DOE OSTI · 3006318
X-ray thermal diffuse scattering as a texture-robust temperature diagnostic for dynamically compressed solids
Abstract
We present a model of x-ray thermal diffuse scattering (TDS) from a cubic polycrystal with an arbitrary crystallographic texture, based on the classic approach of Warren [B. E. Warren, Acta Crystallogr. 6, 803 (1953)]. We compare the predictions of our model with femtosecond x-ray diffraction patterns gathered from ambient and dynamically compressed rolled copper foils obtained at the High Energy Density instrument of the European X-Ray Free-Electron Laser facility and find that the texture-aware TDS model yields more accurate results than does the conventional powder model owed to Warren. Nevertheless, we further show: with sufficient angular detector coverage, the TDS signal is largely unchanged by sample orientation and in all cases strongly resembles the signal from a perfectly random powder; shot-to-shot fluctuations in the TDS signal resulting from grain-sampling statistics are at the percent level, in stark contrast to the fluctuations in the Bragg-peak intensities (which are over an order of magnitude greater); and TDS is largely unchanged even following texture evolution caused by compression-induced plastic deformation. We conclude that TDS is robust against texture variation, making it a flexible temperature diagnostic applicable just as well to off-the-shelf commercial foils as to ideal powders.
Explore related subjects
Keep this discovery
Explore connections, maps & timelines
Heighway, P. G. [Univ. of Oxford (United Kingdom); et al.] (ORCID:0000000162210650), Peake, D. J. [Department of Physics, Clarendon Laboratory, University of Oxford 1 , Parks Road, Oxford OX1 3PU,] (ORCID:0000000259926954), Stevens, T. [Department of Physics, Clarendon Laboratory, University of Oxford 1 , Parks Road, Oxford OX1 3PU,] (ORCID:0009000683553509), Wark, J. S. [Department of Physics, Clarendon Laboratory, University of Oxford 1 , Parks Road, Oxford OX1 3PU,] (ORCID:0000000330553223), Albertazzi, B. [Ecole Polytechnique, Palaiseau, Laboratoire pour l’utilisation des lasers intenses (LULI), CNRS UMR 7605 2 , Route de Saclay, 91128 Palaiseau Cedex,], Ali, S. J. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000318233788), Antonelli, L. [School of Physics, Engineering and Technology, University of York 4 , Heslington, York YO10 5DD,] (ORCID:000000030694948X), Armstrong, M. R. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000323751491), Baehtz, C. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:000000031480511X), Ball, O. B. [SUPA, School of Physics and Astronomy, and Centre for Science at Extreme Conditions, The University of Edinburgh 6 , Edinburgh EH9 3FD,] (ORCID:0000000252150153), Banerjee, S. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:000000019407477X), Belonoshko, A. B. [Frontiers Science Center for Critical Earth Material Cycling, School of Earth Sciences and Engineering, Nanjing University 8 , Nanjing 210023,], Bolme, C. A. [Los Alamos National Laboratory 9 , Los Alamos, New Mexico 87545,] (ORCID:000000021880271X), Bouffetier, V. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000160791260), Briggs, R. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000345885802), Buakor, K. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000302572822), Butcher, T. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0009000309095982), Di Dio Cafiso, S. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,], Cerantola, V. [Dipartimento di Scienze dell’Ambiente e della Terra, Università degli Studi di Milano Bicocca 11 , Piazza della Scienza 1e4, I-20126 Milano,] (ORCID:0000000228082963), Chantel, J. [Univ. Lille, CNRS, INRAE, Centrale Lille, UMR 8207—UMET—Unité Matériaux et Transformations 12 , F-59000 Lille,] (ORCID:0000000283329033), Di Cicco, A. [School of Science and Technology—Physics Division, Università di Camerino 13 , 62032 Camerino,], Coleman, A. L. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000256924400), Collier, J. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0009000120030472), Collins, G. [Laboratory for Laser Energetics (LLE), University of Rochester 14 , 250 East River Road, Rochester, New York 14623-1299,] (ORCID:0000000154366866), Comley, A. J. [Atomic Weapons Establishment (AWE), Materials Science and Research Division (MSRD) 15 , Aldermaston, Berkshire RG7 4PR,] (ORCID:000900022580653X), Coppari, F. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000315923898), Cowan, T. E. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:000000025845000X), Cristoforetti, G. [CNR—Consiglio Nazionale delle Ricerche, Istituto Nazionale di Ottica, CNR—INO) 16 , Largo Enrico Fermi, 6, 50125 Firenze FI,] (ORCID:0000000194209080), Cynn, H. