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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

A survey of pedestal magnetic fluctuations using gyrokinetics and a global reduced model for microtearing stability

This article presents a global reduced model for slab-like microtearing modes (MTMs) in the H-mode pedestal, which reproduces distinctive features of experimentally observed magnetic fluctuations, such as chirping and discrete frequency bands at noncontiguous mode numbers. Our model, importantly, includes the global variation of the diamagnetic frequencies, which is necessary to reproduce the experimental observations. The key insight underlying this model is that MTM instability is enabled by the alignment of a rational surface with the peak in the profile of the diamagnetic frequency. Conversely, MTMs are strongly stabilized for toroidal mode numbers for which these quantities are misaligned. This property explains the discrete fluctuation bands in several DIII-D and JET discharges, which we survey using our reduced model in conjunction with global gyrokinetic simulations. A fast yet accurate reduced model for MTMs enables rapid interpretation of magnetic fluctuation data from a wide range of experimental conditions to help assess the role of MTM in the pedestal.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Neutron-producing gas puff Z-pinch experiments on a fast, low-impedance, 0.5 MA linear transformer driver

A study on the neutron production from single and double gas puff Z-pinches on the CESZAR linear transformer driver with ~0.45 MA current and 170 ns rise time is presented. Total neutron yield measurements made with a LaBr activation detector are compared for three configurations, using a double nozzle setup. When a single, hollow, deuterium gas shell was used, reliable implosions could only be attained at higher load mass than the optimal value to match implosion time with the driver rise time, with neutron yields of ~10 6 per pulse. The use of a double gas puff configuration with a deuterium center jet allowed a reduction in the shell density and operation closer to machine-matched conditions, recording up to (4.1 ± 0.3) × 10 7 neutrons/pulse when either Kr or D 2 was used in the shell. For a comparable mass and implosion time, using a higher atomic-number gas in the outer shell results in more unstable plasma surface and smaller plasma radius at the location of instability bubbles, which, however, do not seem to consistently correlate with a higher neutron yield. Comparing implosion dynamics with models and neutron yields with literature scaling suggests that the machine current is not well coupled to the plasma during the final stages of compression. Optimizing current and energy coupling to the pinched plasma is critical to improving performance, particularly in low-impedance drivers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

The Role of Cloud–Cloud Interactions in the Life Cycle of Shallow Cumulus Clouds

Some of the climate research puzzles relate to a limited understanding of the critical factors governing the life cycle of cumulus clouds. These factors force the initiation and the various mixing processes during cloud life cycles. To shed some light into these processes, we tracked the life cycle of thousands of individual shallow cumulus clouds in a large-eddy simulation during the Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems field campaign in the U.S. southern Great Plains. Concurrent evolution of clouds is tracked and their respective neighboring clouds are examined. Results show that the clouds initially smaller than neighboring clouds can grow larger than the neighboring clouds by a factor of 2 within 20% of their lifetime. Two groups of the tracked clouds with growing and decaying neighboring clouds, respectively, show distinct characteristics in their life cycles. Clouds with growing neighboring clouds form above regions with larger surface heterogeneity, whereas clouds with decaying neighboring clouds are associated with less heterogeneous surfaces. Also, those with decaying neighboring clouds experience larger instability and a more humid boundary layer, indicating evaporation below the cloud base is likely occurring before those clouds are formed. Larger instability leads to higher vertical velocity and convergence within the cloud, which causes stronger surrounding downdrafts and water vapor removal in the surrounding area. The latter appears to be the reason for the decaying neighboring clouds. Finally, understanding those processes provide insights into how cloud–cloud interactions modulate the evolution of cloud population and into how this evolution can be represented in future cumulus parameterizations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

The Scale and Activity of Symmetric Instability Estimated from a Global Submesoscale-Permitting Ocean Model

