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Wang, Lifan

Publications and source records attributed to Wang, Lifan.

Correlating concerted cations with oxygen redox in rechargeable batteries

Rechargeable batteries currently power much of our world, but with the increased demand for electric vehicles (EVs) capable of traveling hundreds of miles on a single charge, new paradigms are necessary for overcoming the limits of energy density, particularly in rechargeable batteries. The emergence of reversible anionic redox reactions presents a promising direction toward achieving this goal; however this process has both positive and negative effects on battery performance. While it often leads to higher capacity, anionic redox also causes several unfavorable effects such as voltage fade, voltage hysteresis, sluggish kinetics, and oxygen loss. However, the introduction of cations with topological chemistry tendencies has created an efficient pathway for achieving long-term oxygen redox with improved kinetics. The cations serve as pillars in the crystal structure and meanwhile can interact with oxygen in ways that affect the oxygen redox process through their impact on the electronic structure. This review delves into a detailed examination of the fundamental physical and chemical characteristics of oxygen redox and elucidates the crucial role that cations play in this process at the atomic and electronic scales. Furthermore, here we present a systematic summary of polycationic systems, with an emphasis on their electrochemical performance, in order to provide perspectives on the development of next-generation cathode materials.

25 ENERGY STORAGE↗

Newly formed dust within the circumstellar environment of SN Ia-CSM 2018evt

Dust associated with various stellar sources in galaxies at all cosmic epochs remains a controversial topic, particularly whether supernovae play an important role in dust production. We report evidence of dust formation in the cold, dense shell behind the ejecta–circumstellar medium (CSM) interaction in the Type Ia-CSM supernova (SN) 2018evt three years after the explosion, characterized by a rise in mid-infrared emission accompanied by an accelerated decline in the optical radiation of the SN. Such a dust-formation picture is also corroborated by the concurrent evolution of the profiles of the Hα emission line. Our model suggests enhanced CSM dust concentration at increasing distances from the SN as compared to what can be expected from the density profile of the mass loss from a steady stellar wind. By the time of the last mid-infrared observations at day +1,041, a total amount of 1.2 ± 0.2 × 10 -2 M ⊙ of new dust has been formed by SN 2018evt, making SN 2018evt one of the most prolific dust factories among supernovae with evidence of dust formation. The unprecedented witness of the intense production procedure of dust may shed light on the perceptions of dust formation in cosmic history.

79 ASTRONOMY AND ASTROPHYSICS↗

The LIGO HET Response (LIGHETR) Project to Discover and Spectroscopically Follow Optical Transients Associated with Neutron Star Mergers

The LIGO HET Response (LIGHETR) project is an enterprise to follow up optical transients (OTs) discovered as gravitational-wave merger sources by the LIGO/Virgo collaboration (LVC). Early spectroscopy has the potential to constrain crucial parameters such as the aspect angle. The LIGHETR collaboration also includes the capacity to model the spectroscopic evolution of mergers to facilitate a real-time direct comparison of models with our data. The principal facility is the Hobby–Eberly Telescope. LIGHETR uses the massively replicated VIRUS array of spectrographs to search for associated OTs and obtain early blue spectra, and in a complementary role, the low-resolution LRS2 spectrograph is used to obtain spectra of viable candidates as well as a densely sampled series of spectra of true counterparts. Once an OT is identified, the anticipated cadence of spectra would match or considerably exceed anything achieved for GW170817 = AT2017gfo for which there were no spectra in the first 12 hr and thereafter only roughly once daily. We describe special HET-specific software written to facilitate the program and attempts to determine the flux limits to undetected sources. We also describe our campaign to follow up OT candidates during the third observational campaign of the LIGO and Virgo Scientific Collaborations. We obtained VIRUS spectroscopy of candidate galaxy hosts for five LVC gravitational-wave events and LRS2 spectra of one candidate for the OT associated with S190901ap. We identified that candidate, ZTF19abvionh = AT2019pip, as a possible Wolf–Rayet star in an otherwise unrecognized nearby dwarf galaxy.

