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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS1985

Tomato responses to ammonium and nitrate nutrition under controlled root-zone pH

Tomato (Lycopersicon esculentum L. Mill. 'Vendor') plants were grown for 21 days in flowing solution culture with N supplied as either 1.0 mM NO3- or 1.0 mM NH4+. Acidity in the solutions was automatically maintained at pH 6.0. Accumulation and distribution of dry matter and total N and net photosynthetic rate were not affected by source of N. Thus, when rhizosphere acidity was controlled at pH 6.0 during uptake, either NO3- or NH4+ can be used efficiently by tomato. Uptake of K+ and Ca2+ were not altered by N source, but uptake of Mg2+ was reduced in NH4(+)-fed plants. This indicates that uptake of Mg2+ was regulated at least partially by ionic balance within the plant.

NASA Program CELSS↗
NASA NTRS1994

Dry matter and nitrogen accumulation are not affected by superoptimal concentration of ammonium in flowing solution culture with pH control

While it is known that superoptimal concentrations of the nitrate (NO3-) ion in solution culture do not increase NO3- uptake or dry matter accumulation, the same is not known for the ammonium (NH4+) ion. An experiment was conducted utilizing flowing solution culture with pH control to investigate the influence of superoptimal NH4+ concentrations on dry matter, nitrogen (N), potassium (K), calcium (Ca), and magnesium (Mg) accumulation by nonnodulated soybean plants. Increasing the NH4+ concentration in solution from 1 to 10 mM did not affect dry matter or N accumulation. Accumulations of K, Ca, and Mg were slightly decreased with increased NH4+ concentration. The NH4+ uptake system, which is saturated at less than 1mM NH4+, is able to regulate uptake of NH4+ at concentrations as high as 10 mM.

NASA Discipline Life Support Systems↗
NASA NTRS1995

Interactions of CO2, temperature and management practices: simulations with a modified version of CERES-Wheat

A new growth subroutine was developed for CERES-Wheat, a computer model of wheat (Triticum aestivum) growth and development. The new subroutine simulates canopy photosynthetic response to CO2 concentrations and light levels, and includes the effects of temperature on canopy light-use efficiency. Its performance was compared to the original CERES-Wheat V-2 10 in 30 different cases. Biomass and yield predictions of the two models were well correlated (correlation coefficient r > 0.95). As an application, summer growth of spring wheat was simulated at one site. Modeled crop responses to higher mean temperatures, different amounts of minimum and maximum warming, and doubled CO2 concentrations were compared to observations. The importance of irrigation and nitrogen fertilization in modulating the wheat crop climatic responses were also analyzed. Specifically, in agreement with observations, rainfed crops were found to be more sensitive to CO2 increases than irrigated ones. On the other hand, low nitrogen applications depressed the ability of the wheat crop to respond positively to CO2 increases. In general, the positive effects of high CO2 on grain yield were found to be almost completely counterbalanced by the negative effects of high temperatures. Depending on how temperature minima and maxima were increased, yield changes averaged across management practices ranged from -4% to 8%.

NASA Discipline Life Support Systems↗
NASA NTRSDate not supplied

Atmospheric Formaldehyde Trend and Its Source Attributions in the Recent Decades

Formaldehyde (CH 2 O) is one of the most important reactive trace gases in the atmosphere with an important role in tropospheric chemistry and in the control of surface air quality. Sources of CH 2 O includes direct emissions and in situ production from the oxidation of volatile organic compounds (VOCs). In this study, we investigate spatial-temporal variations in atmospheric CH 2 O and how changes in CH 2 O couple with tropospheric ozone variability during the past two decades using recently available retrievals from the Ozone Monitoring Instrument (OMI) aboard NASA’s Aura satellite and the RefD1 simulation from the NASA Goddard Earth Observing System Chemistry Climate Model (GEOSCCM). Our initial analysis provides evidence of significant increases in atmospheric CH 2 O concentrations over several of the world’s major anthropogenic regions, including China, India, and the Middle East, and several biomass burning regions, including South America, southern Africa, boreal regions and Indonesia. We furthermore will identify regional source contributions to CH 2 O trends, including anthropogenic VOCs emissions, biogenic isoprene emissions and open fires. In particular, we will focus on anthropogenic emission regions to examine the role of changing anthropogenic VOC emissions on CH 2 O abundance.

