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Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA) Field Campaign Report

With their extensive coverage, low clouds greatly impact global climate. Presently, low clouds are poorly represented in global climate models (GCMs), and the response of low clouds to changes in atmospheric greenhouse gases and aerosols remains the major source of uncertainty in climate simulations. The poor representations of low clouds in GCMs are in part due to inadequate observations of their microphysical and macrophysical structures, radiative effects, and the associated aerosol distribution and budget in regions where the aerosol impact is the greatest. The Eastern North Atlantic (ENA) is a region of persistent but diverse subtropical marine boundary layer (MBL) clouds, whose albedo and precipitation are highly susceptible to perturbations in aerosol properties. Boundary-layer aerosol in the ENA region is influenced by a variety of sources, leading to strong variations in cloud condensation nuclei (CCN) concentration and aerosol optical properties. A permanent ENA site was established by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility on Graciosa Island in the Azores, providing invaluable information on MBL aerosol and low clouds. At the same time, the vertical structures and horizontal variabilities of aerosol, trace gases, cloud, drizzle, and atmospheric thermodynamics are critically needed for understanding and quantifying the budget of MBL aerosol, the radiative properties, precipitation efficiency, and lifecycle of MBL clouds, and the cloud response to aerosol perturbations. Much of this data can be obtained only through aircraft-based measurements. In addition, the interconnected aerosol and cloud processes are best investigated by a study involving simultaneous in situ aerosol, cloud, and thermodynamics measurements. Furthermore, in situ measurements are also necessary for validating and improving ground-based retrieval algorithms at the ENA site. The Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA) project was motivated by the need for comprehensive in situ characterizations of boundary-layer structure, and associated vertical distributions and horizontal variabilities of low clouds and aerosol over the Azores. The ARM Aerial Facility (AAF) Gulfstream-1 (G-1) aircraft was deployed during two intensive measurement periods (IOPs). The first deployment took place from June 21 to July 20, 2017, and the second one took place from January 15 to February 18, 2018. Flights were carried out in the Azores, near the ARM ENA site on Graciosa Island. Deployments during both seasons allow for examination of key aerosol and cloud processes under a variety of representative meteorological and cloud conditions. The science themes for the deployments include: (1) Budget of MBL CCN and its seasonal variation; (2) Effects of aerosol on cloud and precipitation; (3) Cloud microphysical and macrophysical structures, and entrainment mixing; (4) Advancing retrievals of turbulence, cloud, and drizzle; and (5) Model evaluation and processes studies.

Eastern North Atlantic, Graciosa Island, aerosols,↗

Current Status of Multi-Angle Implementation of Atmospheric Correction (MAIAC) Algorithm

A new Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm has been developed for MODIS. MAIAC uses a time series and an image based rather than pixel-based processing to perform simultaneous retrievals of aerosol properties and surface bidirectional reflectance. It is a generic algorithm which works over all land surface types with the exception of snow. MAIAC has an internal Cloud Mask, a dynamic land-water-snow classification and a surface change mask which allows it to flexibly choose processing path over different surfaces. A distinct feature of MAIAC is a high 1 km resolution of aerosol retrievals including optical thickness and fine mode fraction, which is required in different applications including the air quality analysis. An overview of the algorithm, results of AERONET validation, and examples of comparison with MODIS Collection 5 aerosol product, including Deep Blue algorithm, will be presented for different parts of the world including continental USA, Persian Gulf region and India.

Lyapustin, A.↗

Improved Cloud and Snow Screening in MAIAC Aerosol Retrievals Using Spectral and Spatial Analysis

An improved cloud/snow screening technique in the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm is described. It is implemented as part of MAIAC aerosol retrievals based on analysis of spectral residuals and spatial variability. Comparisons with AERONET aerosol observations and a large-scale MODIS data analysis show strong suppression of aerosol optical thickness outliers due to unresolved clouds and snow. At the same time, the developed filter does not reduce the aerosol retrieval capability at high 1 km resolution in strongly inhomogeneous environments, such as near centers of the active fires. Despite significant improvement, the optical depth outliers in high spatial resolution data are and will remain the problem to be addressed by the application-dependent specialized filtering techniques.

