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At least 181 records · Page 10

The oxidizing capacity of the earth's atmosphere - Probable past and future changes

A number of critical atmospheric chemical problems depend on the earth's oxidizing capacity, which is essentially the global burden of oxidants in the lower atmosphere. There is limited direct evidence for changes in the earth's oxidizing capacity since recent preindustrial times when, because of industrial and poulation growth, increasing amounts of O3 precursor trace gases (carbon monoxide, nitrogen oxides, and hydrocarbons) have been released into the atmosphere. The concentrations of O3 and possibly H2O2 have increased over large regions. Models predict that tropospheric O3 will increase about 0.3-1.0 percent per year over the next 50 years with both positive and negative trends possible for OH and H2O2. Models and the observational network for oxidants are improving, but validation of global models is still at an early stage.

Thompson, Anne M.↗

Model capabilities, 2-D

Two dimensional (2-D) atmospheric models provide results for altitude versus latitude as a function of time and are developed primarily for two reasons: to help understand atmospheric occurrences and to give assessments and/or make predictions of future changes in the atmosphere. Historically, the formulation of transport in 2-D models has been a difficult problem. Most current 2-D models have a transport that is either an Eulerian mean circulation with large stratospheric eddy diffusion or a residual (diabatic or Lagragian) mean circulation which typically is accompanied with small stratospheric eddy diffusion. Because of the assumption of zonal averaging, 2-D models are primarily useful in making predictions of atmospheric changes of time scales longer than a season. Although decadel atmospheric changes may be reasonably well represented with a 2-D model, the year to year changes which result from interannual transport differences, stratospheric warmings, semiannual oscillations, or quasi-biennial oscillations may not be well represented in the stratosphere and troposphere.

Jackman, Charles H.↗

Martian Dust Storm Impact on Atmospheric H2o and D/H Observed By Exomars Trace Gas Orbiter

Global dust storms on Mars are rare1,2 but can affect the Martian atmosphere for several months. They can cause changes in atmospheric dynamics and inflation of the atmosphere3, primarily owing to solar heating of the dust3. In turn, changes in atmospheric dynamics can affect the distribution of atmospheric water vapour, with potential implications for the atmospheric photochemistry and climate on Mars4. Recent observations of the water vapour abundance in the Martian atmosphere during dust storm conditions revealed a high-altitude increase in atmospheric water vapour that was more pronounced at high northern latitudes5,6, as well as a decrease in the water column at low latitudes7,8. Here we present concurrent, high-resolution measurements of dust, water and semiheavy water (HDO) at the onset of a global dust storm, obtained by the NOMAD and ACS instruments onboard the ExoMars Trace Gas Orbiter. We report the vertical distribution of the HDO/H2O ratio (D/H) from the planetary boundary layer up to an altitude of 80 kilometres. Our findings suggest that before the onset of the dust storm, HDO abundances were reduced to levels below detectability at altitudes above 40 kilometres. This decrease in HDO coincided with the presence of water-ice clouds. During the storm, an increase in the abundance of H2O and HDO was observed at altitudes between 40 and 80 kilometres. We propose that these increased abundances may be the result of warmer temperatures during the dust storm causing stronger atmospheric circulation and preventing ice cloud formation, which may confine water vapour to lower altitudes through gravitational fall and subsequent sublimation of ice crystals3. The observed changes in H2O and HDO abundance occurred within a few days during the development of the dust storm, suggesting a fast impact of dust storms on the Martian atmosphere.

Ann Carine Vandaele↗

The ERTS-1 investigation (ER-600). Volume 6: ERTS-1 signature extension analysis, July 1972 - June 1973

Feature classification, spatially and temporally, was extended over the Houston test site area. The Earth Resources Technology Satellite (ERTS-1) multispectral scanner data from August, September, and October 1972, of five widely separated lakes were used as statistical training fields and test sites. Short term temporal (same day to 36 days) and moderately long term spatial (within and between three ERTS multispectral scanner frames) signature extensions have been verified with respect to large relatively homogeneous features. The most significant feature dependent variable affecting spatial and short term extension was water turbidity. Long term signature extension will require a model to compensate or modify the ERTS-1 multispectral scanner data for significant sun angle changes. The presence of atmospheric haze changed the absolute signature but always by approximately the same amount so that the measured water signature was always the same. The normally occurring variations in atmospheric haze conditions had no major effect on the water signatures in this study.

