Z ≈ 50 region were populated using a multinucleon transfer reaction with a Cd 106 beam and a Mo 92 target. The beamlike products were identified by the VAMOS + + spectrometer, while the γ rays were detected using the AGATA array. Lifetimes of excited states were determined using the recoil distance Doppler-shift method, employing the Cologne differential plunger. Lifetimes of low-lying states were measured in the even-mass Cd 102 – 108 isotopes. In particular, multiple states with excitation energy up to ≈ 3 MeV, belonging to various bands, were populated in Cd 106 via inelastic scattering. The transition strengths corresponding to the measured lifetimes were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach. Conclusions: Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z = 48 and Z = 50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with β 2 ≈ 0.2 . At this deformation Z = 48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

The GALILEO γ-ray array at the Legnaro National Laboratories

GALILEO, a new 4 pi high-resolution gamma-detection array, based on HPGe detectors, has been developed and installed at the Legnaro National Laboratories. The GALILEO array greatly benefits from a fully-digital readout chain, customized DAQ, and a variety of complementary detectors to improve the resolving power by the detection of particles, ions or high-energy gamma-ray transitions. In this paper, a full description of the array, including electronics and DAQ, is presented together with its complementary instrumentation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Octupole correlations near Te 110

The lifetime of the 2 + and 9 – , 11 – , 13 – , 15 – states in the neutron-deficient 110 Te was measured for the first time using the recoil distance Doppler shift technique. The reported value of the reduced transition probability B(E2; $0$$^{+}_{g.s}$ → 2 + ) = 4.3(8) × 10 3 e 2 fm 4 supports the systematic for even-mass Te isotopes and was interpreted in the framework of the large-scale shell model and cranked shell model calculations. The measured reduced transition probabilities in the negative-parity yrast band revealed the upward trend towards the high spins. Furthermore, the enhanced collectivity is discussed in terms of the tilted axis cranking approach and the symmetry configuration mixing method with the Gogny D1S interaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Isomeric and beta-decay spectroscopy of 173,174 Ho

β-decay spectroscopy of 173,174 Ho (Z = 67, N = 106,107) was conducted at Radioactive Isotope Beam Factory at RIKEN by using in-flight fission of a 345-MeV/u 238 U primary beam. A previously unreported isomeric state at 405 keV with half-life of 3.7(12) μs and a spin and parity of (3/2 + ) is identified in 173 Ho. Moreover, a new state with a spin and parity of 9 - was discovered in 174 Er. The experimental log ft values of 5.84(20) and 5.25(18) suggest an allowed-hindered β decay from the ground state of 174 Ho to the K π = 8 - isomeric state in 174 Er. Configuration-constrained potential energy surface (PES) calculations were performed and the predictions are in reasonable agreement with the experimental results.

150 ≤ A ≤ 189↗