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Vermeulen, Christiaan

Publications and source records attributed to Vermeulen, Christiaan.

The new Device for Indirect Capture Experiments on Radionuclides at LANSCE: Efforts on measuring the resonance(s) responsible for the extremely large 88 Zr (n,γ) cross section

The thermal neutron capture cross section of 88 Zr was recently reported to be the second largest in nature with the largest resonance integral measured. Presumably, these very large values are caused by a resonance or resonances very near thermal energy. Determining their energies and widths, and hence the shape of the cross section away from thermal energies,is useful for applications. The short half-life (83.4 days) and associated large background, renders direct measurements of the neutron capture cross section impossible using current techniques. However, it is possible to measure the total neutron cross section, and hence the resonance properties, using the newly commissioned Device for Indirect Capture Experiments on Radionuclides (DICER) at the Los Alamos Neutron Science Center (LANSCE). Transmission measurements are utilized as a surrogate method to perform capture measurements. The 88 Zr needed for a DICER measurement was produced at the Isotope Production Facility (IPF) and cleanly separated from the production target material. A description of the new instrument, efforts and preliminary results on 88 Zr will be presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The LANSCE experimental program: accelerator requirements

The LANSCE accelerator complex exploits a flexible, high power 800 MeV proton linear accelerator to enable a broad swath of experimental work supporting multiple scientific programs. The beam requirements for these programs are diverse and change over time. The purpose of this document is to record, at a high level, the experimental requirements driving the beam delivery requirements for each experimental facility at LANSCE. Revision 0 serves to baseline the current set of experiments, and we expect to revise the document on an as-needed basis when either the experimental requirements change or are found to require a more complete definition.

43 PARTICLE ACCELERATORS↗

Development of experimental and computational frameworks to predict subcooled flow boiling in the LANL Isotope Production Facility

Cooling is crucial to maintain the integrity of target systems in isotope production facilities. At Los Alamos National Laboratory (LANL)’s Isotope Production Facility (IPF), multiple encapsulated targets are stacked and irradiated in tandem with a 100 MeV, ~250μA proton beam. To facilitate effective heat removal, these stacked targets are separated and cooled via a series of water channels. At these beam currents, this high-energy proton beam heats the target system, likely initiating subcooled flow boiling in the cooling channels. However, in-beam monitoring of the IPF target system is not possible due to the extreme radiation environment, and the necessarily significant shielding. To better understand high-power target performance, we developed ex-situ experimental and computational frameworks to predict the behavior of subcooled flow boiling at IPF. Subcooled flow boiling experiments on Inconel 625 samples under IPF conditions (2 bar pressure, 10 GPM flow rate (i.e., 2249 kg/m 2 /s), 85 K subcooling) revealed that IPF's average operating power is at the early stage of boiling with a heat transfer coefficient of 48,000 W/m 2 /s. The proposed modeling framework enables us to predict a complete boiling curve, i.e., single-phase heat transfer, onset of nucleate boiling, two-phase heat transfer, and critical heat flux (CHF), with specification of input boiling parameters up to intermediate heat flux levels. The estimated CHF under IPF conditions is 5.2 MW/m 2 . Experimental data under reduced conditions (2 bar pressure, 1.5 GPM flow rate (i.e., 337 kg/m 2 /s), 45 K subcooling) served as validation cases for the computational modeling. This computational model can be further extended to more complicated systems replicating the real IPF configuration, for instance, to study void distribution as a function of the incident proton beam profile and coolant velocity profile of multiple cooling channels. Finally, the proposed experimental and computational frameworks provide a means to better understand cooling systems in the isotope production facilities at different accelerators, where in-beam monitoring of the cooling process is not available.

07 ISOTOPE AND RADIATION SOURCES↗