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DOE OSTI · 2575383

Tunable atomically enhanced moiré Berry curvatures in twisted triple bilayer graphene

Abstract

We report a twisted triple bilayer graphene platform consisting of three units of Bernal bilayer graphene consecutively twisted at 1.49° and 1.68°. We demonstrate the atomic reconstruction between the two competing moiré superlattices strongly enhances the Berry curvature of each moiré band insulator state, characterized by measured strong nonlocal valley Hall effect that sensitively depends on the intermoiré competition strength, tunable by manipulating the out-of-plane carrier distribution. Our study sheds light on the microscopic mechanism of atomic and electronic reconstruction in twisted multilayer systems, by systematically investigating transport signatures of moiré Berry curvature and its enhancement from moiré-of-moiré lattice reconstruction. In conclusion, we show that the reconstructed electronic band can be versatilely tuned by electrostatics, providing an approach toward engineering the band structure and its topology for a quantum material platform with designer electrical and optical properties.

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BibTeXRIS

Davydov, Konstantin [Univ. of Minnesota, Minneapolis, MN (United States)] (ORCID:0009000827944411), Zhu, Ziyan [SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)] (ORCID:0000000344635828), Friedman, Noah [Univ. of Minnesota, Minneapolis, MN (United States)] (ORCID:0009000684360012), Gramowski, Ethan [Univ. of Minnesota, Minneapolis, MN (United States)], Li, Yaotian [Univ. of Minnesota, Minneapolis, MN (United States)], Tavakley, Jack [Univ. of Minnesota, Minneapolis, MN (United States)], Watanabe, Kenji [National Institute for Materials Science (NIMS), Tsukuba (Japan)] (ORCID:0000000337018119), Taniguchi, Takashi [National Institute for Materials Science (NIMS), Tsukuba (Japan)] (ORCID:0000000214673105), Luskin, Mitchell [Univ. of Minnesota, Minneapolis, MN (United States)] (ORCID:000000031981199X), Kaxiras, Efthimios [Harvard Univ., Cambridge, MA (United States)] (ORCID:0000000246820165), Wang, Ke [Univ. of Minnesota, Minneapolis, MN (United States)] (ORCID:0000000208954445). 2025-04-23. Tunable atomically enhanced moiré Berry curvatures in twisted triple bilayer graphene. https://doi.org/10.1103/physrevb.111.l161120

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