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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10

Release of the NDI 2.2.0

The Nuclear Data Interface 2.2.0 has been released. It includes the addition of charged particle dE/dx (stopping power) data, the ability to read in NDI-formatted binary data, corrections to TN data, and other minor changes and bug fixes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Release of the NDI 2.2.0alpha

The Nuclear Data Interface 2.2.0alpha has been released. It includes the addition of charged particle dE/dx (stopping power) data, the ability to read in NDI-formatted binary data, corrections to TN data, CP 2011 and CP 2020 data, and other minor changes and bug fixes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Time-Sensitive Quantum Key Distribution (TSQKD)

This is the final report for the Time-Sensitive Quantum Key Distribution (TSQKD) project and summarizes the demonstration and longer-term field testing at an electric utility, EPB of Chattanooga, in Chattanooga, TN. The demonstration was held virtually (due to the COVID pandemic) and successfully executed the tests outlined in a prior report, “Task 10: Develop a QKD Time-Sensitive Networking Test Suite” submitted 9/30/2020. The portable test equipment explained in Task 10 and earlier task reports was tested at GE Research remotely connected with Qubitekk’s QKD equipment in San Diego, CA. Then the equipment was shipped to Qubitekk for physical integration with Qubitekk’s Quantum DataLoc™ Key Server 1570nm (http://qubitekk.com/products/qkd-for-industrial-control-systems-ics/). The portable test equipment was shipped from Qubitekk to EPB for demonstration and extended field testing. A summary of the demonstration and test results are described in this report. The demo and extended field test results are enabled by the NETCONF/YANG IEEE P1913 data management model developed as part of this project (Task 5). The NETCONF/YANG IEEE P1913 data management model demonstrated significant practical utility in providing a common means of monitoring and configuring the QKD system. All data in this report comes from the IEEE P1913 data management model.

24 POWER TRANSMISSION AND DISTRIBUTION↗

High Data Rate Detector for Neutron Reflectometer

Neutron reflectometers are a class of instruments that employ neutron diffraction for measuring the structure of thin films. The technique provides valuable information over a wide variety of scientific and technological applications including chemical aggregation, polymer and surfactant adsorption, structure of thin film magnetic systems, biological membranes, etc. Such instruments are considered to be one of the most important in the neutron science field. Newer facilities place growing demands on the count rate capability of the specialized neutron detectors required. Proportional Technologies completed the Phase I effort successfully with a fully operational prototype detector built at PTI and tested at the CG1A neutron beam of the High Flux Isotope Reactor (HFIR, Oak Ridge, TN). The prototype incorporated 3 panels of 14 copper-walled cells each (total of 42 cells), each lined with 1.3 μm of 10B4C. The detector was tested for efficiency, spatial resolution, count rate linearity, uniformity, overlap and scatter. Testing revealed stable operation, uniform response across cells, and successful resolution of individual cells. The maximum count rate tested in the 3 panels combined was 590 kHz, limited by a deadtime of about 1 μs in the digital electronics. The local rate measured in a single cell showed no deadtime losses up to 810 cps/mm2, indicating that a rate of 20 Mhz can be supported in the 308-cell detector planned for Phase II.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Low-Temperature Electrochemical Wastewater Oxidation

Here, we demonstrated the Clean Sustainable Electrochemical Treatment (CleanSET) process that enables the distributed clean-up of biomass-derived wastewater while simultaneously generating hydrogen (H 2 ). The specific goal of this project is to 1) demonstrate the selective removal of chemical oxygen demand (COD), total carbon (TC), and total nitrogen (TN) of different wastewaters, 2) optimize the electrode composition to improve electrochemical performance, and 3) perform a high-level techno-economic analysis to obtain levelized costs of disposal (LCOD) .

