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Atmospheric transport of pollutants from North America to the North Atlantic Ocean

Ground-based measurements strongly support the hypothesis that pollutant materials of anthropogenic origin are being transported over long distances in the midtroposphere and are a significant source of acid rain, acid snow, trace metal deposition, ozone and visibility-reducing aerosols in remote oceanic and polar regions of the Norhern Hemisphere. Atmospheric sulphur budget calculations and studies of acid rain on Bermuda indicate that a large fraction of pollutant materials emitted into the atmosphere in eastern North America are advected eastwards over the North Atlantic Ocean. The first direct airborne measurements of the vertical distribution of tropospheric aerosols over the western North Atlantic is reported here. A newly developed airborne differential adsorption lidar system was used to obtain continuous, remotely sensed aerosol distributions along its flight path. The data document two episodes of long-distance transport of pollutant materials from North America over the North Atlantic Ocean.

Harriss, R. C.↗

Surface Ocean pCO2 Seasonality and Sea-Air CO2 Flux Estimates for the North American East Coast

Underway and in situ observations of surface ocean pCO2, combined with satellite data, were used to develop pCO2 regional algorithms to analyze the seasonal and interannual variability of surface ocean pCO2 and sea-air CO2 flux for five physically and biologically distinct regions of the eastern North American continental shelf: the South Atlantic Bight (SAB), the Mid-Atlantic Bight (MAB), the Gulf of Maine (GoM), Nantucket Shoals and Georges Bank (NS+GB), and the Scotian Shelf (SS). Temperature and dissolved inorganic carbon variability are the most influential factors driving the seasonality of pCO2. Estimates of the sea-air CO2 flux were derived from the available pCO2 data, as well as from the pCO2 reconstructed by the algorithm. Two different gas exchange parameterizations were used. The SS, GB+NS, MAB, and SAB regions are net sinks of atmospheric CO2 while the GoM is a weak source. The estimates vary depending on the use of surface ocean pCO2 from the data or algorithm, as well as with the use of the two different gas exchange parameterizations. Most of the regional estimates are in general agreement with previous studies when the range of uncertainty and interannual variability are taken into account. According to the algorithm, the average annual uptake of atmospheric CO2 by eastern North American continental shelf waters is found to be between 3.4 and 5.4 Tg C/yr (areal average of 0.7 to 1.0 mol CO2 /sq m/yr) over the period 2003-2010.

interannual variability↗

The East Atlantic - West Russia Teleconnection in the North Atlantic: Climate Impact and Relation to Rossby Wave Propagation

Large-scale winter teleconnection of the East Atlantic - West Russia (EA-WR) over the Atlantic and surrounding regions is examined in order to quantify its impacts on temperature and precipitation and identify the physical mechanisms responsible for its existence. A rotated empirical orthogonal function (REOF) analysis of the upper-tropospheric monthly height field captures successfully the EA-WR pattern and its interannual variation, with the North Atlantic Oscillation as the first mode. EA-WRs climate impact extends from eastern North America to Eurasia. The positive (negative) EA-WR produces positive (negative) temperature anomalies over the eastern US, western Europe and Russia east of Caspian Sea, with negative (positive) anomalies over eastern Canada, eastern Europe including Ural Mountains and the Middle East. These anomalies are largely explained by lower-tropospheric temperature advections. Positive (negative) precipitation anomalies are found over the mid-latitude Atlantic and central Russia around 60E, where lower-level cyclonic (anticyclonic) circulation anomaly is dominant. The eastern Canada and the western Europe are characterized by negative (positive) precipitation anomalies.The EA-WR is found to be closely associated with Rossby wave propagation. Wave activity fluxes show that it is strongly tied to large-scale stationary waves. Furthermore, a stationary wave model (SWM) forced with vorticity transients in the mid-latitude Atlantic (approximately 40N) or diabatic heat source over the subtropical Atlantic near the Caribbean Sea produces well-organized EA-WR-like wave patterns, respectively. Sensitivity tests with the SWM indicate improvement in the simulation of the EA-WR when the mean state is modified to have a positive NAO component that enhances upper-level westerlies between 40-60N.

