Ballistic ion transport through hierarchically-ordered-structure polymer binder

Li, Defu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]; Fang, Chen [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000321011991); Thapa, Santosh [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA]; Sternlicht, Hadas [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA]; Lee, Gi-Hyeok [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]; Ahmed, Faiz [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]; Jin, Xiuyu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000178452371); Miao, Qiusu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, College of Chemistry, University of California, Berkeley, CA, USA]; Giovine, Raynald [College of Chemistry Pines Magnetic Resonance Center – Core Facility, University of California, Berkeley, CA, USA]; Yang, Wanli [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000306668063); Minor, Andrew [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA]; Cheng, Yang-Tse [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA, Department of Chemical and Material engineering, University of Kentucky, Lexington, KY, USA]; Liu, Gao [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000168860507)

doi:10.1039/d4ee06071g

DOE OSTI · 2557561

Ballistic ion transport through hierarchically-ordered-structure polymer binder

Li, Defu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]·Fang, Chen [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000321011991)·Thapa, Santosh [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA]·Sternlicht, Hadas [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA]·Lee, Gi-Hyeok [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]·Ahmed, Faiz [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA]·Jin, Xiuyu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000178452371)·Miao, Qiusu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, College of Chemistry, University of California, Berkeley, CA, USA]·Giovine, Raynald [College of Chemistry Pines Magnetic Resonance Center – Core Facility, University of California, Berkeley, CA, USA]·Yang, Wanli [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000306668063)·Minor, Andrew [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA]·Cheng, Yang-Tse [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA, Department of Chemical and Material engineering, University of Kentucky, Lexington, KY, USA]·Liu, Gao [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000168860507)

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Abstract

Achieving ballistic ion transport in a mixed electronic-ionic conductive polymer, its hierarchically ordered structure (HOS) facilitates ion diffusion and results in solid-state Li + conductivity in the range of 10 −4 to 10 −3 S cm −1 from −20 to 70 °C.

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Li, Defu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA], Fang, Chen [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000321011991), Thapa, Santosh [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA], Sternlicht, Hadas [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA], Lee, Gi-Hyeok [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA], Ahmed, Faiz [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA], Jin, Xiuyu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000178452371), Miao, Qiusu [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, College of Chemistry, University of California, Berkeley, CA, USA], Giovine, Raynald [College of Chemistry Pines Magnetic Resonance Center – Core Facility, University of California, Berkeley, CA, USA], Yang, Wanli [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000306668063), Minor, Andrew [National Center for Electron Microscopy, The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, Department of Materials Science and Engineering, University of California, Berkeley, CA, USA], Cheng, Yang-Tse [Department of Physics and Astronomy, University of Kentucky, Lexington, KY, USA, Department of Chemical and Material engineering, University of Kentucky, Lexington, KY, USA], Liu, Gao [Energy storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA] (ORCID:0000000168860507). 2025-01-01. Ballistic ion transport through hierarchically-ordered-structure polymer binder. https://doi.org/10.1039/d4ee06071g

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