Lyapustin, A.↗

Polarimetric method of estimation of vertical aerosol distribution in application to observations of ozone and NO2

The degree of polarization of skylight at the zenith during twilight depends on the aerosol content in the atmosphere. The long-term observations at the high-mountain research station 'Kislovodsk' (North Caucasus) have shown that the variation of the degree of polarization after the eruption of the El Chichon volcano can serve as the effective parameter characterizing the vertical aerosol stratification in the atmosphere. The results of the measurements are confirmed by the numerical calculations. The algorithm of the retrieval of the vertical aerosol distribution on the base of the measurements of the degree of polarization is proposed. This method can be applied for the increasing of the precision of O3, NO2, and other gas content measurements.

Elansky, Nikolay F.↗

Towards a Strategy of Remote Sensing of Aerosol Direct and Indirect Radiative Forcing

The role of aerosol forcing remains one of the largest uncertainties in estimating man's impact on the global climate system. One school of thought suggests that remote sensing by satellite sensors will provide the data necessary to narrow these uncertainties. Much effort has gone into the development of new satellite sensors specifically designed to retrieve aerosol loading and some information about the sizes of the aerosols. These next generation remote sensing instruments (EOS-MODIS, EOS-MISR, POLDER, ATSR) will provide unprecedented accuracy in the retrieval of aerosol loading. Although the new generation of sensors has excellent accuracy compared to the heritage instruments of the past, they still have measurement limitations. In clean, pristine regions the absolute magnitude of the uncertainty in the aerosol retrieval becomes comparable in magnitude to the signal itself. If much of the aerosol forcing is occurring at very low magnitudes of aerosol concentrations, satellite remote sensing will miss it. This study attempts to quantify remote sensing limitations due to the accuracy limits of the retrieval algorithms. We use a combination of numerical aerosol transport models, ground-based AERONET data and ISCCP cloud climatology to determine how much of the forcing occurs in regions too clean to determine from satellite retrievals. This study is not an intercomparison of global transport models. It is not an estimation of global aerosol forcing. This study is an exercise to determine whether satellite remote sensing can live up to our high expectations. The results show that while remote sensing will be able to measure a majority of the direct forcing, it will miss roughly half of the indirect forcing.

Remer, L. A.↗

Uncertainties in Remote Sensing of Aerosol Radiative Forcing

The role of aerosol forcing remains one of the largest uncertainties in estimating man's impact on the global climate system. One school of thought suggests that remote sensing by satellite sensors will provide the data necessary to narrow these uncertainties. Much effort has gone into the development of new satellite sensors specifically designed to retrieve aerosol loading and some information about the sizes of the aerosols. These next generation remote sensing instruments (EOS-MODIS, EOS-MISR, POLDER, ATSR) will provide unprecedented accuracy in the retrieval of aerosol loading. Although the new generation of sensors has excellent accuracy compared to the heritage instruments of the past, they still have measurement limitations. In clean, pristine regions the absolute magnitude of the uncertainty in the aerosol retrieval becomes comparable in magnitude to the signal itself. If much of the aerosol forcing is occurring at very low magnitudes of aerosol concentrations, satellite remote sensing will miss it. This study attempts to quantify remote sensing limitations due to the accuracy limits of the retrieval algorithms. We use a combination of numerical aerosol transport models, ground-based AERONET data and ISCCP cloud climatology to determine how much of the forcing occurs in regions too clean to determine from satellite retrievals. This study is not an intercomparison of global transport models. It is not an estimation of global aerosol forcing. This study is an exercise to determine whether satellite remote sensing can live up to our high expectations.

