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NASA NTRS · 20060042861

Advanced radioisotope power systems technology development at JPL

Caillat, T.·Sakamato, J.·Jewell, A.·Cheng, J.·Paik, J.·Gascoin, F.·Snyder, J.·Blair, R.·Huang, C. -K.·Fleurial, J. -P.
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Caillat, T., Sakamato, J., Jewell, A., Cheng, J., Paik, J., Gascoin, F., Snyder, J., Blair, R., Huang, C. -K., Fleurial, J. -P.. 2005-06-01. Advanced radioisotope power systems technology development at JPL. https://ntrs.nasa.gov/citations/20060042861

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A review of melt preparation techniques is presented covering necessary phase relationships, synthesis/alloying and crystal growth of thermoelectric materials. The processes described require the knowledge of composition-temperature or composition- temperature-pressure phase diagrams. This knowledge enables the selection of the appropriate method of preparation, apparatus design and processing. The materials, from a technological point of view, will be roughly divided into three categories: low temperature materials (group V chalcogenides based on Bi2Te3), middle temperature materials (group IV chalcogenides based on PbTe) and high temperature materials (Si-Ge solid solutions). All known methods of preparation from melts are described, and a comparative analysis is given. (complete abstract)

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