08 HYDROGEN↗

Uncertainty in Thermal Modeling of Spent Nuclear Fuel Casks

Uncertainty is a key metric in computational modeling that must be evaluated for results to have wide ranging applicability. A well characterized uncertainty range is ideal with clear error bars on results that can be presented to stakeholders. In the field of spent fuel cask modeling, this ideal has been historically difficult to achieve in practice because of the computationally intensive nature of the models used and the difficulty assigning reasonable uncertainties to quantities in as-built systems. The work in this report has been conducted to evaluate the overall state of uncertainty and sensitivity in spent fuel cask models and develop methodologies for evaluating these uncertainties. These methodologies must be practical for engineering applications. They should not require excessive computational resources or calendar time to achieve results. In engineering, the model must be on a scale such that it can be changed and adapted throughout a project as new information is discovered and project goals evolve. This report covers three major modeling task areas that provide an overview of the types of sensitivity and uncertainty present in a spent fuel storage and transportation system. Section 3 discusses sensitivity and uncertainty analysis in the effective thermal conductivity model for the fuel region and applies these results to a single assembly model. Section 4 shows sensitivity analysis of a full cask model in the TN-32B and Section 5 demonstrates the overall uncertainty workflow using Coolant Boiling in Rod Arrays – Spent Fuel Storage and STAR-CCM+ developed from the sensitivity work in the preceding sections.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Preliminary Simulations of Commercial Drying Cycles Using the Advanced Drying Cycle Simulator

The purpose of this report is to document updates on the apparatus to simulate commercial vacuum drying procedures at the Nuclear Energy Work Complex at Sandia National Laboratories. Validation of the extent of water removal in a dry spent nuclear fuel storage system based on drying procedures used at nuclear power plants is needed to close existing technical gaps. Operational conditions leading to incomplete drying may have potential impacts on the fuel, cladding, and other components in the system during subsequent storage and disposal. A general lack of data suitable for model validation of commercial nuclear canister drying processes necessitates well-designed investigations of drying process efficacy and water retention. Scaled tests that incorporate relevant physics and well-controlled boundary conditions are essential to provide insight and guidance to the simulation of prototypic systems undergoing drying processes. This report documents fiscal year 2023 (FY23) updates on the Advanced Drying Cycle Simulator (ADCS). This apparatus was built to simulate commercial drying procedures and quantify the amount of residual water remaining in a pressurized water reactor (PWR) fuel assembly after drying. The ADCS was constructed with a prototypic 17×17 PWR fuel skeleton and waterproof heater rods to simulate decay heat. These waterproof heaters are the next generation design to heater rods developed and tested at Sandia National Laboratories in FY20. In FY23, a series of four simulated commercial drying tests was completed. This report presents the temperature and pressure histories of the drying tests as well as axial temperature profiles that can be compared to data from the Electric Power Research Institute (EPRI) High Burnup Demonstration TN-32B cask. Water content measurements and dew point calculations from a Hiden Analytical HPR-30 mass spectrometer are also presented in this report. Due to familiarization with this first-of-a-kind system, refinements to equipment calibration and test procedures have been identified to better match commercial drying cycles for future simulated tests. However, the presented data demonstrate the successful construction and operation of a viable research platform for quantifying residual water content closely approaching that expected in dry storage canisters during commercial drying procedures.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Thermonuclear Burn in a Multiphysics Code on GPUs

Multiphysics codes links to a library called SINGE for the calculation of thermonuclear (TN) burn rates, but some current multiphysics codes do not attempt to leverage the support for parallel operation that SINGE provides. Our goal is to investigate implementations of the SINGE workflow and analyze how the use of a performance portability layer could reduce run time on CPU archi tectures while also supporting GPU architectures without requiring code modifications. We looked to the Kokkos C++ Performance Portability Ecosystem to implement hardware agnostic parallel patterns.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Temperature-Time Modeling of Spent Fuel Cladding in Dry Storage Casks