Abstract Symmetric instability (SI) extracts kinetic energy from fronts in the surface mixed layer (SML), potentially affecting the SML structure and dynamics. Here, a global submesoscale-permitting ocean model named MITgcm LLC4320 simulation is used to examine the Stone linear prediction of the maximum SI scale to estimate grid spacings needed to begin resolving SI. Furthermore, potential effects of SI on the usable wind work are estimated roughly: this estimate of SI “activity” is useful for assessing if these modes should be resolved or parameterized. The maximum SI scale varies by latitude with median values from 568 to 23 m. Strong seasonality is observed in the SI scale and activity. The median scale in winter is 188 m globally, 2.5 times of that of summer (75 m). SI is more active in winter: 15% of the time compared with 6% in summer. The strongest SI activity is found in the western Pacific, western Atlantic, and Southern Oceans. The required grid spacings for a global model to begin resolving SI eddies in the SML are 24 m (50% of regions resolved) and 7.9 m (90%) in winter, decreasing to 9.4 m (50%) and 3.6 m (90%) in summer. It is also estimated that SI may reduce usable wind work by an upper bound of 0.83 mW m −2 globally, or 5% of the global magnitude. The sensitivity of these estimates to empirical thresholds is provided in the text.

Dong, Jihai↗
DOE OSTI2023

Three-dimensional Dynamics of Strongly Twisted Magnetar Magnetospheres: Kinking Flux Tubes and Global Eruptions

Abstract The origins of the various outbursts of hard X-rays from magnetars (highly magnetized neutron stars) are still unknown. We identify instabilities in relativistic magnetospheres that can explain a range of X-ray flare luminosities. Crustal surface motions can twist the magnetar magnetosphere by shifting the frozen-in footpoints of magnetic field lines in current-carrying flux bundles. Axisymmetric (2D) magnetospheres exhibit strong eruptive dynamics, i.e., catastrophic lateral instabilities triggered by a critical footpoint displacement of ψ crit ≳ π . In contrast, our new three-dimensional (3D) twist models with finite surface extension capture important non-axisymmetric dynamics of twisted force-free flux bundles in dipolar magnetospheres. Besides the well-established global eruption resulting (as in 2D) from lateral instabilities, such 3D structures can develop helical, kink-like dynamics, and dissipate energy locally (confined eruptions). Up to 25% of the induced twist energy is dissipated and available to power X-ray flares in powerful global eruptions, with most of our models showing an energy release in the range of the most common X-ray outbursts, ≲10 43 erg. Such events occur when significant energy builds up while deeply buried in the dipole magnetosphere. Less energetic outbursts likely precede powerful flares, due to intermittent instabilities and confined eruptions of a continuously twisting flux tube. Upon reaching a critical state, global eruptions produce the necessary Poynting-flux-dominated outflows required by models prescribing the fast radio burst production in the magnetar wind—for example, via relativistic magnetic reconnection or shocks.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Predicting Wind Loading and Instability in Solar Tracking PV Arrays

Wind loading and the fluctuating pressure loads it creates on PV panel surfaces are associated with multiple degradation mechanisms and failures. Modest wind speeds create reversing loads that can initiate cell cracks and weather cracked cells. Stronger wind speeds and extreme weather events can lead to larger scale forces and the aerodynamic instability known as torsional galloping. All these effects are dependent on the complex coupling between wind speed, panel orientation, and a myriad of other hardware and site-specific factors. In this work, we present the latest developments from our work to build an open-source, high-performance computing (HPC) fluid dynamics solver to predict and mitigate these effects. This simulation package allows users to easily specify different array layouts, solar-tracking angles, panel geometries, and weather conditions before automatically generating a refined computational mesh and solving for the unsteady loading on each panel surface. Small domains (e.g., a single panel row in isolation) can be solved on a modern laptop, while larger domains or very high-fidelity studies can be solved on distributed or HPC resources with minimal modifications to the underlying problem specification. We present preliminary case studies obtained using this simulation package and highlight how increased wind speeds combined with sub-optimal tracking angles can exacerbate degradation drivers.

