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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS2009

A GCM Study of Responses of the Atmospheric Water Cycle of West Africa and the Atlantic to Saharan Dust Radiative Forcing

The responses of the atmospheric water cycle and climate of West Africa and the Atlantic to radiative forcing of Saharan dust are studied using the NASA finite volume general circulation model (fvGCM), coupled to a mixed layer ocean. We find evidence of an "elevated heat pump" (EHP) mechanism that underlines the responses of the atmospheric water cycle to dust forcing as follow. During the boreal summerr, as a result of large-scale atmospheric feedback triggered by absorbing dust aerosols, rainfall and cloudiness are ehanIed over the West Africa/Eastern Atlantic ITCZ, and suppressed over the West Atlantic and Caribbean region. Shortwave radiation absorption by dust warms the atmosphere and cools the surface, while longwave has the opposite response. The elevated dust layer warms the air over West Africa and the eastern Atlantic. As the warm air rises, it spawns a large-scale onshore flow carrying the moist air from the eastern Atlantic and the Gulf of Guinea. The onshore flow in turn enhances the deep convection over West Africa land, and the eastern Atlantic. The condensation heating associated with the ensuing deep convection drives and maintains an anomalous large-scale east-west overturning circulation with rising motion over West Africa/eastern Atlantic, and sinking motion over the Caribbean region. The response also includes a strengthening of the West African monsoon, manifested in a northward shift of the West Africa precipitation over land, increased low-level westerlies flow over West Africa at the southern edge of the dust layer, and a near surface westerly jet underneath the dust layer overr the Sahara. The dust radiative forcing also leads to significant changes in surface energy fluxes, resulting in cooling of the West African land and the eastern Atlantic, and warming in the West Atlantic and Caribbean. The EHP effect is most effective for moderate to highly absorbing dusts, and becomes minimized for reflecting dust with single scattering albedo at0.95 or higher.

Lau, K. M.↗
NASA NTRS2010

Response of the Water Cycle of West Africa and Atlantic to Radiative Forcing by Saharan Dust

The responses of the atmospheric water cycle and climate of West Africa and the Atlantic to radiative forcing of Saharan dust are studied using the NASA finite volume general circulation model (fvGCM), coupled to a mixed layer ocean. We find evidence in support of the "elevated heat pump" (EHP) mechanism that underlines the responses of the atmospheric water cycle to dust forcing as follow. During the boreal summer, as a result of large-scale atmospheric feed back triggered by absorbing dust aerosols, rainfall and cloudiness are enhanced over the West Africa/Easter Atlantic ITCZ, and suppressed over the West Atlantic and Caribbean. region. Shortwave radiation absorption by dust warms the atmosphere and cools the surface, while long wave has the opposite response. The elevated dust layer warms the air over Nest Africa and the eastern Atlantic. The condensation heating associated with the induced deep convection drives and maintains an anomalous large-scale east-west overturning circulation with rising motion over West Africa/eastern Atlantic, and sinking motion over the Caribbean region. The response also includes a strengthening of the West African monsoon, manifested in northward shift of the West Africa precipitation over land, increased low-level westerlies flow over West Africa at the southern edge of the dust layer, and a near surface energy fluxes, resulting in cooling of the Nest African land and the eastern Atlantic, and a warming in the West Atlantic and Caribbean. The EHP effect is most effective for moderate to highly absorbing dusts, and becomes minimized for reflecting dust with single scattering albedo at 0.95 or higher.

Lau, K. M.↗
NASA NTRS2004

Top-of-Atmosphere Direct Radiative Effect of Aerosols over Global Oceans from Merged CERES and MODIS Observations