Atmospheric Formaldehyde↗
NASA NTRS2022

An Evaluation of Biomass Burning Aerosol Mass, Extinction, and Size Distribution in Geos Using Observations From Camp2EX

Biomass burning aerosol impacts aspects of the atmosphere and Earth system through radiative forcing, serving as cloud condensation nuclei, and air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in numerical weather prediction and climate models or reanalysis products. Using observations collected as part of the Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) in August through October of 2019, aerosol concentration and optical properties are evaluated within the Goddard Earth Observing System (GEOS) and its underlying aerosol module, GOCART. In the operational configuration, GEOS assimilates aerosol optical depth observations at 550 nm to constrain aerosol fields. Particularly for biomass burning aerosol, without the assimilation of aerosol optical depth, aerosol extinction is underestimated compared to observations collected in the Philippines region during the CAMP2Ex campaign. The assimilation process adds excessive amounts of carbon to account for the underestimated extinction, resulting in positive biases in the mass of black and organic carbon, especially within the boundary layer, relative to in situ observations from the Langley Aerosol Research Group Experiment. Counteracting this, GEOS is deficient in sulphate and nitrate aerosol just above the boundary layer. Aside from aerosol mass, extinction within GEOS is a function of ambient relative humidity and an assumed particle size distribution. The relationship between dry and ambient extinction in GEOS reveals that hygroscopic growth is too aggressive within the model for biomass burning aerosol. An additional concern lies in the assumed particle size distribution for GEOS, which has a mode radius that is too small for organic carbon. Variability in the observed particle size distribution for biomass burning aerosol within a single flight also illuminates the fact that a single assumed particle size distribution is not sufficient and that for a proper representation, a more advanced aerosol module with GEOS may be necessary.

Aerosol Mass↗
NASA NTRS1989

Dynamics of carbon dioxide exchange of a wheat community grown in a semi-closed environment

A wheat (Triticum aestivum Yecora Rojo) community was grown in the semi-closed conditions of the NASA/KSC Biomass Production Chamber (BPC). Experiments were conducted to determine whole community carbon dioxide exchange rates as influenced by growth and development, carbon dioxide concentration, time within the photoperiod, irradiance, and temperature. Plants were grown at a population of about 1500 per sq meter using a 20 hour light/4 hour dark daily regime. Light was supplied by HPS vapor lamps and irradiance was maintained in the range of 590 to 675 mu mol per sq meter. The temperature regime was 20 C light/16 C dark and nutrients were supplied hydroponically as a thin film. Fractional interception of PPF by the community increased rapidly during growth reaching a maximum of 0.96, 24 days after planting. This time corresponded to canopy closure and maximum rates of net photosynthesis (NP). Net daily CO2 utilization rates were calculated to day 48 and a 4th order regression equation integrated to obtain total moles of CO2 fixed by the community. This procedure may be useful for monitoring and prediction of biomass yields in a closed ecology life support system (CELSS).

Corey, Kenneth A.↗
NASA NTRS1985

Spatial and temporal patterns in pigment biomass in Gulf Stream warm-core ring 82B and its environs

A chronology of the horizontal and vertical distribution of phytoplankton pigment biomass provides a biological life history of Gulf Stream warm-core ring 82B. Development of ring 82B is followed through three distinct periods: a winter/early spring period of deep convective overturn with uniform and relatively high pigment concentrations to depths of 400 m, a late spring stratification period with subsurface (20-30 m) pigment maxima and relatively high ring center values compared to surrounding waters, and a Gulf Stream interaction period when ring characteristics are dominated by intrusions of low pigment concentration waters. While the ring maintains a unique identity throughout these periods of its life, prolonged deep vertical mixing as well as episodic interactions with its surrounding have a significant influence on pigment distributions within the ring. These interactions generally enhance pigment biomass compared to the water mass from which it is derived. A consistent feature of pigment distribution is the remarkable coherence between this measure of phytoplankton biomass and the corresponding physical hydrodynamic structure of the upper water column.

