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At least 181 records · Page 10

Jump-Start U.S. Manufacturing of High-Performance Permanent Magnets

Gas atomized feedstock powders for Nd-Fe-B based magnets are more robust and cost effective than the strip-cast sheet currently used as feedstock for milling by the magnet industry. However, gas atomized powder’s crystallinity and grain boundary phases are less ideal than the strip cast flake. We proposed to optimize the atomization process as well as the powder chemistry to address this issue and to eliminate heavy rare earth elements from these magnet alloys. Our goal is to help GKN-Hoeganaes, a US metal powder company, who used to make Nd-Fe-B magnets, to bring back US manufacturing of these high energy density permanent magnets.

36 MATERIALS SCIENCE↗

Improved Joint FHC+RHC Sterile Analysis with Nu-on-E Sample

The NOvA experiment measures neutrino oscillations in a nearly pure muon neutrino beam. The neutral current (NC) and the muon neutrino charged current (CC) interaction disappearance are studied to search for active-to-sterile neutrino oscillations. NOvA consists of two functionally identical detectors placed 14 mrad off-axis of Fermilab's NuMI beamline. The Near Detector (ND) is located 100 m underground on-site at Fermilab, while the Far Detector (FD) sits on the surface 810 km away at Ash River, Minnesota. The NuMI beam is capable of running in forward or reverse horn current modes, creating a predominantly neutrino or antineutrino beam, respectively. For this analysis, a simultaneous near and far detector joint fit approach was utilized. Systematic uncertainties constrain the ND while the statistical uncertainties constrain the FD. For the upcoming analysis, we plan on including a dedicated neutrino-on-electron elastic scattering sample. This interaction is advantageous as it is subject to minimal cross-section uncertainties, which will help reduce degeneracies between other uncertainty categories. This thesis presents the sterile neutrino oscillation sensitivity results using 27.2e+20 POT in FHC mode, 12.6e+20 in RHC mode.

Haejun, Stella Oh [Cincinnati U.]↗

Comparison of ACHILLES and GENIE observables for DUNE-PRISM and the SBN program, with new 2p2h predictions

Several DUNE ND off axis locations were simulated using GENIE and ACHILLES, and generator differences and FSI contributions were examined for various observables. Predictions were compared with those of existing experiments, and it is shown that the DUNE ND 20m off axis predictions are similar to that of MicroBooNE for various observables. Finally, the 2p2h interaction mode was simulated for ACHILLES for the first time for ICARUS, and a preliminary comparison is made to MicroBooNE data and simulations from different event generators.

Dumont, Daniel [Fermilab]↗

Life Cycle Inventories and Data Gap Analysis for Rare Earth Elements: Neodymium and Dysprosium from Mining to Magnets

The United States demand for Neodymium-Iron-Boron (NdFeB) magnets, produced from rare earth elements (REEs) such as (Nd) and Dysprosium (Dy), far exceeds its nascent domestic production capacity, rendering it reliant on vulnerable global supply chains dominated by China. To guide research and development investments in securing U.S. REE supply, defensible benchmark metrics across environmental, economic, and social dimensions are needed. In this study, we built globally-representative, process-based cradle-to-cradle life cycle inventories for Nd and Dy in NdFeB magnets lifecycles, encompassing primary material acquisition, beneficiation, smelting and refining, metal processing, specialty alloy and chemical transformation, subcomponent manufacturing, consumer application (use phase) and end-of-life management. We carried out detailed literature review, and applied process engineering principles to build industry-representative upscaled life cycle inventories for both metals. We used these models to conduct bottom-up literature review and gap analysis on existing literature, compilation of data sources for each life cycle stage (and transformations where necessary), and a preliminary technoeconomic analysis (TEA)/life cycle costing analysis (LCCA). Findings from this work emphasize the need for metal specific, representative REE LCIs to establish robust benchmarks for advancing sustainable REE technologies and guiding R&D in REE supply chains.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Probing BSM Oscillatory Signals with the DUNE Detectors and the LBNF Neutrino Beam: NSI and Sterile Neutrino Sensitivities

The Deep Underground Neutrino Experiment (DUNE) is a flagship long-baseline accelerator neutrino experiment under construction in the U.S. With a 1,300 km distance between its Near Detector (ND) and Far Detector (FD), the world’s most intense LBNF (Long-Baseline Neutrino Facility) neutrino beam, and high-resolution LArTPC (Liquid Argon Time Projection Chamber) detectors, DUNE will measure the neutrino oscillation parameters with unprecedented precision. In addition to the determination of the neutrino mass ordering and the potential discovery of Charge-Parity violation in the leptonic sector, DUNE's capabilities present a unique opportunity for probing Beyond the Standard Model (BSM) physics signals with neutrinos. Examples of BSM physics manifestations include the presence of Non-Standard Interactions (NSI) of neutrinos with matter, or the existence of sterile neutrinos that mix with 3-Flavor neutrinos. In this study, we present a joint ND+FD fit to simulated data assessing DUNE's sensitivity to probing neutrino NSI, as well as scenarios including sterile neutrino mixing.