Erb, R. B.↗

NASA's upper atmosphere research satellite: A program to study global ozone change

The Upper Atmosphere Research Satellite (UARS) is a major initiative in the NASA Office of Space Science and Applications, and is the prototype for NASA's Earth Observing System (EOS) planned for launch in the 1990s. The UARS combines a balanced program of experimental and theoretical investigations to perform diagnostic studies, qualitative model analysis, and quantitative measurements and comparative studies of the upper atmosphere. UARS provides theoretical and experimental investigations which pursue four specific research topics: atmospheric energy budget, chemistry, dynamics, and coupling processes. An international cadre of investigators was assembled by NASA to accomplish those scientific objectives. The observatory, its complement of ten state of the art instruments, and the ground system are nearing flight readiness. The timely UARS program will play a major role in providing data to understand the complex physical and chemical processes occurring in the upper atmosphere and answering many questions regarding the health of the ozone layer.

Luther, Michael R.↗

The Hazards of Our Star

The Sun's magnetic field permeates its atmosphere - ranging from the solar photosphere (the visible "surface") to the corona above. Think of this field as a collection of invisible rubber bands that are slowly stretched and twisted until they eventually reach a breaking point, When the field breaks, it releases a small amount of energy, known as a nanoflare. Millions of nanoflares occur every second, and the combined effect heats the solar corona to more than 1 million kelvins, hundreds of times hotter than the photosphere. The super-heated gas emits X-ray and ultraviolet radiation; Earth's upper atmosphere absorbs it, which changes our atmosphere's properties. This can disrupt communication, navigation, and surveillance systems, and also alter the orbits of satellites. On much larger scales, huge sections of the corona explosively erupt in coronal mass ejections (CMEs) and solar flares. CMEs directed toward Earth cause geomagnetic storms, which can wreck havoc on electrical power grids and produce widespread blackouts. Highly energetic particles can damage or even disable critical spacecraft components. Intense radiation from flares has the same effects as nanoflares, but to a greater degree. The need to understand how solar phenomena impact Earth has led to an important science field called space weather.

Klimchuk, James A.↗

Solar Cycle Response and Long-Term Trends in the Mesospheric Metal Layers

The meteoric metal layers (Na, Fe, and K) which form as a result of the ablation of incoming meteors act as unique tracers for chemical and dynamical processes that occur within the upper mesosphere lower thermosphere region. In this work, we examine whether these metal layers are sensitive Fe indicators of decadal long-term changes within the upper atmosphere. Output from a whole-atmosphere climate model is used to assess the response of the Na, K, and Fe layers across a 50 year period (1955-2005). At short timescales, the K layer has previously been shown to exhibit a very different seasonal behavior compared to the other metals. Here we show that this unusual behavior is also exhibited at longer time scales (both the 11 year solar cycle and 50 year periods), where K displays a much more pronounced response to atmospheric temperature changes than either Na or Fe. The contrasting solar cycle behavior of the K and Na layers predicted by the model is confirmed using satellite and lidar observations for the period 2004-2013.

Dawkins, E. C. M.↗

Topographic forcing of the atmosphere and a rapid change in the length of day

During June to September 1992, a special campaign was held to measure rapid changes in Earth's rotation rate and to relate these measurements to variations in the atmosphere's angular momentum, due principally to changes in zonal winds. A strong rise in both length of day and atmospheric momentum during a particular 6-day subperiod is documented, and this example of a short-period perturbation is identified with a specific regional coupling mechanism. Mountain torques within the southern tropics appear to account for most of the rapid momentum transfer between the solid Earth and atmosphere, with those across South America especially important.

Salstein, David A.↗

Modelling atmospheric aerosol backscatter at CO2 laser wavelengths. I - Aerosol properties, modeling techniques, and associated problems. II - Modeled values in the atmosphere. III - Effects of changes in wavelength and ambient conditions

The various methods of calculating the atmospheric aerosol backscattering function, beta(CO2), both from measured aerosol characteristics and from optical measurements made at other wavelengths, are discussed in detail, with limits placed on their accuracy. The most significant factor in determining beta(CO2) is found to be the aerosol size distribution and concentration; this should be known accurately for particle radii up to at least 1 micron for stratospheric particles and 5 microns for tropospheric particles. Results are then presented from the modeling of the aerosol backscattering function at a wavelength of 10.6 microns in the lowest 20 km of the atmosphere. It is found that beta(CO2) varies from 10 to the -6th per m per sr in the planetary boundary layer to less than 10 to the -11th per m per sr in the stratosphere. It is next shown that, with the exception of (NH4)2SO4-containing aerosols, whose size distributions have relatively large numbers of small particles, the variation of backscattering with CO2 wavelength is less than a factor of approximately 3. For such (NH4)2SO4 aerosol distributions, however, the variation of backscatter function with CO2 wavelengths between 9.1 and 11.1 microns may reach one order of magnitude.