aerodynamics↗
DOE OSTI2024

Thermally frustrated phase transition at high pressure in B 2-ordered FeV

X-ray diffraction measurements of equiatomic B2-ordered FeV were performed in a diamond-anvil cell at room temperature at several pressure points up to 80 GPa that showed the cubic phase to be stable with no indication of structural phase transitions. Density functional theory at 0 K predicts Fermi surface nesting, an electronic topological transition, and a phonon dynamical instability within the experimentally investigated pressure range. Nevertheless, the instability is absent in phonon dispersion curves extracted from ab initio molecular dynamics simulations below the critical volume at temperatures as low as 10 K, indicating that thermal atomic displacements can frustrate the phase transition by renormalizing the phonon dispersion curves. Ferrimagnetism is critical for the stability of the cubic phase at low temperature, but thermal atomic displacements are enough to support the structure at and above the Néel temperature.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Effect of H + Exchange and Surface Impurities on Bulk and Interfacial Electrochemistry of Garnet Solid Electrolytes

Contact loss and current constriction pose significant challenges at the Li metal interface of solid-state batteries. For garnet-structured Li 7 La 3 Zr 2 O 12 (LLZO), these effects are amplified by Li + /H + exchange and surface contamination reactions, which lead to conductivity losses and poor Li wetting. In this study, we utilize a variety of surface treatment processes across 37 cells to selectively induce proton exchange and contamination reactions in LLZO. The resulting bulk and surface chemistry is systematically characterized and correlated to changes in electrochemical properties. Additionally, we combine impedance analysis and finite element method modeling to deconvolute sources of impedance contributions at the Li metal interface. Specifically, we show that constriction impedance at the Li metal interface arises not solely from voids, but also from ionically-resistive surface contaminants. Further, these findings emphasize the connection between ionic conductivity and constriction, demonstrating that micron-scale ionically-resistive components increase constriction even with identical contact geometries. Finally, we leverage our comprehensive dataset to highlight unstable overpotential growth as a failure mechanism, additionally showing that the phase of a cell’s impedance is a sensitive indicator for the onset of interfacial instability. Overall, this study clarifies the impacts of proton exchange and surface contamination on electrochemical properties at the Li|solid electrolyte interface and elucidates insights that are generalizable to other solid-state battery systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Modelling and experiment to stabilize disruptive tearing modes in the ITER baseline scenario in DIII-D

Abstract The achievement of high gain, stationary conditions in a tokamak scenario aimed at producing fusion energy in the ITER Project is crucial to the demonstration that this form of energy can be used in future reactors to provide cheap and clean energy globally. Disruptions are a challenge for the fusion energy field, in particular for the ‘ITER Baseline Scenario’ (IBS), as reproduced in the DIII-D tokamak. This work shows that a solution has been found for the m = 2/ n = 1 tearing modes that have consistently caused disruptions in the IBS: stable operation down to zero input torque was achieved by modifying the current density profile at the beginning of the pressure flattop and the ELM character later in the discharges, guided by previous results showing that the most likely cause of these instabilities is the current density profile. The coupling between sawteeth, n>2 modes and the 2/1 TMs is shown to not be statistically significant, nor the leading origin for the evolution towards instability. Ideal and resistive MHD modeling provide positive verification that a steeper ‘well’ in the region of the q = 2 rational surface leads to worse ideal stability, higher tearing index Δ’ and lower threshold Δ’ c for resistive instabilities, consistent with the experimental results. This provides confidence that the methods used in this work can be extrapolated to other devices and applied to avoid disruptions in ITER and pulsed fusion devices worldwide.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Capillary Water in 2-D Drying-Cracking Soil Sub-Grain Models: Morphology and Kinematics of Evaporation and Haines Jumps