This report uses thermal and decay heat modeling to investigate spent fuel performance and the potential for cladding to anneal in dry storage conditions. Annealing is an important feature to investigate in SNF cladding because it has a direct relationship to cladding response in storage, transportation and disposal conditions. Annealed cladding may have lower strength than unannealed cladding, however its increased ductility would provide better protection against rupture in high strain rate situations such as severe accidents. These consequences are the driver for this work however are outside of the scope of this report. The modeling focused on three representative storage systems, the TN-32B, MAGNASTOR with TSC-37 canister, and NUHOMS AHSM with a 32PTH2 canister. This covers the vertical dual-purpose, vertical ventilated and horizontal ventilated casks respectively. Decay heat modeling using high and low enrichment assemblies was used to bound the decay heat curves that might be expected in dry storage. To bound the temperature relationship, the storage casks were modeled starting at the design basis heat loads with heat decaying through time. Although the results are bounding there is not an attempt to maximize conservatism, rather the intent to form a reasonable upper limit on temperature that will be broadly applicable to the U.S. cask fleet. This will allow materials testing to focus on relevant conditions for annealing that may affect the U.S. spent fuel inventory. The results show a clear dependence on heat load pattern in time in Figure S-1 and Figure S-2. This dependence is due to the different assembly decay heat curves for different assemblies in preferentially loaded casks. It shows the need for careful decay heat modeling when examining in service fuel temperatures that are less than the cask design basis heat load. The body of the report shows percent cladding cutoffs of 300°C and 350 °C as well. These results can be used to inform testing and conclusions about cladding performance through time and the potential for cladding annealing during dry storage.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Supplement Analysis for the Proposed Shipment of High Burnup Research Cask to Idaho National Laboratory for Research and Development Purposes

DOE needs to continue with the HBUSFDP and transfer the HBURC to a facility capable of examination and testing of HBU SNF. These types of facilities do not exist at NAPS but are available at DOE national laboratories. The removal and eventual opening of the TN-32B research cask will provide DOE with the opportunity to gather data that will support continued safe storage of SNF at existing nuclear power plants, or a future federal consolidated storage facility. This effort will also help build public trust and confidence by demonstrating DOE’s ability to safely and securely transport commercial SNF using the certified Atlas rail consist.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Integrated Anaerobic Membrane Bioreactor (AnMBR) – electro assisted fermentation platform for total resource recovery from diverse wastewaters

The overall objective of the project was to demonstrate a successful wastewater resource recovery platform comprising an Anaerobic Membrane Bioreactor (AnMBR) to achieve >50% Carbon sequestration efficiency as Volatile Fatty Acids (VFAs) or as methane gas from agricultural (animal feeding operations) wastewater along with the generation of final water exceeding Biological Nutrient Removal (BNR) standards for indirect potable reuse by coupling with constructed wetlands has been successfully accomplished. The AnMBR achieved stable performance over 350 days, removing 80–90% of COD and BOD₅ and recovering methane (0.17±0.07 L CH4/g COD at 66.5±0.03% v/v) at 3-5 LMH flux and 5-9 days HRT with 3-5% w/v total solids. Phosphorus recovery via CaO addition in an 80-L coagulation-flocculation-sedimentation unit ranged from 40.6% to 99.7%, yielding products with 11.4–13.6% P content and citric acid solubility of 32–38.6% P, comparable to rock phosphate mineral. Ammonium adsorption achieved ~94.5% recovery with exchange capacity of 10 – 16 g NH4-N/kg clinoptilolite. The CW polishing step met Kansas discharge standards for BOD5 and TN (<30 and <10 mg /L,) and approached the TP standard (~2.5 – 4 mg P/L). These findings have either already resulted in two peer reviewed publications, two patent applications, and one publication in conference proceedings.

42 ENGINEERING↗

Quantification of LEU Holdup using gamma ray imaging and inverse transport solver

