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At least 181 records · Page 10

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DOE OSTI2021

Effect of Temperature and FEC on Silicon Anode Heat Generation Measured by Isothermal Microcalorimetry

Isothermal microcalorimetry (IMC) was used to better understand parasitic reactions and heat generation from Si electrodes in the first 10 cycles using Li/Si half cells. Heat generation from cell polarization (ohmic heat), entropy changes (reversible heat), and parasitic reactions (parasitic heat) are separated and quantified. The effect of temperature and fluoroethylene carbonate (FEC) as an electrolyte additive are also explored. Our results show that at the C/10 cycling rate used here, ohmic heat makes the largest contribution to overall heat generation while reversible heat is the smallest. Ohmic heat generation increases with cycle number due to increasing internal resistance, though the effect is smaller for cells with FEC. Interestingly, capacity-normalized parasitic heat generation is largely unaffected by changes in temperature despite differing reaction kinetics. We show that this is caused by a decrease in average parasitic reaction enthalpy as temperature is increased. Further, cells with FEC display higher average parasitic reaction enthalpy than cells without. The average parasitic reaction enthalpies for all the Si electrodes we tested were lower than previously reported values for graphite, indicating that the SEI formed on Si is less stable.

25 ENERGY STORAGE↗

NASA NTRS1967

Plasma jet electrode has longer operating life

Water-cooled, silver-infiltrated tungsten electrode has twice the operating lifetime of the pure tungsten electrode used in plasma jet generators. This electrode reduces the erosion rate, ensures excellent heat transfer, and reduces thermal stresses.

Gracey, C. M.↗

NASA NTRS1991

Thermal shock of fiber reinforced ceramic matrix composites

Monolithic silicon carbide and silicon nitride and a Nicalon fiber reinforced silicon carbide composite were subjected to severe thermal shock conditions via impingement of a hydrogen-oxygen flame. Surface heating rates of 1000 C/sec to 2500 C/sec were generated. The performance of the monolithic reference materials are compared and contrasted to the significantly greater thermal shock resistance of the composite. Ultrasonic and radiographic NDE techniques were used to evaluate the integrity of the composite subsequent to thermal shock. Tensile tests were performed to determine the residual tensile strength and modulus. Physical property changes are discussed as a function of number and severity of thermal shock cycles.

Eckel, Andrew J.↗

NASA NTRS1991

Thermal shock fiber-reinforced ceramic matrix composites

Eckel, Andrew J.↗

NASA NTRS2003

Computation of Domain-Averaged Shortwave Irradiance by a One-Dimensional Algorithm Incorporating Correlations between Optical Thickness and Direct Incident Radiation

A one-dimensional radiative transfer algorithm that accounts for correlations between the optical thickness and the incident direct solar radiation is developed to compute the domain-averaged shortwave irradiance profile. It divides the direct irradiance into four components and treats the direct irradiance in two separate, clear and cloudy columns to account for the fact that clouds attenuate the direct irradiance more than clear-sky. The horizontal inhomogeneity of clouds in the cloudy column is treated by the gamma weighted two-stream approximation, which assumes that the optical thickness of clouds follows a gamma distribution. The algorithm inputs the cloud fraction, cumulative cloud fraction as a function of height, and a parameter expressing the shape of the probability density function of the cloud optical thickness distribution in addition to inputs required for a two-stream radiative transfer model. These cloud property inputs can be obtained using ground- and satellite-based instruments. Therefore, the algorithm can treat realistic cloud overlap features and horizontal inhomogeneity of clouds in a framework of one- dimensional radiative transfer. Heating rates computed by the algorithm using cloud fields generated by cloud resolving models agree with those computed with a Monte Carlo model. If optical properties in computational layers that divide a vertically extensive cloud are correlated, the irradiance profile computed by the algorithm further improves.

Kato, S.↗

NASA NTRS1992

Heat generation during overcharge of Ni/H2 cells

Information is given in viewgraph form on the heat generation during overcharge of nickel hydrogen cells. The heat dissipated during various rates of charge and overcharge was measured, using a radiative type calorimeter. Measurements made during the charging of the cell indicated that the total heat was greatest for C/10 charge, compared with C/2 or C/4. The endothermic to exothermic transition occurred at 1.43 V for C/10 charge, and increased to 1.467 V at C/2 charge. The magnitude of the endothermic heat was only 3.7 percent of the total heat generated during charging. Experimentally measured values were compared against those calculated using a thermoneutral potential of 1.51 V. Although there was general agreement between the calculated and measured values, a significant difference existed in the instantaneous heat values for the initial stages of cell discharge. Heat dissipated during self-discharge appears to depend on the charge rate preceding open circuit stand.