Prais, Luiz [Cincinnati U.] (ORCID:000000018224947↗

Charged Pion Production Explorations Using the NOvA Near Detector

The~300T NOvA Near Detector (ND) utilizes segmented liquid scintillator to reconstruct interacting neutrinos arriving from the NuMI Beamline at Fermilab. Given NuMI’s intensity and the ND’s relatively short baseline, NOvA has recorded some of the world’s highest statistics for neutrino interactions around ~2GeV, in great similarity to the forthcoming DUNE experiment. This energy regime is replete with resonant interactions, which will form the plurality of final states in DUNE. NOvA seeks to empower the community with measurements of processes for both semi-exclusive and semi-inclusive charged pion production across muon kinematics and pion angle via single-and multidifferential neutrino scattering cross sections. This poster will review current progress across several related analyses, and look forward to future results.

Roy, Palash K. [Wichita State U.] (ORCID:000000022↗

Abundances of Neutron-capture Elements in 62 Stars in the Globular Cluster Messier 15

M15 is a globular cluster with a known spread in neutron-capture elements. This paper presents abundances of neutron-capture elements for 62 stars in M15. Spectra were obtained with the Michigan/Magellan Fiber System spectrograph, covering a wavelength range from ~4430 to 4630 Å. Spectral lines from Fe I , Fe II , Sr I , Zr II , Ba II , La II , Ce II , Nd II , Sm II , Eu II , and Dy II were measured, enabling classifications and neutron-capture abundance patterns for the stars. Of the 62 targets, 44 are found to be highly Eu-enhanced r-II stars, another 17 are moderately Eu-enhanced r-I stars, and one star is found to have an s-process signature. The neutron-capture patterns indicate that the majority of the stars are consistent with enrichment by the r-process. The 62 target stars are found to show significant star-to-star spreads in Sr, Zr, Ba, La, Ce, Nd, Sm, Eu, and Dy, but no significant spread in Fe. The neutron-capture abundances are further found to have slight correlations with sodium abundances from the literature, unlike what has been previously found; follow-up studies are needed to verify this result. The findings in this paper suggest that the Eu-enhanced stars in M15 were enhanced by the same process, that the nucleosynthetic source of this Eu pollution was the r-process, and that the r-process source occurred as the first generation of cluster stars was forming.

79 ASTRONOMY AND ASTROPHYSICS↗

Adsorption of neodymium, dysprosium, and ytterbium to goethite under varying aqueous chemistry conditions [dataset]

The adsorption of rare earth elements (REEs) to iron oxides can regulate the mobility of REEs in the environment and is heavily influenced by water chemistry. This study utilized batch experiments to examine the adsorption of Nd, Dy, and Yb to goethite under varying pH, electrolyte (type and concentration), and concentrations of dissolved inorganic carbon and citrate. REE adsorption was strongly influenced by pH, with an increase from essentially no adsorption at pH 3.0 to nearly complete adsorption at pH 6.5 and higher. Citrate enhanced the adsorption of REEs at low pH (< 5.0), likely by forming goethite-REE-citrate ternary surface complexes. However, citrate inhibited the adsorption of REEs at higher pH (> 5.0) by forming aqueous REE-citrate complexes. Ionic strength had a small influence on REE adsorption, and the presence of dissolved inorganic carbon had no discernible effect. Equilibrium adsorption was interpreted with a triple layer surface complexation model (SCM). The selection of surface complexation reactions was guided by extended X-ray absorption fine structure spectra. A SCM with a single bidentate inner-sphere surface complexation reaction for Nd and two inner-sphere surface complexation reactions (one monodentate and one bidentate reaction) for Dy and Yb effectively simulated adsorption across a broad range of conditions in the absence of citrate. Accounting for the effects of citrate on REE adsorption required the addition of up to two ternary REE-citrate-goethite surface complexes. The SCM can enable predictions of REE transport in subsurface environments that have goethite as an important adsorbent mineral. This predictive capability could contribute to identifying potential REE sources and facilitating efficient extraction of REEs.