Remer, L.↗

Chapter 10 - Remote Sensing Measurements of Aerosol Properties

Satellite instruments have proven especially capable at monitoring the quantity of airborne particles in columns of atmosphere, globally. This chapter describes the principles of satellite measurements and retrieval algorithms, and surveys current instruments and their capabilities. We outline the issues associated with retrieval algorithms, such as surface characterization and aerosol proximity to clouds, and the challenges with interpretation of the results. The relationship between measured aerosol properties and climate-relevant aerosol properties simulated in models is outlined, as well as how measurements are used to evaluate models. Most space-based aerosol instruments are passive sensors that measure reflected sunlight at multiple wavelengths, some at multiple viewing angles. A few are active sensors that send out their own laser light and measure the returned signal. Except when clouds are present, the excess amount of light scattered back to space, beyond that expected from the surface and atmospheric gas, is attributed to aerosol. Satellite measurements are used in many ways in aerosol research. They often provide the only method for monitoring hazardous phenomena such as major wildfire and volcanic eruption plumes, especially in remote areas. Stable, long-term, near-global-scale satellite data records make it possible to identify regional and global aerosol trends. Aerosol radiative effects on climate can be quantified on a near-global scale and used to estimate the strength of aerosol–radiation and aerosol–cloud interactions as well as to evaluate climate model simulations of these interactions. Aerosol-type mapping from satellite imagery is helpful for source attribution, model validation, and to constrain particle light-absorption properties that are essential for radiative forcing calculations. The range of aerosol properties retrieved from satellite observations has grown considerably since the first global estimates of aerosol optical depth (τ a) over ocean were made in the late 1970s. Methods for retrieving particle size and light-absorption properties were explored in the 1990s using multispectral, multi-angle observations, and polarization in visible and near-infrared wavelengths. Sensitivity to particle light absorption, primarily from black or brown carbon content, improved with the inclusion of UV channels, and sensitivity to very thin aerosol layers in the upper troposphere and lower stratosphere was advanced with the use of limb-sounding instruments and active sensors. There are limitations to every measurement technique, including satellite aerosol remote sensing. For wide-swath, passive instruments, aerosol retrievals near clouds can present substantial challenges as far as 15 km away due to cloud-scattered light contaminating the signal. In nearly all cases, retrievals over bright snow and ice surfaces are precluded because surface reflectance uncertainties can overwhelm the aerosol signal. Similarly, meteorological cloud is identified and masked out where possible. Data from passive sensors also lack vertical resolution except those that view toward the limb or where multi-angle imagery is acquired over plumes from wildfires, erupting volcanoes, and wind-blown dust. Yet, passive sensors provide vastly more coverage than the active instruments that mitigate these issues. Particle microphysical information is qualitative from all remote sensing techniques, relying on proxies to infer particle composition, hygroscopicity, and the amount of light-absorbing material. Further, particles smaller than about 200 nm diameter cannot be distinguished from atmospheric gas molecules with remote sensing, which hinders studies of cloud condensation nuclei and their effects on clouds. Most satellite instruments dedicated to aerosol observations are in low-Earth, near-polar, sun-synchronous orbits, which means they cross the equator at the same local time each day. Most are set on cycles that repeat approximately every 16 days, which makes it difficult to monitor aerosol evolution locally. Geostationary satellites make it possible to observe changes occurring from minutes to hours over regions up to 8000 km in size, but lack coverage of high latitudes, and often provide more limited constraints on aerosol properties. Ground-truth data are vital for satellite aerosol-retrieval validation. The AErosol RObotic NETwork (AERONET) of sun photometers was created in 1993 and has become an established global network of over 350 instruments for validating satellite measurements. The network, as well as global networks of ground-based lidars, solar flux radiometers and other sun photometers, are widely used for evaluating global satellite retrievals and model simulations. NASA's Earth Observing System (EOS) program beginning in 1999 led to improvements in reliability, spatial resolution, and spectral resolution (and hence, to improved particle size discrimination and light absorption properties). Satellite payloads include advanced broad-swath and multi-angle imagers, along with the first space-based active sensor focused largely on long-term aerosol monitoring. Since about 2002, Europe's SENTINEL and operational meteorological satellite fleets are also providing sustained aerosol observations, with planned continuation until at least 2030. Satellite remote sensing instruments offer valuable data for evaluating aerosol representations in global climate models. They have been used to assess aerosol optical and physical properties, trends and distributions, and are applied increasingly as direct model constraints in data assimilation to create global aerosol reanalysis products. Aerosol optical depth is the most common quantity adopted for routine model evaluation, including multiwavelength data to loosely constrain particle-size distributions. These evaluations of multiple models have revealed general biases in their regional aerosol amounts and seasonal patterns of transport and removal. Although satellite measurements have near-global coverage, substantial errors can be introduced into the model observation comparison unless attention is paid to spatial and temporal collocation, cloud screening, subgrid-scale variability, and measurement uncertainties that vary with retrieval conditions.