Vaidyanathan, Hari↗

NASA NTRS1980

Lubrication of optimized-design tapered-roller bearings to 2.4 million DN

The performance of 120.65 mm (4.75 in.) bore high speed design, tapered roller bearings was investigated at shaft speeds to 20,000 rpm (2.4 million DN) under combined thrust and radial load. The test bearing design was computer optimized for high speed operation. Temperature distribution bearing heat generation were determined as a function of shaft speed, radial and thrust loads, lubricant flow rates, and lubricant inlet temperature. The high speed design, tapered roller bearing operated successfully at shaft speeds up to 20,000 rpm under heavy thrust and radial loads. Bearing temperatures and heat generation with the high speed design bearing were significantly less than those of a modified standard bearing tested previously. Cup cooling was effective in decreasing the high cup temperatures to levels equal to the cone temperature.

Parker, R. J.↗

DOE OSTI2020

Iron-Doped Sodium Vanadium Oxyflurophosphate Cathodes for Sodium-Ion Batteries—Electrochemical Characterization and In Situ Measurements of Heat Generation

Sodium-ion batteries (NaIBs) are increasingly being envisioned for grid-scale energy-storage systems because of cost advantages. However, implementation of this vision has been challenged by the low-energy densities delivered by most NaIB cathodes. Toward addressing this challenge, the authors report the synthesis and characterization of a new iron-doped Na 3 Fe 0.3 V 1.7 O(PO 4 ) 2 F 2 cathode using a novel facile hydrothermal route. The synthesized material was characterized using scanning electron microscopy, X-ray diffraction, and Mössbauer spectroscopy techniques. The obtained discharge capacity in the half-cell configuration lies from 119 to 125 to 130 mA h/g at C/10 while tested using three different electrolyte formulations, dimethyl carbonate–ethylene carbonate (EC)–propylene carbonate (PC), diethyl carbonate–EC, and EC–PC, respectively. The synthesized cathodes were also evaluated in full-cell configurations, which delivered an initial discharge capacity of 80 mA h/g with NaTi 2 (PO 4 ) 3 MWCNT as the anode. Ionic diffusivity and interfacial charge transfer kinetics were also evaluated as a function of temperature and sodium concentration, which revealed that electrochemical rate performances in this material were limited by charge-transfer kinetics. To understand the heat generation mechanism of the Na/Na 3 Fe 0.3 V 1.7 O(PO 4 ) 2 F 2 half-cell during charge and discharge processes, an electrochemical isothermal calorimetry measurement was carried out at different current rates for two different temperatures (25 and 45 °C). The results showed that the amount of heat generated was strongly affected by the operating charge/discharge state, C-rate, and temperature. Altogether, this work provides a new synthesis route for the development of iron-doped Na 3 Fe 0.3 V 1.7 O(PO 4 ) 2 F 2 -based high-performance sodium cathode materials aimed at providing a viable pathway for the development and deployment of large-scale energy-storage based on sodium battery systems.

25 ENERGY STORAGE↗

DOE OSTI2022

North Carolina Water Utility Builds Resilience with Distributed Energy Resources

As the frequency and duration of grid outages increase, backup power systems are becoming more important for ensuring that critical infrastructure continues to provide essential services. Most facilities rely on diesel generators, which may be ineffective during long outages owing to limited fuel supplies and high generator failure rates. Distributed energy resources such as solar, storage, and combined-heat-and-power systems, coupled with on-site biofuel production, offer an alternative source of on-site generation that can provide both cost savings and resilience (i.e., the ability to respond to catastrophic events with longer-term consequences). A mixed-integer linear program minimizes costs and maximizes resilience at a wastewater treatment plant in Wilmington, North Carolina. We find that the plant can reduce life-cycle energy costs by 3.1% through the installation of a hybrid combined-heat-and-power, photovoltaic, and storage system. When paired with existing diesel generators, this system can sustain full load for seven days while saving $664,000 over 25 years and reducing diesel fuel use by 48% compared with the diesel-only solution. This analysis informed a decision by the Cape Fear Public Utility Authority to allocate funds for the implementation of a combined-heat-and-power system at the wastewater treatment plant in fiscal year 2023. Finally, the benefits of deploying hybrid combined-heat-and-power technologies and the utilization of on-site biofuel production extend, on a national scale, to thousands of wastewater treatment facilities and other types of critical infrastructure.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2024

