DOE OSTI · 2497861
Li 1.6 AlCl 3.4 S 0.6 : a low-cost and high-performance solid electrolyte for solid-state batteries
Abstract
The Cl–S mixed-anion sublattice of Li 1.6 AlCl 3.4 S 0.6 creates face- and edge-shared octahedra that connect to form 3D ion conduction pathways with low activation energy barriers.
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Poudel, Tej P. [Materials Science and Engineering Program, The Graduate School, Florida State University, 2005 Levy Ave., Tallahassee, FL 32310, USA, Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000347875739), Oyekunle, Ifeoluwa P. [Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000176234493), Deck, Michael J. [Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000164398634), Chen, Yudan [Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000314954289), Hou, Dewen [Center for Nanoscale Materials, Argonne National Laboratory, 9700 S Cass Ave, Lemont, IL 60439, USA] (ORCID:0009000687796559), Ojha, Pawan K. [Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000315030029), Ogbolu, Bright O. [Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0009000125822233), Huang, Chen [Materials Science and Engineering Program, The Graduate School, Florida State University, 2005 Levy Ave., Tallahassee, FL 32310, USA, Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA] (ORCID:0000000329348118), Xiong, Hui [Micron School of Materials Science and Engineering, Boise State University, Boise, ID, 83725, USA] (ORCID:0000000331261476), Hu, Yan-Yan [Materials Science and Engineering Program, The Graduate School, Florida State University, 2005 Levy Ave., Tallahassee, FL 32310, USA, Department of Chemistry and Biochemistry, Florida State University, 95 Chieftan Way, Tallahassee, FL 32306, USA, Center of Interdisciplinary Magnetic Resonance, National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, FL 32310, USA] (ORCID:0000000306775897). 2025-01-01. Li 1.6 AlCl 3.4 S 0.6 : a low-cost and high-performance solid electrolyte for solid-state batteries. https://doi.org/10.1039/d4sc07151d
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