aerosol properties↗

A Portable Ground-Based Atmospheric Monitoring System (PGAMS) for the Calibration and Validation of Atmospheric Correction Algorithms Applied to Aircraft and Satellite Images

Detecting changes in the Earth's environment using satellite images of ocean and land surfaces must take into account atmospheric effects. As a result, major programs are underway to develop algorithms for image retrieval of atmospheric aerosol properties and atmospheric correction. However, because of the temporal and spatial variability of atmospheric transmittance it is very difficult to model atmospheric effects and implement models in an operational mode. For this reason, simultaneous in situ ground measurements of atmospheric optical properties are vital to the development of accurate atmospheric correction techniques. Presented in this paper is a spectroradiometer system that provides an optimized set of surface measurements for the calibration and validation of atmospheric correction algorithms. The Portable Ground-based Atmospheric Monitoring System (PGAMS) obtains a comprehensive series of in situ irradiance, radiance, and reflectance measurements for the calibration of atmospheric correction algorithms applied to multispectral. and hyperspectral images. The observations include: total downwelling irradiance, diffuse sky irradiance, direct solar irradiance, path radiance in the direction of the north celestial pole, path radiance in the direction of the overflying satellite, almucantar scans of path radiance, full sky radiance maps, and surface reflectance. Each of these parameters are recorded over a wavelength range from 350 to 1050 nm in 512 channels. The system is fast, with the potential to acquire the complete set of observations in only 8 to 10 minutes depending on the selected spatial resolution of the sky path radiance measurements

Schiller, Stephen↗

Mapping Aerosol Lidar Ratios Over Ocean for CALIPSO Using Modis AOD-Constrained Retrievals and A Global Aerosol Model

The CALIPSO aerosol algorithms currently assign one lidar ratio value for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms by developing regional and seasonal lidar ratio climatologies. In this study, aerosol lidar ratios are inferred through Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter profiles constrained by collocated aerosol optical depth from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) datasets. The analysis is subsampled for only those profiles that are cloud-free and contain one aerosol type (based on CALIOP feature classification). In addition, the CALIOP profiles are collocated with aerosol volume fractions simulated by the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model. In this talk, the twelve-year (2006-2017) mean spatial distributions of inferred aerosol lidar ratios for CALIOP-classified marine aerosols and the corresponding modeled sea salt volume fractions (SSVF) will be shown. Model-assisted climatological lidar ratio maps on a seasonal scale will also be presented, developed from the empirical relationship found between the modeled SSVF and lidar ratios. A comparison with past studies will be provided as well as results of a sensitivity study regarding the variability of retrieved lidar ratios as a function of horizontal averaging resolution. While the majority of this talk will focus on lidar ratios for CALIOP-classified marine aerosols, preliminary results will be shown for other aerosol types over ocean, such as dust and elevated smoke.

Travis Toth↗

SAGE III/ISS Data Product Improvements

In 2024 the Stratospheric Aerosol and Gas Experiment on the International Space Station (SAGE III/ISS) entered its eighth year of operations. Using a CCD spectrometer to observe solar and lunar occultations through Earth’s limb, the mission has retrieved tens of thousands of vertical profiles for ozone, aerosol, water vapor, and nitrogen dioxide. Retrieval algorithms are constantly under development to enhance these products. The next product version will improve upon previous versions by addressing problems with the aerosol extinction spectrum and recovering hundreds of profiles impeded by the recent proliferation of sunspots. Users of SAGE III/ISS data can also expect improvements to uncertainty estimates and a continued expansion of ancillary products.