Smith, R. C.↗
NASA NTRS2020

Prokaryotic and Fungal Characterization of the Facilities Used to Assemble, Test, and Launch the OSIRIS-REx Spacecraft

To characterize the ATLO (Assembly, Test, and Launch Operations) environment of the OSIRIS-REx spacecraft, we analyzed 17 aluminum witness foils and two blanks for bacterial, archaeal, fungal, and arthropod DNA. Under NASA’s Planetary Protection guidelines, OSIRIS-REx is a Category II outbound, Category V unrestricted sample return mission. As a result, it has no bioburden restrictions. However, the mission does have strict organic contamination requirements to achieve its primary objective of returning pristine carbonaceous asteroid regolith to Earth. Its target, near-Earth asteroid (101955) Bennu, is likely to contain organic compounds that are biologically available. Therefore, it is useful to understand what organisms were present during ATLO as part of the larger contamination knowledge effort—even though it is unlikely that any of the organisms will survive the multi-year deep space journey. Even though these samples of opportunity were not collected or preserved for DNA analysis, we successfully amplified bacterial and archaeal DNA (16S rRNA gene) from 16 of the 17 witness foils containing as few as 7 ± 3 cells per sample. Fungal DNA (ITS1) was detected in 12 of the 17 witness foils. Despite observing arthropods in some of the ATLO facilities, arthropod DNA (COI gene) was not detected. We observed 1,009 bacterial and archaeal sOTUs (sub-operational taxonomic units, 100% unique) and 167 fungal sOTUs across all of our samples (25–84 sOTUs per sample). The most abundant bacterial sOTU belonged to the genus Bacillus. This sOTU was present in blanks and may represent contamination during sample handling or storage. The sample collected from inside the fairing just prior to launch contained several unique bacterial and fungal sOTUs that describe previously uncharacterized potential for contamination during the final phase of ATLO. Additionally, fungal richness (number of sOTUs) negatively correlates with the number of carbon-bearing particles detected on samples. The total number of fungal sequences positively correlates with total amino acid concentration. These results demonstrate that it is possible to use samples of opportunity to characterize the microbiology of low-biomass environments while also revealing the limitations imposed by sample collection and preservation methods not specifically designed with biology in mind.

Aaron B. Regberg↗
NASA NTRSDate not supplied

Evaluation of GEOS Aerosols Using CAMP2Ex Observations

Biomass burning aerosol impacts aspects of the atmosphere and Earth system through direct and semi-direct effects, as well as influencing air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in numerical weather prediction and climate models or reanalysis products. Using observations collected as part of the Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) in August through October of 2019, aerosol concentration and optical properties are evaluated within the Goddard Earth Observing System (GEOS) and its underlying aerosol module, GOCART. In the operational configuration, GEOS assimilates aerosol optical depth observations at 550 nm from AERONET and MODIS to constrain aerosol fields. Particularly for biomass burning aerosol, without the assimilation of aerosol optical depth, aerosol extinction is underestimated compared to observations collected in the Philippines region during the CAMP2Ex campaign. The assimilation process adds excessive amounts of carbon to account for the underestimated extinction, resulting in positive biases in the mass of black and organic carbon, especially within the boundary layer, relative to in situ observations from the Langley Aerosol Research Group Experiment. Counteracting this, GEOS is deficient in sulfate and nitrate aerosol just above the boundary layer. Aerosol extinction within GEOS is a function of the mass of different aerosol species, the ambient relative humidity, the assumed spectral optical properties, and particle size distribution per species. The relationship between dry and ambient extinction in GEOS reveals that hygroscopic growth is too high within the model for biomass burning aerosol. An additional concern lies in the assumed particle size distribution for GEOS, which has a single mode radius that is too small for organic carbon. Variability in the observed particle size distribution for biomass burning aerosol within a single flight also illuminates the fact that a single assumed particle size distribution is not sufficient and that for a proper representation, a more advanced aerosol module within GEOS may be necessary.

Allison Collow↗
NASA NTRS2004

From Surface Chlorophyll a to Phytoplankton Community Composition in Oceanic Waters

The objective of the present study is to examine the potential of using the near-surface total chlorophyll a concentration (C(sub surf)), as it can be derived from ocean color observation, to infer the column-integrated and the vertical distribution of the phytoplanktonic biomass, both in a quantitative way and in a qualitative way (z.e., in terms of community structure). Within this context, a large HPLC (High Performance Liquid Chromatography) pigment database has been analyzed. It includes 2419 vertical pigment profiles, all sampled in Case-1 waters with various trophic states. The relationshps between C(sub surf) and the total chlorophyll alpha vertical distribution, as previously derived by Morel and Berthon, are fully confirmed, as the present results coincide with the previous ones. This agreement allows to go further, namely to examine the possibility of extracting relationships between C(sub surf) and the vertical composition of the algal assemblages. Thanks to the detailed pigment composition available from HPLC measurements, the contribution of three size classes (micro-, nano-, and pico-phytoplankton) to the local total chlorophyll a concentration can be assessed. Corroborating previous findings (e.g., large species dominate in eutrophc environments, whereas tiny phytoplankton prevail in oligotrophic zones), the results lead to a statistically based parameterization. The predictive skill of this parameterization is successfully tested on a separate data set. With such a tool, the vertical total chlorophyll a profiles associated with each size class can be inferred from the sole knowledge of C(sub surf). By combining this tool with satellite ocean color data, it becomes conceivable to quantify on a global scale the phytoplankton biomass associated with each of the three size classes.

