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At least 181 records · Page 10

Weak influence of anthropogenic emissions on aerosol, cloud, and rain in the wet season of the Amazon rainforest

Anthropogenic emissions have been shown to affect new particle formation, aerosol concentrations, and clouds. Such effects vary with region, environmental conditions, and cloud types. In the wet season of Amazonia, anthropogenic emissions emitted from Manaus, Brazil, can significantly increase the cloud condensation nuclei (CCN) concentrations compared to the background of mainly natural aerosols. However, the regional response of cloud and rain to anthropogenic emissions in Amazonia remains very uncertain. Here, we aim to quantify how aerosol concentration, cloud, and rain respond to changes in anthropogenic emissions through parameterized new particle formation and primary aerosol emission in the Manaus region and to understand the underlying mechanisms. We ran the atmosphere-only configuration of the HadGEM3 climate model with a nested regional domain that covers most of the rainforest region (720 km by 1200 km with 3 km resolution) under scaled regional emissions. The 7 d simulations show that, in the areas that are affected by anthropogenic emissions, when aerosol and precursor gas emissions are doubled from the baseline emission inventories, aerosol number concentrations increase by 13 %. The nucleation rate that involves sulfuric acid and biogenic compounds generally increases with pollution levels. However, nucleation is suppressed very close to the pollution source, resulting in lower nucleation and soluble Aitken mode aerosol number concentrations. We also found that doubling the anthropogenic emission can increase the cloud droplet number concentrations ( N d ) by 9 %, but cloud water and rain mass mixing ratios do not change significantly. Even very strong reductions in aerosol number concentrations by a factor of 4, which is an unrealistic condition, cause only a 4 % increase in rain over the domain. If we assume our simulation has a fine enough grid resolution and an accurate representation of the relevant atmospheric processes, the simulated weak and non-linear response of cloud and rain properties to linearly scaled anthropogenic emissions suggests that the interactions among aerosol, cloud, and precipitation in the Amazonian convective environment are buffered by microphysical processes. It also implies that the convective environment is resilient to the changes in Nd that occur in response to localized anthropogenic aerosol perturbations.

Wang, Xuemei [University of Leeds (United Kingdom)↗

Near‐Cloud Aerosol Retrieval Using Machine Learning Techniques, and Implied Direct Radiative Effects

Abstract There is a lack of satellite‐based aerosol retrievals in the vicinity of low‐topped clouds, mainly because reflectance from aerosols is overwhelmed by three‐dimensional cloud radiative effects. To account for cloud radiative effects on reflectance observations, we develop a Convolutional Neural Network and retrieve aerosol optical depth (AOD) with 100–500 m horizontal resolution for all cloud‐free regions regardless of their distances to clouds. The retrieval uncertainty is 0.01 + 5%AOD, and the mean bias is approximately −2%. In an application to satellite observations, aerosol hygroscopic growth due to humidification near clouds enhances AOD by 100% in regions within 1 km of cloud edges. The humidification effect leads to an overall 55% increase in the clear‐sky aerosol direct radiative effect. Although this increase is based on a case study, it highlights the importance of aerosol retrievals in near‐cloud regions, and the need to incorporate the humidification effect in radiative forcing estimates.

54 ENVIRONMENTAL SCIENCES↗

Satellite-Surface Perspectives of Air Quality and Aerosol-Cloud Effects on the Environment: An Overview of 7-SEAS BASELInE

