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At least 181 records · Page 10

Cold Spray Deposition of 304L Stainless Steel to Mitigate Chloride-Induced Stress Corrosion Cracking in Canisters for Used Nuclear Fuel Storage

A feasibility study of the cold spray deposition process of 304L stainless steel on 304L stainless steel substrates as a mitigation method for chloride-induced stress corrosion cracking (CISCC) has been investigated under various substrate conditions. The study is aimed at the application of this technology to mitigate CISCC that may potentially occur in or nearthe fusion welded regions of stainless steel canisters in Dry Cask Storage System (DCSS) for used nuclear fuels. Spherical gas-atomized 304L stainless steel powder, in the size range of 25 µm to 44 µm, was used as a feedstock powder for the cold spray process. The powder was deposited on four types of 304L substrates with various surface conditions: as-polished, oxidized, cold-rolled, plates with prototypical CISCC. The effects of cold spray parameters on quality of cold spray coatings were investigated. Thickness, porosity, and phases in the as-deposited materials were evaluated using scanning electron microscopy (SEM) and X-ray diffraction (XRD), and correlated with microhardness and adhesion strength measured via micro-indentation and ASTM C633 pulling test, respectively. XRD analysis of the coatings was also conducted to examine the effects of cold spray condition on residual stress state in the coating. Detailed cross-sectional examination of coating/substrate interfaces was performed with transmission electron microscopy (TEM) equipped with energy dispersive spectroscopy (EDS). Dense and continuous coatings with good adhesion strength and hardness were produced for the various substrate conditions by adjusting cold spray parameters. The results demonstrate that cold spray stainless steel coating is a viable option to provide a physical barrier against CISCC in fusion weld regions of stainless steel in corrosive chloride salt-bearing environments.

Dry Cask Storage Systems, cold spray, 304L stainle↗

The Need for Integrating the Back End of the Nuclear Fuel Cycle in the United States of America

Current practice for commercial spent nuclear fuel management in the United States of America (US) includes storage of spent fuel in both pools and dry storage cask systems at nuclear power plants. Most storage pools are filled to their operational capacity, and management of the approximately 2,200 metric tons of spent fuel newly discharged each year requires transferring older and cooler fuel from pools into dry storage. In the absence of a repository that can accept spent fuel for permanent disposal, projections indicate that the US will have approximately 134,000 metric tons of spent fuel in dry storage by mid-century when the last plants in the current reactor fleet are decommissioned. Current designs for storage systems rely on large dual-purpose (storage and transportation) canisters that are not optimized for disposal. Various options exist in the US for improving integration of management practices across the entire back end of the nuclear fuel cycle.

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Materials and Dimensional Reference Handbook for the Boiling Water Reactor Dry Cask Simulator.

The performance of commercial nuclear spent fuel dry storage casks is evaluated through detailed analytical modeling of the system’s thermal performance. A recent investigation has been completed that produced a data set that can be used to test the validity of the modeling presently used to determine cladding temperatures in modern vertical dry casks. To produce these data sets under well-controlled boundary conditions, the dry cask simulator (DCS) was built to study the thermal-hydraulic response of fuel under a variety of heat loads, internal vessel pressures, and external configurations [Durbin and Lindgren, 2017]. The experiments were conducted in Albuquerque, New Mexico where the local ambient atmospheric pressure is typically 83 kPa. The purpose of this handbook is to document the pertinent geometric and material property information needed to perform model validation efforts.

