DOE OSTI · 2566007
How does an antisolvent additive affect all interfaces in aqueous Zn–MnO 2 batteries?
Abstract
Low levels of acetonitrile (0.5–2 vol%) have the lowest nucleation, growth, and stripping overpotentials at the Zn anode and highest δ-MnO 2 phase reversibility at cathode suggesting a balance between suppressed conversion and retained Zn 2+ mobility.
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Counihan, Michael J. [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Material Science Division, Argonne National Laboratory, Lemont, Illinois 60439, USA], Roberts, Lacey [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Department of Chemical and Biological Engineering, Materials Science and Engineering Program, Renewable and Sustainable Energy Institute (RASEI), University of Colorado Boulder, Boulder, Colorado 80309, USA], Ilic, Stefan [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Material Science Division, Argonne National Laboratory, Lemont, Illinois 60439, USA], Yang, Yingjie [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Department of Physics, University of Illinois at Chicago, Chicago, Illinois 60607, USA] (ORCID:0000000218988171), Ely, Claire [Department of Chemical and Biological Engineering, Materials Science and Engineering Program, Renewable and Sustainable Energy Institute (RASEI), University of Colorado Boulder, Boulder, Colorado 80309, USA], Klie, Robert F. [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Department of Physics, University of Illinois at Chicago, Chicago, Illinois 60607, USA] (ORCID:0000000347736667), Toney, Michael F. [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Department of Chemical and Biological Engineering, Materials Science and Engineering Program, Renewable and Sustainable Energy Institute (RASEI), University of Colorado Boulder, Boulder, Colorado 80309, USA] (ORCID:0000000275131166), Tepavcevic, Sanja [Joint Center for Energy Storage Research, Argonne National Laboratory, Lemont, Illinois 60439, USA, Material Science Division, Argonne National Laboratory, Lemont, Illinois 60439, USA] (ORCID:0000000301518832). 2025-01-01. How does an antisolvent additive affect all interfaces in aqueous Zn–MnO 2 batteries?. https://doi.org/10.1039/d5ta00951k
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