The objectives of 7-SEASBASELInE (Seven SouthEast Asian Studies Biomass-burning Aerosols and Stratocumulus Environment: Lifecycles and Interactions Experiment) campaigns in spring 2013-2015 were to synergize measurements from uniquely distributed ground-based networks (e.g., AERONET (AErosol RObotic NETwork)), MPLNET ( NASA Micro-Pulse Lidar Network)) and sophisticated platforms (e.g.,SMARTLabs (Surface-based Mobile Atmospheric Research and Testbed Laboratories), regional contributing instruments), along with satellite observations retrievals and regional atmospheric transport chemical models to establish a critically needed database, and to advance our understanding of biomass-burning aerosols and trace gases in Southeast Asia (SEA). We present a satellite-surface perspective of 7-SEASBASELInE and highlight scientific findings concerning: (1) regional meteorology of moisture fields conducive to the production and maintenance of low-level stratiform clouds over land; (2) atmospheric composition in a biomass-burning environment, particularly tracers-markers to serve as important indicators for assessing the state and evolution of atmospheric constituents; (3) applications of remote sensing to air quality and impact on radiative energetics, examining the effect of diurnal variability of boundary-layer height on aerosol loading; (4) aerosol hygroscopicity and ground-based cloud radar measurements in aerosol-cloud processes by advanced cloud ensemble models; and (5) implications of air quality, in terms of toxicity of nanoparticles and trace gases, to human health. This volume is the third 7-SEAS special issue (after Atmospheric Research, vol. 122, 2013; and Atmospheric Environment, vol. 78, 2013) and includes 27 papers published, with emphasis on air quality and aerosol-cloud effects on the environment. BASELInE observations of stratiform clouds over SEA are unique, such clouds are embedded in a heavy aerosol-laden environment and feature characteristically greater stability over land than over ocean, with minimal radar surface clutter at a high vertical spatial resolution. To facilitate an improved understanding of regional aerosol-cloud effects, we envision that future BASELInE-like measurement modeling needs fall into two categories: (1) efficient yet critical in-situ profiling of the boundary layer for validating remote-sensing retrievals and for initializing regional transport chemical and cloud ensemble models; and (2) fully utilizing the high observing frequencies of geostationary satellites for resolving the diurnal cycle of the boundary layerheight as it affects the loading of biomass-burning aerosols, air quality and radiative energetics.

AERONET↗

Effect of Cloud Fraction on Near-Cloud Aerosol Behavior Based on MODIS and CALIPSO Observations

Organizers of the MODIS-VIIRS Science Team Meeting, held May 18-22, 2015 in Silver Spring, MD plan to post the presentations and posters to the NASA MODIS website: http:modis.gsfc.nasa.govsci_teammeetings201505index.php. The MODIS Science Team Meeting is held twice a year, so that the members of the science team may assemble and discuss data they have collected, ideas they have formed, and future issues that apply to the MODIS Mission.

aerosol retrieval↗

Aerosol-Cloud Interactions in the South-East Atlantic: Knowledge Gaps, Planned Observations to Address Them, and Implications for Global Climate Change Modeling

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles, yet the fate of these particles and their influence on regional and global climate is poorly understood. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical Stratocumulus (Sc) cloud decks in the world. The stratocumulus "climate radiators" are critical to the regional and global climate system. They interact with dense layers of BB aerosols that initially overlay the cloud deck, but later subside and are mixed into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects. As emphasized in the latest IPCC report, the global representation of these aerosol-cloud interaction processes in climate models is one of the largest uncertainty in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for global climate change scenarios. We discuss the current knowledge of aerosol and cloud property distributions based on satellite observations and sparse suborbital sampling, and describe planned field campaigns in the region. Specifically, we describe the scientific objectives and implementation of the following four synergistic, international research activities aimed at providing a process-level understanding of aerosol-cloud interactions over the SE Atlantic: 1) ORACLES (Observations of Aerosols above Clouds and their interactions), a five-year investigation between 2015 and 2019 with three Intensive Observation Periods (IOP), recently funded by the NASA Earth-Venture Suborbital Program, 2) CLARIFY-2016 (Cloud-Aerosol-Radiation Interactions and Forcing: Year 2016), a comprehensive observational and modeling programme funded by the UK's Natural Environment Research Council (NERC), and supported by the UK Met Office. 3) LASIC (Layered Atlantic Smoke Interactions with Clouds), a funded deployment of the DOE (Department of Energy) ARM Mobile Facility (AMF1) to Ascension Island, nominally for April 1 2016 - March 31 2017, and 4) ONFIRE (Observations of Fire's Impact on the southeast Atlantic Region), a proposed deployment of the NCAR C-130 aircraft to Sao Tome Island in 2017.