Holdup is the residual amount of special nuclear material (SNM) remaining in a processing facility after the bulk materials have been cleaned out. In commercial uranium processing facilities, quantification of holdup is a major challenge because of the highly variable shapes and sizes of the deposits. Any method that attempts to generalize and calibrate deposit shapes in order to quantify holdup will be prone to high uncertainties. Uncertainties on the order of ±50% are typical in holdup results. In international safeguards applications, a ±50% uncertainty can result in a large amount of material unaccounted for (MUF) thereby increasing the difficulty of detecting material diversion and facility misuse. An imaging-based methodology has been developed with the objective of significantly reducing this uncertainty by using the true deposit shape, instead of relying on oversimplified geometric assumptions. The project is a collaboration between ORNL, Y-12, and the University of Tennessee, Knoxville, TN. Uranium sources of known masses were measured using the Germanium Gamma-ray Imager (GeGI), a high-resolution imaging spectrometer, creating a pixelated map for each spectral bin. Two different gamma imaging methods are employed in this work: coded aperture imaging and Compton imaging. A validated MonteCarlo model of the detector has been developed using the GEANT4 code for determining the intrinsic response of the detector, its enclosure, and the coded aperture mask. An inverse transport solver based on the Markov Chain Monte-Carlo approach known as Differential Evolution Adaptive Metropolis (DREAM) is employed to use the measurement data from the image pixels (coded aperture or Compton) to solve for the mass of 235 U in the deposit. A reliable method based on the DREAM solver has been developed to flag the infinite thickness condition of a uranium deposit. The project team is working towards improving the image reconstruction for Compton imaging so that a better localization of the source can be achieved. Besides treating the coded aperture and Compton imaging methods independently, the project is also evaluating a combined method that uses the Compton scatter data from a coded aperture measurement. GEANT4 simulations are being performed to evaluate the combined approach. The impact on the DREAM optimization as the source thickness progressively approaches infinite thickness is being evaluated. A number of uranium sources available at ORNL have been measured, and the DREAM results have been tested and validated for the coded aperture imaging. A similar effort will be carried out to validate the Compton based method once the development of algorithms for better localization are complete. The imaging based quantification is very amenable to unattended monitoring of holdup accumulation at key measurement points. A proof of concept measurement has been completed to demonstrate this capability The current work used the high energy resolution imager GeGI. However, the approach and methodologies are applicable to other imagers such as the cadmium zin telluride (CZT) based imager manufactured by H3D, Inc.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

2023 Billion-Ton Report

The U.S. Department of Energy Bioenergy Technology Office's (BETO's) 2023 Billion-Ton Report (BT23) is an assessment of renewable carbon resources potentially available in the United States. BT23 explores these resources in terms of quantity, price, geographical density and distribution, and market maturity. Resource quantities in this report are limited by specified economic and environmental sustainability constraints. Good practices are needed to ensure biomass production has positive environmental outcomes. BT23 supports BETO's mission, particularly the 2023 Multi-Year Program Plan. To access 2023 Billion-Ton Report PDFs, appendices, and high-level messages, navigate to the 2023 Billion-Ton Report landing page at https://energy.gov/eere/bioenergy/2023-billion-ton-report-assessment-us-renewable-carbon-resources on the U.S. Department of Energy Bioenergy Technologies Office website. To access information about the quality assumptions used in this report, please see the Biomass Feedstock Library at https://bioenergylibrary.inl.gov/Home/Home.aspx Please cite the 2023 Billion-Ton Report as: U.S. Department of Energy. 2024. 2023 Billion‐Ton Report: An Assessment of U.S. Renewable Carbon Resources. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. ORNL/SPR-2024/3103. doi: 10.23720/BT2023/2316165. Contact Us

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Chapter 1: Background and Introduction

Langholtz, M. H. 2024. “Chapter 1: Background and Introduction.” In 2023 Billion‐Ton Report. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. doi: 10.23720/BT2023/2316166.

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Chapter 2 Biomass Currently Used for Energy and Coproducts

Jacobson, R., and S. Curran. 2024. “Chapter 2: Biomass Currently Used for Energy and Coproducts.” In 2023 Billion‐Ton Report. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. doi: 10.23720/BT2023/2316167.

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Chapter 3: Waste Resources and Byproducts

Milbrandt, A., and A. Badgett. 2024. “Chapter 3: Waste Resources and Byproducts.” In 2023 Billion‐Ton Report. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. doi: 10.23720/BT2023/2316168.

Milbrandt, Anelia↗

Chapter 4: Biomass from the Forested Land Base

Davis, M., L. Lambert, R. Jacobson, D. Rossi, C. Brandeis, J. Fried, B. English, et al. 2024. “Chapter 4: Biomass from the Forested Land Base.” In 2023 Billion‐Ton Report. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. doi: 10.23720/BT2023/2316170.

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Chapter 5: Biomass from Agriculture

Hellwinckel, C., D. de la Torre Ugarte, J. L. Field, and M. Langholtz. 2024. “Chapter 5: Biomass from Agriculture.” In 2023 Billion‐Ton Report. M. H. Langholtz (Lead). Oak Ridge, TN: Oak Ridge National Laboratory. doi: 10.23720/BT2023/2316171.

Hellwinckel, Chad↗