79 ASTRONOMY AND ASTROPHYSICS↗

Constraints on Cosmological Parameters with a Sample of Type Ia Supernovae from JWST

We investigate the potential of using a sample of very high-redshift (2 ≲ z ≲ 6) (VHZ) Type Ia supernovae (SNe Ia) attainable by JWST on constraining cosmological parameters. At such high redshifts, the age of the universe is young enough that the VHZ SN Ia sample comprises the very first SNe Ia of the universe, with progenitors among the very first generation of low-mass stars that the universe has made. We show that the VHZ SNe Ia can be used to disentangle systematic effects due to the luminosity distance evolution with redshifts intrinsic to SN Ia standardization. Assuming that the systematic evolution can be described by a linear or logarithmic formula, we found that the coefficients of this dependence can be determined accurately and decoupled from cosmological models. Systematic evolution as large as 0.15 mag and 0.45 mag out to z = 5 can be robustly separated from popular cosmological models for linear and logarithmic evolution, respectively. The VHZ SNe Ia will lay the foundation for quantifying the systematic redshift evolution of SN Ia luminosity distance scales. When combined with SN Ia surveys at comparatively lower redshifts, the VHZ SNe Ia allow for the precise measurement of the history of the expansion of the universe from z ~ 0 to the epoch approaching reionization.

79 ASTRONOMY AND ASTROPHYSICS↗

Deep drilling in the time domain with DECam: survey characterization

ABSTRACT This paper presents a new optical imaging survey of four deep drilling fields (DDFs), two Galactic and two extragalactic, with the Dark Energy Camera (DECam) on the 4-m Blanco telescope at the Cerro Tololo Inter-American Observatory (CTIO). During the first year of observations in 2021, >4000 images covering 21 deg2 (seven DECam pointings), with ∼40 epochs (nights) per field and 5 to 6 images per night per filter in g, r, i, and/or z have become publicly available (the proprietary period for this program is waived). We describe the real-time difference-image pipeline and how alerts are distributed to brokers via the same distribution system as the Zwicky Transient Facility (ZTF). In this paper, we focus on the two extragalactic deep fields (COSMOS and ELAIS-S1) characterizing the detected sources, and demonstrating that the survey design is effective for probing the discovery space of faint and fast variable and transient sources. We describe and make publicly available 4413 calibrated light curves based on difference-image detection photometry of transients and variables in the extragalactic fields. We also present preliminary scientific analysis regarding the Solar system small bodies, stellar flares and variables, Galactic anomaly detection, fast-rising transients and variables, supernovae, and active Galactic nuclei.

79 ASTRONOMY AND ASTROPHYSICS↗

Snowmass2021 Cosmic Frontier CF6 White Paper: Multi-Experiment Probes for Dark Energy - Transients

This invited Snowmass 2021 White Paper highlights the power of joint-analysis of astronomical transients in advancing HEP Science and presents research activities that can realize the opportunities that come with current and upcoming projects. Transients of interest include gravitational wave events, neutrino events, strongly-lensed quasars and supernovae, and Type~Ia supernovae specifically. These transients can serve as probes of cosmological distances in the Universe and as cosmic laboratories of extreme strong-gravity, high-energy physics. Joint analysis refers to work that requires significant coordination from multiple experiments or facilities so encompasses Multi-Messenger Astronomy and optical transient discovery and distributed follow-up programs.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The Young and Nearby Normal Type Ia Supernova 2018gv: UV-optical Observations and the Earliest Spectropolarimetry