Aerosol-cloud↗

Aerosol-cloud-climate cooling overestimated by ship-track data

The effect of anthropogenic aerosol on the reflectivity of stratocumulus cloud decks through changes in cloud amount is a major uncertainty in climate projections. In frequently occurring nonprecipitating stratocumulus, cloud amount can decrease through aerosol-enhanced cloud-top mixing. The climatological relevance of this effect is debated because ship exhaust only marginally reduces stratocumulus amount. By comparing detailed numerical simulations with satellite analyses, we show that ship-track studies cannot be generalized to estimate the climatological forcing of anthropogenic aerosol. The ship track–derived sensitivity of the radiative effect of nonprecipitating stratocumulus to aerosol overestimates their cooling effect by up to 200%. Further, the offsetting warming effect of decreasing stratocumulus amount needs to be taken into account if we are to constrain the cloud-mediated radiative forcing of anthropogenic aerosol.

54 ENVIRONMENTAL SCIENCES↗

Quantifying the impacts of marine aerosols over the southeast Atlantic Ocean using a chemical transport model: implications for aerosol–cloud interactions

The southeast Atlantic region, characterized by persistent stratocumulus clouds, has one of the highest uncertainties in aerosol radiative forcing and significant variability across climate models. In this study, we analyze the seasonally varying role of marine aerosol sources and identify key uncertainties in aerosol composition at cloud-relevant altitudes over the southeast Atlantic using the GEOS-Chem chemical transport model. We evaluate simulated aerosol optical depth (AOD) and speciated aerosol concentrations against those collected from ground observations and aircraft campaigns such as LASIC, ORACLES, and CLARIFY, conducted during 2017. The model consistently underestimates AOD relative to AERONET, particularly at remote locations like Ascension Island. However, when compared with aerosol mass concentrations from aircraft campaigns during the biomass burning period, it performs adequately at cloud-relevant altitudes, with a normalized mean bias (NMB) between -3.5 % (CLARIFY) and -7.5 % (ORACLES). At these altitudes, in the model, organic aerosols (63 %) dominate during the biomass burning period, while sulfate (41 %) prevails during austral summer, when dimethylsulfide (DMS) emissions peak in the model. Our findings indicate that marine sulfate can account for up to 69 % of total sulfate during the high-DMS period. Sensitivity analyses indicate that refining DMS emissions and oxidation chemistry may increase sulfate aerosol produced from marine sources, highlighting that there remains large uncertainty as to the role of DMS emissions in the marine boundary layer. Additionally, we find marine primary organic aerosol emissions may substantially increase total organic aerosol concentrations, particularly during austral summer. This study underscores the imperative need to refine marine emissions and their chemical transformations, as aerosols from marine sources are a major component of total aerosols at cloud-relevant altitudes and may impact uncertainties in aerosol radiative forcing over the southeast Atlantic.

54 ENVIRONMENTAL SCIENCES↗

Coupled Aerosol-Cloud Systems over Northern Vietnam during 7-SEAS BASELInE: A Radar and Modeling Perspective

The 2013 7-SEASBASELInE campaign over northern Southeast Asia (SEA) provided, for the first time ever, comprehensive ground-based W-band radar measurements of the low-level stratocumulus (Sc) systems that often exist during the spring over northern Vietnam in the presence of biomass-burning aerosols. Although spatially limited, ground-based remote sensing observations are generally free of the surface contamination and signal attenuation effects that often hinder space-borne measurements of these low-level cloud systems. Such observations permit detailed measurements of structures and lifecycles of these clouds as part of a broader effort to study potential impacts of these coupled aerosol-cloud systems on local and regional weather and air quality. Introductory analyses of the W-band radar data show these Sc systems generally follow a diurnal cycle, with peak occurrences during the nighttime and early morning hours, often accompanied by light precipitation. Preliminary results from idealized simulations of Sc development over land based on the observations reveal the familiar response of increased numbers and smaller sizes of cloud droplets, along with suppressed drizzle formation, as aerosol concentrations increase. Slight reductions in simulated W-band reflectivity values also are seen with increasing aerosol concentrations and result primarily from decreased droplet sizes. As precipitation can play a large role in removing aerosol from the atmosphere, and thereby improving air quality locally, quantifying feedbacks between aerosols and cloud systems over this region are essential, particularly given the negative impacts of biomass burning on human health in SEA. Such an endeavor should involve improved modeling capabilities along with comprehensive measurements of time-dependent aerosol and cloud profiles.