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Simulation of Proposed Heat Treatment Methods for the Sister Rods

The High Burnup Spent Fuel Data Project (the 'project'), sponsored by the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE), is focused on experimentally evaluating the effects of long-term dry storage and transportation on high burnup (HBU) pressurized water reactor (PWR) fuel (>45 gigawatt days per metric ton uranium). The goals of the project are to provide confirmatory data for analytical model validation and potential improvement; to provide input to future dry storage cask design; to support license renewals and new licenses for Independent Spent Fuel Storage Installation facilities; and to support transportation licensing for high burnup used fuel. In support of these project goals, an instrumented TN-32B bolted-lid cask (the Research Project Cask or RPC) at the North Anna reactor site will be loaded with intact, HBU PWR fuel assemblies (Project Assemblies) having four different kinds of cladding: standard Zircaloy-4, low-tin Zircaloy-4, ZIRLO{sup R}, and M5{sup R}. In approximately ten years, the instrumented cask will be opened for inspection and several fuel rods from the Project Assemblies will be characterized. The project has also removed 25 'sister rods' from assemblies at North Anna: 9 directly from the project assemblies and 16 from similarly constructed and operated HBU assemblies. The 25 sister rods are all high burnup and cover the range of domestically-used cladding alloys. The 25 sister rods were shipped to Oak Ridge National Laboratory (ORNL) in early 2016 for detailed non-destructive examinations (NDE) followed by destructive examination (DE). Examination of the sister rods will provide a baseline for comparison with the cask rods and will allow for separate effects testing. Dry storage canister loading is completed under water in a designated area of the plant's spent fuel pool. In preparation for dry storage, the fuel assemblies and canister cavity must be drained and dried. Typically, the highest temperatures experienced by the fuel during dry storage are encountered either during drying or transfer of the canister to the storage pad; therefore, as a part of the sister rod testing these temperatures will be simulated in the lab to produce samples that are representative of the peak cladding temperature the fuel experiences either during drying, transfer, or storage. (authors)

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Muon Tracing and Image Reconstruction Algorithms for Cosmic Ray Muon Computed Tomography

Cosmic ray muon-computed tomography (μCT) is a new imaging modality with unique characteristics that could be particularly important for diverse applications including nuclear nonproliferation, spent nuclear fuel monitoring, cargo scanning, and volcano imaging. The strong scattering dependence of muons on atomic number Z in combination with high penetration range could offer a significant advantage over existing techniques when dense, shielded containers must be imaged. However, μCT reconstruction using conventional filtered back-projection is limited due to the overly simple assumptions that do not consider the curved path caused by multiple Coulomb scattering prompting the need for more sophisticated approaches to be developed. Here, we argue that the use of improved muon tracing and scattering angle projection algorithms as well as an algebraic reconstruction technique should produce muon tomographic images with improved quality–or require fewer muons to produce the same image quality–compared to the case where conventional methods are used. We report on the development and assessment of three novel muon tracing methods and two scattering angle projection methods for μCT. Simulated dry storage casks with single and partial missing fuel assemblies were used as numerical examples to assess and compare the proposed methods. The reconstructed images showed an expected improvement in image quality when compared with conventional techniques, even without muon momentum information, which should lead to improved detection capability, even for partial defects.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Non-destructive evaluation and machine learning methods for inspection of spent nuclear fuel canisters: A state-of-the-art review

Nuclear energy is among the cleanest and most efficient energy sources currently available. The operation of nuclear power plants (NPPs) produces large amounts of high-level radioactive waste known as spent nuclear fuel (SNF). Currently, large amounts of SNF is stored in dry cask storage systems (DCSSs) for extended interim storage until a permanent disposal solution becomes available. During the extended interim storage, the DCSS, particularly the SNF canisters, may degrade and abnormal conditions may occur. Therefore, non-destructive evaluation (NDE) and machine learning (ML) approaches are necessary for inspection of SNF canisters. This paper presents a state-of-the-art review of literature by summarizing recent progress made on the applications of NDE and ML for inspection of SNF canisters. Sixteen NDE methods are examined and compared: visual inspection, ultrasonic guided waves (UGWs), laser-based approaches, acoustic emission (AE), eddy current testing (ECT), non-invasive acoustic sensing, dynamic modal testing, cosmic ray muons tomography, neutron imaging, gamma rays detection, fiber optical sensors, through-wall communications, X-ray computed tomography (CT), vibrothermography, monoenergetic photon sources, and surface acoustic wave (SAW) sensors. The technology readiness level (TRL) for each method is assessed and compared. Recent publications on ML-enhanced visual inspection, AE, non-invasive acoustic sensing, dynamic modal testing, and neutron imaging for SNF canisters are summarized and future research needs are identified. In conclusion, this review article provides a convenient reference on the state-of-the-art applications of NDE and ML methods for inspection of SNF canisters.