Morphing of capillary water during the drying of a cluster of three wet grains is imaged and measured. The uniqueness of the tests is in the grains being long cylinders to make the system as close to a 2-D one as possible. In this way, the Laplace pressure depends on the only one curvature of the meniscus, which can easily be followed and is continuously image processed. The motion of liquid/gas interface, and its rate, as well as of contact angle and perimeter, are also monitored. The drying water body has been known to undergo two modes of re-morphing: a slow, evaporation rate-controlled one and a fast, inertia-driven instabilities of the interfaces. Two particular forms of dynamic re-morphing are being followed: one, called classically an “air entry,” which is a meniscus jump before its approaching the throat between the top and a bottom grain and another jump of the bottom contact, with a splitting of the meniscus into two between only two of the three grains. Associated dynamic variables, capillary pressure, and surface tension forces developing prior to and in conjunction with the instabilities of the menisci are presented in a companion paper by Hueckel et al..

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Shock-induced bubble jets: a dual perspective of bubble collapse and interfacial instability theory

Interactions between shock waves and gas bubbles in a liquid can lead to bubble collapse and high-speed liquid jet formation, relevant to biomedical applications such as shock wave lithotripsy and targeted drug delivery. This study reveals a complex interplay between acceleration-induced instabilities that drive jet formation and radial accelerations causing overall bubble collapse under shock wave pressure. Using high-speed synchrotron X-ray phase contrast imaging, the dynamics of micrometre-sized air bubbles interacting with laser-induced underwater shock waves are visualised. These images offer full optical access to phase discontinuities along the X-ray path, including jet formation, its propagation inside the bubble, and penetration through the distal side. Jet formation from laser-induced shock waves is suggested to be an acceleration-driven process. A model predicting jet speed based on the perturbation growth rate of a single-mode Richtmyer–Meshkov instability shows good agreement with experimental data, despite uncertainties in the jet-driving mechanisms. The jet initially follows a linear growth phase, transitioning into a nonlinear regime as it evolves. To capture this transition, a heuristic model bridging the linear and nonlinear growth phases is introduced, also approximating jet shape as a single-mode instability, again matching experimental observations. Upon piercing the distal bubble surface, jets can entrain gas and form a toroidal secondary bubble. Linear scaling laws are identified for the pinch-off time and volume of the ejected bubble relative to the jet’s Weber number, characterising the balance of inertia and surface tension. At low speeds, jets destabilise due to capillary effects, resulting in ligament pinch-off.

Drops and Bubbles: Bubble dynamics↗
DOE OSTI2024

Formation of field-induced breakdown precursors on metallic electrode surfaces

Understanding the underlying factors responsible for higher-than-anticipated local field enhancements required to trigger vacuum breakdown on pristine metal surfaces is crucial for the development of devices capable of withstanding intense operational fields. In this study, we investigate the behavior of nominally flat copper electrode surfaces exposed to electric fields of hundreds of MV/m. Our novel approach considers curvature-driven diffusion processes to elucidate the formation of sharp breakdown precursors. To do so, we develop a mesoscale finite element model that accounts for driving forces arising from both electrostatic and surface-tension-induced contributions to the free energy. Our findings reveal a dual influence: surface tension tends to mitigate local curvature, while the electric field drives mass transport toward regions of high local field density. This phenomenon can trigger the growth of sharper protrusions, ultimately leading to a rapid enhancement of local fields and, consequently, to a runaway growth instability. We delineate supercritical and subcritical regimes across a range of initial surface roughness. Our numerical results are in qualitative agreement with experimentally reported data, indicating the potential practical relevance of field-driven diffusion in the formation of breakdown precursors.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Adhesion-force micro-scale study of desiccating granular material

