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DOE OSTI · 1800016

Topological nanospaser

Abstract

We propose a nanospaser made of an achiral plasmonic–metal nanodisk and a two-dimensional chiral gain medium – a monolayer nanoflake of a transition-metal dichalcogenide (TMDC). When one valley of the TMDC is selectively pumped (e.g. by a circular-polarized radiation), the spaser (surface plasmon amplification by stimulated emission of radiation) generates a mode carrying a topological chiral charge that matches that of the gain valley. There is another, chirally mismatched, time-reversed mode with exactly the same frequency but the opposite topological charge; it is actively suppressed by the gain saturation and never generates, leading to a strong topological protection for the generating matched mode. This topological spaser is promising for use in nano-optics and nanospectroscopy in the near field especially in applications to biomolecules that are typically chiral. Another potential application is a chiral nanolabel for biomedical applications emitting in the far field an intense circularly polarized coherent radiation.

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BibTeXRIS

Ghimire, Rupesh, Wu, Jhih-Sheng, Apalkov, Vadym, Stockman, Mark I.. 2020-03-19. Topological nanospaser. https://doi.org/10.1515/nanoph-2019-0496

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36 MATERIALS SCIENCE↗