58 GEOSCIENCES↗

Adsorption of Rare Earth Elements to Kaolinite [dataset]

Rare earth elements (REEs) are critical components of modern technology behind renewable energy, transportation, and electronics but have a limited current supply. A substantial portion of global REE production relies on ion adsorption deposits. A high abundance of kaolinite in REE enrichment zones within these deposits suggests that kaolinite controls the subsurface migration of REEs. This study aimed to improve the current understanding of REE binding to kaolinite under varying water chemistry conditions. We conducted batch experiments with kaolinite (KGa-2) and three REEs (Nd, Dy, and Yb) at varying pH, electrolyte concentration, dissolved inorganic carbon (DIC), low molecular weight organic acids (citric and oxalic acids), and total REE concentration conditions. Increasing electrolyte concentration inhibits REE adsorption at pH 7, suggesting that ion exchange contributes to adsorption at these pH values. DIC affects adsorption above pH 7−8 by forming strong aqueous complexes with heavy REEs. Citric acid decreases REE adsorption via aqueous complexation of REEs at pH 5 but does not affect adsorption at pH 5. The surface complexation model captures the main adsorption trends with two mechanisms: ion exchange on basal planes at pH ∼6 and inner-sphere surface complexation to edge sites at pH ∼6. Equilibrium constants for surface complexation increase in the order of Yb Dy Nd, indicating a higher strength of adsorption for heavy REEs. This study demonstrates how water chemistry conditions control the adsorption mechanisms that may determine the mobility of REEs in subsurface environments rich in kaolinite.

58 GEOSCIENCES↗

Photoproduction of K0K0-bar with the GlueX Experiment

In this dissertation, we study photoproduction of K0 ?K 0 through the KSKLp and KSKSp ?nal states with the GlueX Phase-I (GlueX-I) data set. We measure the spin-density matrix elements (SDMEs) and di?erential cross section of ?(1020) ! KSKL to better understand photoproduction of light vector mesons. A mass independent Partial Wave Analysis (PWA) of the KSKL and KSKS meson spectrum below 2 GeV is also undertaken to study the meson spectrum with JPC = even++ and odd??. The ?(1020) di?erential cross section is measured at E = 8:2 ? 8:8 GeV and ?t = 0:15 ? 1:00 GeV2. The di?erential cross section is well described by an exponential decay with slope 4:44?0:01 GeV?2 and the integrated cross section is determined to be 295:7?0:4 nb, only statistical uncertainties are quoted. Both measurements are consistent and far more precise than the previous measurement by Ballam et al. [1]. The ?(1020) SDMEs were measured in nine bins of ?t in the same range. At low ?t, we ?nd the data were consistent with s-channel helicity conservation, SCHC, i. e. the only non-zero SDMEs were ?1 1?1 = ?Im(?2 1?1) = 1=2. At higher ?t, the SDMEs deviate from SCHC and the measurements indicate this is due to natural parity exchange since we observe that the SDMEs are consistent with zero unnatural exchange. We also ?find that the contribution from helicity double-flip amplitudes is consistent with zero. The measured SDMEs are in poor agreement with theoretical predictions put forward by JPAC [35]. These measurements will serve as input to re?ne models of production processes, which will be essential for the interpretation of possible signals of exotic mesons in GlueX. Analysis of the spectrum above the ?(1020) indicates the presence of at least three particles at ? 1:50, ? 1:75, and 2:20 GeV. We employ simple parametrizations of the resonance line shape based on relativistic Breit-Wigner functions considering cases with and without interference. The resonance at ? 1:50 GeV is not identifi?ed as any specifi?c resonance, but could be due to interference between the ?(1450) and !(1420). Our models favor the resonance at ~1:75 GeV as the X(1750) rather than the ?(1680). We ?find that introducing a third Breit-Winger into the models improves the ?t quality with the ?2/ndf going from 1.75 to 1.59 and 1.41 to 1.18 for models without and with interference respectively. A PWA of the KSKL spectrum indicates that the spectrum is consistent with exclusively spin-1 contribution up to ? 1:6 GeV. Above ? 1:6 GeV we ?find evidence for a small spin-3 contribution. We also ?nd that the spectrum predominantly positive reflectivity up to ? 1:6 GeV, after which the spectrum becomes a nearly equal mix of both. The KSKS system shows a rich spectrum with multiple resonance structures but is more statistically limited than the KSKL system. Modelling the line shape we ?find evidence at greater than 10? level in favor of a resonance at ? 1:75 GeV. The model parameters suggest this resonance is the f0(1710). The PWA of the KSKS system was inconclusive. However, using a small set of amplitudes suggests that the spin-2 contribution to the spectrum is primarily in the range 1:2?1:6 GeV, where f2(1270), a2(1320) and f02 (1525) are expected.