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Optimization Scheme for Establishing Queues for Shipment of UNF from Shutdown Reactor Sites - 17554

Approximately 14, 815 used nuclear fuel assemblies (5,800 MTHM) are stored in 486 dry storage cask systems located at 12 independent spent fuel storage installations (ISFSIs) located at shutdown reactor sites located across the U.S. that have no access to spent fuel pools. A preliminary evaluation was performed by the University of North Carolina at Charlotte (UNCC) in collaboration with AREVA to establish optimization schemes for establishing queues for the removal of this used/spent nuclear fuel (hence forth identified as UNF) and Greater than Class C low level wastes (GTCC) found at these shutdown reactor sites. These queues assumed the major portion of the shipment of the UNF and GTCC would be by rail, with heavy haul truck or barge potentially utilized to move the UNF from the site to rail for sites not served directly by rail. The destination for these rail shipments were a hypothetical consolidated interim storage facility (CSF) located in West Texas. The queues were developed based on the total costs and time to finish all shipments needed to remove all the UNF from these shutdown sites. Results are presented for optimization schemes based on a continuous flow of shipments using 1, 2, and 3 crews dedicated to individual ISFSIs and discrete shipments using 2 crews capable of performing operations at multiple ISFSIs. (authors)

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High-level waste relocation requires use of new technology in aging nuclear facility - 15269

The West Valley Demonstration Project (WVDP) is preparing to relocate 278 canisters of vitrified high-level waste (HLW) from their current location inside the Main Plant Process Building (MPPB) to an outdoor pad for long-term, on-site storage. The waste was produced at the WVDP between 1996 and 2002 and was originally placed in interim storage inside the MPPB in anticipation of off-site shipment for disposal. Relocation of the canisters to a new on-site location is now necessary as part of WVDP Phase 1 Site Decommissioning work to enable pre-demolition activities inside the MPPB to proceed. The logistics of packaging and moving the HLW canisters within an aging facility to another on-site location has provided numerous technical challenges with subsequent innovations. Significant preparations have taken place to resolve structural inadequacies, including sub-surface soil subsidence issues, antiquated equipment, and facility reconfigurations to support up to 134 metric ton (148 ton) loads. To perform the transfer and storage of the HLW canisters, new equipment and fabrications were required including a robust storage system consisting of stainless steel canister overpacks within steel-reinforced concrete storage casks, three specialty cask transporters, a remotely operated welding system and construction of an outdoor engineered storage pad to store the 56 casks containing the relocated HLW canisters. Packaging and relocation of vitrified canisters is scheduled to begin in 2015. (authors)

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Storage and Transport Cask Data For Used Commercial Nuclear Fuel

This document is a compilation of publicly available information on spent/used nuclear fuel storage and transport casks in use in the United States as of the summer of 2013. As such, it is a functional update and extension of JAI-582, “Shipping and Storage Cask Data For Commercial Spent Nuclear Fuel,” originally published by JAI Corporation in March 2005. This report is intended to provide a convenient reference for those with interest in, or those engaged in the production, handling, storage, transport, and disposition of spent/used commercial nuclear fuel. Data for each cask is tabulated in a standardized table format to facilitate rapid access to key design and performance information, and to enable the document user to more rapidly conduct comparative analyses of cask design and performance parameters. Multiple-assembly “canisters,” and both canister-based and non-canistered packages are included in the main body of the report. Packages that have been used in the past, but which are no longer in active use in the U.S., are included in Appendix A.