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000346585764), Descamps, A. [School of Mathematics and Physics, Queen’s University Belfast 17 , University Road, Belfast BT7 1NN,] (ORCID:0000000317086376), Dorchies, F. [Université de Bordeaux, CNRS, CEA, CELIA, UMR 5107 18 , F-33400 Talence,] (ORCID:0000000259229585), Duff, M. J. [SUPA, School of Physics and Astronomy, and Centre for Science at Extreme Conditions, The University of Edinburgh 6 , Edinburgh EH9 3FD,], Dwivedi, A. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0009000874970444), Edwards, C. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,], Eggert, J. H. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000157307108), Errandonea, D. [Departamento de Fisica Aplicada—ICMUV, Universidad de Valencia—UV 19 , C/Dr. Moliner 50 Burjassot, E-46100 Valencia,] (ORCID:0000000301894221), Fiquet, G. [Sorbonne Université, Muséum National d’Histoire Naturelle, UMR CNRS 7590, Insitut de Minéralogie, de Physique, des Matériaux, et de Cosmochinie, IMPMC 20 , Paris 75005,] (ORCID:0000000189613281), Galtier, E. [SLAC National Accelerator Laboratory 21 , 2575 Sand Hill Road, Menlo Park, California 94025,] (ORCID:000000020396285X), Laso Garcia, A. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0000000276710901), Ginestet, H. [Univ. Lille, CNRS, INRAE, Centrale Lille, UMR 8207—UMET—Unité Matériaux et Transformations 12 , F-59000 Lille,] (ORCID:0000000269314062), Gizzi, L. [CNR—Consiglio Nazionale delle Ricerche, Istituto Nazionale di Ottica (CNR—INO) 22 , Via G. Moruzzi, 1-56124 Pisa,] (ORCID:0000000165726492), Gleason, A. [SLAC National Accelerator Laboratory 21 , 2575 Sand Hill Road, Menlo Park, California 94025,] (ORCID:0000000277365118), Goede, S. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,], Gonzalez, J. M. [Department of Physics, University of South Florida 23 , Tampa, Florida 33620,] (ORCID:0000000170389726), Gorman, M. G. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000195676166), Harmand, M. [Sorbonne Université, Muséum National d’Histoire Naturelle, UMR CNRS 7590, Insitut de Minéralogie, de Physique, des Matériaux, et de Cosmochinie, IMPMC 20 , Paris 75005,; PIMM, Arts et Metiers Institute of Technology, CNRS, Cnam, HESAM University 24 , 151 boulevard de l’Hopital, 75013 Paris,] (ORCID:0000000307135824), Hartley, N. J. [SLAC National Accelerator Laboratory 21 , 2575 Sand Hill Road, Menlo Park, California 94025,] (ORCID:0000000262682436), Hernandez-Gomez, C. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0009000595461989), Higginbotham, A. [School of Physics, Engineering and Technology, University of York 4 , Heslington, York YO10 5DD,] (ORCID:0000000152119933), Höppner, H. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0009000019295097), Humphries, O. S. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000167480422), Husband, R. J. [Deutsches Elektronen-Synchrotron DESY 25 , Notkestr. 85, 22607 Hamburg,] (ORCID:000000027666401X), Hutchinson, T. M. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000318823702), Hwang, H. [Deutsches Elektronen-Synchrotron DESY 25 , Notkestr. 85, 22607 Hamburg,] (ORCID:0000000284983811), Keen, D. A. [ISIS Facility, STFC Rutherford Appleton Laboratory 26 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0000000303762767), Kim, J. [Department of Physics, Hanyang University 27 , 17 Haengdang dong, Seongdong gu, Seoul 133-791,] (ORCID:0000000317873775), Koester, P. [CNR—Consiglio Nazionale delle Ricerche, Istituto Nazionale di Ottica, CNR—INO) 16 , Largo Enrico Fermi, 6, 50125 Firenze FI,] (ORCID:0000000216174633), Konopkova, Z. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000189056307), Kraus, D. [Universität Rostock, Institut für Physik 28 , D-18051 Rostock,] (ORCID:0000000263504180), Krygier, A. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000161781195), Labate, L. [CNR—Consiglio Nazionale delle Ricerche, Istituto Nazionale di Ottica, CNR—INO) 16 , Largo Enrico Fermi, 6, 50125 Firenze FI,] (ORCID:0000000208044548), Lazicki, A. E. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,], Lee, Y. [Department of Earth System Sciences, Yonsei University 29 , 50 Yonsei-ro Seodaemun-gu, Seoul 03722,] (ORCID:0000000220430804), Liermann, H.-P. [Deutsches Elektronen-Synchrotron DESY 25 , Notkestr. 85, 22607 Hamburg,] (ORCID:0000000150391183), Mason, P. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0000000182409819), Masruri, M. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0000000225216241), Massani, B. [SUPA, School of Physics and Astronomy, and Centre for Science at Extreme Conditions, The University of Edinburgh 6 , Edinburgh EH9 3FD,] (ORCID:0000000258171780), McBride, E. E. [School of Mathematics and Physics, Queen’s University Belfast 17 , University Road, Belfast BT7 1NN,] (ORCID:0000000288216126), McGuire, C. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,], McHardy, J. D. [SUPA, School of Physics and Astronomy, and Centre for Science at Extreme Conditions, The University of Edinburgh 6 , Edinburgh EH9 3FD,] (ORCID:0000000226308092), McGonegle, D. [Atomic Weapons Establishment (AWE), Materials Science and Research Division (MSRD) 15 , Aldermaston, Berkshire RG7 4PR,] (ORCID:0000000153291081), McWilliams, R. S. [SUPA, School of Physics and Astronomy, and Centre for Science at Extreme Conditions, The University of Edinburgh 6 , Edinburgh EH9 3FD,] (ORCID:0000000237308661), Merkel, S. [Univ. Lille, CNRS, INRAE, Centrale Lille, UMR 8207—UMET—Unité Matériaux et Transformations 12 , F-59000 Lille,] (ORCID:000000032767581X), Morard, G. [Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, IRD, Univ. Gustave Eiffel, ISTerre 30 , 38000 Grenoble,] (ORCID:0000000242250767), Nagler, B. [SLAC National Accelerator Laboratory 21 , 2575 Sand Hill Road, Menlo Park, California 94025,] (ORCID:0009000257367842), Nakatsutsumi, M. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000308684745), Nguyen-Cong, K. [Department of Physics, University of South Florida 23 , Tampa, Florida 33620,] (ORCID:0000000342996208), Norton, A.-M. [School of Physics, Engineering and Technology, University of York 4 , Heslington, York YO10 5DD,] (ORCID:0000000177120615), Oleynik, I. I. [Department of Physics, University of South Florida 23 , Tampa, Florida 33620,] (ORCID:0000000253486484), Otzen, C. [Institut für Geo- und Umweltnaturwissenschaften, Albert-Ludwigs-Universität Freiburg 31 , Hermann-Herder-Straße 5, 79104 Freiburg,] (ORCID:0000000208092355), Ozaki, N. [Graduate School of Engineering Science, Osaka University 32 , 1-3 Machikaneyama Toyonaka, Osaka 560-8531,] (ORCID:0000000273209871), Pandolfi, S. [Sorbonne Université, Muséum National d’Histoire Naturelle, UMR CNRS 7590, Insitut de Minéralogie, de Physique, des Matériaux, et de Cosmochinie, IMPMC 20 , Paris 75005,] (ORCID:0000000308559434), Pelka, A. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0009000133085376), Pereira, K. A. [Department of Chemistry, University of Massachusetts Amherst 33 , 690 N. Pleasant St., Physical Sciences Building, Amherst, Massachusetts 01003-9303,] (ORCID:0000000222522999), Phillips, J. P. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0000000324720144), Prescher, C. [Institut für Geo- und Umweltnaturwissenschaften, Albert-Ludwigs-Universität Freiburg 31 , Hermann-Herder-Straße 5, 79104 Freiburg,] (ORCID:0000000295561032), Preston, T. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:0000000312282263), Randolph, L. [European XFEL 10 , Holzkoppel 4, 22869 Schenefeld,] (ORCID:000000019587404X), Ranjan, D. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0000000286414794), Ravasio, A. [Ecole Polytechnique, Palaiseau, Laboratoire pour l’utilisation des lasers intenses (LULI), CNRS UMR 7605 2 , Route de Saclay, 91128 Palaiseau Cedex,] (ORCID:0000000220776493), Rips, J. [Universität Rostock, Institut für Physik 28 , D-18051 Rostock,] (ORCID:0009000247645618), Santamaria-Perez, D. [Departamento de Fisica Aplicada—ICMUV, Universidad de Valencia—UV 19 , C/Dr. Moliner 50 Burjassot, E-46100 Valencia,] (ORCID:0000000211195056), Savage, D. J. [Los Alamos National Laboratory 9 , Los Alamos, New Mexico 87545,] (ORCID:0000000199732030), Schoelmerich, M. [Paul Scherrer Institut 34 , Forschungsstrasse 111, 5232 Villigen,] (ORCID:0000000247901565), Schwinkendorf, J.-P. [Helmholtz-Zentrum Dresden-Rossendorf (HZDR) 5 , Bautzner Landstraße 400, 01328 Dresden,] (ORCID:0009000287037641), Singh, S. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000202869549), Smith, J. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0009000993340509), Smith, R. F. [Lawrence Livermore National Laboratory 3 , Livermore, California 94550,] (ORCID:0000000256755731), Sollier, A. [CEA, DAM, DIF 35 , 91297 Arpajon,; Université Paris-Saclay, CEA, Laboratoire Matière en Conditions Extrêmes 36 , 91680 Bruyères-le-Châtel,] (ORCID:000000015067954X), Spear, J. [Central Laser Facility (CLF), STFC Rutherford Appleton Laboratory 7 , Harwell Campus, Didcot OX11 0QX,] (ORCID:0009000149335325). 2025-10-21. X-ray thermal diffuse scattering as a texture-robust temperature diagnostic for dynamically compressed solids. https://doi.org/10.1063/5.0295250
Cite the original work for its findings. Save a collection to share your selection of sources.