The direct radiative effect of aerosols (DREA) is defined as the difference between radiative fluxes in the absence and presence of aerosols. In this study, the direct radiative effect of aerosols is estimated for 46 months (March, 2000 to December, 2003) of merged CERES and MODIS Terra global measurements over ocean. This analysis includes the contribution from clear regions in both clear and partly cloudy CERES footprints. MODIS-CERES narrow-to-broadband regressions are developed to convert clear-sky MODIS narrowband radiances to broadband SW radiances, and CERES clear-sky Angular Distribution Models (ADMs) are used to estimate the corresponding TOA radiative fluxes needed to determine the DREA. Clear-sky MODIS pixels are identified using two independent cloud masks: (i) the NOAA-NESDIS algorithm used for inferring aerosol properties from MODIS on the CERES Single Scanner Footprint TOA/Surface Fluxes and Clouds (SSF) product (NOAA-SSF); and (ii) the standard algorithm used by the MODIS aerosol group to produce the MODO4 product (MODO4). Over global oceans, direct radiative cooling by aerosols for clear scenes identified from MODO4 is estimated to be 5.5 W m-2, compared to 3.8 W m-2 for clear scenes from NOAA-SSF. Regionally, differences are largest in areas affected by dust aerosol, such as oceanic regions adjacent to the Saharan and Saudi Arabian deserts, and in northern Pacific Ocean regions influenced by dust transported from Asia. The net total-sky (clear and cloudy) DREA is negative (cooling) and is estimated to be -2.0 W m-2 from MOD04, and -1.6 W m-2 from NOAA-SSF. The DREA is shown to have pronounced seasonal cycles in the Northern Hemisphere and large year-to-year fluctuations near deserts. However, no systematic trend in deseasonalized anomalies of the DREA is observed over the 46-month time series considered.

Loeb, N. G.↗
NASA NTRS2020

Aerosol Layer Height with Enhanced Spectral Coverage Achieved by Synergy between VIIRS and OMPS-NM Measurements

This letter presents a near production-ready algorithm to retrieve the height of biomass burning smoke and mineral dust aerosols as part of National Aeronautics and Space Administration (NASA)’s Deep Blue aerosol data product suite. It utilizes the enhanced spectral coverage achieved by using colocated data from the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM), both aboard the Suomi National Polar-orbiting Partnership (S-NPP) satellite. In particular, the 412-nm top-of-atmosphere (TOA) reflectance from VIIRS and the ultraviolet aerosol index from OMPS-NM are used to determine the height and single-scattering albedo of the absorbing aerosols simultaneously. Constraints on aerosol optical depth at 550 nm and surface reflectance for the 412-nm band are provided by the operational VIIRS Deep Blue aerosol product. Wildfire smoke layer heights obtained from the algorithm over North America, where smoke plumes often stretched thousands of kilometers, are shown to agree with those from Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements, with an uncertainty generally within 1–1.5 km. This new height data set will be included in the upcoming Version 2 VIIRS Deep Blue aerosol product.

aerosol↗
NASA NTRS2020

Aerosol Layer Height With Enhanced Spectral Coverage Achieved by Synergy Between VIIRS and OMPS-NM Measurements

This study presents a near production-ready algorithm to retrieve the height of biomass burning smoke and mineral dust aerosols as part of NASA’s Deep Blue aerosol data product suite. It utilizes the enhanced spectral coverage achieved by using co-located data from the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM), both aboard the Suomi National Polar-orbiting Partnership (S-NPP) satellite. Specifically, the 412 nm top-of-atmosphere reflectance from VIIRS and the ultraviolet aerosol index from OMPS-NM are used to determine the height and single-scattering albedo of the absorbing aerosols simultaneously. Constraints on aerosol optical depth at 550 nm and surface reflectance for the 412 nm band are provided by the operational VIIRS Deep Blue aerosol product. Wildfire smoke layer heights obtained from the algorithm over North America, where smoke plumes often stretched thousands of kilometers, are shown to agree with those from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements, with an uncertainty generally within 1-1.5 km. This new height data set will be included in the upcoming Version 2 VIIRS Deep Blue aerosol product.