The nondetection of companion stars in SN Ia progenitor systems lends support to the notion of double-degenerate systems and explosions triggered by the merging of two white dwarfs. This very asymmetric process should lead to a conspicuous polarimetric signature. By contrast, observations consistently find very low continuum polarization as the signatures from the explosion process largely dominate over the pre-explosion configuration within several days. Critical information about the interaction of the ejecta with a companion and any circumstellar matter is encoded in the early polarization spectra. In this study, we obtain spectropolarimetry of SN 2018gv with the ESO Very Large Telescope at -13.6 days relative to the B-band maximum light, or ~5 days after the estimated explosion—the earliest spectropolarimetric observations to date of any SN Ia. These early observations still show a low continuum polarization (lesssim0.2%) and moderate line polarization (0.30% ± 0.04% for the prominent Si ii λ6355 feature and 0.85% ± 0.04% for the high-velocity Ca component). The high degree of spherical symmetry implied by the low-line and continuum polarization at this early epoch is consistent with explosion models of delayed detonations and is inconsistent with the merger-induced explosion scenario. Finally, the dense UV and optical photometry and optical spectroscopy within the first ~100 days after the maximum light indicate that SN 2018gv is a normal SN Ia with similar spectrophotometric behavior to SN 2011fe.

79 ASTRONOMY AND ASTROPHYSICS↗

ASASSN-15LH: A Superluminous Ultraviolet Rebrightening Observed by Swift and Hubble

We present and discuss ultraviolet and optical photometry from the Ultraviolet/Optical Telescope, X-ray limits from the X-Ray Telescope on Swift, and imaging polarimetry and ultraviolet/optical spectroscopy with the Hubble Space Telescope, all from observations of ASASSN-15lh. It has been classified as a hydrogen-poor superluminous supernova (SLSN I), making it more luminous than any other supernova observed. ASASSN-15lh is not detected in the X-rays in individual or co-added observations. From the polarimetry we determine that the explosion was only mildly asymmetric. We find the flux of ASASSN-15lh to increase strongly into the ultraviolet, with an ultraviolet luminosity 100 times greater than the hydrogen-rich, ultraviolet-bright SLSN II SN2008es. We find that objects as bright as ASASSN-15lh are easily detectable beyond redshifts of ∼4 with the single-visit depths planned for the Large Synoptic Survey Telescope. Deep near-infrared surveys could detect such objects past a redshift of ∼20, enabling a probe of the earliest star formation. A late rebrightening-most prominent at shorter wavelengths -is seen about two months after the peak brightness, which is itself as bright as an SLSN. The ultraviolet spectra during the rebrightening are dominated by the continuum without the broad absorption or emission lines seen in SLSNe or tidal disruption events (TDEs) and the early optical spectra of ASASSN-15lh. Our spectra show no strong hydrogen emission, showing only Lyα absorption near the redshift previously found by optical absorption lines of the presumed host. The properties of ASASSN-15lh are extreme when compared to either SLSNe or TDEs.

Brown, Peter J.↗

Evidence for Type Ia Supernova Diversity from Ultraviolet Observations with the Hubble Space Telescope

We present ultraviolet (UV) spectroscopy and photometry of four Type Ia supernovae (SNe 2004dt, 2004ef, 2005M, and 2005cf) obtained with the UV prism of the Advanced Camera for Surveys on the Hubble Space Telescope, This dataset provides unique spectral time series down to 2000 A. Significant diversity is seen in the near-maximum-light spectra (approx.2000-3500 A) for this small sample. The corresponding photometric data, together with archival data from Swift Ultraviolet/Optical Telescope observations, provide further evidence of increased dispersion in the UV emission with respect to the optical. The peak luminosities measured in the uvw lIF250W filter are found to correlate with the B-band light-curve shape parameter .(Delta)m15(B), but with much larger scatter relative to the correlation in the broad-band B band (e.g., approx. 0.4 mag versus approx. 0.2 mag for those with 0.8 <.(Delta)m15(B) < 1.7 mag). SN 2004dt is found as an outlier of this correlation (at> 3(sigma), being brighter than normal SNe Ia such as SN 2005cf by approx. 0,9 mag and approx. 2.0 mag in the uvwl1F250W and uvm2/F220W filters, respectively. We show that different progenitor metallicity or line-expansion velocities alone cannot explain such a large discrepancy. Viewing-angle effects, such as due to an asymmetric explosion, may have a significant influence on the flux emitted in the UV region. Detailed modeling is needed to disentangle and quantify the above effects

Wang, Xiaofeng↗