Robert Manion↗

Correcting for Trace Gas Absorption When Retrieving Aerosol Optical Depth from Satellite Observations of Reflected Shortwave Radiation

Retrieving aerosol optical depth (AOD) from top-of-atmosphere (TOA) satellite measured radiance requires separating the aerosol signal from the total observed signal. Total TOA radiance includes signal from underlying surface and from atmospheric constituents such as aerosols, clouds and gases. Multispectral retrieval algorithms, such as the dark-target (DT) algorithm that operates upon Moderate Resolution Imaging Spectroradiometer (MODIS, onboard Terra and Aqua satellites) and Visible Infrared Imaging Radiometer Suite (VIIRS, onboard Suomi-NPP) sensors, use wavelength bands in "window" regions. However, while small, the gas absorptions in these bands are non-negligible and require correction. In this paper we use High-resolution TRANsmission (HITRAN) database and Line-by-Line Radiative Transfer Model (LBLRTM) to derive consistent gas corrections for both MODIS and VIIRS wavelength bands. Absorptions from H2O, CO2 and O3 are considered, as well as other trace gases. Even though MODIS and VIIRS bands are "similar", they are different enough that applying MODIS specific gas corrections to VIIRS observations results in an underestimate of global mean AOD (by 0.01), but with much larger regional AOD biases up to 0.07. As recent studies are attempting to create a long-term data record by joining multiple satellite datasets, including MODIS and VIIRS, the consistency of gas correction becomes even more crucial.

Satellite Remote Sensing↗

Applying the Dark Target Aerosol Algorithm with Advanced Himawari Imager Observations During the KORUS-AQ Field Campaign

For nearly 2 decades we have been quantitatively observing the Earth's aerosol system from space at one or two times of the day by applying the Dark Target family of algorithms to polar-orbiting satellite sensors, particularly MODIS and VIIRS. With the launch of the Advanced Himawari Imager (AHI) and the Advanced Baseline Imagers (ABIs) into geosynchronous orbits, we have the new ability to expand temporal coverage of the traditional aerosol optical depth (AOD) to resolve the diurnal signature of aerosol loading during daylight hours. The Korean–United States Air Quality (KORUS-AQ) campaign taking place in and around the Korean peninsula during May–June 2016 initiated a special processing of full-disk AHI observations that allowed us to make a preliminary adoption of Dark Target aerosol algorithms to the wavelengths and resolutions of AHI. Here,we describe the adaptation and show retrieval results from AHI for this 2-month period. The AHI-retrieved AOD is collocated in time and space with existing AErosol RObotic NETwork stations across Asia and with collocated Terra and Aqua MODIS retrievals. The new AHI AOD product matches AERONET, and the standard MODIS product does as well, and the agreement between AHI and MODIS retrieved AOD is excellent, as can be expected by maintaining consistency in algorithm architecture and most algorithm assumptions. Furthermore, we show that the new product approximates the AERONET-observed diurnal signature. Examining the diurnal patterns of the new AHI AOD product we find specific areas over land where the diurnal signal is spatially cohesive. For example, in Bangladesh the AOD in-creases by 0.50 from morning to evening, and in northeast China the AOD decreases by 0.25. However, over open ocean the observed diurnal cycle is driven by two artifacts, one associated with solar zenith angles greater than 70t hat may be caused by a radiative transfer model that does not properly represent the spherical Earth and the other artifact associated with the fringes of the 40 degree glint angle mask. This opportunity during KORUS-AQ provides encouragement to move towards an operational Dark Target algorithm for AHI. Future work will need to re-examine masking including snow mask, reevaluate assumed aerosol models for geosynchronous geometry, address the artifacts over the ocean, and investigate size parameter retrieval from the over-ocean algorithm.

Gupta, Pawan↗

Multiangle Implementation of Atmospheric Correction (MAIAC):: Radiative Transfer Basis and Look-up Tables - 1