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Thermal Analysis Capability of UNF-ST&DARDS

In the United States, approximately 2,500 casks are loaded with commercial spent nuclear fuel (SNF) that has transitioned from wet storage (spent fuel pools) to dry storage. The number of loaded dry storage casks is increasing by approximately 200 each year. Over time, cask designs have evolved to enhance safety and to accommodate more fuel and higher heat loads. Also, higher burnup fuel is being transitioned into dry storage. The SNF is being stored in dry casks for longer times than specified in the original certification period. Several degradation mechanisms related to fuel assemblies and canisters are affected by temperature. For the cladding, temperature-dependent phenomena include creep and annealing, hydride reorientation and embrittlement, and the ductile-to-brittle transition. Temperature can also influence phenomena that affect the long-term integrity of the storage system, including deliquescence, corrosion, and stress-corrosion cracking. Therefore, accurate determination of the temperatures of various components is needed to evaluate potential safety-related issues during transportation after extended storage and to ensure SNF retrievability. The Used Nuclear Fuel-Storage, Transportation & Disposal Analysis Resource and Data System (UNF ST&DARDS) is being developed for the US Department of Energy Office of Nuclear Energy to streamline analyses for the waste management system [1]. Lastly, the thermal analysis capability within UNF-ST&DARDS and example results are discussed herein.

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Dry Canister Storage System Inspection and Robotic Delivery System Development

EPRI is working to develop and demonstrate technologies capable of inspecting welded stainless steel canisters used in dry cask storage systems in situ, without the need to remove them from their concrete casks. This involves the coupling of specialized cameras and inspection devices with small remotely operated vehicles (ROVs). The objective is to demonstrate the capability to identify any presence of (or precursors to) stress corrosion cracking (SCC) and other anomalies that may require additional investigation. (authors)

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Long-term Prediction of Spent Fuel Storage Canisters - Issues and Approaches - 18112

The considerations involved in aging management of stainless steel canisters used in dry cask storage of spent fuel are discussed in this paper in a probabilistic framework. The two important modes of degradation in the long-term performance of the casks are localized corrosion and stress corrosion cracking initiating from the external surface. These degradation modes are determined by the evolution of the electrochemical behavior and the strain rate of the stainless steel. Laboratory data suggest that Type 304L/316L stainless steels should suffer from localized corrosion and SCC under salt deposits. However, field inspection of the canisters has not indicated extensive pitting or stress corrosion cracking. This discrepancy can be understood in terms of the joint probabilities of various factors that must come together to cause these failure modes. A Bayesian network approach is suggested as the framework for modeling the probability of failure of canisters and long-term management of aging. The gaps in knowledge to conduct a Bayesian network analysis are discussed. (authors)

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Used Fuel Disposition Campaign - Baseline Studies for Ring Compression Testing of High-Burnup Fuel Cladding

Structural analyses of high-burnup fuel require cladding mechanical properties and failure limits to assess fuel behavior during long-term dry cask storage and transportation. Pre-storage drying-transfer operations and early stage storage subject cladding to higher temperatures and much higher pressure-induced tensile hoop stresses relative to in-reactor operation and pool storage. Under these conditions, radial hydrides may precipitate during slow cooling and provide an additional embrittlement mechanism as the cladding temperature decreases below the ductile-to-brittle transition temperature (DBTT). On the basis of previous test results, susceptibility to radial-hydride precipitation depends on cladding material, microstructure, and pre-drying distribution of hydrides across the cladding wall, as well as peak hoop stresses and temperatures during drying operations and storage. Susceptibility to embrittlement depends on the extent of radial-hydride precipitation and the thickness of the outer-surface hydride rim. These results highlight the importance of determining the DBTT for high-burnup cladding as a function of peak drying-storage temperatures and stresses and including the relevant mechanical properties in cask structural analyses. Additional testing is needed at lower (and perhaps more realistic) peak drying-storage temperatures and stresses, for which the DBTT is expected to decrease.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Addressing Facility Needs for Concrete Assessment Using Ultrasonic Testing: Mid-year Report

