DOE OSTI · 1008336
Imaging Nonequilibrium Atomic Vibrations with X-ray Diffuse Scattering
Abstract
We use picosecond x-ray diffuse scattering to image the nonequilibrium vibrations of the lattice following ultrafast laser excitation. We present images of nonequilibrium phonons in InP and InSb throughout the Brillouin-zone which remain out of equilibrium up to nanoseconds. The results are analyzed using a Born model that helps identify the phonon branches contributing to the observed features in the time-resolved diffuse scattering. In InP this analysis shows a delayed increase in the transverse acoustic (TA) phonon population along high-symmetry directions accompanied by a decrease in the longitudinal acoustic (LA) phonons. In InSb the increase in TA phonon population is less directional.
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Trigo, M., Chen, J., Vishwanath, V. H., Sheu, Y. M., Graber, T., Henning, R., Reis, D. 2011-03-03. Imaging Nonequilibrium Atomic Vibrations with X-ray Diffuse Scattering. https://www.osti.gov/biblio/1008336
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