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DOE OSTI · 2566430

Next-generation neutron detection using a 6 Li glass scintillator composite

Favalli, Andrea [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); European Commission, Ispra (Italy). Joint Research Centre (JRC)] (ORCID:0000000229161700)·Wiggins, Brenden W. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·Iliev, Metodi [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·Richards, Cameron G. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·Ogren, Kristofer [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·McLean, Thomas D. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·Ianakiev, Kiril D. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]·Hehlen, Markus P. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)] (ORCID:0000000259207108)
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Abstract

Neutron detectors are crucial in fundamental science, nuclear security, safeguards, and civil applications. 3 He-filled gas proportional counters are the gold standard for thermal neutron detection, prized for their efficiency, neutron/gamma discrimination, and stability; however, the scarcity of 3 He has prompted the search for alternatives. Here, we introduce a neutron detector design based on a scintillating composite consisting of 6 Li glass scintillator particles dispersed in an organic matrix. A detector consisting of this scintillating composite, photomultiplier tubes (PMTs) for optical detection, and electronics for reading out the PMT signal in both pulse and current modes was prototyped and characterized using various neutron and gamma sources. The prototype achieves a measured intrinsic detection efficiency of 6.70 ± 0.01%, a die-away time of 10.3 ± 0.1 μs, a negligible gamma misidentification probability, and response linearity up to at least 3.7 × 10 6 incident neutrons/s established via a cross-calibration technique. This detector holds the potential to outperform traditional 3 He-gas-based neutron detection systems, offering a viable alternative amidst the ongoing 3 He shortage and promising advancements in neutron detection technology.

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BibTeXRIS

Favalli, Andrea [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); European Commission, Ispra (Italy). Joint Research Centre (JRC)] (ORCID:0000000229161700), Wiggins, Brenden W. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Iliev, Metodi [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Richards, Cameron G. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Ogren, Kristofer [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], McLean, Thomas D. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Ianakiev, Kiril D. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Hehlen, Markus P. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)] (ORCID:0000000259207108). 2025-01-04. Next-generation neutron detection using a 6 Li glass scintillator composite. https://doi.org/10.1038/s42005-024-01903-3

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