Simulations of radiatively cooled magnetic reconnection driven by pulsed power

Magnetic reconnection is an important process in astrophysical environments, as it reconfigures magnetic field topology and converts magnetic energy into thermal and kinetic energy. In extreme astrophysical systems, such as black hole coronae and pulsar magnetospheres, radiative cooling modifies the energy partition by radiating away internal energy, which can lead to the radiative collapse of the reconnection layer. In this paper, we perform two- and three-dimensional simulations to model the MARZ (Magnetic Reconnection on Z) experiments, which are designed to access cooling rates in the laboratory necessary to investigate reconnection in a previously unexplored radiatively cooled regime. These simulations are performed in GORGON, an Eulerian two-temperature resistive magnetohydrodynamic code, which models the experimental geometry comprising two exploding wire arrays driven by 20 MA of current on the Z machine (Sandia National Laboratories). Radiative losses are implemented using non-local thermodynamic equilibrium tables computed using the atomic code Spk, and we probe the effects of radiation transport by implementing both a local radiation loss model and P 1/3 multi-group radiation transport. The load produces highly collisional, super-Alfvénic (Alfvén Mach number M A ≈ 1.5), supersonic (Sonic Mach number M S ≈ 4–5) strongly driven plasma flows which generate an elongated reconnection layer (Aspect Ratio L/δ≈100 , Lundquist number S L ≈ 400). The reconnection layer undergoes radiative collapse when the radiative losses exceed the rates of ohmic and compressional heating (cooling rate/hydrodynamic transit rate = τ$^{–1}_{cool}$/τ$^{–1}_{H}$ ≈100); this generates a cold strongly compressed current sheet, leading to an accelerated reconnection rate, consistent with theoretical predictions. Lastly, the current sheet is also unstable to the plasmoid instability, but the magnetic islands are extinguished by strong radiative cooling before ejection from the layer.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Estimation of 14 MeV neutron rate from triton burn-up in future W7-X deuterium plasma campaigns

Fast ion confinement is of major importance for the ignition of a burning fusion plasma. In future deuterium plasma campaigns of the Wendelstein 7-X stellarator, W7-X, the amount of triton burn-up is one possible measure for fast ion confinement. A well-established technique to observe triton burn-up is the 14 MeV neutron rate. In this paper, it is estimated whether an existing scintillating fibre neutron detector is also suited to measure triton burn-up in W7-X with sufficient accuracy. In this work, an estimation is presented, which can be applied to any tokamak or stellarator design and is one-dimensional in the minor radius. The inputs are profiles of density, temperature, and differential volume element as well as the triton slowing-down time. The estimation calculates the thermal deuteron fusion rate and the associated deuteron-triton fusion rate; thus, the triton burn-up generated 14 MeV neutron rate. It neither takes triton diffusion nor explicit losses into account. This thermally generated fusion rate is compared to the neutral beam injection heating induced beam-plasma fusion rate.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Stretchable Photodiodes with Polymer-Engineered Semiconductor Nanowires for Wearable Photoplethysmography

Healthcare systems worldwide have been stressed to provide sufficient resources to serve the increasing and aging population in our society. The situation became more challenging at the time of pandemic. Technology advancement, especially the adoption of wearable health monitoring devices, has provided an important supplement to current clinical equipment. Most health monitoring devices are rigid, however, human tissues are soft. Such a difference has prohibited intimate contact between the two and jeopardized wearing comfortableness, which hurdles measurement accuracy especially during longtime usage. Here, in this work, we report a soft and stretchable photodiode that can conformally adhere onto the human body without any pressure and measure cardiovascular variables for an extended period with higher reliability than commercial devices. The photodiode used a composite light absorber consisting of an organic bulk heterojunction embedded into an elastic polymer matrix. It is discovered that the elastic polymer matrix not only improves the morphology of the bulk heterojunction for obtaining the desired mechanical properties but also alters its electronic band structure and improves the electrical properties that lead to a reduced dark current and enhanced photovoltage in the stretchable photodiode. The work has demonstrated high fidelity measurements and longtime monitoring of heat rate variability and oxygen saturation, potentially enabling next-generation wearable photoplethysmography devices for point-of-care diagnosis of cardiovascular diseases in a more accessible and affordable way.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

NASA NTRS1977

Toxicity studies of a polyurethane rigid foam

Relative toxicity tests were performed on a polyurethane foam containing a trimethylopropane-based polyol and an organophosphate flame retardant. The routine screening procedure involved the exposure of four Swiss albino male mice in a 4.2 liter hemispherical chamber to the products generated by pyrolyzing a 1.00 g sample at a heating rate of 40 deg C/min from 200 to 800 C in the absence of air flow. In addition to the routine screening, experiments were performed with a very rapid rise to 800 C, with nominal 16 and 48 ml/sec air flow and with varying sample rates. No unusual toxicity was observed with either gradual or rapid pyrolysis to 800 C. Convulsions and seizures similar to those previously reported were observed when the materials were essentially flash pyrolyzed at 800 C in the presence of air flow, and the toxicity appeared unusual because of low sample weights required to produce death.

