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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS2011

The Dolinar Receiver in an Information Theoretic Framework

Optical communication at the quantum limit requires that measurements on the optical field be maximally informative, but devising physical measurements that accomplish this objective has proven challenging. The Dolinar receiver exemplifies a rare instance of success in distinguishing between two coherent states: an adaptive local oscillator is mixed with the signal prior to photodetection, which yields an error probability that meets the Helstrom lower bound with equality. Here we apply the same local-oscillator-based architecture with aninformation-theoretic optimization criterion. We begin with analysis of this receiver in a general framework for an arbitrary coherent-state modulation alphabet, and then we concentrate on two relevant examples. First, we study a binary antipodal alphabet and show that the Dolinar receiver's feedback function not only minimizes the probability of error, but also maximizes the mutual information. Next, we study ternary modulation consistingof antipodal coherent states and the vacuum state. We derive an analytic expression for a near-optimal local oscillator feedback function, and, via simulation, we determine its photon information efficiency (PIE). We provide the PIE versus dimensional information efficiency (DIE) trade-off curve and show that this modulation and the our receiver combination performs universally better than (generalized) on-off keying plus photoncounting, although, the advantage asymptotically vanishes as the bits-per-photon diverges towards infinity.

optical communications↗
NASA NTRS1988

Ultralow threshold graded-index separate-confinement heterostructure single quantum well (Al, Ga) As lasers

Broad area graded-index separate-confinement heterostructure single quantum well lasers grown by molecular-beam epitaxy (MBE) with threshold current density as low as 93 A/sq cm (520 microns long) have been fabricated. Buried lasers formed from similarly structured MBE material with liquid phase epitaxy regrowth had threshold currents at submilliampere levels when high reflectivity coatings were applied to the end facets. A CW threshold current of 0.55 mA was obtained for a laser with facet reflectivities of about 80 percent, a cavity length of 120 micron, and an active region stripe width of 1 micron. These devices driven directly with logic level signals have switch-on delays less than 50 ps without any current prebias. Such lasers permit fully on-off switching while at the same time obviating the need for bias monitoring and feedback control.

Derry, P. L.↗
NASA NTRS1993

Analytic Theory and Control of the Motion of Spinning Rigid Bodies

Numerical simulations are often resorted to, in order to understand the attitude response and control characteristics of a rigid body. However, this approach in performing sensitivity and/or error analyses may be prohibitively expensive and time consuming, especially when a large number of problem parameters are involved. Thus, there is an important role for analytical models in obtaining an understanding of the complex dynamical behavior. In this dissertation, new analytic solutions are derived for the complete attitude motion of spinning rigid bodies, under minimal assumptions. Hence, we obtain the most general solutions reported in the literature so far. Specifically, large external torques and large asymmetries are included in the problem statement. Moreover, problems involving large angular excursions are treated in detail. A new tractable formulation of the kinematics is introduced which proves to be extremely helpful in the search for analytic solutions of the attitude history of such kinds of problems. The main utility of the new formulation becomes apparent however, when searching for feedback control laws for stabilization and/or reorientation of spinning spacecraft. This is an inherently nonlinear problem, where standard linear control techniques fail. We derive a class of control laws for spin axis stabilization of symmetric spacecraft using only two pairs of gas jet actuators. Practically, this could correspond to a spacecraft operating in failure mode, for example. Theoretically, it is also an important control problem which, because of its difficulty, has received little, if any, attention in the literature. The proposed control laws are especially simple and elegant. A feedback control law that achieves arbitrary reorientation of the spacecraft is also derived, using ideas from invariant manifold theory. The significance of this research is twofold. First, it provides a deeper understanding of the fundamental behavior of rigid bodies subject to body-fixed torques. Assessment of the analytic solutions reveals that they are very accurate; for symmetric bodies the solutions of Euler's equations of motion are, in fact, exact. Second, the results of this research have a fundamental impact on practical scientific and mechanical applications in terms of the analysis and control of all finite-sized rigid bodies ranging from nanomachines to very large bodies, both man made and natural. After all, Euler's equations of motion apply to all physical bodies, barring only the extreme limits of quantum mechanics and relativity.

