Search NASA⌕ Search

DOE OSTI · 1358027

Nuclear Data Sheets for A=189

Abstract

Evaluated experimental data are presented for 13 known mass 189 nuclides (Hf, Ta, W, Re, Os, Ir, Pt, Au, Hg, Tl, Pb, Bi, Po). Since the 2003Wu02 publication, structure and decay data from 25 new and primary publications have been incorporated in the current work, while adding a new 189 Hf nuclide. New data have been added for all nuclides except 189 Au and 189 Hg. Moreover, several previous datasets were modified for β-decay Q values and conversion coefficients even when no new publications appeared since 2003Wu02. In spite of large amounts of data available for A=189 nuclides, several deficiencies remain, which are pointed out below in the hope that further experimental work may improve our knowledge of structure of these nuclides. For 189 Hf and 189 Ta, ground-state half-lives, and their decay schemes are unknown. An isomer in 189 Ta has recently been established but its decay characteristics are unknown, even though several gamma rays were connected with its decay. No excited states are known in 189 W and only one in 189 Po. The decay scheme of 189 W is known poorly with most gamma rays left as unassigned. The decay schemes of 189 Au and 189 Pb g.s. suffer from incompleteness, while those for the g.s. and isomer of 189 Tl are almost absent. The decay schemes of g.s. and isomer of 189 Hg are very complex as apparent from the study by 1996Wo04. Evaluators feel that these two decay schemes could be improved with modern gamma-ray detector arrays. While several isomers are known in many of the A=189 nuclides, there is in general lack of information of level half-lives, thus limiting the knowledge of transition probabilities. High-spin structures, including SD bands in 189 Hg and 189 Tl, are known in 189 Re, 189 Ir, 189 Pt, 189 Au, 189 Hg, 189 Tl, 189 Pb and 189 Bi. Single-particle transfer data are available for 189 Re, 189 Os, and 189 Pt; and two-neutron transfer data for 189 Ir.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Johnson, T. D., Singh, Balraj. 2017-04-26. Nuclear Data Sheets for A=189. https://doi.org/10.1016/j.nds.2017.04.001

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related reports

Design-informed neutronics assessment of long-lived fission product transmutation in a tokamak fusion reactor blanket

This study presents a neutronics-based assessment of the feasibility and viability of transmuting six major long-lived fission products (LLFPs) from light-water reactors, namely 99 Tc, 129 I, 79 Se, 93 Zr, 126 Sn, and 135 Cs, within the blanket region of a tokamak fusion reactor, using the MIT ARC design as a concrete fusion configuration. Monte Carlo neutronics simulations were performed to evaluate LLFP transmutation and to compare the results with a reference boiling water reactor (BWR). The results indicate that transmutation of all six LLFPs is neutronics-feasible in fusion reactors, with transmutation half-lives significantly shorter than their natural decay half-lives. For elemental targets, transmutation of 135 Cs, 126 Sn, and 93 Zr was found potentially viable, as the net mass transmuted exceeded that achievable in the reference BWR under identical target volume and irradiation time. When isotopically separated targets were considered, transmutation of 126 Sn and 93 Zr appeared potentially viable. A parametric study demonstrated that plasma geometry modifications can enhance local neutron flux, increasing the transmuted 93 Zr mass by approximately 33% and reducing the transmutation half-life from approximately 240 years to 180 years. Repositioning the target and adjusting material layer thickness reduced the transmutation half-life of 93 Zr to 67 years and increased the net mass transmuted by a factor of 50. Furthermore, these results demonstrate that fusion reactors can enable LLFP transmutation beyond the practical limits of thermal fission reactors and highlight the critical role of reactor and blanket design optimization. Engineering and fuel-cycle considerations required for deployment are beyond the scope of this neutronics-focused study.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A hybrid Monte Carlo-deterministic second moment method with efficient variance reduction

In this work, we present a hybrid method that combines Monte Carlo with deterministic finite element methods to solve a linear Boltzmann transport equation. Our hybrid method runs orders of magnitude faster than Monte Carlo, without sacrificing accuracy, for a proxy problem from radiative transfer that contains both optically-thick and optically-thin material. We believe that this is the first demonstration of a hybrid Second Moment Method in more than one spatial dimension, the first to consider more than one material, and the first to use variance reduction. Our variance reduction approach arises from an asymptotic analysis in which we show that the magnitude of the scattering source grows without bound. We transform the problem to compute the deviation of the radiation intensity from isotropy. The magnitude of the source in the transformed problem is bounded, and the quality of the hybrid method solution is dramatically improved by a substantial reduction in the variance.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