Uitz, Julia↗
NASA NTRS2020

Global Carbon Cycle and Climate Feedbacks in the NASA GISS ModelE2.1

We present results from the NASA GISS ModelE2.1‐G‐CC Earth System Model with coupled climate‐carbon cycle simulations that were submitted to the sixth phase of the Coupled Model Intercomparison Project (CMIP6) Coupled Climate‐Carbon Cycle MIP (C4MIP). Atmospheric CO2 concentration and carbon budgets for the land and ocean in the historical simulations were generally consistent with observations. Low simulated atmospheric CO2 concentrations during 1850‐1950 were due to excess uptake from prescribed land cover change, which erroneously replaced arid shrublands with higher biomass crops, and assumed high 2004 LAI values in vegetated lands throughout the historical simulation. At the end of the historical period, slightly higher simulated CO2 than observed resulted from the land being an insufficient net carbon sink, despite the net effect of CO2 fertilization and warming‐induced increases to leaf photosynthetic capacity. The global ocean carbon uptake agreed well with the observations with the largest discrepancies in the low latitudes. Future climate projection at 2091‐2100 agreed with CMIP5 models in the northward shift, of temperate deciduous forest climate and expansion across Eurasia along 60 °N latitude, and dramatic regional biome shifts from drying and warming in continental Europe. Carbon feedback parameters were largely similar to the CMIP5 model ensemble. For our model, the variation of land feedback parameters within the uncertainty arises from the fertilization feedback being less sensitive due to lack of increased vegetation growth, and the comparably more negative ocean carbon‐climate feedback is due to the large slowdown of the Atlantic overturning circulation.

Carbon cycle↗
NASA NTRS2009

Further Studies on the Physical and Biogeochemical Causes for Large Interannual Changes in the Patagonian Shelf Spring-Summer Phytoplankton Bloom Biomass

A very strong and persistent phytoplankton bloom was observed by ocean color satellites during September - December 2003 along the northern Patagonian shelf. The 2003 bloom had the highest extent and chlorophyll a (Chl-a) concentrations of the entire Sea-viewing Wide Field-of-view Sensor (SeaWiFS) period (1997 to present). SeaWiFS-derived Chl-a exceeded 20 mg/cu m in November at the bloom center. The bloom was most extensive in December when it spanned more than 300 km across the shelf and nearly 900 km north-south (35degS to 43degS). The northward reach and the deep penetration on the shelf of the 2003 bloom were quite anomalous when compared with other years, which showed the bloom more confined to the Patagonian shelf break (PSB). The PSB bloom is a conspicuous austral spring-summer feature detected by ocean color satellites and its timing can be explained using the Sverdrup critical depth theory. Based on high-resolution numerical simulations, in situ and remote sensing data, we provide some suggestions for the probable mechanisms responsible for that large interannual change of biomass as seen by ocean color satellites. Potential sources of macro and micro (e.g., Fe) nutrients that sustain the high phytoplankton productivity of the Patagonian shelf waters are identified, and the most likely physical processes that maintain the nutrient balance in the region are discussed.

Signorini, Sergio R.↗
NASA NTRS2002

Dust, Pollution, and Biomass Burning Aerosols in Asian Pacific: A Column Surface/Satellite Perspective

Many recent field experiments are designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern/southeastern Asia and along the rim of the western Pacific. For example, the phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Springtime is also the peak season for biomass burning in southeastern Asia. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS (Moderate Resolution Imaging Spectroradiometer), SeaWiFS (Sea-viewing Wide Field-of-view Sensor), TOMS (Total Ozone Mapping Spectrometer) and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. A column satellite-surface perspective of Asian aerosols will be presented and will discuss their implications in regional-to-global effects on climate, fresh water redistribution, and health issues. (to be presented in Hawaii, April 28 - May 3, and Beijing, China, May 6 - 10, 2002)