The UFD Gap Analysis to Support Extended Storage of Used Nuclear Fuel (June 30, 2011) emphasizes the need for the development of monitoring techniques and technologies for dry storage cask materials. A high priority is given to the development of 'systems for early detection of confinement boundary degradation.' This requires both new techniques for monitoring and inspection, as well as new measurable parameters to quantify mechanical degradation. The use of Nonlinear Elastic Wave Spectroscopy (NEWS) has been shown to provide sensitive parameters correlating to mechanical degradation in a wide variety of materials. Herein we report upon recent research performed to address the high priority of concrete degradation using a selection of these techniques and compare to a ASTM standard ultrasonic technique. Also reported are the near term plans to continue this research in the remaining FY and into the coming years. This research was conducted at Los Alamos National Laboratory (LANL) in the Acoustics Lab of the Geophysics group in the Earth and Environmental Sciences division, and in collaboration with the Laboratory for Nondestructive Evaluation at the University of the Mediterranean (Aix en Provence, France) and the Electrical Power Research Institute (EPRI). The objective of this research project was to determine the feasibility of using an NDE technique based on non-linear ultrasound for determining the depth and degree of microcracking in the near surface of concrete and to assess the degree of sensitivity of such technique. This objective is reached by the means of combining linear and nonlinear measurements, associated with numerical simulation. We first study the global effect of thermal damage on concrete's linear and nonlinear properties by resonance inspection techniques. We show that standard pulse wave speed techniques are not relevant to extract mechanical properties of concrete. The high sensitivity of measured nonlinearity is shown and serves as a validation tool for the rest of the study, i.e., probing the material nonlinearity at various depths through the use of Time Reversal Elastic Nonlinearity Diagnostic (TREND). The basic idea of probing the material nonlinearity at various depths by changing the frequency is validated by exhibiting a similar trend as nonlinear resonance measurements. We address at the end of this report, the potentialities of applying these procedures to real concrete structures.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Experimental Seismic Response of Scaled Storage Containments under Identical Loading Conditions - 16318

Dry Storage Casks (DSCs) store spent nuclear fuel (SNF), usually at sites contiguous to nuclear power plants known as Independent Spent Fuel Storage Installation (ISFSI). DSCs have been considered as a temporary storage solution, and are usually licensed for 20 years, which can be extended up to an operating periods of 60 years. Recently, however, DSCs have been considered as a potential mid-term solution for hundreds of years. This consideration requires reevaluation of DSC performance under a larger seismic hazard. That leads to larger horizontal and vertical accelerations. This study is a part of a research project evaluating the seismic response of free-standing DSCs under long return period seismic events. This article assess whether the response of free-standing structures under seismic excitation is repeatable. For this purpose, experimental tests were conducted using a six degree-of-freedom (6DOF) shake table. During the experimental tests, several ground motions were repeated multiple times to obtain the dynamic response under identical loading conditions. Scaled casks of four aspect ratios (radius to centroidal height ratio, r/h{sub cg}) were studied: 0.39, 0.43, 0.55 and 0.62. The specimens studied are considered to be 1:2.5 and 1:3.5 scaled model of generic prototype casks. The experimental results show that a small change in initial conditions leads to change in the boundary condition of moving bodies and in combination with acceleration being applied at different frequencies contained within the applied ground motions may lead to a large variation in the response. (authors)

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Sister Rod Nondestructive Examination Final Report

This report documents work performed under the Spent Fuel and Waste Disposition for the US Department of Energy (DOE) Office of Nuclear Energy (NE) Spent Fuel and Waste Science and Technology program. This work was performed to fulfill the Level 2 Milestone M2SF-17OR010201021, “Documentation of Non-destructive Tests on Sister Pins,” within work package SF-17OR01020102. The High Burnup Spent Fuel Data Project, sponsored by DOE-NE, is focused on understanding the effects of long-term storage and transportation on high burnup (HBU) (>45 gigawatt days per metric ton uranium) light water reactor fuel. The goals of the project are to “provide confirmatory data for model validation and potential improvement, provide input to future spent nuclear fuel (SNF) dry storage cask design, support license renewals and new licenses for Independent Spent Fuel Storage Installations (ISFSIs), and support transportation licensing for high burnup SNF". In support of project goals, 25 sister rods were removed from fuel assemblies at the North Anna Power Station. Nine rods were removed from the project assemblies, and 16 rods were removed from similar HBU assemblies. The 25 sister rods were shipped to Oak Ridge National Laboratory (ORNL) Irradiated Fuels Examination Laboratory (IFEL) in early 2016 for detailed nondestructive examination (NDE) and destructive examination (DE). The detailed examinations will provide essential information on the physical state of the HBU rods and the fuel contained in the rods prior to loading, drying, and long-term dry storage. Similar tests will be performed at the end of the long-term storage period to identify any changes in the fuel rods’ properties during the dry storage period.