Aerosol↗
NASA NTRS2013

Tropical Atlantic Dust and Smoke Aerosol Variations Related to the Madden-Julian Oscillation in MODIS and MISR Observations

In this study, Moderate Resolution Imaging Spectroradiometer (MODIS) fine mode fraction and Multi-angle Imaging SpectroRadiometer (MISR) nonspherical fraction data are used to derive dust and smoke aerosol optical thickness (T(sub dust) and T(sub smoke)) over the tropical Atlantic in a complementary way: due to its wider swath, MODIS has 3-4 times greater sampling than MISR, but MISR dust discrimination is based on particle shape retrievals, whereas an empirical scheme is used for MODIS. MODIS and MISR show very similar dust and smoke winter climatologies. T(sub dust) is the dominant aerosol component over the tropical Atlantic, accounting for 40-70 percent of the total aerosol optical thickness (AOT), whereas T(sub smoke) is significantly smaller than T(sub dust). The consistency and high correlation between these climatologies and their daily variations lends confidence to their use for investigating the relative dust and smoke contributions to the total AOT variation associated with the Madden-Julian Oscillation (MJO). The temporal evolution and spatial patterns of the τdus anomalies associated with the MJO are consistent between MODIS and MISR: the magnitude of MJO-realted T(sub dust) anomalies is comparable to or even larger than that of the total T, while the T(sub smoke) anomaly represents about 15 percent compared to the total, which is quite different from their relative magnitudes to the total T on the climatological time scale. This suggests that dust and smoke are not influenced by the MJO in the same way. Based on correlation analysis, dust is strongly influenced by the MJO-modulated trade wind and precipitation anomalies, and can last as long as one MJO phase, whereas smoke is less affected.

Madden-Julian Oscillation↗
NASA NTRS2020

Impact of Dust-Cloud-Radiation-Precipitation Dynamical Feedback on Subseasonal-to-Seasonal Variability of the Asian Summer Monsoon in Global Variable-Resolution Simulations With MPAS-CAM5

In this study, we investigate the effects of increased dust emission from the Middle East deserts on subseasonal-to-seasonal (S2S) variability of the Asian summer monsoon (ASM). Numerical experiments are performed using the Model for Prediction Across Scales (MPAS) coupled with the Community Atmosphere Model (CAM5) physics, with regional refinement at 30 km grid resolution over South Asia and the surrounding regions. Result shows that increased dust emission and transport from the Middle East/West Asia region induces a strong dust-cloud-radiation-precipitation-circulation feedback, resulting in a colder surface over the desert regions and the western Tibetan Plateau, but warmer and moister troposphere with enhanced cloudiness and precipitation over the Pakistan/Northwest India (PNWI) region. The latter changes are amplified by the dust aerosol induced Elevated Heat Pump (EHP) mechanism along the West Himalayas/Iranian Plateau foothill regions, most pronounced during May- June. During July-August, cloud radiation feedback further enhances the warming of the upper troposphere, and cooling of the land surface over the PNWI and adjacent regions overWest Asia. The upper tropospheric heating and increased precipitation over PNWI spur a large-scale anomalous Rossby wavetrain and a northward displacement of the subtropical jetstream, manifesting in a contraction of the South Asian High and westward shift of the Western Pacific Subtropical High. As a result, the entire ASM precipitation-cloud system is displaced westward. Precipitation and cloudiness are intensified over northwest and western India and west Asia, but suppressed over southern and central East Asia. Analyses of the S2S variability of the upper level vorticity balance suggests that heating by Middle East dust plays an important role in exciting, and anchoring a teleconnection pattern through interactions among dust cloud radiation, precipitation heating over the PNWI, the development of an upper level Rossby wavetrain, and the northward shift of the boreal summer jetstream over Eurasia.

Asian summer monsoon↗
DOE OSTI2024

Numerical coupling of aerosol emissions, dry removal, and turbulent mixing in the E3SM Atmosphere Model version 1 (EAMv1) – Part 2: A semi-discrete error analysis framework for assessing coupling schemes

