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Xu, Hongmei

Publications and source records attributed to Xu, Hongmei.

Evaluating fine-resolution, regional outputs of a variable resolution global climate model

Climate models have been used to study water resources and regional hydrologic responses to climate change, but climate model outputs must be downscaled to provide relevant regional data. However, the accuracy of this regional data is limited by uncertainties across and within downscaling methods, uncertainty across global outputs, and discontinuities at downscaled boundaries. A new alternative to traditional downscaling is a variable resolution model that incorporates fine-resolution regions directly into a coarse-resolution, global climate simulation in order to capture contiguous dynamics across resolution boundaries. In this study, we used the Variable-Resolution Community Earth System Model (VR-CESM) to generate one-eighth degree (14 km) fine-resolution outputs for the western U.S. and eastern China from 1970-2006. We focus our evaluation on precipitaiton, temperature, snow pack, solar radiation, and wind. We compare the model outputs with remote-sensing-based precipitation data, and both reanalysis and gridded weather station data for precipitation and temperature. VR-CESM generally has a cold bias in winter and a warm bias in summer in the western U.S., which compensate each other to reduce the annual bias. In eastern China, however, the sign of temperature biases are more consistent throughout the year with cold biases in the higher mountains and warm biases throughout most of the rest of the region. Precipitation biases are dependent upon reference data, and show slight overestimation in high mountain regions in both the U.S. and China with respect to gridded weather station data. Simulated snow cover in the western U.S. is reasonable compared to remote sensing data, but snow cover and snow water equivalent have larger biases when compared to reanalysis data. In eastern China there are widespread snow cover biases compared to remote sensing data. VR-CESM underestimates downward shortwave radiation to a greater degree in summer than in winter, and underestimates surface layer windspeed over mountains to a greater degree than in other areas. Comparison between VR-CESM and a coarser simulation (1-degree Beijing Climate Center model) shows reduced precipitation biases in the mountainous regions with finer resolution, indicating the value of variable-resolution modeling for reigonal studies.

Di Vittorio, Alan↗

Evaluating Variable‐Resolution CESM Over China and Western United States for Use in Water‐Energy Nexus and Impacts Modeling

Abstract Climate models are critical tools to study earth system processes and are often further downscaled to provide refined‐resolution data sets for regional water‐energy impact analyses. In this study, the Variable‐Resolution Community Earth System Model (VR‐CESM), a new dynamical downscaling method, is employed to generate 1/8° simulations for China and the western United States over 1970–2006. Precipitation, temperature, snowpack, radiation, and wind speed are compared with two 1° global climate models, regional climate model ensemble, and reference data sets to evaluate their fidelity. Simulated precipitation skill is dependent upon the reference data sets used, a slight (<+10%) and spatially consistent wet bias in China during summer and the western United States during winter. Precipitation bias in VR‐CESM is the smallest among models and demonstrates the added value provided by resolution refinement. However, temperature biases are generally greater than precipitation due to more complicated interactions among processes. VR‐CESM simulates +2°C warm bias in the low‐elevation regions in China but −2°C cold bias in mountains. However, DJF cold bias (−2.23°C to−3.37°C) and JJA warm bias (+1.13°C to +1.87°C) exist in the western United States. The modeling skills of precipitation and temperature at various topographies are similar in the two evaluated regions. The cold bias was likely affected by downward shortwave radiation deficit (−15%) and slow bias of surface wind speeds (−16% to −29%). Despite the wet and cold bias, snow water equivalent and snow cover are underestimated in mountains. We conclude that VR‐CESM outperforms other models evaluated and provides the best estimation of downscaled climate model data for water‐energy studies.

54 ENVIRONMENTAL SCIENCES↗

Synthesis and Photophysical Properties of Light-Harvesting Gold Nanoclusters Fully Functionalized with Antenna Chromophores

The development of efficient light-harvesting systems is important to understand the key aspects of solar-energy conversion processes and to utilize them in various photonic applications. In this study, atomically well-defined gold nanoclusters are reported as a new platform to fabricate artificial light-harvesting systems. An efficient amide coupling method is developed to synthesize water-soluble Au 22 clusters fully protected with pyrene chromophores by taking advantage of their facile phase-transfer reaction. The synthesized Au 22 clusters with densely packed 18 pyrene chromophores (Au 22 –PyB 18 ) exhibit triple-emission in blue, green, and red wavelength regions arising respectively from pyrene monomer, pyrene excimer, and Au 22 emission, producing bright white light emission together. The photoluminescence of Au 22 is enhanced by more than tenfold, demonstrating that pyrenes at the periphery efficiently channel the absorbed energy to the luminescent Au 22 at the center. A combination of femtosecond transient absorption and anisotropy measurements of Au 22 –PyB 18 explicitly reveals three main decay components of 220 fs, 3.5 ps, and 160 ps that can be assigned to energy migration between pyrenes and energy transfer processes from pyrene monomer and excimer to the central Au 22 , respectively.

14 SOLAR ENERGY↗

Assessing concurrent effects of climate change on hydropower supply, electricity demand, and greenhouse gas emissions in the Upper Yangtze River Basin of China

Hydropower importantly provides flexible low-carbon electricity, however, climate change will affect the hydropower system through altering hydrologic regimes while also affecting electricity demands for heating and cooling that hydropower resources serve. This study assesses the effect of climate change on hydropower and electricity demand in the Upper Yangtze River Basin (UYRB) in China on the regional net electric load and greenhouse gas (GHG) emissions. This is accomplished by using climate projections from five global climate models (GCMs) to simultaneously force (1) a physically-based hydrological model and a statistically-based hydropower model to estimate the future generating capacity of 21 large hydropower plants in the UYRB and (2) an empirical electricity demand model accounting for socioeconomic and climatic factors. Under climate change, the projected hydropower generation in the UYRB tends to increase in the 21st century but is far less than the increase in electricity demand, increasing the gap between demand and supply. Future increases in overall electricity demand are driven by GDP growth, but climate change will alter the distribution of the seasonal electricity demand. Climate warming decreases electricity demand for heating in winter and increases electricity demand for cooling in summer, but ultimately increases demand. Meanwhile, there is an increasing mismatch between electricity demand and hydropower supply associated with inter- and intra-annual variations, owing to the temporal climate change and increase in compound climate extremes (droughts and heatwaves). Finally, meeting the gap between supply and demand due to climate change is estimated to contribute 79.0–184.6 and 50.6–316.2 MMT CO 2e /yr of additional GHG emissions by the mid and end of 21st century, respectively.

13 HYDRO ENERGY↗