Experiments on five-, four-, three- and two-wet-hydrophilic-grain clusters were performed to investigate evolution of adhesion of granular media during drying on the micro-scale. The experiments show that the adhesion-force of a cluster initially grows at most to three times the original value before decreasing to zero by the end of evaporation. The adhesion-force is composed of capillary pressure force acting over the liquid/solid contact surface area, and surface tension forces acting over the three-phase contact perimeter length. This is in contrast with most macro-scale phenomenological models, in which the only desaturation process variables affecting strength are suction and saturation. Both the contact surface area and contact perimeter length are reduced to zero upon complete liquid evaporation. The morphology of an evaporating water body evolves through slow flow controlled by evaporation rate, interrupted by various modes of fast air entry, which are non-equilibrium jumps of liquid/gas interfaces (Haines jumps). The instabilities involve large adhesion force discontinuities and substantial water mass reconfiguration with water flow in an extremely short time, which makes the process transient. The reconfigurations can reduce the original multi-grain water clusters to four-, three- and two-grain clusters by way of three different instability modes: of thin-sheet instability, or meniscus snap-through instability, depending on the sign of the Gauss curvature of the liquid surface, or finally, for two-grain bridges only, a liquid wire pinch-off. For larger meso-scale assemblies, however, the global adhesion-force evolution is little affected by the jumps. The air entries are potential sites for drying cracks. The (approximately) calculated capillary pressure for two- and three-grain clusters, in no cases is seen to reach high values, predicted from water retention curves.

Engineering↗
DOE OSTI2020

An In Situ Formed Surface Coating Layer Enabling LiCoO 2 with Stable 4.6 V High‐Voltage Cycle Performances

Abstract The development of high‐voltage LiCoO 2 is essential for achieving lithium‐ion batteries with high volumetric energy density, however, it faces a great deal of challenges owing to the materials, structure and interfacial instability issues. In this work, a strategy is developed, through heat annealing a precoated surface layer to in situ form a high‐voltage‐stable surface coating layer, which is demonstrated to be highly effective to improve the high‐voltage performance of LiCoO 2 . It is discovered that LiCoO 2 reacts with Li 1.5 Al 0.5 Ti 1.5 (PO 4 ) 3 (LATP) at 700 °C to form exclusively spinel phases in addition to Li 3 PO 4 , which are structurally coherent to the layered lattice of LiCoO 2 . The heat annealing of the precoated thin layer of LATP enables the formation of a high‐quality surface layer. Spinel phases possess high‐voltage‐stable structures with much weaker oxidizing ability of lattice oxygen than layered structure. In addition, the Li 3 PO 4 is a good lithium‐ion conductor with excellent chemical stability at high voltages. All these benefits contribute to the construction of a uniform and conformal high‐voltage‐stable surface layer with favorable lithium conducting kinetics at the LiCoO 2 surface. The modified LiCoO 2 shows excellent 4.6 V high‐voltage cycle performance at both room temperature and 45 °C. The thermal stability is greatly enhanced as well.

Wang, Yi↗
DOE OSTI2020

Design of Cylindrical Implosion Experiments to Demonstrate Scale-Invariant Rayleigh-Taylor Instability Growth

Radiation-hydrodynamics simulations are used to design laser-driven cylindrical implosion experiments to directly measure hydrodynamic instability growth in convergent geometry. Designs for two different size targets, varying in radial dimension by a factor of three, are presented. A set of beam pointings and powers are identified for each scale design that result in a nearly axially uniform implosion of an embedded marker layer. The implosion trajectories are shown to be scale-invariant between designs, with nearly identical scaled acceleration profiles. Finally, linear theory and radiation-hydrodynamics simulations predict that Rayleigh-Taylor instability growth of an azimuthal perturbation, machined on the inner surface of the embedded marker, is also scale-invariant between designs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Resolving Chemical and Spatial Heterogeneities at Complex Electrochemical Interfaces in Li-Ion Batteries