Abstract. Part 1 (Wan et al., 2024) of this study discusses the motivation and empirical evaluation of a revision to the aerosol-related numerical process coupling in the atmosphere component of the Energy Exascale Earth System Model version 1 (EAMv1) to address the previously reported issue of strong sensitivity of the simulated dust aerosol lifetime and dry removal rate to the model's vertical resolution. This paper complements that empirical justification of the revised scheme with a mathematical justification leveraging a semi-discrete analysis framework for assessing the splitting error of process coupling methods. The framework distinguishes the error due to numerical splitting from the error due to the time integration method(s) used for each individual process. Such a distinction results in a framework that provides an intuitive understanding of the causes of the splitting error. The application of this framework to the dust life cycle in EAMv1 confirms (i) that the original EAMv1 scheme artificially strengthens the effect of dry removal processes and (ii) that the revised splitting reduces that artificial strengthening. While the error analysis framework is presented in the context of the dust life cycle in EAMv1, the framework can be broadly leveraged to evaluate process coupling schemes, both in other physical problems and for any number of processes. This framework will be particularly powerful when the various process implementations support a variety of time integration approaches. Whereas traditional local truncation error approaches require separate consideration of each combination of time integration methods, this framework enables evaluation of coupling schemes independent of particular time integration approaches for each process while still allowing for the incorporation of these specific time integration errors if so desired. The framework also explains how the splitting error terms result from (i) the integration of individual processes in isolation from other processes and (ii) the choices of input state and time step size for the isolated integration of processes. Such a perspective has the potential for the rapid development of alternative coupling approaches that utilize knowledge both about the desired accuracy and about the computational costs of individual processes.

58 GEOSCIENCES↗
DOE OSTI2025

Dust Direct Radiative Effect Including Large Particles and Component Minerals

The direct radiative effect (DRE) of dust aerosols in Earth system models (ESMs) remains highly uncertain, largely due to inadequate representations of particle size distribution (PSD) and mineral composition. Using NASA's Earth Surface Mineral Dust Source Investigation (EMIT) soil mineralogy data and observed PSD in an ESM that resolves dust mineral composition and emitted diameters from 0.1 to 70 μm, we find a near-neutral global dust net DRE (−0.057 W m −2 ), weaker than most previous estimates. Large dust (diameter >10 μm) contributes 30% of the global longwave dust optical depth, providing observational constraints on large-particle abundance, and offsets 20% of the dust shortwave cooling over major source regions. Incorporation of EMIT mineralogy reduces shortwave uncertainty by more than 50%. The remaining uncertainty mainly exists in processes controlling dust abundance, particularly the poorly understood transport of large dust, and longwave optical properties, which require additional observational constraints to more accurately quantify the dust DRE.

Li, Longlei [Cornell Univ., Ithaca, NY (United Sta↗
DOE OSTI2022

Relative importance of high-latitude local and long-range-transported dust for Arctic ice-nucleating particles and impacts on Arctic mixed-phase clouds

Dust particles, serving as ice-nucleating particles (INPs), may impact the Arctic surface energy budget and regional climate by modulating the mixed-phase cloud properties and lifetime. In addition to long-range transport from low-latitude deserts, dust particles in the Arctic can originate from local sources. However, the importance of high-latitude dust (HLD) as a source of Arctic INPs (compared to low-latitude dust, LLD) and its effects on Arctic mixed-phase clouds are overlooked. In this study, we evaluate the contribution to Arctic dust loading and INP population from HLD and six LLD source regions by implementing a source-tagging technique for dust aerosols in version 1 of the US Department of Energy's Energy Exascale Earth System Model (E3SMv1). Our results show that HLD is responsible for 30.7 % of the total dust burden in the Arctic, whereas LLD from Asia and North Africa contributes 44.2 % and 24.2 %, respectively. Due to its limited vertical transport as a result of stable boundary layers, HLD contributes more in the lower troposphere, especially in boreal summer and autumn when the HLD emissions are stronger. LLD from North Africa and East Asia dominates the dust loading in the upper troposphere with peak contributions in boreal spring and winter. The modeled INP concentrations show better agreement with both ground and aircraft INP measurements in the Arctic when including HLD INPs. The HLD INPs are found to induce a net cooling effect (-0.24 W m -2 above 60 °N) on the Arctic surface downwelling radiative flux by changing the cloud phase of the Arctic mixed-phase clouds. The magnitude of this cooling is larger than that induced by North African and East Asian dust (0.08 and -0.06 W m -2 , respectively), mainly due to different seasonalities of HLD and LLD. Uncertainties of this study are discussed, which highlights the importance of further constraining the HLD emissions.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2012

Size Resolved Measurements of Springtime Aerosol Particles over the Northern South China Sea

