DOE OSTI · 1809065
Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy
Abstract
We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.
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Sun, Yanwen, Carini, Gabriella, Chollet, Matthieu, Decker, Franz-Josef, Dunne, Mike, Fuoss, Paul, Hruszkewycz, Stephan O., Lane, Thomas J., Nakahara, Kazutaka, Nelson, Silke, Robert, Aymeric, Sato, Takahiro, Song, Sanghoon, Stephenson, G. Brian, Sutton, Mark, Van Driel, Tim B., Weninger, Clemens, Zhu, Diling. 2021-07-28. Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy. https://doi.org/10.1103/physrevlett.127.058001
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