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Zhujun Li

Publications and source records attributed to Zhujun Li.

Approximating the Lidar Ratio of Modeled Aerosol Species to Help Inform Lidar Ratio Selection for Marine Aerosols in the Forthcoming Version 5 CALIPSO Data Products

- After 16+ years, the NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission will soon retire. - Narrow window of opportunity exists to improve quality of CALIPSO aerosol retrievals by advancing knowledge of aerosol lidar ratios for different aerosol types; - For CALIOP, the elastic backscatter lidar aboard CALIPSO, an aerosol lidar ratio (i.e., extinction-to-backscatter ratio) is generally assumed to retrieve vertical profiles of aerosol extinction and subsequently column-integrated aerosol optical depth (AOD). - Current CALIPSO lidar ratio selection process uses a single lidar ratio for each of the 7 CALIPSO tropospheric aerosol types, with large uncertainties for most aerosol types. Goal of this study: creation of regional and seasonal climatological lidar ratio maps for marine aerosols by leveraging passive aerosol retrievals (MODIS) and global model simulations (GEOS/GOGART).

Travis D Toth↗

Regional Energy Budget Over Ocean Derived From Satellite Observations

The uncertainty in regional surface energy flux derived by summing all energy flux components is known to be large. In addition, quantifying the regional energy flux uncertainty considering all flux component uncertainties is very difficult. However, this approach is needed to understand regional energy flux components and how these components change with time. The CERES surface radiation budget data product, Edition 4.1 EBAF combined with reanalysis products was used to assess regional surface energy budget over ocean in earlier studies. The CERES team revised the data product and released Edition 4.2 EBAF product in February 2023. Prominent differences from the earlier edition are: 1) no geostationary satellite derived cloud properties are used for surface irradiance computations and 2) MERRA-2 provides temperature and humidity profiles. Combined with surface turbulent fluxes from various products, this study uses the revised EBAF surface irradiances and addresses regional energy budget over ocean. In addition, the uncertainty in regional surface radiation and energy budgets is discussed.

Seiji Kato↗

Creating Seasonal Climatologies of Aerosol Lidar Ratios Over Ocean Using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The current CALIPSO algorithms assign one lidar ratio (i.e., extinction-to-backscatter ratio; LR) value globally for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms through the development of regional and seasonal LR climatologies. In this work, aerosol LRs are inferred through CALIOP backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type (e.g., marine). The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. In this poster, we show twelve-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine aerosols and how they correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). Near land masses, smaller SSVFs and larger LRs are found (due to the influence of over-land aerosols). In the remote ocean regions (likely less impacted by over-land aerosols), larger SSVFs and smaller LRs are found. The developed relationship between the GOCART model SSVFs and MODIS AOD constrained LRs is used to create model-assisted seasonal LR maps. Additionally, we show maps of inferred LRs from constrained retrievals using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) product and comparisons with those from the MODIS analyses. The technique demonstrated here benefits CALIPSO in the near-term, but similar methods can also be applied to the next generation space-based elastic backscatter lidars with collocated passive sensors, such as those of the upcoming NASA Atmosphere Observing System (AOS).

Travis Toth↗

Mapping Aerosol Lidar Ratios Over Ocean Using Constrained Retrievals and A Global Aerosol Model

The current NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) algorithms assign one lidar ratio (i.e., extinction-to-backscatter ratio; LR) value globally for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms through the development of regional and seasonal LR climatologies. In this work, aerosol LRs are inferred through Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type (e.g., marine). The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. In this presentation, we show that the twelve-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine aerosols correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). For example, smaller SSVFs (< 65%) and larger LRs (> 55 sr), are found near land masses. This is indicative of the influence of over-land aerosols (e.g., pollution and biomass burning smoke). In the remote oceans (i.e., regions likely less impacted by non-sea salt aerosols), larger SSVFs (> 95%) and smaller LRs (< 25 sr) are found. The developed relationship between the GOCART SSVFs and MODIS AOD constrained LRs (polynomial fit intersect values of ~56 sr for SSVF of 0% and ~21 sr for SSVF of 100%) is used to produce model-assisted climatological LR maps on seasonal scales. Additionally, we show maps of inferred LRs from constrained retrievals using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) product and comparisons with those from the MODIS analyses. The technique demonstrated in this study not only benefits CALIPSO in the near-term, but similar methods can be applied to future spaceborne elastic backscatter lidars with collocated passive sensors, such as those associated with the upcoming NASA Atmosphere Observing System (AOS).

Travis Toth↗

Creating Regional and Seasonal Climatologies of Marine and Dusty Marine Aerosol Lidar Ratios using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The CALIPSO aerosol algorithms currently assign one lidar ratio (LR) value globally for each of the seven tropospheric aerosol types. In this study, MODIS total column aerosol optical depths (AODs) are used to constrain collocated CALIOP backscatter profiles in a Fernald inversion that infers aerosol LRs for CALIOP-classified marine and dusty marine aerosols. The GOCART aerosol model is leveraged to estimate the sea salt volume fractions (SSVFs) that are collocated with the CALIOP+MODIS LR retrievals. An inverse empirical relationship is found between the SSVFs and LRs (i.e., smaller SSVFs and larger LRs near coastlines, but the opposite in the remote oceans). This SSVF/LR relationship is applied to create regional and seasonal hybrid (i.e., retrieval & model-assisted) climatological LR maps so as to develop more robust LR selections for marine and dusty marine aerosols in the CALIPSO algorithms. These analyses also provide critical LR information for the next generation of spaceborne elastic backscatter lidars.

