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DOE OSTI · 1800614

Phase-matching analysis in high-order harmonic generation with nonzero orbital angular momentum Laguerre-Gaussian beams

Jin, Cheng·Li, Baochang·Wang, Kan·Xu, Chenhui·Tang, Xiangyu·Yu, Chao·Lin, C. D.
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Abstract

Through high-order harmonic generation driven by intense ultrashort vortex infrared or midinfrared lasers, a nonzero orbital angular momentum can be imprinted onto extreme ultraviolet (XUV) or soft-x-ray (SXR) light pulses. Here we simulate the generation of vortex XUV harmonics in the gas medium as well as their propagation in vacuum till reaching the far field. In this work, we find that the intensity and phase of generated high harmonics are very sensitive to the position of gas jet with respect to the laser focus. The topological charge of the $\textit{q}$th harmonic is found to be $\textit{q}$ times that of the driving Laguerre-Gaussian beam. Each harmonic in the far field appears as a single ring in the transverse plane with an invariant diameter which is scalable with the fundamental topological charge only when the gas jet is placed after the laser focus. The underlying phase-matching mechanism is analyzed by examining the spatial map of the coherence length and by calculating the evolution of harmonic emission in the medium. We anticipate this work to stimulate interest in generating intense vortex XUV or SXR attosecond pulses for probing dynamics of molecules where special molecular features are difficult to be detected with linear or circular XUV or SXR pulses.

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Jin, Cheng, Li, Baochang, Wang, Kan, Xu, Chenhui, Tang, Xiangyu, Yu, Chao, Lin, C. D.. 2020-09-25. Phase-matching analysis in high-order harmonic generation with nonzero orbital angular momentum Laguerre-Gaussian beams. https://doi.org/10.1103/physreva.102.033113

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