This paper describes a radiative transfer basis of the algorithm MAIAC which performs simultaneous retrievals of atmospheric aerosol and bidirectional surface reflectance from the Moderate Resolution Imaging Spectroradiometer (MODIS). The retrievals are based on an accurate semianalytical solution for the top-of-atmosphere reflectance expressed as an explicit function of three parameters of the Ross-Thick Li-Sparse model of surface bidirectional reflectance. This solution depends on certain functions of atmospheric properties and geometry which are precomputed in the look-up table (LUT). This paper further considers correction of the LUT functions for variations of surface pressure/height and of atmospheric water vapor, which is a common task in the operational remote sensing. It introduces a new analytical method for the water vapor correction of the multiple ]scattering path radiance. It also summarizes the few basic principles that provide a high efficiency and accuracy of the LUT ]based radiative transfer for the aerosol/surface retrievals and optimize the size of LUT. For example, the single-scattering path radiance is calculated analytically for a given surface pressure and atmospheric water vapor. The same is true for the direct surface-reflected radiance, which along with the single-scattering path radiance largely defines the angular dependence of measurements. For these calculations, the aerosol phase functions and kernels of the surface bidirectional reflectance model are precalculated at a high angular resolution. The other radiative transfer functions depend rather smoothly on angles because of multiple scattering and can be calculated at coarser angular resolution to reduce the LUT size. At the same time, this resolution should be high enough to use the nearest neighbor geometry angles to avoid costly three ]dimensional interpolation. The pressure correction is implemented via linear interpolation between two LUTs computed for the standard and reduced pressure levels. A linear mixture and a modified linear mixture methods are used to represent different aerosol types in the aerosol/surface retrievals from several base models of the fine and coarse aerosol fractions. In summary, the developed LUT algorithm allows fast high-accuracy simulations of the outgoing radiance with full variability of the atmospheric and surface bidirectional reflectance properties for the aerosol/surface remote sensing.

Lyapustin, Alexei↗

A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations

Cloud condensation nuclei (CCN) are mediators of aerosol–cloud interactions (ACIs), contributing to the largest uncertainties in the understandings of global climate change. We present a novel remote-sensing-based algorithm that quantifies the vertically resolved CCN number concentrations (N CCN ) using aerosol optical properties measured by a multiwavelength lidar. The algorithm considers five distinct aerosol subtypes with bimodal size distributions. The inversion used the lookup tables developed in this study, based on the observations from the Aerosol Robotic Network, to efficiently retrieve optimal particle size distributions from lidar measurements. The method derives dry aerosol optical properties by implementing hygroscopic enhancement factors in lidar measurements. The retrieved optically equivalent particle size distributions and aerosol-type-dependent particle composition are utilized to calculate critical diameters using κ-Köhler theory and N CCN at six supersaturations ranging from 0.07 % to 1.0 %. Sensitivity analyses indicate that uncertainties in extinction coefficients and relative humidity greatly influence the retrieval error in N CCN . The potential of this algorithm is further evaluated by retrieving N CCN using airborne lidar from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign and is validated against simultaneous measurements from the CCN counter. The independent validation with robust correlation demonstrates promising results. Furthermore, the N CCN has been retrieved for the first time using a proposed algorithm from spaceborne lidar – Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) – measurements. The application of this new capability demonstrates the potential for constructing a 3D CCN climatology at a global scale, which helps to better quantify ACI effects and thus reduce the uncertainty in aerosol climate forcing.

54 ENVIRONMENTAL SCIENCES↗

MISR Aerosol Product Attributes and Statistical Comparisons with MODIS

In this paper, Multi-angle Imaging SpectroRadiometer (MISR) aerosol product attributes are described, including geometry and algorithm performance flags. Actual retrieval coverage is mapped and explained in detail using representative global monthly data. Statistical comparisons are made with coincident aerosol optical depth (AOD) and Angstrom exponent (ANG) retrieval results from the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument. The relationship between these results and the ones previously obtained for MISR and MODIS individually, based on comparisons with coincident ground-truth observations, is established. For the data examined, MISR and MODIS each obtain successful aerosol retrievals about 15% of the time, and coincident MISR-MODIS aerosol retrievals are obtained for about 6%-7% of the total overlap region. Cloud avoidance, glint and oblique-Sun exclusions, and other algorithm physical limitations account for these results. For both MISR and MODIS, successful retrievals are obtained for over 75% of locations where attempts are made. Where coincident AOD retrievals are obtained over ocean, the MISR-MODIS correlation coefficient is about 0.9; over land, the correlation coefficient is about 0.7. Differences are traced to specific known algorithm issues or conditions. Over-ocean ANG comparisons yield a correlation of 0.67, showing consistency in distinguishing aerosol air masses dominated by coarse-mode versus fine-mode particles. Sampling considerations imply that care must be taken when assessing monthly global aerosol direct radiative forcing and AOD trends with these products, but they can be used directly for many other applications, such as regional AOD gradient and aerosol air mass type mapping and aerosol transport model validation. Users are urged to take seriously the published product data-quality statements.