The high specific capacities of Ni-rich transition metal oxides have garnered immense interest for improving the energy density of Li-ion batteries (LIBs). Despite the potential of these materials, Ni-rich cathodes suffer from interfacial instabilities that lead to crystallographic rearrangement of the active material surface as well as the formation of a cathode electrolyte interphase (CEI) layer on the composite during electrochemical cycling. While changes in crystallographic structure can be detected with diffraction-based methods, probing the chemistry of the disordered, heterogeneous CEI layer is challenging. In this work, we use a combination of ex situ solid-state nuclear magnetic resonance (SSNMR) spectroscopy and X-ray photoemission electron microscopy (XPEEM) to provide chemical and spatial information, on the nanometer length scale, on the CEI deposited on LiNi 0.8 Mn 0.1 Co 0.1 O 2 (NMC811) composite cathode films. XPEEM elemental maps offer insight into the lateral arrangement of the electrolyte decomposition products that comprise the CEI and paramagnetic interactions (assessed with electron paramagnetic resonance (EPR) and relaxation measurements) in 13 C SSNMR provide information on the radial arrangement of the CEI from the NMC811 particles outward. Using this approach, here we find that LiF, Li 2 CO 3 , and carboxy-containing structures are directly appended to NMC811 active particles, whereas soluble species detected during in situ 1 H and 19 F solution NMR experiments (e.g., alkyl carbonates, HF, and vinyl compounds) are randomly deposited on the composite surface. We show that the combined approach of ex situ SSNMR and XPEEM, in conjunction with in situ solution NMR, allows spatially-resolved, molecular-level characterization of paramagnetic surfaces and new insights into electrolyte oxidation mechanisms in porous electrode films.

36 MATERIALS SCIENCE↗
DOE OSTI2023

New linear stability parameter to describe low-β electromagnetic microinstabilities driven by passing electrons in axisymmetric toroidal geometry

In magnetic confinement fusion devices, the ratio of the plasma pressure to the magnetic field energy, β, can become sufficiently large that electromagnetic microinstabilities become unstable, driving turbulence that distorts or reconnects the equilibrium magnetic field. In this paper, a theory is proposed for electromagnetic, electron-driven linear instabilities that have current layers localised to mode-rational surfaces and binormal wavelengths comparable to the ion gyroradius. The model retains axisymmetric toroidal geometry with arbitrary shaping, and consists of orbit-averaged equations for the mode-rational surface layer, with a ballooning space kinetic matching condition for passing electrons. The matching condition connects the current layer to the large scale electromagnetic fluctuations, and is derived in the limit that β is comparable to the square root of the electron-to-ion-mass ratio. Electromagnetic fluctuations only enter through the matching condition, allowing for the identification of an effective β that includes the effects of equilibrium flux surface shaping. The scaling predictions made by the asymptotic theory are tested with comparisons to results from linear simulations of micro-tearing and electrostatic microinstabilities in MAST discharge #6252, showing excellent agreement. In particular, it is demonstrated that the effective β can explain the dependence of the local micro-tearing mode (MTM) growth rate on the ballooning parameter θ 0 – possibly providing a route to optimise local flux surfaces for reduced MTM-driven transport.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Vertical control of DIII-D discharges with strong negative triangularity

Through predictive modeling validated by a series of experiments on DIII-D, the vertical stability of low β diverted plasmas with strong negative triangularity (NT) ($\delta\sim-0.6$) is assessed. As a result of their unique magnetic geometry, NT plasmas feature larger Shafranov shifts and more elongated inner flux surfaces than positive triangularity counterparts, typically leading to enhanced vertical instability growth rates. However, coupling with the non-conformal vessel DIII-D wall reduces these growth rates to controllable values, providing a path forward for stabilizing strongly NT plasma with a diverted geometry. These discharges are used to validate GSdesign (part of the TokSys code suite) stability calculations in strong NT plasmas on DIII-D, with errors of no more than ~20% observed between modeled and experimentally measured growth rates. Additions of diagnostic noise and power supply tuning to the TokSys model are needed to accurately capture the time dependence of DIII-D NT discharges, assisting with the design of control schemes specific to the DIII-D poloidal field coils. Lastly, implications of these results on a future NT reactor are briefly described.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