aerosol cloud interactions↗

On the prolonged lifetime of the El Chichon sulfuric acid aerosol cloud

The observed decay of the aerosol mixing ratio following the eruption of El Chichon appears to have been 20-30 percent slower than that following the eruption of Fuego in 1974, even though the sulfuric acid droplets were observed to grow to considerably larger sizes after El Chichon. This suggests the possible presence of a condensation nuclei and sulfuric acid vapor source and continued growth phenomena occurring well after the El Chichon eruption. It is proposed that the source of these nuclei and the associated vapor may be derived from annual evaporation and condensation of aerosol in the high polar regions during stratospheric warming events, with subsequent spreading to lower latitudes.

Hofmann, D. J.↗

Near-Cloud Aerosol Properties from the 1 Km Resolution MODIS Ocean Product

This study examines aerosol properties in the vicinity of clouds by analyzing high-resolution atmospheric correction parameters provided in the MODIS (Moderate Resolution Imaging Spectroradiometer) ocean color product. The study analyzes data from a 2 week long period of September in 10 years, covering a large area in the northeast Atlantic Ocean. The results indicate that on the one hand, the Quality Assessment (QA) flags of the ocean color product successfully eliminate cloud-related uncertainties in ocean parameters such as chlorophyll content, but on the other hand, using the flags introduces a sampling bias in atmospheric products such as aerosol optical thickness (AOT) and Angstrom exponent. Therefore, researchers need to select QA flags by balancing the risks of increased retrieval uncertainties and sampling biases. Using an optimal set of QA flags, the results reveal substantial increases in optical thickness near clouds-on average the increase is 50% for the roughly half of pixels within 5 km from clouds and is accompanied by a roughly matching increase in particle size. Theoretical simulations show that the 50% increase in 550nm AOT changes instantaneous direct aerosol radiative forcing by up to 8W/m2 and that the radiative impact is significantly larger if observed near-cloud changes are attributed to aerosol particles as opposed to undetected cloud particles. These results underline that accounting for near-cloud areas and understanding the causes of near-cloud particle changes are critical for accurate calculations of direct aerosol radiative forcing.

near-cloud aerosols↗

The detection of clouds, aerosols and marine atmospheric boundary layer characteristics from simulated GLAS data

Scheduled for launch in 2001 as part of NASA's Earth Observing System (EOS), the Geoscience Laser Altimeter System (GLAS) will provide continuous laser sounding of the earth's atmosphere from space for the first time. From its polar orbit about 600 km above the surface, GLAS will employ a 40 Hz solid state laser operating at 1064 nm to measure topography to an accuracy of 10 cm. Simultaneously, the atmospheric channels (1064 and 532 nm) of GLAS will provide profiles of atmospheric backscatter from 40 km to the ground with 75 meter vertical resolution (Spinhirne and Palm, 1996). These measurements will give scientists an unprecedented global data set on the vertical structure of clouds and aerosols which will greatly aid research efforts aimed at understanding their effects on climate and their role in climate change (Hartman, 1994). To better understand and predict the performance of the GLAS atmospheric channels, a computer model was developed to simulate the type of signal that the instrument would likely produce. The model uses aircraft lidar data and provides realistic simulated GLAS data sets over large areas spanning a wide range of atmospheric conditions. These simulated GLAS datasets are invaluable for designing and testing algorithms for the retrieval of parameters such as cloud and aerosol layer height, optical depth and extinction cross section. This work is currently proceeding and in this paper we will present results of the cloud and aerosol detection algorithm with emphasis on the detection of Marine Atmospheric Boundary Layer (MABL) aerosol. In addition, we use a recently developed technique to ascertain the feasability of estimating MABL moisture and temperature structure from spaceborne systems such as GLAS.