Large sources of aerosol particles and their precursors are ubiquitous in East Asia. Such sources are known to impact the South China Sea (henceforth SCS), a sometimes heavily polluted region that has been suggested as particularly vulnerable to climate change. To help elucidate springtime aerosol transport into the SCS, an intensive study was performed on the remote Dongsha (aka Pratas) Islands Atoll in spring 2010. As part of this deployment, a Davis Rotating-drum Uniform size-cut Monitor (DRUM) cascade impactor was deployed to collect size-resolved aerosol samples at the surface that were analyzed by X-ray fluorescence for concentrations of selected elements. HYSPLIT backtrajectories indicated that the transport of aerosol observed at the surface at Dongsha was occurring primarily from regions generally to the north and east. This observation was consistent with the apparent persistence of pollution and dust aerosol, along with sea salt, in the ground-based dataset. In contrast to the sea-level observations, modeled aerosol transport suggested that the westerly flow aloft (w700 hPa) transported smoke-laden air toward the site from regions from the south and west. Measured aerosol optical depth at the site was highest during time periods of modeled heavy smoke loadings aloft. These periods did not coincide with elevated aerosol concentrations at the surface, although the model suggested sporadic mixing of this free-tropospheric aerosol to the surface over the SCS. A biomass burning signature was not clearly identified in the surface aerosol composition data, consistent with this aerosol type remaining primarily aloft and not mixing strongly to the surface during the study. Significant vertical wind shear in the region also supports the idea that different source regions lead to varying aerosol impacts in different vertical layers, and suggests the potential for considerable vertical inhomogeneity in the SCS aerosol environment.

South China Sea↗
NASA NTRS2006

Aerosol-Water Cycle Interaction: A New Challenge in Monsoon Climate Research

Long recognized as a major environmental hazard, aerosol is now known to have strong impacts on both regional and global climate. It has been estimated that aerosol may reduce by up to 10% of the seasonal mean solar radiation reaching the earth surface, producing a global cooling effect that opposes global warming (Climate Change 2001). This means that the potential perils that humans have committed to global warming may be far greater than what we can detect at the present. As a key component of the Earth climate system, the water cycle is profoundly affected by the presence of aerosols in the atmosphere. Through the so-called direct effect , aerosol scatters and/or absorbs solar radiation, thus cooling the earth surface and changing the horizontal and vertical radiational heating contrast in the atmosphere. The heating contrast drives anomalous atmospheric circulation, resulting in changes in convection, clouds, and rainfall. Another way aerosol can affect the water cycle is through the so-called indirect effects, whereby aerosol increases the number of cloud condensation nuclei, prolongs life time of clouds, and inhibits the growth of cloud drops to raindrops. This leads to more clouds, and increased reflection of solar radiation, and further cooling at the earth surface. In monsoon regions, the response of the water cycle to aerosol forcing is especially complex, not only because of presence of diverse mix of aerosol species with vastly different radiative properties, but also because the monsoon is strongly influenced by ocean and land surface processes, land use, land change, as well as regional and global greenhouse warming effects. Thus, sorting out the impacts of aerosol forcing, and interaction with the monsoon water cycle is a very challenging problem. In this talk, I will offer some insights into how aerosols may impact the Asian monsoon based on preliminary results from satellite observations and climate model experiments. Specifically, I will discuss the elevated heat pump hypothesis, involving atmospheric heating by absorbing aerosols (dust and black carbon) over the southern slopes of the Himalayas, and feedback with the deep convection, in modifying monsoon water cycle over South .and East Asia. The role of aerosol forcing relative to those due to sea surface temperature and land surface processes, as well as observation requirements to verify such a hypothesis will also be discussed.