Tsay, Si-Chee↗
NASA NTRS1985

Distribution and metabolism of quaternary amines in salt marshes

Quaternary amines such as glycine betaine (GBT) are common osmotically active solutes in much of the marine biota. GBT is accumulated by various bacteria, algae, higher plants, invertebrates, and vertebrates in response to salinity or water stresses; in some species, GBT occurs at tens to hundreds of millimolar concentrations and can account for a significant fraction of total nitrogen. Initial studies suggest that GBT is readily converted to two potential methane precursors, trimethylamine (TMA) and acetate, in anoxic sediments. TMA is apparently the most important methane precursor in surface sediments containing sulfate reducing bacteria. In salt marshes, the bulk of the methane formed may be due to the metabolism of TMA rather than other substrates. Current research is focussed on testing this hypothesis and on determining the role of quaternary amino osmoregulatory solutes in methane fluxes from marine environments. Preliminary studies have dealt with several problems: (1) determination of GBT concentrations in the dominant flora and fauna of salt marshes; (2) synthesis of radiolabelled GBT for metabolic studies; and (3) determination of fates of BGT in marine sediments using radiotracers. Both GC and HPLC techniques have been used to assay GBT concentrations in plant and animal tissues. S. alterniflora is probably the only significant source of GBT (and indirectly of methane) since the biomass and distribution of most other species is limited. Current estimates suggest that S. alterniflora GBT could account for most of the methane efflux from salt marshes.

King, Gary M.↗
NASA NTRS2018

A13H-2546: Intercomparison of biomass burning aerosol properties from in-situ and remote-sensing instruments in ORACLES-2016

The magnitude of the cumulative effects of aerosols, both directly and on cloud properties, remains the biggest source of uncertainty in our understanding of anthropogenic radiative forcing on the climate. The magnitude of aerosol effects in any given region will depend on not just the aerosol concentration, but also on the characteristics of the aerosol under consideration. The NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign was conducted in 2016-2018 over three deployments in the Southeast Atlantic Ocean (SEA), with the goal of making observations of seasonal biomass burning (BB) smoke plumes overlying persistent stratocumulus cloud decks. During the first ORACLES deployment (September 2016), two NASA aircraft (a P-3 and an ER-2) were flown with a suite of aerosol, cloud, radiation, and meteorological instruments for remote-sensing and in-situ observations. In ORACLES, data collected by eight different instrument teams are used to derive aerosol properties over this region by independent methods. Here we present a comparison of results from the different instrument retrievals with a focus on the measures of aerosol absorption. We focus on specific cases with near-coincident measurements from in-situ (PSAP or PTI for aerosol absorption combined with a nephelometer for aerosol scattering) and remote sensing (4STAR, AirMSPI, RSP, and SSFR) instruments from coordinated flights between the two aircraft. We use the single scattering albedo (SSA), a measure of the relative absorption versus total extinction by aerosols, as the main comparable property between the various remote sensing and in-situ methods. For the remote sensing instruments, we see general good agreement in the total aerosol loading (aerosol optical depth, AOD), though see some differences in the absorbing component (AAOD). We report values for the retrieved aerosol parameters measured in the ORACLES flights and comment upon the observed variability between different instruments. Finally, we discuss these ORACLES results in the context of previous measurements of BB aerosol over the SEA.

Kristina Pistone↗
NASA NTRSDate not supplied

FUTURE LEVELS OF AEROSOLS & RADIATIVE FORCING OVER THE ARCTIC

The Arctic Monitoring and Assessment Programme (AMAP) is currently assessing the impacts of Short-Lived Climate Forcers (SLCF) on Arctic climate and air quality. In support of the assessment, we used the NASA Goddard Institute of Space Sciences (GISS) Earth System Model (modelE2.1), with prescribed sea surface temperature and sea-ice fraction, to simulate SLCF concentrations globally between 1995 and 2015. Two simulations were conducted, using the One-Moment Aerosol (OMA) and the Multiconfiguration Aerosol TRacker of mIXing state (MATRIX) aerosol modules. OMA is a mass-based scheme in which aerosols are assumed to remain externally mixed and have a prescribed and constant size distribution, while MATRIX is an aerosol microphysics scheme based on the quadrature method of moments, which is able to explicitly simulate the mixing state of aerosols. Anthropogenic emissions from the ECLIPSE v6b emissions database were used, along with emissions from aircrafts and open biomass burning from the Coupled Model Intercomparison Project Phase 6 (CMIP6), while the natural emissions of sea salt, DMS, isoprene and dust are calculated interactively. The simulated monthly surface concentrations of sulfate (SO4), black carbon (BC), organic carbon (OA), and ozone (O3) are compared with observations from a set of Arctic stations, extracted from the EBAS and IMPROVE databases, as well as a few additional locations. Simulated aerosol optical depths (AOD) are also compared with Advanced Very-High Resolution Radiometer (AVHRR). The study will present the evaluation of the modelE2.1 in simulating SLCF levels over the Arctic using different aerosol schemes, along with observed and simulated trends of SLCFs over the Arctic between 1995 and 2015.