Palm, Stephen P.↗

Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) Science Plan

Coastal cities provide the opportunity to characterize marine clouds and the substantial effects of manmade particles on cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties.

54 ENVIRONMENTAL SCIENCES↗

Remote sensing of cloud, aerosol, and water vapor properties from the moderate resolution imaging spectrometer (MODIS)

The authors describe the status of MODIS-N and its companion instrument MODIS-T (tilt), a tiltable cross-track scanning spectrometer with 32 uniformly spaced channels between 0.410 and 0.875 micron. They review the various methods being developed for the remote sensing of atmospheric properties using MODIS, placing primary emphasis on the principal atmospheric applications of determining the optical, microphysical, and physical properties of clouds and aerosol particles from spectral reflection and thermal emission measurements. In addition to cloud and aerosol properties, MODIS-N will be used for determining the total precipitable water vapor and atmospheric stability. The physical principles behind the determination of each of these atmospheric products are described, together with an example of their application to aircraft and/or satellite measurements.

King, Michael D.↗

Investigating Spatial Variability of Aerosol, Cloud Condensation Nuclei, and Ice Nucleating Particles in Mountainous Terrain Field Campaign Report

The U.S. Department of Energy Atmospheric System Research (ASR)-supported Surface Atmosphere Integrated Field Laboratory (SAIL) campaign in the East River Watershed (ERW) of the Upper Colorado River Basin in southwestern Colorado ran from fall 2021 to spring 2023. Two monitoring sites were deployed in the ERW as part of SAIL. The two sites were the Aerosol Observation System (AOS) located on Crested Butte Ski Mountain, and the second ARM Mobile Facility (AMF2), located at the Rocky Mountain Biological Laboratory in Gothic, Colorado. To gain a more comprehensive understanding of aerosols in complex, mountainous terrain, Handix Scientific deployed SAIL-Net, a distributed network of six measurement nodes spanning the domain of the SAIL research area from October 2021 to July 2023. Each node measured aerosol particles between 140 nm and 3.4 μm in diameter using a small portable optical particle spectrometer (POPS; Gao et al. 2016), cloud condensation nuclei (CNN) using a miniature CCN counter (CloudPuck), and ice nucleating particles (INP) using the time-resolved aerosol filter sampler (TRAPS; Creamean et al. 2018). Our approach was similar to other studies that aimed to better characterize and understand aerosols and gas-phase pollutants using networks of lower-cost sensors (Caubel et al. 2019, Kelly et al. 2021, Asher et al. 2022). Such studies have identified neighborhood-level variations in pollutant concentrations (Schneider et al. 2017, Popoola et al. 2018, Caubel et al. 2019). Small-scale variations such as this are poorly represented in models and poorly measured by a single monitoring system (Caubel et al. 2019). Previous work has shown the representation error (the ability of measurements to represent a larger area) increases with complex orography, leading to decreases in model accuracy (Schutgens et al. 2017). The overall goal of SAIL-Net was to improve our understanding of the variability of aerosol in the ERW, thus increasing our knowledge of aerosol-cloud interactions in this region and informing the usefulness of distributed networks of measurements for future studies. We met this goal by answering the following science questions: 1. What is the aerosol temporal variability, and how does aerosol inhomogeneity vary seasonally? Is there significant seasonal variability in sources, or are short-term meteorological conditions the most important determining factor in sources for cloud nuclei? 2. What is the aerosol spatial variability? What are the aerosol characteristics at cloud base, presumably the particles most representative of those acting as cloud nuclei? 3. How should measurement networks be designed to capture aerosol-cloud interactions, and what do they need to measure? Can a single measurement site accurately represent aerosol properties in regions of complex terrain? SAIL-Net consisted of six measurement nodes spread across the ERW near Crested Butte, Colorado. The primary objective in site placement was to select locations that captured the vertical variation in aerosol properties while also spanning the domain of the SAIL campaign. The elevation of the sites ranged from roughly 2750 m along the valley floor of the ERW to approximately 3500 m near the top of Crested Butte Mountain, which is one of the taller peaks in the ERW. The farthest distance between sites was 14 km, while the closest two sites were approximately 1 km apart. Two of the sites were collocated with the ARM SAIL sites; our instruments sat on top of one of the trailers at AOS and another one of our sites was located in a meadow just above AMF2.

