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DOE OSTI · 3675554

A holistic platform for accelerating sorbent-based carbon capture

Abstract

Abstract Reducing carbon dioxide (CO 2 ) emissions urgently requires the large-scale deployment of carbon-capture technologies. These technologies must separate CO 2 from various sources and deliver it to different sinks 1,2 . The quest for optimal solutions for specific source–sink pairs is a complex, multi-objective challenge involving multiple stakeholders and depends on social, economic and regional contexts. Currently, research follows a sequential approach: chemists focus on materials design 3 and engineers on optimizing processes 4,5 , which are then operated at a scale that impacts the economy and the environment. Assessing these impacts, such as the greenhouse gas emissions over the plant’s lifetime, is typically one of the final steps 6 . Here we introduce the PrISMa (Process-Informed design of tailor-made Sorbent Materials) platform, which integrates materials, process design, techno-economics and life-cycle assessment. We compare more than 60 case studies capturing CO 2 from various sources in 5 global regions using different technologies. The platform simultaneously informs various stakeholders about the cost-effectiveness of technologies, process configurations and locations, reveals the molecular characteristics of the top-performing sorbents, and provides insights on environmental impacts, co-benefits and trade-offs. By uniting stakeholders at an early research stage, PrISMa accelerates carbon-capture technology development during this critical period as we aim for a net-zero world.

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BibTeXRIS

Charalambous, Charithea (ORCID:0000000346066534), Moubarak, Elias (ORCID:0000000182716800), Schilling, Johannes (ORCID:0000000180135439), Sanchez Fernandez, Eva, Wang, Jin-Yu (ORCID:0000000318014139), Herraiz, Laura, Mcilwaine, Fergus (ORCID:0000000153007941), Peh, Shing, Garvin, Matthew, Jablonka, Kevin (ORCID:0000000348944660), Moosavi, Seyed (ORCID:0000000203575729), Van Herck, Joren, Ozturk, Aysu (ORCID:0000000269582323), Pourghaderi, Alireza (ORCID:0000000176066864), Song, Ah-Young (ORCID:0000000179310148), Mouchaham, Georges (ORCID:0000000186969733), Serre, Christian (ORCID:0000000330402564), Reimer, Jeffrey (ORCID:0000000241913725), Bardow, André (ORCID:0000000238310691), Smit, Berend (ORCID:0000000346538562), Garcia, Susana (ORCID:000000023713311X). 2024-07-17. A holistic platform for accelerating sorbent-based carbon capture. https://doi.org/10.1038/s41586-024-07683-8

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