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DOE OSTI · 2283359

Manipulating Interlayer Excitons for Near-Infrared Quantum Light Generation

Zhao, Huan·Zhu, Linghan·Li, Xiangzhi·Chandrasekaran, Vigneshwaran·Baldwin, Scott Jon Kevin·Pettes, Michael Thompson·Piryatinski, Andrei·Yang, Li·Htoon, Han
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Abstract

Interlayer excitons (IXs) formed at the interface of van der Waals materials possess various novel properties. In parallel development, strain engineering has emerged as an effective means for creating 2D quantum emitters. Here, exploring the intersection of these two exciting areas, we use MoS2/WSe2 heterostructure as a model system and demonstrate how strain, defects, and layering can be utilized to create defect-bound IXs capable of bright, robust, and tunable quantum light emission in the technologically important near-infrared spectral range. Our work presents defect-bound IXs as a promising platform for pushing the performance of 2D quantum emitters beyond their current limitations.

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2D heterostructures77 NANOSCIENCE AND NANOTECHNOLOGYTMDCdefectsexcitonsheterostructuresinterlayer excitonlayered materialslayersquantum emitters

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BibTeXRIS

Zhao, Huan, Zhu, Linghan, Li, Xiangzhi, Chandrasekaran, Vigneshwaran, Baldwin, Scott Jon Kevin, Pettes, Michael Thompson, Piryatinski, Andrei, Yang, Li, Htoon, Han. 2023-12-01. Manipulating Interlayer Excitons for Near-Infrared Quantum Light Generation. https://doi.org/10.1021/acs.nanolett.3c03296

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