Tsiotras, Panagiotis↗
NASA NTRS2010

Single Spatial-Mode Room-Temperature-Operated 3.0 to 3.4 micrometer Diode Lasers

Compact, highly efficient, 3.0 to 3.4 m light emitters are in demand for spectroscopic analysis and identification of chemical substances (including methane and formaldehyde), infrared countermeasures technologies, and development of advanced infrared scene projectors. The need for these light emitters can be currently addressed either by bulky solid-state light emitters with limited power conversion efficiency, or cooled Interband Cascade (IC) semiconductor lasers. Researchers here have developed a breakthrough approach to fabrication of diode mid-IR lasers that have several advantages over IC lasers used for the Mars 2009 mission. This breakthrough is due to a novel design utilizing the strain-engineered quantum-well (QW) active region and quinternary barriers, and due to optimization of device material composition and growth conditions (growth temperatures and rates). However, in their present form, these GaSb-based laser diodes cannot be directly used as a part of sensor systems. The device spectrum is too broad to perform spectroscopic analysis of gas species, and operating currents and voltages are too high. In the current work, the emitters were fabricated as narrow-ridge waveguide index-guided lasers rather than broad stripe-gain guided multimode Fabry-Perot (FP) lasers as was done previously. These narrow-ridge waveguide mid-IR lasers exhibit much lower power consumptions, and can operate in a single spatial mode that is necessary for demonstration of single-mode distributed feedback (DBF) devices for spectroscopic applications. These lasers will enable a new generation of compact, tunable diode laser spectrometers with lower power consumption, reduced complexity, and significantly reduced development costs. These lasers can be used for the detection of HCN, C2H2, methane, and ethane.

Frez, Clifford F.↗
DOE OSTI2020

Scheme for stabilising the phase and arrival time of ultrashort laser pulses in a coherent beam combining fibre system

An algorithm has been demonstrated for simultaneously measuring the phase and arrival time of optical pulses relative to pulses in a reference channel using one detector array. Based on this algorithm, a simple optoelectronic pulse phase and arrival time stabilisation scheme has been designed for operation in a coherent beam combining fibre system for ultrashort pulses (including chirped ones). We have studied the performance of the stabilisation scheme. In particular, we have reached a phase measurement rate of 25 000 cps, demonstrated an ∼ 2 kHz limiting phase stabilisation frequency in a feedback loop, and obtained an arrival time measurement accuracy of ∼ 5 % of the transform-limited pulse duration at a measurement rate of 5 cps. In experiments concerned with coherent beam combining for two channels of a pulsed fibre system at a wavelength of 1030 nm, we have demonstrated phase stabilisation with an accuracy better than λ/100 and delay setting accuracy of 10 fs at a transform-limited pulse duration of ∼ 200 fs and obtained 94 % beam combining efficiency. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

Efficient Preparation of Dicke States

Here, we present an algorithm utilizing midcircuit measurement and feedback that prepares Dicke states with polylogarithmically many ancillae and polylogarithmic depth. Our algorithm uses only global midcircuit projective measurements and adaptively chosen global rotations. This improves over prior work that was only efficient for Dicke states of low weight or was not efficient in both depth and width. Our algorithm can also naturally be implemented in a cavity QED context using logarithmic time, zero ancillae, and atom-photon coupling scaling with the square root of the system size.

cavity methods↗
DOE OSTI2021

Giant nonlinear optical responses from photon-avalanching nanoparticles

Avalanche phenomena use steeply nonlinear dynamics to generate disproportionately large responses from small perturbations, and are found in a multitude of events and materials. Photon avalanching enables technologies such as optical phase-conjugate imaging, infrared quantum counting and efficient upconverted lasing. However, the photon-avalanching mechanism underlying these optical applications has been observed only in bulk materials and aggregates, limiting its utility and impact. In this study we report the realization of photon avalanching at room temperature in single nanostructures-small, Tm 3+ -doped upconverting nanocrystals-and demonstrate their use in super-resolution imaging in near-infrared spectral windows of maximal biological transparency. Avalanching nanoparticles (ANPs) can be pumped by continuous-wave lasers, and exhibit all of the defining features of photon avalanching, including clear excitation-power thresholds, exceptionally long rise time at threshold, and a dominant excited-state absorption that is more than 10,000 times larger than ground-state absorption. Beyond the avalanching threshold, ANP emission scales nonlinearly with the 26th power of the pump intensity, owing to induced positive optical feedback in each nanocrystal. This enables the experimental realization of photon-avalanche single-beam super-resolution imaging with sub-70-nanometre spatial resolution, achieved by using only simple scanning confocal microscopy and without any computational analysis. Pairing their steep nonlinearity with existing super-resolution techniques and computational methods, ANPs enable imaging with higher resolution and at excitation intensities about 100 times lower than other probes. The low photon-avalanching threshold and excellent photostability of ANPs also suggest their utility in a diverse array of applications, including sub-wavelength imaging and optical and environmental sensing.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Efficient Energy Funneling in Quasi‐2D Perovskites: From Light Emission to Lasing