EA/WR↗

Cropland abandonment between 1986 and 2018 across the United States: spatiotemporal patterns and current land uses

Knowing where and when croplands have been abandoned or otherwise removed from cultivation is fundamental to evaluating future uses of these areas, e.g. as sites for ecological restoration, recultivation, bioenergy production, or other uses. However, large uncertainties remain about the location and time of cropland abandonment and how this process and the availability of associated lands vary spatially and temporally across the United States. Here, we present a nationwide, 30 m resolution map of croplands abandoned throughout the period of 1986–2018 for the conterminous United States (CONUS). We mapped the location and time of abandonment from annual cropland layers we created in Google Earth Engine from 30 m resolution Landsat imagery using an automated classification method and training data from the U.S. Department of Agriculture Cropland Data Layer. Our abandonment map has overall accuracies of 0.91 and 0.65 for the location and time of abandonment, respectively. From 1986 to 2018, 12.3 (±2.87) million hectares (Mha) of croplands were abandoned across CONUS, with areas of greatest change over the Ogallala Aquifer, the southern Mississippi Alluvial Plain, the Atlantic Coast, North Dakota, northern Montana, and eastern Washington state. The average annual nationwide abandoned area across our study period was 0.51 Mha per year. Annual abandonment peaked between 1997 and 1999 at a rate of 0.63 Mha year –1 , followed by a continuous decrease to 0.41 Mha year –1 in 2009–2011. Among the abandoned croplands, 53% (6.5 Mha) changed to grassland and pasture, 18.6% (2.28 Mha) to shrubland and forest, 8.4% (1.03 Mha) to wetlands, and 4.6% (0.56 Mha) to non-vegetated lands. Of the areas that we mapped as abandoned, 19.6% (2.41 Mha) were enrolled in the Conservation Reserve Program as of 2020. Our new map highlights the long-term dynamic nature of agricultural land use and its relation to various competitive pressures and land use policies in the United States.

54 ENVIRONMENTAL SCIENCES↗

Cold-air outbreaks in the continental US: Connections with stratospheric variations

Mid-latitude Northern Hemisphere extreme cold events continue to occur despite overall winter warming trends. These events have been linked to weakened stratospheric polar vortex (SPV) states. In this study, we analyze both the upper and lower polar stratosphere for links to extreme winter cold and snow in the continental US, finding two SPV variations of interest. The first features an upper-level vortex displaced toward western Canada and linked to northwestern US severe winter weather. The second features a weakened upper-level vortex displaced toward the North Atlantic and linked to central-eastern US severe winter weather. Both variations feature lower-level stretched vortices and stratospheric wave reflection. Since 2015, a northwestward shift in severe winter weather across the US is concurrent with an increase in the frequency of the westward-focused variation relative to the eastward-focused variation and a shift to more negative phases of the El Niño–Southern Oscillation.

Science & Technology - Other Topics↗

Changes in Tropical Cyclone Intensity Over the Past 30 Years: A Global and Dynamic Perspective

The hurricane season of 2005 was the busiest on record and Hurricane Katrina (2005) is believed to be the costliest hurricane in U. S. history. There are growing concerns regarding whether this increased tropical cyclone activity is a result of global warming, as suggested by Emanuel(2005) and Webster et al. (2005), or just a natural oscillation (Goldenberg et al. 2001). This study examines the changes in tropical cyclone intensity to see what were really responsible for the changes in tropical cyclone activity over the past 30 years. Since the tropical sea surface temperature (SST) warming also leads to the response of atmospheric circulation, which is not solely determined by the local SST warming, this study suggests that it is better to take the tropical cyclone activities in the North Atlantic (NA), western North Pacific (WNP) and eastern North Pacific (ENP) basins as a whole when searching for the influence of the global-scale SST warming on tropical cyclone intensity. Over the past 30 years, as the tropical SST increased by about 0.5 C, the linear trends indicate 6%, 16% and 15% increases in the overall average intensity and lifetime and the annual frequency. Our analysis shows that the increased annual destructiveness of tropical cyclones reported by Emanuel(2005) resulted mainly from the increases in the average lifetime and annual frequency in the NA basin and from the increases in the average intensity and lifetime in the WNP basin, while the annual destructiveness in the ENP basin generally decreased over the past 30 years. The changes in the proportion of intense tropical cyclones reported by Webster et a1 (2005) were due mainly to the fact that increasing tropical cyclones took the tracks that favor for the development of intense tropical cyclones in the NA and WNP basins over the past 30 years. The dynamic influence associated with the tropical SST warming can lead to the impact of global warming on tropical cyclone intensity that may be very different from our current assessments, which were mainly based on the thermodynamic theory of tropical cyclone intensity.