Lau, William K. M.↗
NASA NTRS2006

Aerosol-Water Cycle Interaction: A New Challenge in Monsoon Climate Research

Long recognized as a major environmental hazard, aerosol is now known to have strong impacts on both regional and global climate. It has been estimated that aerosol may reduce by up to 10% of the seasonal mean solar radiation reaching the earth surface, producing a global cooling effect that opposes global warming (Climate Change 2001). This means that the potential perils that humans have committed to global warming may be far greater than what we can detect at the present. As a key component of the Earth climate system, the water cycle is profoundly affected by the presence of aerosols in the atmosphere. Through the so-called "direct effect", aerosol scatters and/or absorbs solar radiation, thus cooling the earth surface and changing the horizontal and vertical radiational heating contrast in the atmosphere. The heating contrast drives anomalous atmospheric circulation, resulting in changes in convection, clouds, and rainfall. Another way aerosol can affect the water cycle is through the so-called "indirect effects", whereby aerosol increases the number of cloud condensation nuclei, prolongs life time of clouds, and inhibits the growth of cloud drops to raindrops. This leads to more clouds, and increased reflection of solar radiation, and further cooling at the earth surface. In monsoon regions, the response of the water cycle to aerosol forcing is especially complex, not only because of presence of diverse mix of aerosol species with vastly different radiative properties, but also because the monsoon is strongly influenced by ocean and land surface processes, land use, land change, as well as regional and global greenhouse warming effects. Thus, sorting out the impacts of aerosol forcing, and interaction with the monsoon water cycle is a very challenging problem. In this talk, I will offer some insights into how aerosols may impact the Asian monsoon based on preliminary results from satellite observations and climate model experiments. Specifically, I will discuss the "elevated heat pump" hypothesis, involving atmospheric heating by absorbing aerosols (dust and black carbon) over the southern slopes of the Himalayas, and feedback with the deep convection, in modifying monsoon water cycle over South and East Asia. The role of aerosol forcing relative to those due to sea surface temperature and land surface processes, as well as observation requirements to verify such a hypothesis will also be discussed.

Lau, William K. M.↗
NASA NTRS2018

Interactions Between Asian Air Pollution and Monsoon System: South Asia (ROSES-2014 ACMAP)

Asia's rapid economic growth over the past several decades has brought a remarkable increase in air pollution levels in that region. High concentrations of aerosols (also known as particulate matter or PM) from pollution sources pose major health hazards to half of the world population in Asia including South Asia. How do pollution and dust aerosols regulate the monsoon circulation and rainfall via scattering and absorbing solar radiation, changing the atmospheric heating rates, and modifying the cloud properties? We conducted a series of regional model experiments with NASA-Unified Weather Research and Forecast (NUWRF) regional model with coupled aerosol-chemistry-radiation-microphysics processes over South Asia for winter, pre-monsoon, and monsoon seasons to address this question. This study investigates the worsening air quality problem in South Asia by focusing on the interactions between pollution and South Asian monsoon, not merely focusing on the increase of pollutant emissions.

regional model experiments with NASA-Unified Weath↗
NASA NTRS1978

Retrieving the complex refractive index of atmospheric aerosols from ratios of solar spectral extinction measurements

The technique proposed by Fymat (1976) for retrieving the complex refractive index of atmospheric aerosols using narrowband spectral transmission ratios, taken within an overall narrow spectral interval, is investigated in the case of modelled polydispersions of rural, maritime-continental, maritime-sea spray and meteoric dust aerosols. It is confirmed that for not too broad size distributions most of the information comes from a narrow size range of 'active' aerosols so that, under these circumstances, the refractive index components can indeed be retrieved essentially independently of the size distribution. For 0.1% accurate data in three colors, the technique can provide the real and imaginary components of the index respectively within 0.07% and 0.3% accuracy.

Fymat, A. L.↗
NASA NTRS2014

Operational Dust Prediction

Over the last few years, numerical prediction of dust aerosol concentration has become prominent at several research and operational weather centres due to growing interest from diverse stakeholders, such as solar energy plant managers, health professionals, aviation and military authorities and policymakers. Dust prediction in numerical weather prediction-type models faces a number of challenges owing to the complexity of the system. At the centre of the problem is the vast range of scales required to fully account for all of the physical processes related to dust. Another limiting factor is the paucity of suitable dust observations available for model, evaluation and assimilation. This chapter discusses in detail numerical prediction of dust with examples from systems that are currently providing dust forecasts in near real-time or are part of international efforts to establish daily provision of dust forecasts based on multi-model ensembles. The various models are introduced and described along with an overview on the importance of dust prediction activities and a historical perspective. Assimilation and evaluation aspects in dust prediction are also discussed.