Abstract Quasi‐2D Ruddlesden–Popper halide perovskites with a large exciton binding energy, self‐assembled quantum wells, and high quantum yield draw attention for optoelectronic device applications. Thin films of these quasi‐2D perovskites consist of a mixture of domains having different dimensionality, allowing energy funneling from lower‐dimensional nanosheets (high‐bandgap domains) to 3D nanocrystals (low‐bandgap domains). High‐quality quasi‐2D perovskite (PEA) 2 (FA) 3 Pb 4 Br 13 films are fabricated by solution engineering. Grazing‐incidence wide‐angle X‐ray scattering measurements are conducted to study the crystal orientation, and transient absorption spectroscopy measurements are conducted to study the charge‐carrier dynamics. These data show that highly oriented 2D crystal films have a faster energy transfer from the high‐bandgap domains to the low‐bandgap domains (<0.5 ps) compared to the randomly oriented films. High‐performance light‐emitting diodes can be realized with these highly oriented 2D films. Finally, amplified spontaneous emission with a low threshold 4.16 µJ cm −2 is achieved and distributed feedback lasers are also demonstrated. These results show that it is important to control the morphology of the quasi‐2D films to achieve efficient energy transfer, which is a critical requirement for light‐emitting devices.

Lei, Lei↗
DOE OSTI2024

Probabilistic inference of the structure and orbit of Milky Way satellites with semi-analytic modelling

Semi-analytic modelling furnishes an efficient avenue for characterizing dark matter haloes associated with satellites of Milky Way-like systems, as it easily accounts for uncertainties arising from halo-to-halo variance, the orbital disruption of satellites, baryonic feedback, and the stellar-to-halo mass (SMHM) relation. We use the SatGen semi-analytic satellite generator, which incorporates both empirical models of the galaxy–halo connection as well as analytic prescriptions for the orbital evolution of these satellites after accretion onto a host to create large samples of Milky Way-like systems and their satellites. By selecting satellites in the sample that match observed properties of a particular dwarf galaxy, we can infer arbitrary properties of the satellite galaxy within the cold dark matter paradigm. For the Milky Way’s classical dwarfs, we provide inferred values (with associated uncertainties) for the maximum circular velocity v max and the radius r max at which it occurs, varying over two choices of baryonic feedback model and two prescriptions for the SMHM relation. While simple empirical scaling relations can recover the median inferred value for v max and r max , this approach provides realistic correlated uncertainties and aids interpretability. We also demonstrate how the internal properties of a satellite’s dark matter profile correlate with its orbit, and we show that it is difficult to reproduce observations of the Fornax dwarf without strong baryonic feedback. Furthermore, the technique developed in this work is flexible in its application of observational data and can leverage arbitrary information about the satellite galaxies to make inferences about their dark matter haloes and population statistics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

A spin-wave magnetometer with a positive feedback

In this work, we demonstrate experimentally the operation of a spin-wave magnetometer integrated into a circuit with a positive feedback. The circuit consists of the passive magnetic and active electric parts. The magnetic part includes a sensing element, which is a magnetic cross junction made of Y 3 Fe 2 (FeO 4 ) 3 . The electric part includes a non-linear amplifier and a phase shifter. The electric and magnetic parts are connected via micrometer size antennae. Spin waves are excited by two of these antennae while the output inductive voltage produced by the interfering spin waves is detected by the third antenna. Spin waves propagating in the orthogonal arms of the cross can accumulate significantly different phase shifts, depending on the direction and the strength of the external magnetic field. The output inductive voltage reaches its maximum in the case of constructive spin wave interference. The positive feedback provides further signal amplification. It appears possible to enhance the response function, compared to the passive circuits without a feedback, by a factor of ×100 without an increase in the noise level. The experimental data show a prominent response to the external magnetic field variation, exceeding 5 x 10 3 V/T. The intrinsic noise spectral density of the device can be as low as 10 -16 V 2 /Hz. The estimated sensitivity of the prototype device is 2 x 10 -12 T/√Hz at room temperature. We argue that spin-wave magnetometers can potentially be as sensitive as SQUIDs while operating at room temperature.

