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DOE OSTI · 2574159

Active microrheology and dynamic phases for pattern-forming systems with competing interactions

Abstract

We consider the driven dynamics of a probe particle moving through an assembly of particles with competing long-range repulsive and short-range attractive interactions, which form crystal, stripe, labyrinth, and bubble states as the ratio of attraction to repulsion is varied. We show that the probe particle exhibits a depinning-like threshold from an elastic regime, where the probe particle is trapped by interactions with the other particles, to a plastic flow regime, where the probe particle can break bonds in the surrounding medium. For a fixed particle density, the depinning threshold and sliding velocity of the probe particle vary nonmonotonically as the attraction term is increased. A velocity minimum appears near the crystal to stripe crossover, and there is a significant increase in the depinning threshold in the bubble regime when the probe particle is strongly confined inside the bubbles. For fixed attractive interaction but increasing particle density, the behavior is also nonmonotonic, and there are jumps and drops in the velocity and depinning threshold corresponding to points at which the system transitions between different structures. There are also several distinct flow states that can be characterized by the amount of plastic deformation induced by the probe particle in the surrounding medium. Each flow state generates a different amount of effective drag on the probe particle, and there can be jumps in the velocity-force curve at transitions between the states. In conclusion, we also find that when oriented stripes are present, the probe particle can move along the stripe in an edge transport state that has a finite Hall angle.

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BibTeXRIS

Reichhardt, Charles [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)] (ORCID:000000020193189X), Reichhardt, Cynthia Jane O. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)] (ORCID:0000000234875089). 2025-05-19. Active microrheology and dynamic phases for pattern-forming systems with competing interactions. https://doi.org/10.1103/physreve.111.055406

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36 MATERIALS SCIENCE