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DOE OSTI · 3378224

Emergence of low-energy spin waves in superconducting electron-doped cuprates

Krighaar, Kristine M. L. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute] (ORCID:0000000314155815)·Cederholm, Jeppe J. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Inst. Laue-Langevin (ILL), Grenoble (France); Ecole Polytechnique Federale Lausanne (EPFL) (Switzerland)] (ORCID:0009000065228039)·Schriver, Ellen M. S. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute]·Jacobsen, Henrik [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Data Management and Software Centre, Kongens Lyngby (Denmark)] (ORCID:0000000169503990)·Lauritzen, Christine P. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Utrecht University (Netherlands)]·Zaliznyak, Igor [Brookhaven National Laboratory (BNL), Upton, NY (United States)] (ORCID:0000000285487924)·Qvistgaard, Cédric H. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Technical Univ. of Denmark, Lyngby (Denmark)] (ORCID:0009000733414508)·Hansen, Ursula B. [Inst. Laue-Langevin (ILL), Grenoble (France)] (ORCID:0000000152704091)·Alshemi, Ahmed [Lund Univ. (Sweden)] (ORCID:0000000302715299)·Stampfl, Anton P. J. [Australian Nuclear Science and Technology Organisation (ANSTO), Lucas Heights, NSW (Australia)] (ORCID:0000000256014319)·Grivel, Jean-Claude [Technical Univ. of Denmark, Lyngby (Denmark)]·Song, Dongjoon [Univ. of British Columbia, Vancouver, BC (Canada)] (ORCID:0000000337599646)·Lefmann, Kim [Univ. of Copenhagen (Denmark). The Niels Bohr Institute] (ORCID:000000034282756X)·Kamminga, Machteld E. [Utrecht University (Netherlands)] (ORCID:0000000230716996)
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Abstract

In order to fully utilize the technological potential of unconventional superconductors, an enhanced understanding of the superconducting mechanism is necessary. In the best performing superconductors, the cuprates, superconductivity is intimately linked with magnetism, although the details of this coupling remain elusive. Here, we address this gap by studying the electron-doped cuprate Nd 1.85 Ce 0.15 CuO 4−δ that has an antiferromagnetic ground state when synthesized and only becomes superconducting after a reductive annealing process. Using neutron spectroscopy, we show that the as-grown crystal exhibits a large spin pseudogap in the magnetic fluctuation spectrum. Annealing removes defects introduced by the commonly employed synthesis method and significantly reduces the spin pseudogap. While the spin pseudogap in the annealed sample likely arises from superconductivity, in the as-grown sample it results from the absence of long-wavelength spin waves. These results reveal a direct connection between defects, magnetism, and superconductivity, offering new insight into the mechanisms underlying high-temperature superconductivity and guiding the design of improved superconducting materials.

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Krighaar, Kristine M. L. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute] (ORCID:0000000314155815), Cederholm, Jeppe J. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Inst. Laue-Langevin (ILL), Grenoble (France); Ecole Polytechnique Federale Lausanne (EPFL) (Switzerland)] (ORCID:0009000065228039), Schriver, Ellen M. S. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute], Jacobsen, Henrik [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Data Management and Software Centre, Kongens Lyngby (Denmark)] (ORCID:0000000169503990), Lauritzen, Christine P. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Utrecht University (Netherlands)], Zaliznyak, Igor [Brookhaven National Laboratory (BNL), Upton, NY (United States)] (ORCID:0000000285487924), Qvistgaard, Cédric H. [Univ. of Copenhagen (Denmark). The Niels Bohr Institute; Technical Univ. of Denmark, Lyngby (Denmark)] (ORCID:0009000733414508), Hansen, Ursula B. [Inst. Laue-Langevin (ILL), Grenoble (France)] (ORCID:0000000152704091), Alshemi, Ahmed [Lund Univ. (Sweden)] (ORCID:0000000302715299), Stampfl, Anton P. J. [Australian Nuclear Science and Technology Organisation (ANSTO), Lucas Heights, NSW (Australia)] (ORCID:0000000256014319), Grivel, Jean-Claude [Technical Univ. of Denmark, Lyngby (Denmark)], Song, Dongjoon [Univ. of British Columbia, Vancouver, BC (Canada)] (ORCID:0000000337599646), Lefmann, Kim [Univ. of Copenhagen (Denmark). The Niels Bohr Institute] (ORCID:000000034282756X), Kamminga, Machteld E. [Utrecht University (Netherlands)] (ORCID:0000000230716996). 2026-05-01. Emergence of low-energy spin waves in superconducting electron-doped cuprates. https://doi.org/10.1038/s42005-026-02650-3

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