36 MATERIALS SCIENCE↗
NASA NTRS2009

Complexity for Survival of Living Systems

A logical connection between the survivability of living systems and the complexity of their behavior (equivalently, mental complexity) has been established. This connection is an important intermediate result of continuing research on mathematical models that could constitute a unified representation of the evolution of both living and non-living systems. Earlier results of this research were reported in several prior NASA Tech Briefs articles, the two most relevant being Characteristics of Dynamics of Intelligent Systems (NPO- 21037), NASA Tech Briefs, Vol. 26, No. 12 (December 2002), page 48; and Self-Supervised Dynamical Systems (NPO- 30634) NASA Tech Briefs, Vol. 27, No. 3 (March 2003), page 72. As used here, living systems is synonymous with active systems and intelligent systems. The quoted terms can signify artificial agents (e.g., suitably programmed computers) or natural biological systems ranging from single-cell organisms at one extreme to the whole of human society at the other extreme. One of the requirements that must be satisfied in mathematical modeling of living systems is reconciliation of evolution of life with the second law of thermodynamics. In the approach followed in this research, this reconciliation is effected by means of a model, inspired partly by quantum mechanics, in which the quantum potential is replaced with an information potential. The model captures the most fundamental property of life - the ability to evolve from disorder to order without any external interference. The model incorporates the equations of classical dynamics, including Newton s equations of motion and equations for random components caused by uncertainties in initial conditions and by Langevin forces. The equations of classical dynamics are coupled with corresponding Liouville or Fokker-Planck equations that describe the evolutions of probability densities that represent the uncertainties. The coupling is effected by fictitious information-based forces that are gradients of the information potential, which, in turn, is a function of the probability densities. The probability densities are associated with mental images both self-image and nonself images (images of external objects that can include other agents). The evolution of the probability densities represents mental dynamics. Then the interaction between the physical and metal aspects of behavior is implemented by feedback from mental to motor dynamics, as represented by the aforementioned fictitious forces. The interaction of a system with its self and nonself images affords unlimited capacity for increase of complexity. There is a biological basis for this model of mental dynamics in the discovery of mirror neurons that learn by imitation. The levels of complexity attained by use of this model match those observed in living systems. To establish a mechanism for increasing the complexity of dynamics of an active system, the model enables exploitation of a chain of reflections exemplified by questions of the form, "What do you think that I think that you think...?" Mathematically, each level of reflection is represented in the form of an attractor performing the corresponding level of abstraction with more details removed from higher levels. The model can be used to describe the behaviors, not only of biological systems, but also of ecological, social, and economics ones.

Zak, Michail↗
DOE OSTI2020

Influence of zonal flow and density on resistive drift wave turbulent transport

The generations of zonal flow (ZF) and density (ZD) and their feedback on the resistive drift wave turbulent transport are investigated within the modified Hasegawa-Wakatani model. With proper normalization, the system is only controlled by an effective adiabatic parameter, a, where the ZF dominates the collisional drift wave (DW) turbulence in the adiabatic limit a > 1. By conducting direct numerical simulations, we found that the ZF can significantly reduce the transport by trapping the DWs in the vicinities of its extrema for a > 1, whereas the ZD itself has little impact on the turbulence but can only assist ZF to further decrease the transport by flattening the local plasma density gradient.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

High-Sensitivity rf Detection Using an Optically Pumped Comagnetometer Based on Natural-Abundance Rubidium with Active Ambient-Field Cancellation