54 ENVIRONMENTAL SCIENCES↗

Strong Dependence of Atmospheric Feedbacks on Mixed-Phase Microphysics and Aerosol-Cloud Interactions in HadGEM3

We analyze the atmospheric processes that explain the large changes in radiative feed-backs between the two latest climate configurations of the Hadley Centre Global Environmental model. We use a large set of atmosphere-only climate-change simulations (amip and amip-p4K) to separate the contributions to the differences in feedback parameter from all the atmospheric model developments between the two latest model configurations. We show that the differences are mostly driven by changes in the shortwave cloud radiative feedback in the midlatitudes, mainly over the Southern Ocean. Two new schemes explain most of the differences: the introduction of a new aerosol scheme; and the development of a new mixed-phase cloud scheme. Both schemes reduce the strength of the pre-existing shortwave negative cloud feedback in the midlatitudes. The new aerosol scheme dampens a strong aerosol-cloud interaction, and it also suppresses a negative clear-sky shortwave feedback. The mixed-phase scheme increases the amount of cloud liquid water path (LWP) in the present-day, thereby reducing the radiative effciency of the increase of LWP in the warmer climate. It also enhances a strong, pre-existing, positive cloud fraction feedback. We assess the realism of the changes by comparing present-day simulations against observations, and discuss avenues that could help constrain the relevant processes.

HadGEM3↗

Clouds, aerosols, and photochemistry in the Jovian atmosphere

An assessment is made of the development status of concepts for cloud and aerosol compositions, vertical and horizontal distributions, and microphysical properties, in the Jovian upper troposphere and stratosphere. Attention is given to several key photochemical species' relationships to aerosol formation as well as their transport process implications, treating photochemistry in the context of comparative planetology and noting differences and similarities among the outer planet atmospheres; since this approach emphasizes observational data, a variegated assortment of ground-based and spacecraft observations is assembled. Current views on the tropospheric distribution of clouds are challenged, and a rationale is presented for alternative accounts.

West, R. A.↗

The Atmosphere Observing System (AOS): Synergistic Aerosol, Cloud, Convection and Precipitation Measurement and Modeling Systems

The 2017 Decadal Survey (DS) highlighted Earth System Science themes, science and application questions, and several high priority objectives that have led to the inclusion of Aerosols (A) and Clouds-Convection-Precipitation (CCP) as Designated Observables (DOs). On June 1, 2018, several NASA centers (GSFC, LaRC, JPL, MSFC, GRC and ARC) submitted a joint Study Plan to the NASA Earth Science Division for the Aerosol (A) and Cloud, Convection, and Precipitation (CCP) Pre-formulation Study (ACCP), with the ACCP Study concluding in early 2021. The new mission now in pre-phase A is being referred to as the Atmosphere Observing System (AOS), an integral part of NASA’s Earth System Observatory (ESO) strategy. The DS and the ACCP team recognized the science merit in combining the A and CCP DOs for both enhancing the ability to address a number of science objectives and also to provide an expanded capability to address additional objectives beyond those of the individual DOs. A critical element of the ACCP observing strategy is to make extensive use of new passive and active sensors as well as of the so-called Program-of-Record (PoR), complemented by a fully integrated sub-orbital component. In order to achieve maximum benefit, all these observations need to be integrated into comprehensive observing and modeling/data assimilation systems. Such an approach requires comprehensive model-data synthesis capabilities that needs to be conceived in conjunction with the space-based and suborbital components of AOS. In this presentation we will summarize the major science goals of AOS including cloud feedbacks, atmospheric convection, emphasizing aerosol processes and aerosol radiative effects, and the synergistic aspects of clouds-precipitation-aerosol interactions. We will describe examples of how AOS data will be used across space and time to better initialize forecasts and train modeling systems, and to infuse models and data assimilation systems with AOS data for advancing operational predictions and to generate expanded hindcasts and reconstruction of the climate record.

Arlindo da Silva↗