assimilation↗
DOE OSTI2023

Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts

Soil dust aerosols are a key component of the climate system, as they interact with short- and long-wave radiation, alter cloud formation processes, affect atmospheric chemistry and play a role in biogeochemical cycles by providing nutrient inputs such as iron and phosphorus. The influence of dust on these processes depends on its physicochemical properties, which, far from being homogeneous, are shaped by its regionally varying mineral composition. The relative amount of minerals in dust depends on the source region and shows a large geographical variability. However, many state-of-the-art Earth system models (ESMs), upon which climate analyses and projections rely, still consider dust mineralogy to be invariant. The explicit representation of minerals in ESMs is more hindered by our limited knowledge of the global soil composition along with the resulting size-resolved airborne mineralogy than by computational constraints. In this work we introduce an explicit mineralogy representation within the state-of-the-art Multiscale Online Nonhydrostatic AtmospheRe CHemistry (MONARCH) model. We review and compare two existing soil mineralogy datasets, which remain a source of uncertainty for dust mineralogy modeling and provide an evaluation of multiannual simulations against available mineralogy observations. Soil mineralogy datasets are based on measurements performed after wet sieving, which breaks the aggregates found in the parent soil. Our model predicts the emitted particle size distribution (PSD) in terms of its constituent minerals based on brittle fragmentation theory (BFT), which reconstructs the emitted mineral aggregates destroyed by wet sieving. Our simulations broadly reproduce the most abundant mineral fractions independently of the soil composition data used. Feldspars and calcite are highly sensitive to the soil mineralogy map, mainly due to the different assumptions made in each soil dataset to extrapolate a handful of soil measurements to arid and semi-arid regions worldwide. For the least abundant or more difficult-to-determine minerals, such as iron oxides, uncertainties in soil mineralogy yield differences in annual mean aerosol mass fractions of up to ~ 100 %. Although BFT restores coarse aggregates including phyllosilicates that usually break during soil analysis, we still identify an overestimation of coarse quartz mass fractions (above 2 µm in diameter). In a dedicated experiment, we estimate the fraction of dust with undetermined composition as given by a soil map, which makes up ~ 10 % of the emitted dust mass at the global scale and can be regionally larger. Changes in the underlying soil mineralogy impact our estimates of climate-relevant variables, particularly affecting the regional variability of the single-scattering albedo at solar wavelengths or the total iron deposited over oceans. All in all, this assessment represents a baseline for future model experiments including new mineralogical maps constrained by high-quality spaceborne hyperspectral measurements, such as those arising from the NASA Earth Surface Mineral Dust Source Investigation (EMIT) mission.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

Quantifying the Influence of Mechanistic Representation of Particle Dry Deposition on Historical Changes in Aerosol-Climate Interactions

Dry deposition removes short-lived climate forcers and their precursors from the atmosphere. The aerosol dry deposition schemes in many global climate models have been untouched for decades. Previous work hints that aerosol dry deposition is an uncertainty with respect to aerosol impacts on climate change. Here we demonstrate the impact of a more mechanistic aerosol dry deposition parameterization on the historical aerosol direct and cloud albedo effects using the NASA GISS global chemistry-climate model. We investigate two aerosol configurations – a “bulk” mass-based scheme and a modal scheme that more explicitly represents internal mixing and microphysics – of the global model. Both configurations show ~20% larger historical increases in non-dust aerosols globally with more mechanistic dry deposition. Changes to particle dry deposition, which are strongly a function of particle diameter, have a greater influence on the cloud albedo effect (up to 0.1 W m-2) when aerosols are more explicitly resolved in the modal scheme. On the other hand, impacts on the direct aerosol effect are small for both model configurations. In both aerosol configurations, the global climate effects are relatively insensitive to uncertainty in the strength of the uptake to dry deposition as suggested by (limited) measurements. In general, the low number of aerosol flux measurements and strong variability across existing observations challenge confidence in our understanding of dry depositional processes and changes with environmental conditions. Nonetheless, our work suggests that changes in dry deposition may be important for accurately estimating increases in aerosol abundances over the historical period, which is key for correct inferences about how cooling from aerosols has offset warming from greenhouse gases.

Dry deposition↗