To detect a specific radio-frequency (rf) magnetic field, rf optically pumped magnetometers (OPMs) require a static magnetic field to set the Larmor frequency of the atoms equal to the frequency of interest. However, unshielded and variable magnetic field environments (e.g., an rf OPM on a moving platform) pose a problem for rf OPM operation. Here, we demonstrate the use of a natural-abundance rubidium vapor to make a comagnetometer to address this challenge. Our implementation builds upon the simultaneous application of several OPM techniques within the same vapor cell. First, we use a modified implementation of an OPM variometer based on 87 Rb to detect and actively cancel unwanted external fields at frequencies ≲60 Hz using active feedback to a set of field control coils. In this experiment, we exploit this stabilized field environment to implement a high-sensitivity rf magnetometer using 85 Rb. Using this approach, we demonstrate the ability to measure rf fields with a sensitivity of approximately 9 fT Hz -1/2 inside a magnetic shield in the presence of an applied field of approximately 20 μT along three mutually orthogonal directions. This demonstration opens up a path toward completely unshielded operation of a high-sensitivity rf OPM.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Systematizing the effective theory of self-interacting dark matter

If dark matter has strong self-interactions, future astrophysical and cosmological observations, together with a clearer understanding of baryonic feedback effects, might be used to extract the velocity dependence of the dark matter scattering rate. To interpret such data, we should understand what predictions for this quantity are made by various models of the underlying particle nature of dark matter. In this paper, we systematically compute this function for fermionic dark matter with light bosonic mediators of vector, scalar, axial vector, and pseudoscalar type. We do this by matching to the nonrelativistic effective theory of self-interacting dark matter and then computing the spin-averaged viscosity cross section nonperturbatively by solving the Schrödinger equation, thus accounting for any possible Sommerfeld enhancement of the low-velocity cross section. In the pseudoscalar case, this requires a coupled-channel analysis of different angular momentum modes. We find, contrary to some earlier analyses, that nonrelativistic effects only provide a significant enhancement for the cases of light scalar and vector mediators. Scattering from light pseudoscalar and axial vector mediators is well described by tree-level quantum field theory.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

An Electrical Resistance Diagnostic for Conductivity Monitoring in Laser Powder Bed Fusion

With the growing interest in metal additive manufacturing using laser powder bed fusion (LPBF), there is a need for advanced in-situ nondestructive evaluation (NDE) methods that can dynamically monitor manufacturing process-related variations, that can be used as a feedback mechanism to further improve the manufacturing process, leading to parts with improved microstructural properties and mechanical properties. Current NDE techniques either lack sensitivity beyond build layer, are costly or time-consuming, or are not compatible for in-situ integration. In this research, we develop an electrical resistance diagnostic for in-situ monitoring of powder fused regions during laser powder bed fusion printing. The technique relies on injecting current into the build plate and detecting voltage differences from conductive variations during printing using a simple, cheap four-point electrode array directly connected to the build plate. A computational model will be utilized to determine sensitivities of the approach, and preliminary experiments will be performed during the printing process to test the overall approach.