Linera, Gabriel Rodriguez↗

Predicting Missing Regions in Charged Particle Tracks Using a Sparse 3D Convolutional Neural Network

The 2x2 Demonstrator is a prototype of ND-LAr, the liquid argon time-projection chamber of the Deep Underground Neutrino Experiment’s Near Detector complex. Both the 2x2 Demonstrator and ND-LAr are modular detectors that will have pixelated charge readouts and inactive regions wherein there is no sensitivity to charge deposition and light signals that arise from charged particle interactions with liquid argon. In the 2x2, these inactive regions are located in between the active detector modules, which introduces the challenge of inferring what charge signals ought to look like in these regions. This study explores the use of a Sparse 3D Convolutional Neural Network (ConvNet) to infer missing regions in charged particle tracks. Hits corresponding to energy depositions are voxelized into a three-dimensional grid for each track. Voxels that fall into predefined inactive regions are removed to simulate the lack of detector output. The model is trained to infer the topology of the missing track voxels, with the ultimate goal of inferring the missing charge or energy values in these voxels as well. Results indicate that this approach shows promise in prediction of missing track regions with some accuracy.

Utaegbulam, Hilary↗

Searching for Neutrino Tridents in the NOvA Near Detector

This dissertation presents a search for neutrino trident production in the NOvA near detector through the coherent ``dimuon" channel: $\nu_\mu +\hspace{1pt}\text{X} \rightarrow \nu_\mu + \mu^- + \mu^+ +\hspace{1pt}\text{X}$. Trident production is a rare, purely electroweak process with sensitivity to physics beyond the Standard Model. The theoretical background, motivation for studying the process, and previous experimental measurements are reviewed. The analysis uses data collected by the NOvA near detector (ND) from Fermilab's Neutrinos at the Main Injector (NuMI) beam between November 2014 and February 2024, corresponding to an exposure of $25.5\times 10^{20}$ protons on target. The ND is a segmented tracking calorimeter located 800~m from the beam target, receiving neutrinos with a mean energy of 2~GeV. A multi-pass background reduction strategy is implemented, including the development of a novel dimuon-specific tracking technique. Trident candidates are identified using a boost ed decision tree classifier trained on simulated signal and background events. Limited background Monte Carlo statistics necessitate the use of functional fits to sideband data, which are extrapolated to estimate backgrounds in the signal region. The unblinded data contain 9 trident-like events, with an estimated background of 5.66 $\pm$ 5.15 events. This yields a best fit estimate of 3.34 tridents compared to the Standard Model prediction of 4.66. A profiled Feldman-Cousins method is used to determine a 90\% confidence interval of [0,9.1] on the number of signal events, corresponding to an upper limit of 1.95$\times$ the Standard Model prediction. This result represents the lowest energy search for trident events to date, and the first experimental contribution to the process in 27 years.

Bowles, Reed Scott [Indiana U.]↗

Comparison of ACHILLES and GENIE Observables for DUNE-PRISM and the SBN Program, with New 2p2h Predictions

The DUNE near detector LAr-TPC can be moved to different off-axis positions to sample different neutrino fluxes, which in turn will yield different cross section distributions for observables. Several DUNE ND off axis locations were simulated using GENIE and ACHILLES, and generator differences and FSI contributions were examined for various observables. Additionally, the predictions were compared with those of existing experiments, and it is shown that the DUNE ND 20m off axis predictions are similar to that of MicroBooNE for various observables. Finally, the 2p2h interaction mode was simulated for ACHILLES for the first time for ICARUS, and a preliminary comparison is made to MicroBooNE data and simulations from different event generators.

