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DOE OSTI · 2565633

Nanoscale engineering and dynamic stabilization of mesoscopic spin textures

Harkins, Kieren [University of California, Berkeley, CA (United States)] (ORCID:0009000835926782)·Fleckenstein, Christoph [KTH Royal Inst. of Technology, Stockholm (Sweden)]·D’Souza, Noella [University of California, Berkeley, CA (United States)] (ORCID:0009000175244726)·Schindler, Paul M. [Max Planck Society, Dresden (Germany). Max Planck Inst. for the Physics of Complex Systems] (ORCID:0000000309735444)·Marchiori, David [University of California, Berkeley, CA (United States)] (ORCID:0000000197383674)·Artiaco, Claudia [KTH Royal Inst. of Technology, Stockholm (Sweden)] (ORCID:0000000201411878)·Reynard-Feytis, Quentin [University of California, Berkeley, CA (United States)] (ORCID:0000000173351491)·Basumallick, Ushoshi [University of California, Berkeley, CA (United States)]·Beatrez, William [University of California, Berkeley, CA (United States)] (ORCID:0000000240719402)·Pillai, Arjun [University of California, Berkeley, CA (United States)] (ORCID:0000000295001887)·Hagn, Matthias [University of California, Berkeley, CA (United States)] (ORCID:0009000701324436)·Nayak, Aniruddha [University of California, Berkeley, CA (United States)] (ORCID:000000034407803X)·Breuer, Samantha [University of California, Berkeley, CA (United States)]·Lv, Xudong [University of California, Berkeley, CA (United States); California Institute of Technology (CalTech), Pasadena, CA (United States)] (ORCID:0000000256013789)·McAllister, Maxwell [University of California, Berkeley, CA (United States)] (ORCID:0000000213335198)·Reshetikhin, Paul [University of California, Berkeley, CA (United States)] (ORCID:0000000322367359)·Druga, Emanuel [University of California, Berkeley, CA (United States)]·Bukov, Marin [Max Planck Society, Dresden (Germany). Max Planck Inst. for the Physics of Complex Systems] (ORCID:0000000236889599)·Ajoy, Ashok [University of California, Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); CIFAR Azrieli Global Scholars Program (Canada)] (ORCID:0000000332422913)

Abstract

Thermalization, while ubiquitous in physics, has traditionally been viewed as an obstacle to be mitigated. In contrast, we demonstrate here the use of thermalization in the generation, control, and readout of “shell-like” spin textures with interacting 13 C nuclear spins in diamond, wherein spins are polarized oppositely on either side of a critical radius. The textures span several nanometers and encompass many hundred spins; they are created and interrogated without manipulating the nuclear spins individually. Long-time stabilization is achieved via prethermalization to a Floquet-engineered Hamiltonian under the electronic gradient field: The texture is therefore metastable and robust against spin diffusion. This enables the state to endure over multiple minutes before it decays. Our work on spin-state engineering paves the way for applications in quantum simulation and nanoscale imaging.

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BibTeXRIS

Harkins, Kieren [University of California, Berkeley, CA (United States)] (ORCID:0009000835926782), Fleckenstein, Christoph [KTH Royal Inst. of Technology, Stockholm (Sweden)], D’Souza, Noella [University of California, Berkeley, CA (United States)] (ORCID:0009000175244726), Schindler, Paul M. [Max Planck Society, Dresden (Germany). Max Planck Inst. for the Physics of Complex Systems] (ORCID:0000000309735444), Marchiori, David [University of California, Berkeley, CA (United States)] (ORCID:0000000197383674), Artiaco, Claudia [KTH Royal Inst. of Technology, Stockholm (Sweden)] (ORCID:0000000201411878), Reynard-Feytis, Quentin [University of California, Berkeley, CA (United States)] (ORCID:0000000173351491), Basumallick, Ushoshi [University of California, Berkeley, CA (United States)], Beatrez, William [University of California, Berkeley, CA (United States)] (ORCID:0000000240719402), Pillai, Arjun [University of California, Berkeley, CA (United States)] (ORCID:0000000295001887), Hagn, Matthias [University of California, Berkeley, CA (United States)] (ORCID:0009000701324436), Nayak, Aniruddha [University of California, Berkeley, CA (United States)] (ORCID:000000034407803X), Breuer, Samantha [University of California, Berkeley, CA (United States)], Lv, Xudong [University of California, Berkeley, CA (United States); California Institute of Technology (CalTech), Pasadena, CA (United States)] (ORCID:0000000256013789), McAllister, Maxwell [University of California, Berkeley, CA (United States)] (ORCID:0000000213335198), Reshetikhin, Paul [University of California, Berkeley, CA (United States)] (ORCID:0000000322367359), Druga, Emanuel [University of California, Berkeley, CA (United States)], Bukov, Marin [Max Planck Society, Dresden (Germany). Max Planck Inst. for the Physics of Complex Systems] (ORCID:0000000236889599), Ajoy, Ashok [University of California, Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); CIFAR Azrieli Global Scholars Program (Canada)] (ORCID:0000000332422913). 2025-03-28. Nanoscale engineering and dynamic stabilization of mesoscopic spin textures. https://doi.org/10.1126/sciadv.adn9021

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