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Higher harmonic ultrasonic guided waves for structural integrity assessment of dry storage canisters - 15381

Dry storage of used fuel from nuclear power plants has gone from an interim storage solution to a longer-term solution, which necessitates monitoring the integrity of the stainless steel canister that confines the used fuel. Since the storage facilities are located around the country in a variety of different environments there is a wide range of degradation mechanisms that could occur over time in the cylindrical canister. One potential degradation mode that has created significant concern is stress corrosion cracking. We propose using higher harmonic ultrasonic guided waves as a tool to nondestructively inspect used fuel canisters. Higher harmonics are generated when a wave propagates through a nonlinear elastic media. These higher harmonics have been shown to be quite sensitive to microstructural features such as dislocation substructures, persistent slip bands, precipitates, etc. The use of ultrasonic guided waves to inspect the canister is attractive due to the size of the canister and the ability of guided waves to inspect a reasonably large domain relative to traditional bulk wave ultrasonics. We will highlight our recent progress on theory, numerical simulations, and laboratory experiments to develop higher harmonic guided waves as a tool to detect microstructural changes that precede macro-scale damage. Analyzed structures include plates and hollow cylinders, and we focus on localized damage initiation, as is the case for stress corrosion cracking. Recent experiments focus on using magnetostrictive transducers in activating the fundamental shear horizontal mode (SH0) and the third harmonic that is generated due to the material nonlinearity. The magnetostrictive transducer comprises a thin iron-cobalt foil, a meandering electric coil, and a permanent magnet. These transducers are inexpensive, easy to use, and are very efficient at generating shear waves. In applications where the wavelength is larger than the plate thickness, the waves are guided by the traction free boundary conditions and propagate in the plane of the plate. For this canister application, the shear horizontal waves energize the entire thickness of the canister and propagate along the shell in the direction dictated by the meander coil. Experiments indicate that magnetostrictive transducers can generate waves that propagate in plate thicknesses of 1 mm to at least 16 mm. The SH0 mode is nondispersive and generates a third harmonic of the same mode that is shown to be sensitive to localized plastic strain and unseen fatigue damage. It has a strong potential to detect the very early stages of stress corrosion cracking. Due to the geometric configuration of dry storage casks, the transducers will need to be delivered to the inspection points by a robotic system that navigates through the cask ventilation system. (authors)

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Accident analysis of spent fuel storage and transportation cask with Gd based neutron absorber

The shortage of nuclear spent fuel storage pool has been issued. The spent fuel storage and transportation cask is one of the major alternatives for storing spent fuel. The use of advanced neutron absorber is important for effective storage of spent fuel in spent fuel cask. Gadolinium based neutron absorber is chosen since it has high neutron absorption cross section in thermal neutron region compared to boron and it does not produce any gas element when it reacts with a neutron. The major requirement for neutron absorbing materials in the spent fuel cask system is to maintain subcriticality in normal, off-normal and accident conditions. In this study, the criticality calculations under accident conditions are conducted to ensure the safety of spent fuel cask. Major accident conditions are flood and cask tip-over. The full and partial flooded condition is analyzed and 100% flooded condition has the highest reactivity. The water density is selected as 1 g/cm{sup 3} because k{sub eff} is highest at this condition. When the cask tip-over, the flux trap reduces. In this case, a huge increase in reactivity of 800 pcm takes place. (authors)

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