Dumont, Daniel [Fermilab]↗

Challenges in selecting appropriate electrodes for high-temperature molten salt systems

Based on a specific molten salt (e.g., chloride, fluoride, iodide) investigated, different working and reference electrode materials can be selected considering the chemical and thermal stability of the electrochemical cell components. In this talk, the electrode materials and challenges encountered with a spectro-electrochemical setup installed inside a glovebox, and the solutions implemented to address these challenges, specifically for the chloride and iodide molten salts will be presented. For molten chlorides, the fundamental interactions between neodymium chloride (NdCl3) and Nd metal in lithium chloride-potassium chloride eutectic salt were investigated at 773 K. The electrochemical transitions Nd2+,3+/Nd(s) were analyzed using an inert W electrode with cyclic voltammetry and chronoamperometry techniques, coupled with in-situ UV-Vis spectroscopy to elucidate the kinetic pathways of this disproportionation reaction (eq. 1). Nd(s) + NdCl3 = NdCl2 (1) For molten iodides, the challenges related to working electrode selectivity and present spectro-electrochemical results obtained from cyclic voltammetry measurements conducted at 673 K will be discussed.

36 - MATERIALS SCIENCE↗

From Detector Layout to Signal Analysis: Geometry Optimization and Neutron-Gamma Tagging in Plastic Scintillator Detectors

Neutrinos are elementary particles with many properties still unknown. Their masses so far have only upper and lower limits. Still, due to neutrino oscillations, it is clear that they are not massless, as stated by the Standard Model of Elementary Particles. Neutrinos are also present in the Universe in vast amounts, but they rarely interact with the surrounding matter. Their abundance makes them very interesting for many theories beyond the Standard Model, e.g., dark matter searches and CP symmetry violation in the leptonic sector, which could be (partially) responsible for the observed matter-antimatter asymmetry in today's Universe.\\ The Deep Underground Neutrino Experiment (DUNE) is a next-generation accelerator-based neutrino oscillation experiment that will study neutrinos with unprecedented precision and may answer many open questions. DUNE uses a powerful neutrino beam from Fermilab. It consists of a Near Detector (ND) complex to measure neutrinos before oscillat ion, and a Far Detector (FD) complex $1300\ \mathrm{km}$ away to measure them after oscillation. As part of the ND complex, measurements are also possible with different angles to the neutrino beam. This enables excellent control of systematic uncertainties of e.g., neutrino cross section measurements.\\ One detector in the near detector complex is The Muon Spectrometer (TMS), an extension of a Liquid Argon (LAr) detector that measures the charge and momentum of muons produced in neutrino interactions within the LAr. The design of this detector, which consists of alternating layers of steel and plastic scintillator bars, must be optimized for the expected muon energies.\\ In this thesis, a study of the optimal module orientation plan is presented, which is necessary for the physics performance of the near detector complex and, by extension, DUNE. As part of this study, the event reconstruction was also developed and improved. Simulated muons are then reconstructed, and the performan ce of different module orientation plans is tested.\\ As a second part, a study of neutron and gamma tagging using a Pulse Shape Discriminating (PSD) plastic scintillator is presented. The properties of this material allow particle differentiation based on the temporal distribution of emitted light. A novel approach to using the individual light signals was successfully tested using data from a small, local test setup.

Nehm, Asa [Mainz U.]↗

NOvA Sterile Neutrino Search with Additional Systematic Constraints

The NOvA experiment measures neutrino oscillations in a nearly pure muon neutrino beam. The neutral current (NC) and the muon neutrino charged current (CC) interaction disappearance are studied to search for active-to-sterile neutrino oscillations. NOvA consists of two functionally identical detectors placed 14 mrad off-axis of the Fermi National Accelerator Laboratory's NuMI beamline. The Near Detector (ND) is located 100 meters underground on-site at Fermilab, while the Far Detector (FD) is situated on the surface 810 kilometers away at Ash River, Minnesota. The NuMI beam is capable of operating in either forward or reverse horn current modes, producing predominantly neutrino or antineutrino beams, respectively. For this analysis, a simultaneous near and far detector joint fit approach was utilized. Systematic uncertainties constrain the ND while the statistical uncertainties constrain the FD. In addition to the dual baseline approach, the neutrino-on-electron elastic scattering sample was included. This interaction is advantageous as it is subject to minimal cross-section uncertainties, which will help reduce degeneracies between other uncertainty categories. This thesis presents the sterile neutrino oscillation sensitivity results using 27.2e+20 POT in FHC mode, 12.6e+20 in RHC mode, with the nu-on-e sample of 13.6e+20 POT in FHC.

Oh, Haejun [Cincinnati U.]↗