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DOE OSTI · 3016264

Current-Activated Reactive Ultrafast Joining (CARUJ)

Abstract

We have demonstrated Current Activated Reactive Ultrafast Joining (CARUJ) as a novel approach for rapid fabrication of similar and dissimilar materials, such as ceramic-ceramic and ceramic-metal joint assemblies. The CARUJ technology utilizes resistive heating of carbon-based materials to apply localized heat at, (through or around) joint zones at rates of 10 1 -10 2 ˚C/min, enabling joining at time scales considerably shorter (several minutes as opposed to hours) than conventional approaches for similar systems. Herein, we present our findings while evaluating the CARUJ concept. Three methods of heat application were evaluated: (i) using carbon joule heating elements to apply heat directly through the joint interface; (ii) using flexible joule heating elements to locally apply heat around the assembly interface; and (iii) non-contact heating of the joint assembly using inductive power. Schemes (ii) and (iii) proved to be the most effective in producing mechanically sound reliable joints. We demonstrated single-step fabrication of dense SiC-SiC joints with a Si- SiC interface using minimal pressure (1–2 MPa) in under 30 minutes. Measured average joint strengths of about 15 MPa are initially achieved for joined bodies when tested in single lap offset (SLO) compressive shear, while tuning of the interfacial composition along with a reduction in interlayer thickness, results in improved joint strengths of approximately 43 MPa. We further demonstrated SiC-SiC joining using Active Brazing Alloys (ABAs) proof of concept joining of tubular geometries. The versatility of CARUJ is demonstrated by utilizing non-contact heating via induction, to join dissimilar materials systems of SiC, SS316 and MAX phase ceramics with ABA interlayers. The localized and rapid heat application realizes a versatile material joining technique that can be extended for joining components at the plant site.

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BibTeXRIS

Singh, Dileep [Argonne National Laboratory (ANL), Argonne, IL (United States)], Barua, Bipul [Argonne National Laboratory (ANL), Argonne, IL (United States)] (ORCID:0000000247184113), Lee, Tae [Argonne National Laboratory (ANL), Argonne, IL (United States)], Messner, Mark [Argonne National Laboratory (ANL), Argonne, IL (United States)] (ORCID:0000000200404385), Luo, Jian [Univ. of California, San Diego, CA (United States)], Sivakumar, Sashank [Univ. of California, San Diego, CA (United States)]. 2025-05-01. Current-Activated Reactive Ultrafast Joining (CARUJ). https://doi.org/10.2172/3016264

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36 MATERIALS SCIENCE