Wu, Liguang↗

Identification of major moisture sources across the Mediterranean Basin

We employ a Lagrangian based moisture back trajectory method on an ensemble of four reanalysis datasets to provide a comprehensive understanding of moisture sources over the Mediterranean land region (30° N–49.5° N and 9.75° W–61.5° E) at seasonal timescales for 1980–2013 period. Using a source region between 10° S–71.35° N along the latitude and 80° W–84.88° E along the longitude that is subdivided into ten complimentary sub-regions, our analyses is able to backtrack up to > 90% of seasonal precipitation at each grid point within the target region. Our results indicate a significant role of moisture advected from the North Atlantic and Mediterranean Sea, and locally recycled moisture over the target region in shaping the spatial organization of seasonal precipitation. However, a clear east–west contrast is witnessed in determining the relative importance of each of these major moisture sources where the North Atlantic dictates the moisture supply over the western Mediterranean while moisture from Mediterranean Sea and local recycling play a key role over the eastern Mediterranean. Our analyses also demonstrate a major footprint of the North Atlantic Oscillation (NAO) on precipitation variability over the Mediterranean land as dynamic and thermodynamic anomalies during the negative phase of NAO match with those during wet years and vice versa. The findings reported here are generally consistent across the four reanalysis datasets. Overall, this study establishes the relative roles of adjacent and far-off oceanic and terrestrial evaporative sources over the Mediterranean land and should help in understanding the drivers of precipitation variability and change at varying timescales.

54 ENVIRONMENTAL SCIENCES↗

On isostasy at Atlantic-type continental margins

The concept of isostasy describes the manner in which topographic features on the earth's surface are compensated at depth. The present investigation is concerned with the isostatic mechanism at Atlantic-type continental margins. Particular attention is given to the question whether the flexure model of isostasy, which has successfully been used at other geological features in oceans, is applicable at margins. Cross-spectral techniques are used to analyze the relationship between free air gravity and topography at Atlantic-type continental margins. The relatively old eastern North America is found to be associated with the highest value of the effective elastic thickness in the range 10-20 km, while the relatively young Coral Sea/Lord Howe rise is associated with the lowest value of less than 5 km. The differences in estimates of effective elastic thickness between margins can be explained by a simple model in which the flexural strength of the basement increases with age.

Karner, G. D.↗

Evaluation of Space-Based Constraints on Global Nitrogen Oxide Emissions with Regional Aircraft Measurements over and Downwind of Eastern North America

We retrieve tropospheric nitrogen dioxide (NO 2) columns for May 2004 to April 2005 from the SCIAMACHY satellite instrument to derive top-down emissions of nitrogen oxides (NO(x) = NO + NO2) via inverse modeling with a global chemical transport model (GEOS-Chem). Simulated NO 2 vertical profiles used in the retrieval are evaluated with airborne measurements over and downwind of North America (ICARTT); a northern midlatitude lightning source of 1.6 Tg N/yr minimizes bias in the retrieval. Retrieved NO2 columns are validated (r2 = 0.60, slope = 0.82) with coincident airborne in situ measurements. The top-down emissions are combined with a priori information from a bottom-up emission inventory with error weighting to achieve an improved a posteriori estimate of the global distribution of surface NOx emissions. Our a posteriori NOx emission inventory for land surface NOx emissions (46.1 Tg N/yr) is 22% larger than the GEIA-based a priori bottom-up inventory for 1998, a difference that reflects rising anthropogenic emissions, especially from East Asia A posteriori NOx emissions for East Asia (9.8 Tg N/yr) exceed those from other continents. The a posteriori inventory improves the GEOS-Chem simulation of NOx, peroxyacetylnitrate, and nitric acid with respect to airborne in situ measurements over and downwind of New York City. The a posteriori is 7% larger than the EDGAR 3.2FT2000 global inventory, 3% larger than the NEI99 inventory for the United States, and 68% larger than a regional inventory for 2000 for eastern Asia. SCIAMACHY NO2 columns over the North Atlantic show a weak plume from lightning NO(x).