Kent, G.S.↗

Shortwave feedbacks and El Nino-Southern Oscillation: Forced ocean coupled ocean-atmosphere experiments

Changes in tropical sea surface temperature (SST) can produce changes in cloudiness that modify incoming solar shortwave (SW) radiation, which in turn affects SST. The effects of this negative feedback on Pacific interannual variability are examined in forced ocean model and hybrid coupled ocean-atmosphere model simulations. Two empirical schemes are used to model the large-scale, low-frequency response of surface SW to SST anomalies. The first scheme attempts to account for the nonlocal nature of the atmospheric response to SST based patterns of covariability analyzed through singular value decomposition. In the observations the primary coupled mode of variability is composed of a SW anomaly in the central Pacific that covaries with anomalous SST in the eastern Pacific. This is applied in the model as a nonlocal feedback. The second scheme examines the effects of a purely local feedback with a spatially varying coefficient of magnitude chosen similar to the first scheme. In almost all cases the second scheme behaved similarly to the first, presumably because the correlation scale of SST is large enough for El Nino-Southern Oscillation (ENSO) dynamics that there is little sensitivity to the local approximation in the SW feedback. In simulations forced by time series of observed wind stress the SW feedback induced very minor SST damping. Results for a simpified heat budget analysis showed that while the SW feedback increased the local heat flux damping on SST, it also induced a mean shallowing of the mixed layer. The resulting changes in both the local mean vertical temperature gradient and the zonal velocity response to the wind stress acted to oppose the local heat flux damping effects. When the observed SW anomalies were applied to forced simulations, the simulated SST anomalies were modified as expected, and agreement with observed SST improved. In coupled simulations the SW feedbacks had greater impact than in the case of specified stress. The main effects were to decrease the magnitude of the warm and cold SST anomalies in the central Pacific, while leaving the pattern and evolution of ENSO anomalies essentially unchanged elsewhere. The SW feedbacks thus produce a modest improvement of the model ENSO SST pattern compared with observations, although they tended to shorten the period of the model ENSO cycle. Overall the results suggest that large-scale SW feedbacks are of quantitative importance to simulating some aspects of the ENSO cycle but are not critical to the overall occurrence of the phenomenon.

Waliser, Duane E.↗

Mars - The role of the regolith in determining atmospheric pressure and the atmosphere's response to insolation changes

A quantitative model for atmosphere-regolith exchange of CO2 on Mars is presented. The model, based on new laboratory measurements of CO2 adsorption on ground rock at 158, 175, 196, and 231 K for CO2 pressures from 1.0 to 80 mbar, is consistent with Viking observations, while models involving a massive residual CO2 cap and no long-term atmosphere-regolith CO2 exchange are not consistent. The model indicates: (1) the atmosphere-plus-cap system is buffered on a long-term basis by exchangeable CO2 adsorbed in the regolith; (2) if the atmosphere-plus-cap system suddenly disappeared, the system would eventually be almost completely restored by reequilibration with the regolith; (3) exchange with the adsorbed phase in the regolith has greatly restricted O-18 enrichment of the atmosphere; (4) the layered terrain primarily represents current periodic pressure increases; and (5) pressures of 100-300 nbar might have existed during the early history of the planet.

Fanale, F. P.↗

Large-scale short-period sea ice atmosphere interaction

Changes in the microwave brightness temperature measured by the Electrically Scanning Microwave Radiometer (ESMR) flown on board the Nimbus V satellite reveal large-scale sea ice fluctuations in the Antarctic marginal ice zone. These ice margin fluctuations arre predominantly wave numbers 1-4, with phase speeds of about 3 m/s independent of wave number. The spatial pattern and eastward advection of the sea ice anomalies match those of the atmospheric sea level pressure, and are consistent with sea ice displacement due to surface wind stress. Examination of the outgoing longwave radiation indicates that suppression of high clouds in regions of increased sea ice inc reases the radiative cooling which contributes to maintaining the ice. Data from three winter seasons indicate about a one-third probability of occurence of this large scale high frequency sea ice atmosphere interaction during any given 2-week period in winter.

Cahalan, Robert F.↗

NSA Site Science: Use of ARM Observations from Northern Alaska to Evaluate and Improve Prediction Capabilities