Travis D. Toth↗

Creating Regional and Seasonal Climatologies of Marine and Dusty Marine Aerosol Lidar Ratios using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The CALIPSO aerosol algorithms currently assign one lidar ratio (LR) value globally for each of the seven tropospheric aerosol types. In this study, MODIS total column aerosol optical depths (AODs) are used to constrain collocated CALIOP backscatter profiles in a Fernald inversion that infers aerosol LRs for CALIOP-classified marine and dusty marine aerosols. The GOCART aerosol model is leveraged to estimate the sea salt volume fractions (SSVFs) that are collocated with the CALIOP+MODIS LR retrievals. An inverse empirical relationship is found between the SSVFs and LRs (i.e., smaller SSVFs and larger LRs near coastlines, but the opposite in the remote oceans). This SSVF/LR relationship is applied to create regional and seasonal hybrid (i.e., retrieval & model-assisted) climatological LR maps so as to develop more robust LR selections for marine and dusty marine aerosols in the CALIPSO algorithms. These analyses also provide critical LR information for the next generation of spaceborne elastic backscatter lidars.

Travis D. Toth↗

Mapping Aerosol Lidar Ratios Over Ocean using MODIS AOD Constrained Retrievals and GOCART Model Simulations

After 17 years, the NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission ceased science operations in August 2023. For the final CALIPSO data products release (Version 5), the CALIPSO project seeks to improve the accuracy of its aerosol extinction by advancing knowledge of aerosol lidar ratios (i.e., extinction-to-backscatter ratios; LRs) for various aerosol types. The current algorithm assigns one LR value globally for each of the seven tropospheric aerosol types. The CALIPSO team aims to improve the retrieval algorithm through the development of regional and seasonal LR climatologies for the same aerosol types. In this study, aerosol LRs are inferred through Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data over oceans during daytime. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type. The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. This presentation will reveal findings that the 12-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine and dusty marine aerosols correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). For example, smaller SSVFs (< 65%) and larger LRs (> 55 sr), are found near land masses (Fig. 1). This indicates the influence of advected anthropogenic aerosols (e.g., pollution and biomass burning smoke). In the remote oceans (i.e., regions likely less impacted by non-sea salt aerosols), the SSVFs are larger (> 95%) and the LRs are smaller (< 25 sr) (Fig. 1). A polynomial fit of the MODIS AOD constrained LRs to the corresponding GOCART SSVFs (intersect values of ~58 sr for SSVF of 0% and ~21 sr for SSVF of 100%) is further used to produce model-assisted climatological LR maps on seasonal scales. Additionally, we will show results of a LR validation analysis for which we compare the revised CALIPSO AODs obtained by applying the seasonal/regional constrained LRs against CALIPSO Version 4.51 Ocean Derived Column Optical Depth (ODCOD). While the majority of the presentation will focus on LRs for CALIOP-classified marine and dusty marine aerosols, an overview of LR results will show preliminary results for other aerosol types over ocean, such as dust and elevated smoke. The technique demon-strated in this study highlights the benefits not only to the final planned CALIPSO data release in 2025, but similar methods can be applied to future spaceborne elastic backscatter lidars with collocated passive sensors (e.g., such as those associated with NASA’s proposed Atmosphere Observing System).

Travis D Toth↗

Variable Lidar Ratios for Marine and Dusty Marine Using MODIS AOD Constrained Retrievals and GOCART Model Simulations and their Impact on Level 2 CALIPSO Data Products in Version 5

The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard CALIPSO provided global measurements of attenuated backscatter profiles of various tropospheric aerosol species from June 2006 through June 2023. Extinction profiles are retrieved from these backscatter measurements by assuming a value for the extinction-to-backscatter or lidar ratio (LR). Up until version V4.51 of the data products, only a constant global value for each of the species has been used, spatially and temporally. However, it has been well known from various ground-based measurements that LRs of each aerosol species can potentially vary spatially as well seasonally. For the forthcoming Version 5 of the CALIPSO products, the CALIPSO team will implement variable lidar ratios at 532 nm for the species classified as “marine” and “dusty marine”. Here we present the essential elements of this scheme, which involves estimating lidar ratios by constraining Fernald solutions for the CALIOP particulate backscatter profiles using aerosol optical depths (AOD) from collocated MODIS retrievals. To account for the lack of measurements in various regions and seasons (e.g., Arctic winters), we leverage collocated model sea-salt volume fractions (SSVF) simulated by the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model and use an empirical relationship between the SSVF and LR to build hybrid climatological maps for the entire globe, i.e., using the modelled values when reliable values of the constrained LRs are not available. Initial evaluation of the resulting extinction profiles and corresponding AODs, both globally and in specific regions are presented using a limited amount of data. The primary improvement in AOD occurs in the coastal areas, like the Arabian Sea and Bay of Bengal. The estimated marine LR values in these regions are significantly higher than the constant value of 23 sr used in previous data releases, likely due to mixing with offshore pollution which results in higher AODs. Initial validation results using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) retrievals and ground-based AERONET AOD measurements are presented.

CALIPSO↗