Martin, Randall V.↗

Estuarine Dissolved Organic Carbon Flux From Space: With Application to Chesapeake and Delaware Bays

This study uses a neural network model trained with in situ data, combined with satellite data and hydrodynamic model products, to compute the daily estuarine export of dissolved organic carbon (DOC) at the mouths of Chesapeake Bay (CB) and Delaware Bay (DB) from 2007 to 2011. Both bays show large flux variability with highest fluxes in spring and lowest in fall as well as interannual flux variability (0.18 and 0.27 Tg C/year in 2008 and 2010 for CB; 0.04 and 0.09 Tg C/year in 2008 and 2011 for DB). Based on previous estimates of total organic carbon (TOCexp) exported by all Mid-Atlantic Bight estuaries (1.2 Tg C/year), the DOC export (CB + DB) of 0.3 Tg C/year estimated here corresponds to 25% of the TOCexp. Spatial and temporal covariations of velocity and DOC concentration provide contributions to the flux, with larger spatial influence. Differences in the discharge of fresh water into the bays (74 billion cu. m/year for CB and 21 billion cu. m/year for DB) and their geomorphologies are major drivers of the differences in DOC fluxes for these two systems. Terrestrial DOC inputs are similar to the export of DOC at the bay mouths at annual and longer time scales but diverge significantly at shorter time scales (days to months). Future efforts will expand to the Mid-Atlantic Bight and Gulf of Maine, and its major rivers and estuaries, in combination with coupled terrestrial-estuarine-ocean biogeochemical models that include effects of climate change, such as warming and CO2 increase.

Estuarine DOC export↗

Secular Changes in the Solar Semidiurnal Tide of the Western North Atlantic Ocean

An analysis of twentieth century tide gauge records reveals that the solar semidiurnal tide S, has been decreasing in amplitude along the eastern coast of North America and at the mid-ocean site Bermuda. In relative terms the observed rates are unusually large, of order 10% per century. Periods of greatest change, however, are inconsistent among the stations, and roughly half the stations show increasing amplitude since the late 1990s. Excepting the Gulf of Maine, lunar tides are either static or slightly increasing in amplitude; a few stations show decreases. Large changes in solar, but not lunar, tides suggest causes related to variable radiational forcing, but the hypothesis is at present unproven. Citation: Ray, R. D. (2009), Secular changes in the solar semidiurnal tide of the western North Atlantic Ocean

Ray, Richard D.↗

Convective transport over the central United States and its role in regional CO and ozone budgets

We have constructed a regional budget for boundary layer carbon monoxide over the central United States (32.5 deg - 50 deg N, 90 deg - 105 deg W), emphasizing a detailed evaluation of deep convective vertical fluxes appropriate for the month of June. Deep convective venting of the boundary layer (upward) dominates other components of the CO budget, e.g., downward convective transport, loss of CO by oxidation, anthropogenic emissions, and CO produced from oxidation of methane, isoprene, and anthropogenic nonmethane hydrocarbons (NMHCs). Calculations of deep convective venting are based on the method pf Pickering et al.(1992a) which uses a satellite-derived deep convective cloud climatology along with transport statistics from convective cloud model simulations of observed prototype squall line events. This study uses analyses of convective episodes in 1985 and 1989 and CO measurements taken during several midwestern field campaigns. Deep convective venting of the boundary layer over this moderately polluted region provides a net (upward minus downward) flux of 18.1 x 10(exp 8) kg CO/month to the free troposphere during early summer. Shallow cumulus and synoptic-scale weather systems together make a comparable contribution (total net flux 16.2 x 10(exp 8) kg CO/month). Boundary layer venting of CO with other O3 precursors leads to efficient free troposheric O3 formation. We estimate that deep convective transport of CO and other precursors over the central United States in early summer leads to a gross production of 0.66 - 1.1 Gmol O3/d in good agreement with estimates of O3 production from boundary layer venting in a continental-scale model (Jacob et al., 1993a, b). On this respect the central U.S. region acts as s `chimney' for the country, and presumably this O3 contributes to high background levels of O3 in the eastern United States and O3 export to the North Atlantic.

