DOE OSTI · 2587415
Radiochronometric discordance in cast uranium metal: a multi-laboratory intercomparison exercise
Abstract
Here, the model age of a nuclear material is crucial in nuclear forensic analysis. Uranium metals with complex production histories often exhibit discordant model ages from the 230 Th– 234 U and 231 Pa– 235 U chronometers. Recent studies involving targeted uranium metal castings have enhanced our understanding of decay product behavior during casting, aiding nuclear forensic interpretation. Building on this prior work, forensics laboratories at Atomic Weapons Establishment (AWE), Lawrence Livermore National Laboratory (LLNL), and Los Alamos National Laboratory (LANL) conducted an interlaboratory comparison to investigate spatial heterogeneity in uranium metal cast under controlled conditions. Each laboratory measured samples of a mixed feedstock and its corresponding cast product. This work furthers our understanding of discordant model ages and the use of discordance as a signature to enhance confidence in interpretations of radiochronometric data for nuclear forensics.
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Higginson, Matthew A. [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)] (ORCID:0009000766422256), Chen, Christine Yifeng [Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)], Denton, Joanna S. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Steiner, Robert E. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Ainge, Alexander [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Cross, Sam [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Cocciadiferro, Ashley [Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)], Dunne, James A. [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Edwards, Mark A. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Engel, John [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Gaffney, Amy M. [Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)], Gilligan, Chris R. D. [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Johnson, Adelicia [Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)], Kaye, Philip [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Kayzar-Boggs, Theresa M. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], LaMont, Stephen P. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Rice, Natalie T. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Sanborn, Matthew E. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)], Shilling, Alice [Atomic Weapons Establishment (AWE), Berkshire (United Kingdom)], Wende, Allison M. [Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)]. 2025-08-19. Radiochronometric discordance in cast uranium metal: a multi-laboratory intercomparison exercise. https://doi.org/10.1007/s10967-025-10311-y
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