Kahn, Ralph A.↗

Creating Regional and Seasonal Climatologies of Marine and Dusty Marine Aerosol Lidar Ratios using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The CALIPSO aerosol algorithms currently assign one lidar ratio (LR) value globally for each of the seven tropospheric aerosol types. In this study, MODIS total column aerosol optical depths (AODs) are used to constrain collocated CALIOP backscatter profiles in a Fernald inversion that infers aerosol LRs for CALIOP-classified marine and dusty marine aerosols. The GOCART aerosol model is leveraged to estimate the sea salt volume fractions (SSVFs) that are collocated with the CALIOP+MODIS LR retrievals. An inverse empirical relationship is found between the SSVFs and LRs (i.e., smaller SSVFs and larger LRs near coastlines, but the opposite in the remote oceans). This SSVF/LR relationship is applied to create regional and seasonal hybrid (i.e., retrieval & model-assisted) climatological LR maps so as to develop more robust LR selections for marine and dusty marine aerosols in the CALIPSO algorithms. These analyses also provide critical LR information for the next generation of spaceborne elastic backscatter lidars.

Travis D. Toth↗

Creating Regional and Seasonal Climatologies of Marine and Dusty Marine Aerosol Lidar Ratios using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The CALIPSO aerosol algorithms currently assign one lidar ratio (LR) value globally for each of the seven tropospheric aerosol types. In this study, MODIS total column aerosol optical depths (AODs) are used to constrain collocated CALIOP backscatter profiles in a Fernald inversion that infers aerosol LRs for CALIOP-classified marine and dusty marine aerosols. The GOCART aerosol model is leveraged to estimate the sea salt volume fractions (SSVFs) that are collocated with the CALIOP+MODIS LR retrievals. An inverse empirical relationship is found between the SSVFs and LRs (i.e., smaller SSVFs and larger LRs near coastlines, but the opposite in the remote oceans). This SSVF/LR relationship is applied to create regional and seasonal hybrid (i.e., retrieval & model-assisted) climatological LR maps so as to develop more robust LR selections for marine and dusty marine aerosols in the CALIPSO algorithms. These analyses also provide critical LR information for the next generation of spaceborne elastic backscatter lidars.

Travis D. Toth↗

An Automatic Cloud Mask Algorithm Based on Time Series of MODIS Measurements

Quality of aerosol retrievals and atmospheric correction depends strongly on accuracy of the cloud mask (CM) algorithm. The heritage CM algorithms developed for AVHRR and MODIS use the latest sensor measurements of spectral reflectance and brightness temperature and perform processing at the pixel level. The algorithms are threshold-based and empirically tuned. They don't explicitly address the classical problem of cloud search, wherein the baseline clear-skies scene is defined for comparison. Here, we report on a new CM algorithm which explicitly builds and maintains a reference clear-skies image of the surface (refcm) using a time series of MODIS measurements. The new algorithm, developed as part of the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm for MODIS, relies on fact that clear-skies images of the same surface area have a common textural pattern, defined by the surface topography, boundaries of rivers and lakes, distribution of soils and vegetation etc. This pattern changes slowly given the daily rate of global Earth observations, whereas clouds introduce high-frequency random disturbances. Under clear skies, consecutive gridded images of the same surface area have a high covariance, whereas in presence of clouds covariance is usually low. This idea is central to initialization of refcm which is used to derive cloud mask in combination with spectral and brightness temperature tests. The refcm is continuously updated with the latest clear-skies MODIS measurements, thus adapting to seasonal and rapid surface changes. The algorithm is enhanced by an internal dynamic land-water-snow classification coupled with a surface change mask. An initial comparison shows that the new algorithm offers the potential to perform better than the MODIS MOD35 cloud mask in situations where the land surface is changing rapidly, and over Earth regions covered by snow and ice.

Lyapustin, Alexei↗