Aersosols↗
NASA NTRS2007

Fine Aerosol Bulk Composition Measured on WP-3D Research Aircraft in Vicinity of the Northeastern United States - Results from NEAQS

During the New England Air Quality Study (NEAQS) in the summer of 2004, airborne measurements were made of the major inorganic ions and the water-soluble organic carbon (WSOC) of the submicron (PM(sub 1.0)) aerosol. These and ancillary data are used to describe the overall aerosol chemical characteristics encountered during the study. Fine particle mass was estimated from particle volume and a calculated density based on measured particle composition. Fine particle organic matter (OM) was estimated from WSOC and a mass balance analysis. The aerosol over the northeastern United States (U.S.) and Canada was predominantly sulfate and associated ammonium, and organic components, although in unique plumes additional ionic components were also periodically above detection limits. In power generation regions, and especially in the Ohio River Valley region, the aerosol tended to be predominantly sulfate (approximately 60% micro gram /micro gram) and apparently acidic, based on an excess of measured anions compared to cations. In all other regions where sulfate concentrations were lower and a smaller fraction of overall mass, the cations and anions were balanced suggesting a more neutral aerosol. In contrast, the WSOC and estimated OM were more spatially uniform and the fraction of OM relative to PM mass was largely influenced by sources of sulfate. The study median OM mass fraction was 40%. Throughout the study region, sulfate and organic aerosol mass were highest near the surface and decreased rapidly with increasing altitude. The relative fraction of organic mass to sulfate was similar throughout all altitudes within the boundary layer (altitude less than 2.5 km), but was significantly higher at altitude layers in the free troposphere (above 2.5 km). A number of distinct biomass burning plumes from fires in Alaska and the Yukon were periodically intercepted, mostly at altitudes between 3 and 4 km. These plumes were associated with highest aerosol concentrations of the study and were largely comprised of organic aerosol components (approximtely 60%).

Peltier, R. E.↗
NASA NTRS2012

Size Resolved Measurements of Springtime Aerosol Particles over the Northern South China Sea

Large sources of aerosol particles and their precursors are ubiquitous in East Asia. Such sources are known to impact the South China Sea (henceforth SCS), a sometimes heavily polluted region that has been suggested as particularly vulnerable to climate change. To help elucidate springtime aerosol transport into the SCS, an intensive study was performed on the remote Dongsha (aka Pratas) Islands Atoll in spring 2010. As part of this deployment, a Davis Rotating-drum Uniform size-cut Monitor (DRUM) cascade impactor was deployed to collect size-resolved aerosol samples at the surface that were analyzed by X-ray fluorescence for concentrations of selected elements. HYSPLIT backtrajectories indicated that the transport of aerosol observed at the surface at Dongsha was occurring primarily from regions generally to the north and east. This observation was consistent with the apparent persistence of pollution and dust aerosol, along with sea salt, in the ground-based dataset. In contrast to the sea-level observations, modeled aerosol transport suggested that the westerly flow aloft (w700 hPa) transported smoke-laden air toward the site from regions from the south and west. Measured aerosol optical depth at the site was highest during time periods of modeled heavy smoke loadings aloft. These periods did not coincide with elevated aerosol concentrations at the surface, although the model suggested sporadic mixing of this free-tropospheric aerosol to the surface over the SCS. A biomass burning signature was not clearly identified in the surface aerosol composition data, consistent with this aerosol type remaining primarily aloft and not mixing strongly to the surface during the study. Significant vertical wind shear in the region also supports the idea that different source regions lead to varying aerosol impacts in different vertical layers, and suggests the potential for considerable vertical inhomogeneity in the SCS aerosol environment.

South China Sea↗