36 MATERIALS SCIENCE↗
NASA NTRSDate not supplied

X-Ray Missions Based on LTD Technologies

Microcalorimeter arrays used as imaging spectrometers will enable ground-breaking science in X-ray astrophysics. Their development has been one of the driving applications of the low temperature detector community since the early 1980s. While their application in space remains in relative infancy, we are on the verge of an era in which microcalorimeter spectrometers are likely to dominate instrumentation for high-energy astrophysics missions. NASA sounding rocket experiments such as the X-ray Quantum Calorimeter (XQC) and Micro-X have now paved the way for orbital observatories. JAXA’s Astro-H gave us a glimpse of this fantastic new capability before its unfortunate demise. The launch of XRISM later this year should finally demonstrate the sort of large suite of observations that X-ray microcalorimeter arrays will make major contributions to. In the mid-2030s, we will see the launch of ESA’s flagship Athena mission, that will further advance the imaging and spectroscopic capabilities for the high-energy X-ray community enormously. Numerous other potential new mission concepts using X-ray microcalorimeters have been studied in detail such as NASA’s Lynx and the Light Element Mapper (LEM), JAXA’s Super-DIOS, and China’s Hot Universe Baryon Surveyor (HUBS). In the first half of this presentation, I will review the development and desired requirements of the X-ray microcalorimeter missions and concepts, and describe the current progress and status missions being implemented and proposed. In the second half of this presentation, I will focus on The Line Emission Mapper (LEM) which is a probe-class mission concept under study by NASA that is designed to provide unprecedented insight into the physics of galaxy formation, including stellar and black-hole feedback and flows of baryonic matter into and out of galaxies. LEM incorporates a light-weight X-ray optic with 10” angular resolution and a large-format microcalorimeter array with a 15” pixel pitch over a 29’ field of view (FOV). The main microcalorimeter array and readout design takes advantage of mature technology that has been developed for Athena X-IFU. The central 7’ region of the array consists of ~ 800 transition-edge sensors (TESs), optimized for a bandpass of 0.3-2 keV and with an energy resolution of 1.2 eV at 1 keV. The rest of the FOV is covered by 4-pixel TES hydras with 2.5 eV energy resolution at 1 keV. Hydras are position-sensitive (‘thermally multiplexed’) detectors that enable extremely large numbers of effective pixels in an array, without a commensurate increase in the number of wires, bias circuit, and readout components. In total the array will have ~ 4k TESs with ~ 14k imaging elements on a 290 micron-pitch. The array will be read out with state-of-the-art time-division multiplexing (TDM), implement with 59 pixels (and 1 dark pixel) in each of the 69 TDM columns. Here we present a detailed overview of the baseline microcalorimeter detector design and present first results from both single pixel TESs and 4-pixel hydras. Our prototype LEM pixels utilize 15um x 50um Mo/Au TESs with a transition temperature of around 58 mK. These pixels incorporate high-fill-factor Au absorbers of thickness 0.54um. We have demonstrated an energy resolution of 0.90+/-0.02 eV and 1.90 +/-0.02 eV at 1.5 keV for single pixel and 4-pixel hydras, respectively, meeting the performance requirements of LEM. We show how the position discrimination in the hydra pixels can be achieved, down to energies of a few 100 eV, using the measured pulse rise-times. Finally, we will show that the properties of the LEM pixels are well optimized for the proposed TDM read out architecture.

Simon Richard Bandler↗
DOE OSTI2022

High resolution atomic force microscopy with an active piezoelectric microcantilever

Active microcantilevers with on-chip sensing and actuation provide significant advantages in tapping mode Atomic Force Microscopy (AFM). Collocated transduction allows for effective manipulation of cantilever dynamics through feedback control, enabling higher scan rates. However, the adjacency of the sensing and actuation electrodes is known to result in a high level of feedthrough, leading to a low imaging resolution. Readout circuit noise further deteriorates the imaging precision. Here, we investigate the noise sources that affect AFM microcantilevers with collocated aluminum nitride (AlN) actuator–sensor pairs. We reported these cantilevers in earlier work and demonstrated that they display a very low level of feedthrough between the actuation and sensing electrodes. We present a high signal-to-noise ratio (SNR) sensing method that enables us to demonstrate high-resolution AFM on a calibration grating with nm-step silicon carbide (SiC) terraces. In conclusion, measuring the Lorentzian response of the cantilever’s Brownian motion with the on-chip active sensor at resonance enables us to calibrate the dynamic stiffness at the first fundamental resonance mode, without utilizing an optical sensor.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Dynamically controlled random lasing with colloidal titanium carbide MXene

Control of lasing properties through tailorable and dynamically tunable materials and reconfigurable compositions can augment the performance of random lasers for a wide range of applications. Here, a colloid of randomly dispersed weakly scattering single-layer titanium carbide (Ti 3 C 2 T x ) MXene flakes embedded within rhodamine 101 gain medium is experimentally shown to provide feedback for random lasing. Additionally, in contrast to previously reported random laser systems where the optical properties of scatterers are static, the relative permittivity of Ti 3 C 2 T x MXene flakes can be varied under optical pumping due to the saturable absorption properties. Numerical simulations indicate that the observed nonlinear response of Ti 3 C 2 T x MXene flakes enables dynamically tunable random lasing. Thus, pumping the Ti 3 C 2 T x MXene flakes with a second optical source decreases the gain threshold required to obtain random lasing. Also, using numerical simulations, it is shown that the control over the intensity of the second pump enables tuning the field distribution of the random lasing modes. Considering the diversity of the MXenes family, the proposed MXene colloidal metamaterial design opens up a new avenue to advanced control of lasing properties for photonic applications.

36 MATERIALS SCIENCE↗