Thompson, Anne M.↗

Global and Regional Trends of Aerosol Optical Depth over Land and Ocean Using SeaWiFS Measurements from 1997 to 2010

Both sensor calibration and satellite retrieval algorithm play an important role in the ability to determine accurately long-term trends from satellite data. Owing to the unprecedented accuracy and long-term stability of its radiometric calibration, the SeaWiFS measurements exhibit minimal uncertainty with respect to sensor calibration. In this study, we take advantage of this well-calibrated set of measurements by applying a newly-developed aerosol optical depth (AOD) retrieval algorithm over land and ocean to investigate the distribution of AOD, and to identify emerging patterns and trends in global and regional aerosol loading during its 13-year mission. Our results indicate that the averaged AOD trend over global ocean is weakly positive from 1998 to 2010 and comparable to that observed by MODIS but opposite in sign to that observed by AVHRR during overlapping years. On a smaller scale, different trends are found for different regions. For example, large upward trends are found over the Arabian Peninsula that indicate a strengthening of the seasonal cycle of dust emission and transport processes over the whole region as well as over downwind oceanic regions. In contrast, a negative-neutral tendency is observed over the desert/arid Saharan region as well as in the associated dust outflow over the north Atlantic. Additionally, we found decreasing trends over the eastern US and Europe, and increasing trends over countries such as China and India that are experiencing rapid economic development. In general, these results are consistent with those derived from ground-based AERONET measurements.

Hsu, N. C.↗

Marine Magnetic Anomalies and the Reconstruction of the World

Until the middle of the 20th century little was known about magnetic anomalies in the oceans. Then it was discovered that there are relatively large anomalies in most of the oceans and they were unrelated to any geological structure known at that time. In the early 1950's large anomalies had been found over the Mid-Atlantic Ridge, and linear anomalies over the eastern continental shelf of North America and, shortly after that, off the west coast. A survey of the ridge south of Iceland showed that the anomalies were linear, parallel to the ridge axis, and symmetrical about the axis. Using the theory that the anomalies were caused by geomagnetic field reversals and seafloor spreading it was possible to greatly extend the time scale of geomagnetic reversals, to determine the velocity of seafloor spreading and estimate the time of opening of the North Atlantic. Lamont had a world-wide collection of marine magnetic profiles. These were used, systematically, to determine the positions of most of the land masses of the world since the beginnings of the world's present oceans.

Heirtzler, James R.↗

Analysis of North Atlantic Aircraft Data on Oxygenated Intermediate Species Using an Adapted Regional Chemistry-Transport Model

Our study is on the interaction of nitrogen oxides with organics as they are exported from their complex sources in Eastern North America. Both urban and specific industrial emissions contribute the nitrogen of the C-H-O-N compounds that affect the global atmosphere, helping determine both ozone and the self-cleaning radical chemistry of the troposphere mediated by the OH radical. Different industrial sources, urban, and natural emissions contribute the organic C. Peroxyacetyl nitrate, CH3C(double bonds O)OONO2 is the most interesting compound for which we can measure the outflow to the full depth of the Atlantic troposphere. As we adapt the 3-d chemical model to describe outflow for specific periods with sufficient accuracy, we are analyzing some valuable information in the NARE-97 complete airborne dataset. (NARE: North Atlantic Regional Experiment). Ames researchers find that there are substantial puzzles in the ratios of PAN/NO2. Peroxy acetyl nitrate provides one of the major long-distance export pathways for active nitrogen from Eastern North America. It should be closely linked with NO, (defined as the sum NO + NO2) by simple thermal association and decomposition reactions, at least when the ambient temperature is substantially above 5 C.