The Arctic is warming at a rate nearly double that of the rest of the planet, leading to profound changes in atmospheric, oceanic, and ice processes. The U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility has played a significant role in Arctic research, operating observatories in Alaska's North Slope for over 25 years. These observatories provide a rich, and wide-reaching dataset that offers insight into atmospheric processes in northern Alaska. This report details the results of a nine-year research project (2015–2024) supported by the DOE Atmospheric Systems Research (ASR) program, that leverages data from ARM’s deployment of observing facilities at Utqiaġvik (known as the North Slope of Alaska, or NSA, site) and Oliktok Point, Alaska. The project was conducted in two phases: - Phase 1 (2015–2019): Focused on understanding key atmospheric processes at Oliktok Point, including cloud formation, high-latitude precipitation, aerosol-cloud interactions, and cloud properties. - Phase 2 (2019–2024): Extended the research to the broader North Slope region, using data from both Oliktok Point and Utqiaġvik. Topics explored included surface energy budgets, atmospheric stability, ice nucleation processes, and microphysics in Arctic clouds. The project resulted in numerous research products, including 50 peer-reviewed publications and dissertations, 169 presentations, and 10 data products. These products cover a variety of topics, including: - Cloud Macro- and Microphysical Properties: Arctic clouds play a crucial role in energy transfer, and accurate representation in models is critical. The study explored cloud transitions, ice crystal shapes, and dual-wavelength radar data to understand ice crystal habits and size distributions. - Aerosol Properties and Processes: The team examined aerosol sources in the Arctic, including industrial emissions and natural sources. Observations showed significant spatial gradients in aerosol concentrations due to human activities and wildfire smoke. The influence of aerosols on cloud formation and the surface energy budget was also assessed. - Aerosol-Cloud Interactions: Research revealed that aerosols might suppress cloud ice production, affecting cloud radiative forcing and precipitation. The impact of local industrial emissions on cloud properties was also investigated. - Contextualizing the North Slope of Alaska in the context of the broader Arctic: To understand broader trends, the project evaluated large-scale circulation patterns and the influence of weather systems on the Arctic. Studies indicated that large-scale processes play a significant role in temperature patterns and the timing of snowmelt. - Advancing ARM Observational and Modeling Capabilities: The project developed new radar data products and advanced measurement techniques, including clutter mitigation and drizzle detection. Uncrewed aerial systems (UAS) and tethered balloon systems (TBS) were deployed to gather detailed atmospheric data. Additionally, the project supported 10 early career scientists, providing training and mentorship to undergraduate interns, graduate students, postdoctoral researchers, and early career researchers. These efforts contributed to the advancement of ARM research capabilities and fostered a new generation of scientists skilled in Arctic atmospheric research. Ultimately, this ASR-supported project has provided valuable insights into Arctic atmospheric processes and their broader climate implications. Recommendations for future work include continuing support for long-term observing at Arctic locations to foster additional research, further exploration of aerosol-cloud interactions and the potential impacts of enhanced industrialization of the Arctic, and expanded use of uncrewed systems to gather data in this remote and harsh environment. Additionally, the data products developed by this work, and the data products developed through the ARM infrastructure, leave a treasure-trove of additional information that should be explored for many years to come to gain additional insight into physical processes in the Arctic atmosphere that drive the rapid changes occurring in at high latitudes and their global impact.

58 GEOSCIENCES↗

The impact of emissions from space transport systems on the state of the atmosphere

The exhaust products of space transport systems contain many substances, some of which can lead to ozone destruction. Significant changes in atmospheric constituents were calculated in a local area within a few kilometers of the exhaust trail of rockets (i.e., over 80% decreases in local ozone), although these effects are simulated to last only a few hours. Relatively small changes in atmospheric constituents are computed for regional areas within 1000 km of the exhaust trail (i.e. less than 10% decreases in column ozone), and even smaller changes are computed on a global scale (i.e., less than 0.03% decreases in total global ozone depletion).

Jackman, Charles H.↗

The observed day-to-day variability of Mars atmospheric water vapor

The present evaluation of Viking water column abundance measurements of the Martian atmosphere notes observed changes to be due to atmospheric water vapor vertical column abundance variations, as well as to apparent changes resulting from abundance changes of atmospheric aerosols, relative vertical distribution changes of water vapor and aerosol, or systematic viewing-geometry variations. Variability noted in several major regions by visible and thermal-IR observations is found to very accurately coincide with the occurrence of water ice clouds and hazes.

Jakosky, Bruce M.↗

Measurements of solar wind helium in the lunar atmosphere

Measurements of lunar atmospheric helium during 1973 from the Apollo 17 surface mass spectrometer are presented. The average helium abundance is shown to be about 70% of the theoretical model value, suggesting that the solar wind helium flux in 1973, during sunspot minimum, was substantially less than the expected average flux. Large-amplitude transients in the helium data indicate rapid response of the lunar atmosphere to changes in solar wind. The atmospheric helium abundance is shown to be correlated with the geomagnetic index Kp.

Hodges, R. R., Jr.↗

Studies conducted as a search for physical mechanisms relating solar variability and the troposphere

Chains of causative mechanisms that are hypothesized to relate solar variability to the behavior of the Earth's lower atmosphere were assessed. Solar variations believed most likely to constitute the forcing functions in hypothesized solar terrestrial atmosphere chain, changes in the Earth's atmospheric electrical characteristics due to solar variability, and the observed variations in atmospheric behavior that are influenced by solar variability were also examined.

Wu, S. T.↗