Hilado, C. J.↗

NASA NTRS1985

A new mechanism for excitation of electrostatic ion cyclotron waves and associated perpendicular ion heating

A new mechanism for exciting the kinetic ion cyclotron waves in the presence of a nonuniform electric field perpendicular to the external magnetic field is given. Application of this instability to various space plasmas is discussed. The new instability mechanism may provide a more efficient agent for perpendicular ion heating than other EIC generation processes, since the linear growth rate is insensitive to the temperature ratio.

Ganguli, G.↗

NASA NTRS1989

Cloud-generated radiative heating and its generation of available potential energy

The generation of zonal available potential energy (APE) by cloud radiative heating is discussed. The APE concept was mathematically formulated by Lorenz (1955) as a measure of the maximum amount of total potential energy that is available for conversion by adiabatic processes to kinetic energy. The rate of change of APE is the rate of the generation of APE minus the rate of conversion between potential and kinetic energy. By radiative transfer calculations, a mean cloud-generated radiative heating for a well defined set of cloud classes is derived as a function of cloud optical thickness. The formulation is suitable for using a general cloud parameter data set and has the advantage of taking into account nonlinearities between the microphysical and macrophysical cloud properties and the related radiation field.

Stuhlmann, R.↗

NASA NTRS1991

Linear stability of free planetary waves in the presence of radiative-photochemical feedbacks

The diabatic effects of Newtonian cooling and ozone-dynamics interaction on the linear stability of free planetary waves in the atmosphere have been studied using a simple beta-plane model. The model couples radiative transfer, ozone advection, and ozone photochemistry with the quasi-geostrophic dynamical circulation. An analytical expression is derived which demonstrates the following: (1) the influence of meridional ozone advection on wave growth or decay depends on the wave and basic state vertical structures; and (2) photochemically accelerated cooling, which predominates in the upper stratosphere, augments the Newtonian cooling rate and is stabilizing. Attention is also given to the 1D linear stability problem which is numerically solved for a Charney basic state and for zonal mean basic states. It is shown that ozone heating generated by ozone-dynamics interaction in the stratosphere can reduce (enhance) the damping rates due to Newtonian cooling by as much as 50 percent for planetary waves of large vertical scale and maximum amplitude in the stratosphere.

Nathan, Terrence R.↗

NASA NTRS1984

Comparison of predicted and experimental thermal performance of angular-contact ball bearings

Predicted bearing heat generation and bearing temperature were verified by experimental data for ball bearings over a range of sizes, shaft speeds, and lubricant flow rates. The computer program Shaberth requires, as input, a factor which describes the air-oil mixture in the bearing cavity for calculation of the ball drag contribution to bearing heat generation. An equation for this lubricant percent volume in the bearing cavity was derived and appears to be valid over the range of test conditions including bearing bore sizes from 35 to 167 mm and shaft speeds from 1.0 to 3.0 million DN.

Parker, R. J.↗

NASA NTRS1998

Engineering Aerothermal Analysis for X-34 Thermal Protection System Design

Design of the thermal protection system for any hypersonic flight vehicle requires determination of both the peak temperatures over the surface and the heating-rate history along the flight profile. In this paper, the process used to generate the aerothermal environments required for the X-34 Testbed Technology Demonstrator thermal protection system design is described as it has evolved from a relatively simplistic approach based on engineering methods applied to critical areas to one of detailed analyses over the entire vehicle. A brief description of the trajectory development leading to the selection of the thermal protection system design trajectory is included. Comparisons of engineering heating predictions with wind-tunnel test data and with results obtained using a Navier- Stokes flowfield code and an inviscid/boundary layer method are shown. Good agreement is demonstrated among all these methods for both the ground-test condition and the peak heating flight condition. Finally, the detailed analysis using engineering methods to interpolate the surface-heating-rate results from the inviscid/boundary layer method to predict the required thermal environments is described and results presented.

Wurster, Kathryn E.↗