Chatfield, Robert↗

A Comparison between the TOPEX/POSEIDON Data and a Global Ocean General Circulation Model during 1992-1993

The TOPEX/POSEIDON altimetric sea level observation during 1992-1993 was used to validate the simulation made by a global ocean general circulation model (OGCM) forced by the daily wind stress and heat flux derived from the National Meteorological Center operational analysis. The OGCM is a version of the modular ocean model with a horizontal resolution of 2 deg longitude and 1 deg latitude and 22 levels in the vertical. The model simulation is compared to the observation at spatial scales of the order of 500 km and larger. Only the temporal variations are examined. The variability is composed primarily of the annual cycle and intraseasonal fluctuations (periods shorter than 100 days). The basic features of the annual cycle are simulated well by the model. Major discrepancies are found in the eastern tropical Pacific, as well as the eastern North Pacific and most of the interior of the North Atlantic. The culprit is suspected to be the inadequate heat forcing and mixing parameterizations of the model. Significant intraseasonal variability is found in the central North Pacific and the Southern Ocean. The simulation is highly correlated with the observation at periods from 20 to 100 days. The spatial scales are larger than 1000 km in many places. These variabilities are apparently the barotropic response of the ocean to wind forcing. The results of the study provide a basis for future assimilation of the data into the OGCM for improved description of the large-scale ocean variabilities.

Chao, Yi↗

Does The Nile Reflect Solar Variability?

Historical records of the Nile water level provide a unique opportunity to investigate the possibility that solar variability influences the Earth's climate. Particularly important are the annual records of the water level, which are uninterrupted for the years 622-1470 A.D. These records are non-stationary, so that standard spectral analyses cannot adequately characterize them. Here the Empirical Mode Decomposition technique, which is designed to deal with nonstationary, nonlinear time series, becomes useful. It allows the identification of two characteristic time scales in the water level data that can be linked to solar variability: the 88 year period and a time scale of about 200 years. These time scales are also present in the concurrent aurora data. Auroras are driven by coronal mass ejections and the rate of auroras is an excellent proxy for solar variability. Analysis of auroral data contemporaneous with the Nile data shows peaks at 88 years and about 200 years. This suggests a physical link between solar variability and the low frequency variations of the Nile water level. The link involves the influence of solar variability on the North Annual Mode of atmospheric variability and its North Atlantic and Indian Oceans patterns that affect rainfall over Eastern Equatorial Africa where the Nile originates.

statistical methods↗

Exceptional Warmth in the Northern Hemisphere during January through March of 2020: The Roles of Unforced and Forced Modes of Atmospheric Variability

Much of northern Eurasia experienced record high temperatures during the first three months of 2020, and the eastern United States experienced a significant heat wave during March. In this study, we show that the above episodes of extraordinary warmth reflect to a large extent the unusual persistence and large amplitude of three well-known modes of atmospheric variability: the Arctic Oscillation (AO), the North Atlantic Oscillation (NAO), and the Pacific–North American (PNA) pattern. We employ a “replay” approach in which simulations with the NASA GEOS AGCM are constrained to remain close to MERRA-2 over specified regions of the globe in order to identify the underlying forcings and regions that acted to maintain these modes well beyond their typical submonthly time scales. We show that an extreme positive AO played a major role in the surface warming over Eurasia, with forcing from the tropical Pacific and Indian Ocean regions acting to maintain its positive phase. Forcing from the tropical Indian Ocean and Atlantic regions produced positive NAO-like responses, contributing to the warming over eastern North America and Europe. The strong heat wave that developed over eastern North America during March was primarily associated with an extreme negative PNA that developed as an instability of the North Pacific jet, with tropical forcing providing support for a prolonged negative phase. A diagnosis of the zonally symmetric circulation shows that the above extratropical surface warming occurred underneath a deep layer of tropospheric warming, driven by stationary eddy-induced changes in the mean meridional circulation.

Northern Hemisphere↗